Spin-based Quantum Information Processing Research Articles

High-fidelity spin readout via the double latching mechanism

Projective measurement of single-electron spins, or spin readout, is among the most fundamental technologies for spin-based quantum information processing. Implementing spin readout with both high-fidelity and scalability is indispensable for developing fault-tolerant quantum computers in large-scale spin-qubit arrays. To achieve high fidelity, a latching mechanism is useful. However, the fidelity can be decreased by spin relaxation and charge state leakage, and the scalability is currently challenging. Here, we propose and demonstrate a double-latching high-fidelity spin readout scheme, which suppresses errors via an additional latching process. We experimentally show that the double-latching mechanism provides significantly higher fidelity than the conventional latching mechanism and estimate a potential spin readout fidelity of 99.94% using highly spin-dependent tunnel rates. Due to isolation from error-inducing processes, the double-latching mechanism combined with scalable charge readout is expected to be useful for large-scale spin-qubit arrays while maintaining high fidelity.

Cavity-Mediated Entanglement of Parametrically Driven Spin Qubits via Sidebands

We consider a pair of quantum dot-based spin qubits that interact via microwave photons in a superconducting cavity and that are also parametrically driven by separate external electric fields. For this system, we formulate a model for spin qubit entanglement in the presence of mutually off-resonant qubit and cavity frequencies. We show that the sidebands generated via the driving fields enable highly tunable qubit-qubit entanglement using only ac control and without requiring the qubit and cavity frequencies to be tuned into simultaneous resonance. The model we derive can be mapped to a variety of qubit types, including detuning-driven one-electron spin qubits in double quantum dots and three-electron resonant exchange qubits in triple quantum dots. The high degree of nonlinearity inherent in spin qubits renders these systems particularly favorable for parametric drive-activated entanglement. We determine multiple common resonance conditions for the two driven qubits and the cavity and identify experimentally relevant parameter regimes that enable the implementation of entangling gates with suppressed sensitivity to cavity photon occupation and decay. The parametrically driven sideband resonance approach that we describe provides a promising route toward scalability and modularity in spin-based quantum information processing through drive-enabled tunability that can also be implemented in micromagnet-free electron and hole systems for spin-photon coupling. Published by the American Physical Society 2024

Coherent manipulation of nuclear spins in the strong driving regime

Spin-based quantum information processing makes extensive use of spin-state manipulation. This ranges from dynamical decoupling of nuclear spins in quantum sensing experiments to applying logical gates on qubits in a quantum processor. Fast manipulation of spin states is highly desirable for accelerating experiments, enhancing sensitivity, and applying elaborate pulse sequences. Strong driving using intense radio-frequency (RF) fields can, therefore, facilitate fast manipulation and enable broadband excitation of spin species. In this work, we present an antenna for strong driving in quantum sensing experiments and theoretically address challenges of the strong driving regime. First, we designed and implemented a micron-scale planar spiral RF antenna capable of delivering intense fields to a sample. The planar antenna is tailored for quantum sensing experiments using the diamond’s nitrogen-vacancy (NV) center and should be applicable to other solid-state defects. The antenna has a broad bandwidth of 22 MHz, is compatible with scanning probes, and is suitable for cryogenic and ultrahigh vacuum conditions. We measure the magnetic field induced by the antenna and estimate a field-to-current ratio of G/A, representing a six-fold increase in efficiency compared to the state-of-the-art, crucial for cryogenic experiments. We demonstrate the antenna by driving Rabi oscillations in 1H spins of an organic sample on the diamond surface and measure 1H Rabi frequencies of over 500 kHz, i.e. -pulses shorter than 1 —an order of magnitude faster than previously reported in NV-based nuclear magnetic resonance (NMR). Finally, we discuss the implications of driving spins with a field tilted from the transverse plane in a regime where the driving amplitude is comparable to the spin-state splitting, such that the rotating wave approximation does not describe the dynamics well. We present a simple recipe to optimize pulse fidelity in this regime based on a phase and offset-shifted sine drive, which may be optimized in situ without numerical optimization procedures or precise modeling of the experiment. We consider this approach in a range of driving amplitudes and show that it is particularly efficient in the case of a tilted driving field. The results presented here constitute a foundation for implementing fast nuclear spin control in various systems.

A DDS-based integrated microwave source for fast frequency sweeping in quantum magnetic-resonance systems

Magnetic resonance is a fundamental method to manipulate qubits in spin-based quantum information processing. In such areas, the functionality of fast frequency sweeping is required to determine the resonance of the system. We provide a hardware-synchronized sweeping microwave source with a minimal latency in the sub-μs level based on the direct digital synthesizer technique. The output frequency can be up-converted to match the requirement for particular applications. We demonstrate this module in an optically detected magnetic resonance experiment for a nitrogen-vacancy center, and the spectrum is obtained much faster than conventional schemes with high resolution. Comparing with commercial vector signal generators, our module is highly integrated on a single board with a limited area, especially suitable for engineering of quantum sensors and devices in the future.

Strong long-range spin-spin coupling via a Kerr magnon interface

Strong long-range coupling between distant spins is crucial for spin-based quantum information processing. However, achieving such a strong spin-spin coupling remains challenging. Here we propose to realize a strong coupling between two distant spins via the Kerr effect of magnons in a yttrium-iron-garnet nanosphere. By applying a microwave field on this nanosphere, the Kerr effect of magnons can induce the magnon squeezing, so that the coupling between the spin and the squeezed magnons can be exponentially enhanced. This in turn allows the spin-magnon distance increased from nano- to micrometer scale. By considering the virtual excitation of the squeezd magnons in the dispersive regime, strong spin-spin coupling mediated by the squeezed magnons can be achieved, and a remote quantum-state transfer, as well as the nonlocal two-qubit iSWAP gate with high fidelity becomes implementable. Our approach offers a feasible scheme to perform quantum information processing among distant spins.

Analyzing nuclear spins in diamond at room temperature based on traversal periodic-signal identification

Detecting and imaging nuclear spins are of fundamental importance for spin-based quantum information processing in diamond. It is often realized by means of dynamical decoupling (DD) strategies, where a high-efficiency method for DD spectral analysis is required. Previously, a deep-learning-based algorithm is developed and applied on a cryogenic nitrogen-vacancy center experiment. Here, we improve the method by using a traversal periodic-signal identification approach before the deep-learning processing. With this improvement, low-resolution DD spectra with overlapped peaks could be well separated. This enables the deep-learning procedure being generally used in room-temperature experiments, where the measured spectra are often broadened with temperature. We apply this improved method in experiment, and its produced results match well with expectation. This method promises a wide range of applications in other spin-based systems.

Anisotropic g -tensors in hole quantum dots: Role of transverse confinement direction

Qubits encoded in the spin state of heavy holes confined in Si- and Ge-based semiconductor quantum dots are currently leading the efforts toward spin-based quantum information processing. The virtual absence of spinful nuclei in purified samples yields long qubit coherence times and the intricate coupling between spin and momentum in the valence band can provide very fast spin-orbit-based qubit control, e.g., via electrically induced modulations of the heavy-hole $g$-tensor. A thorough understanding of all aspects of the interplay between spin-orbit coupling, the confining potentials, and applied magnetic fields is thus essential for the development of the optimal hole-spin-based qubit platform. Here we theoretically investigate the manifestation of the effective $g$-tensor and effective mass of heavy holes in two-dimensional hole gases as well as in lateral quantum dots. We include the effects of the anisotropy of the effective Luttinger Hamiltonian (particularly relevant for Si-based systems) and we focus on the detailed role of the orientation of the transverse confining potential. We derive general analytic expressions for the anisotropic $g$-tensor and we present a general and straightforward way to calculate corrections to this $g$-tensor for localized holes due to various types of spin-orbit interaction, exemplifying the approach by including a simple linear Rashba-like term. Our results thus contribute to the understanding needed to find optimal points in parameter space for hole-spin qubits, where confinement is effective and spin-orbit-mediated electric control over the spin states is efficient.

Spin Digitizer for High-Fidelity Readout of a Cavity-Coupled Silicon Triple Quantum Dot

An important requirement for spin-based quantum information processing is reliable and fast readout of electron spin states, allowing for feedback and error correction. However, common readout techniques often require additional gate structures hindering device scaling or impose stringent constraints on the tuning configuration of the sensed quantum dots. Here, we operate an in-line charge sensor within a triple quantum dot, where one of the dots is coupled to a microwave cavity and used to readout the charge states of the other two dots. Owing to the proximity of the charge sensor, we observe a near-digital sensor response with a power signal-to-noise ratio >450 at an integration time of $t_{\rm int}$ = 1 $\mu$s. Despite small singlet-triplet splittings $\approx$40 $\mu$eV, we further utilize the sensor to measure the spin relaxation time of a singlet-triplet qubit, achieving an average single-shot spin readout fidelity >99%. Our approach enables high-fidelity spin readout, combining minimal device overhead with flexible qubit operation in semiconductor quantum devices.

Controlling directed atomic motion and second-order tunneling of a spin-orbit-coupled atom in optical lattices

We theoretically explore the tunneling dynamics for the tight-binding (TB) model of a single spin-orbit-coupled atom trapped in an optical lattice subjected to lattice shaking and to time-periodic Zeeman field. By means of analytical and numerical methods, we demonstrate that the spin-orbit (SO) coupling adds some new results to the tunneling dynamics in both multiphoton resonance and far-off-resonance parameter regimes. When the driving frequency is resonant with the static Zeeman field (multi-photon resonances), we obtain an unexpected new dynamical localization (DL) phenomenon where the single SO-coupled atom is restricted to making perfect two-site Rabi oscillation accompanied by spin flipping.By using the unconventional DL phenomenon, we are able to generate a ratchetlike effect which enables directed atomic motion towards different directions and accompanies periodic spin-flipping under the action of SO coupling. For the far-off-resonance case, we show that by suppressing the usual inter-site tunneling alone, it is possible to realize a type of spin-conserving second-order tunneling between next-nearest-neighboring sites, which is not accessible in the conventional lattice system without SO coupling. We also show that simultaneous controls of the usual inter-site tunneling and the SO-coupling-related second-order-tunneling are necessary for quasienergies flatness (collapse) and completely frozen dynamics to exist. These results may be relevant to potential applications such as spin-based quantum information processing and design of novel spintronics devices.

Real-Time Feedback Control of Charge Sensing for Quantum Dot Qubits

Measurement of charge configurations in few-electron quantum dots is a vital technique for spin-based quantum information processing. While fast and high-fidelity measurement is possible by using proximal quantum dot charge sensors, their operating range is limited and prone to electrical disturbances. Here we demonstrate realtime operation of a charge sensor in a feedback loop to maintain its sensitivity suitable for fast charge sensing in a Si/SiGe double quantum dot. Disturbances to the charge sensitivity, due to variation of gate voltages for operating the quantum dot and $1/f$ charge fluctuation, are compensated by a digital PID controller with the bandwidth of $\approx 100\,{\rm kHz}$. The rapid automated tuning of a charge sensor enables unobstructed charge stability diagram measurement facilitating realtime quantum dot tuning and submicrosecond single-shot spin readout without compromising the performance of a charge sensor in time-consuming experiments for quantum information processing.

Magnetic field induced delocalization in hybrid electron-nuclear spin ensembles

We use field-cycling-assisted dynamic nuclear polarization and continuous radio-frequency (RF) driving over a broad spectral range to demonstrate magnetic-field-dependent activation of nuclear spin transport from strongly-hyperfine-coupled 13C sites in diamond. We interpret our observations with the help of a theoretical framework where nuclear spin interactions are mediated by electron spins. In particular, we build on the results from a 4-spin toy model to show how otherwise localized nuclear spins must thermalize as they are brought in contact with a larger ancilla spin network. Further, by probing the system response to a variable driving field amplitude, we witness stark changes in the RF-absorption spectrum, which we interpret as partly due to contributions from heterogeneous multi-spin sets, whose 'zero-quantum' transitions become RF active thanks to the hybrid electron-nuclear nature of the system. These findings could prove relevant in applications to dynamic nuclear polarization, spin-based quantum information processing, and nanoscale sensing.

Designed polynuclear lanthanide complexes for quantum information processing.

The design of dissymmetric organic ligands featuring combinations of 1,3-diketone and 2,6-diacetylpyridine coordination pockets has been exploited to produce dinuclear and trinuclear lanthanide-based coordination compounds. These molecules exhibit two or more non-equivalent Ln ions, most remarkably enabling the access to well-defined heterolanthanide compositions. The site-selective disposition of each metal ion within the molecular entities allows the study of each centre individually as a spin-based quantum bit, affording unparalleled versatility for quantum gate design. The inherent weak interaction between the Ln ions permits the performance of multi-qubit quantum logical operations realized through their derived magnetic states, or implementing quantum-error correction protocols. The different studies performed to date on these systems are revised, showing their vast potential within spin-based quantum information processing.

Robust energy-selective tunneling readout of singlet-triplet qubits under large magnetic field gradient

Fast and high-fidelity quantum state detection is essential for building robust spin-based quantum information processing platforms in semiconductors. The Pauli spin blockade (PSB)-based spin-to-charge conversion and its variants are widely used for the spin state discrimination of two-electron singlet–triplet (ST0) qubits; however, the single-shot measurement fidelity is limited by either the low signal contrast, or the short lifetime of the triplet state at the PSB energy detuning, especially due to strong mixing with singlet states at large magnetic field gradients. Ultimately, the limited single-shot measurement fidelity leads to low visibility of quantum operations. Here, we demonstrate an alternative method to achieve spin-to-charge conversion of ST0 qubit states using energy-selective tunneling between doubly occupied quantum dots (QDs) and electron reservoirs. We demonstrate a single-shot measurement fidelity of 90% and an S–T0 oscillation visibility of 81% at a field gradient of 100 mT (~500 MHz h (g*·μB)−1); this allows single-shot readout with full electron charge signal contrast and, at the same time, long and tunable measurement time with negligible effect of relaxation even at strong magnetic field gradients. Using an rf-sensor positioned opposite to the QD array, we apply this method to two ST0 qubits and show high-visibility readout of two individual single-qubit gate operations is possible with a single rf single-electron transistor sensor. We expect our measurement scheme for two-electron spin states can be applied to various hosting materials and provides a simplified and complementary route for multiple qubit state detection with high accuracy in QD-based quantum computing platforms.

Spin-controlled generation of indistinguishable and distinguishable photons from silicon vacancy centres in silicon carbide

Quantum systems combining indistinguishable photon generation and spin-based quantum information processing are essential for remote quantum applications and networking. However, identification of suitable systems in scalable platforms remains a challenge. Here, we investigate the silicon vacancy centre in silicon carbide and demonstrate controlled emission of indistinguishable and distinguishable photons via coherent spin manipulation. Using strong off-resonant excitation and collecting zero-phonon line photons, we show a two-photon interference contrast close to 90% in Hong-Ou-Mandel type experiments. Further, we exploit the system’s intimate spin-photon relation to spin-control the colour and indistinguishability of consecutively emitted photons. Our results provide a deep insight into the system’s spin-phonon-photon physics and underline the potential of the industrially compatible silicon carbide platform for measurement-based entanglement distribution and photonic cluster state generation. Additional coupling to quantum registers based on individual nuclear spins would further allow for high-level network-relevant quantum information processing, such as error correction and entanglement purification.

Single-electron pumping in a ZnO single-nanobelt quantum dot transistor

Diluted magnetic semiconductors (DMSs) have traditionally been employed to implement spin-based quantum computing and quantum information processing. However, their low Curie temperature is a major hurdle in their use in this field, which creates the necessity for wide bandgap DMSs operating at room temperature. In view of this, a single-electron transistor (SET) with a global back-gate was built using a wide bandgap ZnO nanobelt (NB). Clear Coulomb oscillations were observed at 4.2 K. The periodicity of the Coulomb diamonds indicates that the Coulomb oscillations arise from single quantum dots of uniform size, whereas quasi-periodic Coulomb diamonds correspond to the contribution of multi-dots present in the ZnO NB. By applying an AC signal to the global back-gate across a Coulomb peak with varying frequencies, single-electron pumping was observed; the increase in current was equal to the production of electron charge and frequency. The current accuracy of about 1% for both single- and double-electron pumping was achieved at a high frequency of 25 MHz. This accurate single-electron pumping makes the ZnO NB SET suitable for single-spin injection and detection, which has great potential for applications in quantum information technology.

Resonant microwave-mediated interactions between distant electron spins

Nonlocal qubit interactions are a hallmark of advanced quantum information technologies1-5. The ability to transfer quantum states and generate entanglement over distances much larger than qubit length scales greatly increases connectivity and is an important step towards maximal parallelism and the implementation of two-qubit gates on arbitrary pairs of qubits6. Qubit-coupling schemes based on cavity quantum electrodynamics2,7,8 also offer the possibility of using high-quality-factor resonators as quantum memories3,9. Extending qubit interactions beyond the nearest neighbour is particularly beneficial for spin-based quantum computing architectures, which are limited by short-range exchange interactions10. Despite the rapidly maturing device technology for silicon spin qubits11-16, experimental progress towards achieving long-range spin-spin coupling has so far been restricted to interactions between individual spins and microwave photons17-20. Here we demonstrate resonant microwave-mediated coupling between two electron spins that are physically separated by more than four millimetres. An enhanced vacuum Rabi splitting is observed when both spins are tuned into resonance with the cavity, indicating a coherent interaction between the two spins and a cavity photon. Our results imply that microwave-frequency photons may be used to generate long-range two-qubit gates between spatially separated spins.

Electrically controlled nuclear polarization of individual atoms.

Nuclear spins serve as sensitive probes in chemistry1 and materials science2 and are promising candidates for quantum information processing3-6. NMR, the resonant control of nuclear spins, is a powerful tool for probing local magnetic environments in condensed matter systems, which range from magnetic ordering in high-temperature superconductors7,8 and spin liquids9 to quantum magnetism in nanomagnets10,11. Increasing the sensitivity of NMR to the single-atom scale is challenging as it requires a strong polarization of nuclear spins, well in excess of the low polarizations obtained at thermal equilibrium, as well as driving and detecting them individually4,5,12. Strong nuclear spin polarization, known as hyperpolarization, can be achieved through hyperfine coupling with electron spins2. The fundamental mechanism is the conservation of angular momentum: an electron spin flips and a nuclear spin flops. The nuclear hyperpolarization enables applications such as in vivo magnetic resonance imaging using nanoparticles13, and is harnessed for spin-based quantum information processing in quantum dots14 and doped silicon15-17. Here we polarize the nuclear spins of individual copper atoms on a surface using a spin-polarized current in a scanning tunnelling microscope. By employing the electron-nuclear flip-flop hyperfine interaction, the spin angular momentum is transferred from tunnelling electrons to the nucleus of individual Cu atoms. The direction and magnitude of the nuclear polarization is controlled by the direction and amplitude of the current. The nuclear polarization permits the detection of the NMR of individual Cu atoms, which is used to sense the local magnetic environment of the Cu electron spin.

Enhanced quantum coherence in exchange coupled spins via singlet-triplet transitions.

Manipulation of spin states at the single-atom scale underlies spin-based quantum information processing and spintronic devices. These applications require protection of the spin states against quantum decoherence due to interactions with the environment. While a single spin is easily disrupted, a coupled-spin system can resist decoherence by using a subspace of states that is immune to magnetic field fluctuations. Here, we engineered the magnetic interactions between the electron spins of two spin-1/2 atoms to create a "clock transition" and thus enhance their spin coherence. To construct and electrically access the desired spin structures, we use atom manipulation combined with electron spin resonance (ESR) in a scanning tunneling microscope. We show that a two-level system composed of a singlet state and a triplet state is insensitive to local and global magnetic field noise, resulting in much longer spin coherence times compared with individual atoms. Moreover, the spin decoherence resulting from the interaction with tunneling electrons is markedly reduced by a homodyne readout of ESR. These results demonstrate that atomically precise spin structures can be designed and assembled to yield enhanced quantum coherence.

Measurement of the Overhauser field in a two-dimensional electron system at weak magnetic fields

Optically induced polarization of electron spins has been able to generate nuclear polarization via dynamic nuclear polarization (DNP), and control of this nuclear spin polarization has extensive application potentiality in spin-based quantum information processing and quantum computation. Here, we report optically induced DNP measurements in a two-dimensional electron gas embedded in a GaAs/AlGaAs heterostructure. We are able to obtain the Overhauser field Bn and show that it is proportional to the external magnetic field Bext when the latter is weak. We also show that the proportionality coefficient k between Bn and Bext can be manipulated by varying the intensity and helicity of the pump light.

A silicon metal-oxide-semiconductor electron spin-orbit qubit

The silicon metal-oxide-semiconductor (MOS) material system is a technologically important implementation of spin-based quantum information processing. However, the MOS interface is imperfect leading to concerns about 1/f trap noise and variability in the electron g-factor due to spin–orbit (SO) effects. Here we advantageously use interface–SO coupling for a critical control axis in a double-quantum-dot singlet–triplet qubit. The magnetic field-orientation dependence of the g-factors is consistent with Rashba and Dresselhaus interface–SO contributions. The resulting all-electrical, two-axis control is also used to probe the MOS interface noise. The measured inhomogeneous dephasing time, T_{{mathrm{2m}}}^ star, of 1.6 μs is consistent with 99.95% 28Si enrichment. Furthermore, when tuned to be sensitive to exchange fluctuations, a quasi-static charge noise detuning variance of 2 μeV is observed, competitive with low-noise reports in other semiconductor qubits. This work, therefore, demonstrates that the MOS interface inherently provides properties for two-axis qubit control, while not increasing noise relative to other material choices.