When assessing text, supervised natural language processing (NLP) models have traditionally been used to measure targeted constructs in the organizational sciences. However, these models require significant resources to develop. Emerging “off-the-shelf” large language models (LLM) offer a way to evaluate organizational constructs without building customized models. However, it is unclear whether off-the-shelf LLMs accurately score organizational constructs and what evidence is necessary to infer validity. In this study, we compared the validity of supervised NLP models to off-the-shelf LLM models (ChatGPT-3.5 and ChatGPT-4). Across six organizational datasets and thousands of comments, we found that supervised NLP produced scores were more reliable than human coders. However, and even though not specifically developed for this purpose, we found that off-the-shelf LLMs produce similar psychometric properties as supervised models, though with slightly less favorable psychometric properties. We connect these findings to broader validation considerations and present a decision chart to guide researchers and practitioners on how they can use off-the-shelf LLM models to score targeted constructs, including guidance on how psychometric evidence can be “transported” to new contexts.