Bistable laminates have potential applications in areas such as buffer and soft robotics due to their two stable states and ability to deform through both snap-through and snap-back processes. However, conventional orthotropic bistable laminates with two stable state configurations and snap loads are similar in magnitude. There is a problem that the deformation cannot be easily driven when the laminate stiffness is high. To solve this problem, a clever design is needed to reduce the snap-back load and increase the snap-through load so that the driven deformation can be realized more easily. In this paper, we propose a design method to suppress and control the deformation of bistable laminates by utilizing the shape memory of 3D-printed shape memory polymers (SMP), which enables the laminates to increase the stiffness while reducing the driving force. First, a numerical model of viscoelasticity of the laminate is established to study its deformation characteristics, and the numerical results are compared with experimental results with good agreement. The effect of SMPs on the snap load and principal curvature of bistable laminates is also investigated. Finally, the interlayer interface bonding of the bistable laminates is examined in microscopic perspective. The results demonstrate that 3D printed SMPs can effectively enhance the snap-through load and reduce the snap-back load of bistable laminates, achieving deformation suppression and control while maintaining good interlaminar bonding with carbon fiber composites. This study provides new insights and practical significance for the deformation suppression and active control of bistable structures.