Single-scattering Properties Of Particles Research Articles

Effect of host medium absorption on polarized radiative transfer in dispersed media

This paper focuses on polarized radiative transfer in a thin layer composed of titanium dioxide particles while considering the effect of host medium absorption on particle scattering. The single-scattering properties of particles in an absorbing medium are calculated using the modified Lorenz-Mie program recently developed based on the first-principles theory of electromagnetic scattering, and the vector radiative transfer equation is solved by using the spectral element method. The relative errors of Stokes parameters caused by using the conventional Lorenz-Mie theory are systemically investigated. The results show that neglecting the effect of host medium absorption on particle scattering has a more significant impact on the radiation intensity than the polarization components in most cases. Meanwhile, the relative errors of Stokes parameters induced by using the conventional Lorenz-Mie theory obviously increase with the increase of the host medium absorption index and particle size parameter. Due to the larger scattering coefficients and scattering albedos (i.e., for the case of particle size parameter x=10.0 in this study), the relative errors of Stokes parameters of monodisperse particles are obviously larger than those of polydisperse particles. Moreover, it is found that the relative errors of the Stokes parameters change nonlinearly with the particle volume fraction, especially for large size particles.

Multiple scattering of polarized light by particles in an absorbing medium.

We study multiple scattering of light by particles embedded in an absorbing host medium using a recently developed single-scattering and vector radiative-transfer methodology directly based on the Maxwell equations. The first-principles results are compared with those rendered by the conventional heuristic approach according to which the single-scattering properties of particles can be computed by assuming that the host medium is nonabsorbing. Our analysis shows that the conventional approach yields very accurate results in the case of aerosol and cloud particles suspended in an absorbing gaseous atmosphere. In the case of air bubbles in water, the traditional approach can cause large relative errors in reflectance, but only when strong absorption in the host medium makes the resulting reflectance very small. The corresponding polarization errors are substantially smaller.

Scattering and absorption of light by ice particles: Solution by a new physical-geometric optics hybrid method

A new physical-geometric optics hybrid (PGOH) method is developed to compute the scattering and absorption properties of ice particles. This method is suitable for studying the optical properties of ice particles with arbitrary orientations, complex refractive indices (i.e., particles with significant absorption), and size parameters (proportional to the ratio of particle size to incident wavelength) larger than ∼20, and includes consideration of the edge effects necessary for accurate determination of the extinction and absorption efficiencies. Light beams with polygon-shaped cross sections propagate within a particle and are traced by using a beam-splitting technique. The electric field associated with a beam is calculated using a beam-tracing process in which the amplitude and phase variations over the wavefront of the localized wave associated with the beam are considered analytically. The geometric-optics near field for each ray is obtained, and the single-scattering properties of particles are calculated from electromagnetic integral equations. The present method does not assume additional physical simplifications and approximations, except for geometric optics principles, and may be regarded as a “benchmark” within the framework of the geometric optics approach. The computational time is on the order of seconds for a single-orientation simulation and is essentially independent of the size parameter. The single-scattering properties of oriented hexagonal ice particles (ice plates and hexagons) are presented. The numerical results are compared with those computed from the discrete-dipole-approximation (DDA) method.