Experimental control of quantum systems has been pursued widely since the invention of quantum mechanics. In the first part of the 20th century, atomic physics helped provide a test bed for quantum mechanics through studies of atoms’ internal energy differences and their interaction with radiation. The advent of spectrally pure, tunable radiation sources such as microwave oscillators and lasers dramatically improved these studies by enabling the coherent control of atoms’ internal states to deterministically prepare superposition states, as, for example, in the Ramsey method (Ramsey, 1990). More recently this control has been extended to the external (motional) states of atoms. Laser cooling and other refrigeration techniques have provided the initial states for a number of interesting studies, such as Bose-Einstein condensation. Similarly, control of the quantum states of artificial atoms in the context of condensed-matter systems is achieved in many laboratories throughout theworld. To give proper recognition to all of these works would be a daunting task; therefore, I will restrict these notes to experiments on quantum control of internal and external states of trapped atomic ions. The precise manipulation of any system requires lownoise controls and isolation of the system from its environment. Of course the controls can be regarded as part of the environment, so we mean that the system must be isolated from the uncontrolled or noisy parts of the environment. A simple example of quantum control comes from nuclear magnetic resonance, where the spins of a macroscopic ensemble of protons in the state j #i (spin antiparallel to an applied magnetic field) can be deterministically placed in a superposition state j #i þ j i (j j2 þ j j2 1⁄4 1) by application of a resonant rf field for a specified duration. Although the ensemble is macroscopic, in this example each spin is independent of the others and behaves as an individual quantum system. But already in 1935, Erwin Schrodinger (Schrodinger, 1935) realized that, in principle, quantum mechanics should apply to a macroscopic system in a more complex way, which could then lead to bizarre consequences. In his specific example, the system is composed of a single radioactive particle and a cat placed together with a mechanism such that if the particle decays, poison is released, which kills the cat. Quantum mechanically we represent the quantum states of the radioactive particle as undecayed 1⁄4 j i or decayed 1⁄4 j #i, and live and dead states of the cat as jLi and jDi. If the system is initialized in the state represented by the wave function j ijLi, then after a duration equal to the half life of the particle, quantum mechanics says the system evolves to a superposition state where the cat is alive and dead simultaneously, expressed by the superposition wave function