Sapphire Chirped Pulse Amplification Laser Research Articles

Investigation and suppression of pre-pulses on nanosecond time scale in the SULF-1PW laser.

It is of crucial significance to investigate and suppress pre-pulses on nanosecond time scale because the intense pre-plasma generated by them may have enough time to expand and, thus, cause fatal impact on laser-matter interactions. In this research, we analyze the potential origins of pre-pulses on nanosecond time scale in a typical Ti:sapphire chirped pulse amplification laser system. Based on the analysis, the initial status of these generated pre-pulses in the SULF-1PW laser is measured and investigated. Then different measures, including fine control on the time synchronization and the replacement for the Ti:sapphire, are adopted in the SULF-1PW laser to suppress these pre-pulses with respective origins, which can promote the energy ratio between the main pulse and these pre-pulses by 2-3 orders of magnitude. This research not only improves the temporal contrast of the SULF-1PW laser on nanosecond time scale but also provides beneficial guidance for the design and construction of similar laser facilities.

Reducing temporal pedestal in a Ti:sapphire chirped-pulse amplification system by using a stretcher based on two concave mirrors.

We demonstrate the temporal pedestal suppression in a Ti:sapphire chirped-pulse amplification laser system. The far-field spectral phase noise can be avoided by using a stretcher based on two concave mirrors in the system, reducing the intensity and the time range of the amplified pulse's pedestal. At the amplified energy of 1.7 J, the contrast measurement showed that the pedestal intensity was at a level of about 10-10 within a 10 ps time window near the main pulse. In the proton acceleration experiment, a 10 nm thickness CH target was irradiated by the high-contrast pulse with the focused intensity of ∼1.4×1020W/cm2, which generated a proton beam with a cutoff energy of 16 MeV.

Petawatt Femtosecond Laser Pulses from Titanium-Doped Sapphire Crystal

Ultra-high intensity femtosecond lasers have now become excellent scientific tools for the study of extreme material states in small-scale laboratory settings. The invention of chirped-pulse amplification (CPA) combined with titanium-doped sapphire (Ti:sapphire) crystals have enabled realization of such lasers. The pursuit of ultra-high intensity science and applications is driving worldwide development of new capabilities. A petawatt (PW = 1015 W), femtosecond (fs = 10−15 s), repetitive (0.1 Hz), high beam quality J-KAREN-P (Japan Kansai Advanced Relativistic ENgineering Petawatt) Ti:sapphire CPA laser has been recently constructed and used for accelerating charged particles (ions and electrons) and generating coherent and incoherent ultra-short-pulse, high-energy photon (X-ray) radiation. Ultra-high intensities of 1022 W/cm2 with high temporal contrast of 10−12 and a minimal number of pre-pulses on target has been demonstrated with the J-KAREN-P laser. Here, worldwide ultra-high intensity laser development is summarized, the output performance and spatiotemporal quality improvement of the J-KAREN-P laser are described, and some experimental results are briefly introduced.

On the effect of third-order dispersion on phase-matched terahertz generation via interfering chirped pulses

High-energy narrowband terahertz (THz) pulses, relevant for a plethora of applications, can be created from the interference of two chirped-pulse drive lasers. The presence of third order dispersion, an intrinsic feature of many high-energy drive lasers, however, can significantly reduce the optical-to-THz conversion efficiency and have other undesired effects. Here, we present a detailed description of the effect of third-order dispersion (TOD) in the pump pulse on the generation of THz radiation via phase-matching of broadband highly chirped pulse trains. Although the analysis is general, we focus specifically on parameters typical to a Ti:Sapphire chirped-pulse amplification laser system for quasi-phase-matching in periodically-poled lithium niobate (PPLN) in the range of THz frequencies around 0.5 THz. Our analysis provides the tools to optimize the THz generation process for applications requiring high energy and to control it to produce desired THz waveforms in a variety of scenarios.

High-Power Ultrashort Pulse Lasers to Pump Plasma-Based Soft X-Ray Lasers

High-energy ultrashort pulse optical lasers operating at high repetition rate are required to drive intense compact coherent soft X-ray sources, including soft X-ray lasers, for applications in nanoscience and nanotechnology, material studies, and high field science. This paper reviews two types of high-power solid-state laser systems developed at Colorado State University to pump compact, high repetition rate, and plasma-based soft X-ray lasers. One is a flashlamp-pumped, petawatt-class Ti:sapphire chirped-pulse amplification laser that generates 0.85 PW pulses of 30 fs duration at 3.3 Hz repetition rate. Using a fraction of the output energy from this laser, we have demonstrated gain-saturated, compact, repetitive lasers down to 6.85 nm in Ni-like Gd and have observed gain in shorter wavelength transitions, down to 5.85 nm in Ni-like Dy. The second type of pump laser is an all diode-pumped chirped-pulse amplification system based on cryogenically cooled Yb:YAG active mirror amplifiers that produces 1 J pulses of picosecond duration at 500 Hz repetition rate. These compact diode-pumped laser systems have enabled new advances in high-average-power tabletop soft X-ray lasers that include 100 Hz demonstrations at wavelengths ranging from 10.9 to 18.9 nm, as well long duration operation at these high repetition rates for periods up to one hour. These and other recent results that include the operation of an 18.9 nm laser Ni-like Mo laser at 400 Hz repetition rate open a path to compact kilohertz repetition rate soft X-ray lasers.

Improvement of the focusing ability by double deformable mirrors for 10-PW-level Ti: sapphire chirped pulse amplification laser system.

Double deformable mirrors (DMs) with different actuator densities are cascaded to optimize the wavefront aberrations to improve the focus intensity of the Shanghai super-intense ultrafast laser facility (SULF), which plans to generate 10 PW laser pulse. The beam aberrations near the focal spot are corrected from 0.556 um to 0.112 um in RMS by a 300-mm DM with a large stroke installed after the compressor. After then, it is further optimized to 0.041 um using a 130-mm DM with a high spatial resolution working after the main amplifier. The corrected beam is focused to 2.75 × 2.87 um2 at the full width at half maximum (FWHM) with an f/2.5 off-axis parabolic mirror (OAP), which contains approximately 27.69% energy. A peak intensity of 2 × 1022 W/cm2 is achieved at the output of 5.4 PW, and it could exceed 1023 W/cm2 in the SULF 10 PW laser facility using an f/1.8 OAP.

High-Contrast, High-Intensity Petawatt-Class Laser and Applications

A high-contrast high-intensity petawatt-class Ti:sapphire chirped-pulse amplification laser has been developed for research on high field science. A saturable absorber and a low-gain optical parametric chirped-pulse amplification preamplifier in the front-end have improved the temporal contrast in the system to ∼ <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"><tex-math>$2 \times 10^{12}$</tex-math></inline-formula> on the subnanosecond time scale at the ∼70 TW power level. In addition to the high-contrast broadband high-energy output from the final amplifier has been achieved with a flat-top spatial profile with a filling factor of ∼70%. This is the result of pump beam spatial profile homogenization with diffractive optical elements. The system produces the uncompressed output pulse energy of 29 J, indicating the capability for reaching a peak power of ∼600 TW. We discuss in detail the design, performance, and characterization of the laser including output power, pulse duration, and spatiotemporal beam quality. We also describe the on-going upgrade of the laser system and some applications for the laser in relativistic dominated laser–matter interactions.

Enhancement of Amplified Spontaneous Emission Contrast With a Novel Front-End Based on NOPA and SHG Processes

Employing a novel front-end based on femtosecond noncollinear optical-parametric amplification and second-harmonic generation processes in a Ti:sapphire chirped pulse amplification laser system, we first demonstrate the efficient enhancement of amplified spontaneous emission (ASE) contrast. Cleaned seed pulses of 100-μJ energy generated by the front-end are amplified to 0.75 J before compressor. After compression and under pulse peak power of 7 TW, the ASE contrast is promoted from original ~ 108 to ~ 1011. The experimental results for nanometer film target interactions also demonstrate the improvement of the contrast. Finally, the evolution of the ASE contrast under different seed pulse energy is demonstrated experimentally, which can be used to design the higher power laser with higher ASE contrast.

Experimental research and application of pulse clean technique based on cross polarized wave generation

Cross polarized wave (XPW) generation technique is used to improve the contrast of the output pulses from a 800 nm Ti: sapphire femtosecond (fs) laser. The measured temporal contrast of the cleaned pulse is 1011 (limited by the dynamic range of the third-order auto-correlator), which is 3 orders of magnitude higher than the temporal contrast ratio of the initial pulse. The efficiency of XPW is 22%. And the bandwidth of the cleaned pulse is broadened after the XPW nonlinear process. Through the dispersion compensation using double chirped mirrors and fused silica plate, the 25 fs pulse duration is achieved. With the cleaned pulse used as the seed of a TW-level Ti: sapphire chirped-pulse amplification laser system, the 250 mJ/50 fs pulses corresponding to 5 TW peak power are obtained. And the 1011 temporal contrast is demonstrated on the time scale of hundreds of picoseconds before the main femtosecond pulse.

Efficient Spherical Wavefront Correction near the Focus for the 0.89 PW/29.0 fs Ti:Sapphire Laser Beam

We demonstrate a new loop system of the spherical wavefront (SW) correction near the beam focus to effectively improve the focusability of 0.89 PW/29.0 fs Ti:sapphire chirped pulse amplification laser. After wavefront correction, the Strehl ratio is improved to reach 0.91, and the focal spot size using the f/4 off-axis parabola is reduced to 6.34 × 6.94 μm2 (corresponding to 1.63 × 1.78 times diffraction limitation). With full peak power of 0.89 PW, the peak intensity of 2.59 × 1021 W/cm2 is obtained. The experimental results show that the SW correction scheme near the beam focus is comparatively simple, economic and high-efficient.

Contrast enhancement in a Ti:sapphire chirped-pulse amplification laser system with a noncollinear femtosecond optical-parametric amplifier

We experimentally demonstrated the contrast enhancement in a Ti:sapphire chirped-pulse amplification (CPA) laser with a noncollinear femtosecond optical-parametric amplifier. A total gain of 3.4 × 10(4) and pulse energy of 26 μJ were achieved. With the clean high-energy seeding pulse, the contrast ratio of the main amplified laser pulse to the amplified spontaneous emission in the Ti: sapphire CPA laser system was improved to around 10(10) within the time scale of hundreds of picoseconds.

High temporal and spatial quality petawatt-class Ti:sapphire chirped-pulse amplification laser system

Optical parametric chirped-pulse amplification (OPCPA) operation with low gain by seeding with high-energy, clean pulses is shown to significantly improve the contrast to better than 10(-10) to 10(-11) in a high-intensity Ti:sapphire laser system that is based on chirped-pulse amplification. In addition to the high-contrast broadband, high-energy output from the final amplifier is achieved with a flat-topped spatial profile of filling factor near 77%. This is the result of pump beam spatial profile homogenization with diffractive optical elements. Final pulse energies exceed 30 J, indicating capability for reaching peak powers in excess of 500 TW.

Amplified spontaneous emission contrast of CPA laser

The influence on the level of amplified spontaneous emission (ASE) contrast resulting from the different seed pulse energies has been experimentally studied in a 10-TW-level femtosecond Ti:sapphire chirped pulse amplification laser. It is found that, with the seed pulse energy increasing, the ASE pedestal is suppressed more efficiently, and the ASE contrast is improved with a saturable tendency. The measurement of ~2×10-8 ASE contrast in the range of more than 50 ps before the main pulse is achieved in the laser.

Prepulse-free, multi-terawatt, sub-30-fs laser system

We have built a prepulse-free, multi-terawatt, ultrashort pulse laser system, which combines both conventional laser amplification and optical parametric chirped pulse amplification (OPCPA) techniques. By employing an OPCPA system after the regenerative amplifier in a Ti:sapphire chirped pulse amplification laser chain, we have dramatically enhanced the prepulse contrast by 6 orders of magnitude. A prepulse contrast of better than 4.4 x 10-11 has been measured with a high energy broadband pulse of 24 mJ at 10 Hz repetition rate from the OPCPA system. Using a subsequent four-pass Ti:sapphire amplifier, we have achieved an amplified energy of 279 mJ and an ultrashort recompressed amplified pulse duration of 23.5 fs, corresponding to the peak powers for OPCPA and four-pass amplifier of 0.5 TW and 5.9 TW, respectively.

Contrast and phase characterization of a high-peak-power 20-fs laser pulse

We fully characterize a high-peak-power, ultrashort laser pulse in a Ti:sapphire chirped-pulse amplification laser system. The contrast, temporal, and spectral phases of the 20-fs pulse are determined by using high-dynamic-range cross-correlation and frequency-resolved optical gating techniques. Minimization of the total phase error can be achieved by balancing the phase terms of the group delay dispersion and quartic. The laser system is currently being applied to perform high-field atomic ionization experiments at 1020 W/cm2.

Short pulsed laser machining: How short is short enough?

Machined feature quality is examined, and the effects of laser pulse width (and thus peak power or intensity) are investigated for the following four laser systems: (1) a millisecond-class, free-running Nd:YAG; (2) a 100-nanosecond-class, Q-switched Nd:YAG laser; (3) a 100-picosecond-class, mode locked Nd:YAG laser; and (4) a 100-femtosecond-class, Ti:sapphire chirped pulse amplification laser. The effect of shorter laser wavelength is also examined by using the second harmonic wavelength of the Nd:YAG laser in the Q-switched and the mode locked pulse formats. Hole drilling and cutting of superalloy, ceramic, and composite materials are studied. The machined feature quality is improved as the pulse width becomes shorter and the peak intensity becomes higher. The shorter wavelength provides another significant improvement. Finally, an attempt is made to view these quality improvements in the context of process throughput and cost of ownership.

High-repetition rate 1-J green laser system

A laser-diode-pumped high-repetition-rate zigzag slab Nd:YAG oscillator-amplifier system is developed as the pumping source of a high-average-power and terawatt Ti:sapphire chirped pulse amplification laser system. This system can produce a greater than 2-J high-energy fundamental laser pulse at a repetition rate of 100 Hz. The frequency-doubled energy with a diffusion-bonded KTP crystal is 1 J at a repetition rate of 100 Hz.