The Great Proterozoic Accretionary Orogeny along the southern and southeastern margin of Laurentia is arguably the first long-lived, modern-style active plate margin on Earth, representing significant crustal growth and reworking. Here, we present new detrital zircon U–Pb and Hf data, along with zircon and monazite metamorphic ages, from tectonic domains in the southwestern Grenville Province that represent depositional basins formed and reworked during a series of events between 2.2 and 1.2 Ga. As such, the data allow a glimpse into the evolution and assembly of this extensive margin. The Nepewassi domain contains Archean basement overlain by mature sandstone characterized by near-unimodal, ca. 2.7–2.6 Ga detrital zircon peaks and likely correlative with Superior Province basement and its Huronian cover. The Nepewassi domain underwent both Archean (ca. 2.65 Ga) and Killarnean (ca. 1.76 Ga) metamorphism. In addition, all units preserve evidence of Grenvillian high-grade metamorphism between ca. 1.05 and 0.99 Ga. The structurally highest parts of the Nepewassi domain also contain younger sedimentary rocks that received detritus from Killarnean sources, with evolved Hf isotopic compositions indicative of reworked Archean crust. Sedimentary rocks in the Tomiko domain preserve detrital zircon of Penokean and Killarnean age (1.9–1.7 Ga) with evolved Hf compositions, along with Labradorian (1.7–1.6 Ga) grains of more juvenile composition. Detrital zircon from the Kiosk domain yield Penokean through Labradorian ages, with Hf compositions ranging from evolved to juvenile. In contrast to the sedimentary rocks found in these Laurentia-derived parautochthonous domains, similar rocks from younger, more allochthonous units, including the Shawanaga and basal Parry Sound domain, dominantly contain zircon ranging from Pinwarian (ca. 1.45 Ga) through ca. 1.20 Ga that show exclusively juvenile isotopic compositions. The data show that sedimentary basins received detritus from nearby active sources as well as from the nearby Superior continent, and that successively younger sources and basins became increasingly less influenced by continental input as the margin grew wider. The data add to a growing database of similar data from other parts of this several thousand-kilometer-long margin that seemingly displayed little along-strike variation in overall evolution, implying the existence of a vast, Pacific-scale ocean.
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