Small Optical Nonlinearity Research Articles

Ultrashort low-loss \u03a8 gates for linear optical logic on Si photonics platform

Nonlinear optical gates are usually considered as fundamental building blocks for universal optical computation. However, the performance is severely limited by small optical nonlinearity, thereby bounding their operation speed, consumption energy, and device size. In this paper, we propose and experimentally demonstrate linear optical logic operations with ~3 μm-long Si wire “Ψ” gates consist of 3 × 1 optical combiners including auxiliary bias port, which maximizes the binary contrast of the output in telecom wavelength. We have demonstrated 20 Gbps Boolean “AND” operation with experimentally measured small signal loss (1.6 dB experimentally). A single Ψ gate can perform representative Boolean operations by changing the bias power and relative phases. We have also demonstrated wavelength-independent operation by seven wavelengths, which leads to wavelength-division multiplexed parallel computation. This ultrashort, highly-integrable, low-loss, and energy-efficient optical logic gates pave the way for ultralow latency optical pattern matching, recognition, and conversion.

Ultrafast and energy-efficient all-optical switching with graphene-loaded deep-subwavelength plasmonic waveguides

All-optical switches have attracted attention because they can potentially overcome the speed limitation of electric switches. However, ultrafast, energy-efficient all-optical switches have been challenging to realize due to the intrinsically small optical nonlinearity in existing materials. As a solution, we propose graphene-loaded deep-subwavelength plasmonic waveguides (30 nm x 20 nm). Thanks to extreme light confinement, we have significantly enhanced optical nonlinear absorption in graphene, and achieved ultrafast all-optical switching with a switching energy of 35 fJ and a switching time of 260 fs. The switching energy is four orders of magnitudes smaller than that in previous graphene-based devices and is the smallest value ever reported for any all-optical switch operating at a few picoseconds or less. This device can be efficiently connected to conventional Si waveguides and employed in Si photonic integrated circuits. We believe that this graphene-based device will pave the way towards on-chip ultrafast and energy-efficient photonic processing.

Nonreciprocal photon blockade in a two-mode cavity with a second-order nonlinearity

It is shown that the Fizeau drag can be used to cause nonreciprocity. We propose the use of a nanostructured toroid cavity made of $\chi^{(2)}$ nonlinear materials to achieve nonreciprocal photon blockade (PB) through the Fizeau drag. Under the weak driving condition, we discuss the origins of the PB based on the doubly resonant modes with good spatial overlap at the fundamental and second-harmonic frequencies. We also find that for the fundamental mode, the PB happens when we drive the system from one side but the photon-induced tunneling happens when we drive the system from the other side. However, there is no such phenomenon in the second-harmonic mode. Remarkably, the PB phenomenon occurs with a reasonably small optical nonlinearity thus bringing the system parameters closer to the reasonably achievable realm by the current technology.

Parametric Amplification of a Superconducting Plasma Wave.

Many applications in photonics require all-optical manipulation of plasma waves1, which can concentrate electromagnetic energy on sub-wavelength length scales. This is difficult in metallic plasmas because of their small optical nonlinearities. Some layered superconductors support Josephson plasma waves (JPWs)2,3, involving oscillatory tunneling of the superfluid between capacitively coupled planes. Josephson plasma waves are also highly nonlinear4, and exhibit striking phenomena like cooperative emission of coherent terahertz radiation5,6, superconductor-metal oscillations7 and soliton formation8. We show here that terahertz JPWs can be parametrically amplified through the cubic tunneling nonlinearity in a cuprate superconductor. Parametric amplification is sensitive to the relative phase between pump and seed waves and may be optimized to achieve squeezing of the order parameter phase fluctuations9 or single terahertz-photon devices.

An organic dye with very large Stokes-shift and broad tunability of fluorescence: Potential two-photon probe for bioimaging and ultra-sensitive solid-state gas sensor

Light-emitting nonlinear optical molecules, especially those with large Stokes shifts and broad tunability of their emission wavelength, have attracted considerable attention for various applications including biomedical imaging and fluorescent sensors. However, most fluorescent chromophores have only limited potential for such applications due to small Stokes shifts, narrow tunability of fluorescence emissions, and small optical nonlinearity in highly polar solvents. In this work, we demonstrate that a two-photon absorbing stilbene chromophore exhibits a large two-photon absorption action cross-section (ηδ = 320 GM) in dimethylsulfoxide (DMSO) and shows broad fluorescence tunability (125 nm) by manipulating the polarity of the surrounding medium. Importantly, a very large Stokes shift of up to 227 nm is achieved in DMSO. Thanks to these features, this chromophore can be utilized as a two-photon probe for bioimaging applications and in an ultrasensitive solid-state gas detector.

Nonlinear optical grating diffraction in dye-doped blue-phase liquid crystals

Low-power cw lasers are employed to study grating formation in blue-phase liquid crystals. We observed that undoped samples exhibit vanishingly small optical nonlinearities whereas methyl-red-dye doped samples produce strong nonlinear self-diffraction effects. The nonlinearities are attributed to director axis reorientation, disorder, and lattice distortion by the laser-excited dye molecules. The magnitude of the observed intensity-dependent index coefficient is in the range of 10(-4)-10(-3) cm2/Watt.

Coherent control of quantum-well excitons in a resonant semiconductor microcavity for high-speed all-optical switching

Coherent control of excitons in quantum wells embedded in a resonant planar semiconductor microcavity versus in quantum wells without the cavity at high repetition rates is investigated theoretically to determine the practical constraints for application in high bit-rate optical switching. It is shown that /spl pi/-shifted pulse pairs are optimal to coherently populate and depopulate the QW on the 100-fs timescale. For the cavity-free case, the small optical nonlinearity will require devices incorporating /spl sim/100 quantum wells; the resonant enhancement of the confined mode for the case of the cavity leads to an effective increase in the optical nonlinearity and thus a reduction of the required number of quantum wells to /spl sim/10. In addition, switch architectures that avoid interferometers, and thus will have superior temperature and mechanical stability, based on the microcavity are proposed. We believe that although room-temperature operation of a 100-Gb/s switch based on this principle may be difficult, operation at liquid-nitrogen temperature should be feasible.