Resonant Photon Research Articles

An integrated sensor chip of resonant cavity light emitter and photon detector for wearable optical medicine

An integrated sensor chip of resonant cavity light emitter and photon detector for wearable optical medicine

Magnetic field-engineered optical nonlinearity in germanene nanotubes

Abstract The linear and nonlinear optical properties of germanene nanotubes (GeNTs) under the influence of magnetic fields are investigated through theoretical analysis. By employing a tight-binding model beyond the Dirac cone approximation, the electronic band structure, density of states, dipole matrix elements, and third-order nonlinear optical susceptibilities are calculated. The application of a magnetic field induces a Zeeman splitting of the energy levels, breaking the band degeneracy. Consequently, the dipole matrix elements exhibit a magnetic field dependence, altering the intensity and number of allowed transitions. In the infrared and ultraviolet energy regions, the linear optical absorption spectrum displays the splitting of peaks into dual neighboring peaks, with the splitting distance linearly dependent on the magnetic field strength. The third-order nonlinear optical susceptibilities, χTHG(3)3ω and χIDIR(3)ω, reveal the emergence of multiple resonance peaks in different energy regions due to two-photon and three-photon absorption processes. The magnetic field significantly influences the number, position, and height of these optical peaks, enabling effective control over the nonlinear optical response. By investigating the scaled energy (E/E_g) dependence, a universal behavior is observed for the three- and two photon resonance peaks, where their positions remain constant, but their peak intensities are significantly enhanced under the influence of the magnetic field. These findings demonstrate the potential of GeNTs as tunable nonlinear optical materials, with the magnetic field serving as an effective parameter for engineering their optical properties for various applications in optoelectronics, photonics, and related fields.

Gamma-ray irradiation-induced effects on Er3+-doped Li2O-Bi2O3-B2O3-TeO2 glass: Structural, Optical, Luminescence, and Radiation Shielding Properties

In the present study, we report the gamma (γ) ray irradiation-induced structural, optical, luminescence and radiation shielding properties of Er3+-doped Li2O-Bi2O3-B2O3-TeO2 glasses prepared by melt-quenching technique. It was evidence of the slight reductions in density and refractive index while maintaining stable optical properties upon the γ irradiation. Additionally, increased molar volume and polarizability indicated a less compact network. Raman spectroscopy shows broadened peaks and intensity reductions at key vibrational modes. The UV-Vis-NIR absorption spectra reveal the shift in the absorption edge and reduction in the intensities of Er³⁺ absorption bands (around 450, 520, 550, and 650 nm) with higher radiation doses, indicating radiation-induced damage. It was found that the band gap values decreased from 2.58 eV to 1.30 eV for un-irradiated glass to 90 kGy irradiated glass, and Urbach energy was found to increase from 0.18 to 1 eV respectively, indicating structural disorder and localized states within the band gap. PL emission spectra demonstrated intensity changes and peak shifts with γ radiation dose while maintaining a dominant green emission from 4S3/2 → 4I15/2 and 2H11/2 → 4I15/2 transitions, supported by the CIE diagram analysis. The NIR emission spectra also displayed a peak at 1530 nm with decreasing intensity, indicating defect-induced non-radiative recombination centres. Luminescence lifetime decay profiles indicated reduced lifetimes at higher γ doses, suggesting introduced non-radiative decay pathways. Furthermore, Phy-X software analysis highlighted effective γ-ray shielding influenced by chemical composition and photon flux, with MAC sharply decreasing to 1.8 cm2/g at 0.1 MeV and stabilizing, while LAC showed reduced attenuation efficiency at higher energies. HVL and TVL increased with energy, stabilizing around 4-5 cm and 15-16 cm, respectively, necessitating thicker materials for effective shielding at higher photon energies. MFP rapidly increased to 6-7 cm at 2 MeV, stabilizing at higher energies, while Zeff decreased sharply before stabilizing around 1 MeV. The EBF and EABF trends exhibited higher values at low energies, stabilizing at higher energies, indicating effective photon interaction and resonance effects.

Counterdiabatic Driving for Periodically Driven Systems.

Periodically driven systems have emerged as a useful technique to engineer the properties of quantum systems, and are in the process of being developed into a standard toolbox for quantum simulation. An outstanding challenge that leaves this toolbox incomplete is the manipulation of the states dressed by strong periodic drives. The state-of-the-art in Floquet control is the adiabatic change of parameters. Yet, this requires long protocols conflicting with the limited coherence times in experiments. To achieve fast control of nonequilibrium quantum matter, we generalize the notion of variational counterdiabatic driving away from equilibrium focusing on Floquet systems. We derive a nonperturbative variational principle to find local approximations to the adiabatic gauge potential for the effective Floquet Hamiltonian. It enables transitionless driving of Floquet eigenstates far away from the adiabatic regime. We discuss applications to two-level, Floquet band, and interacting periodically driven models. The developed technique allows us to capture nonperturbative photon resonances and obtain high-fidelity protocols that respect experimental limitations like the locality of the accessible control terms.

Readout error mitigated quantum state tomography tested on superconducting qubits

Quantum technologies rely heavily on accurate control and reliable readout of quantum systems. Current experiments are limited by numerous sources of noise that can only be partially captured by simple analytical models and additional characterization of the noise sources is required. We test the ability of readout error mitigation to correct noise found in systems composed of quantum two-level objects (qubits). To probe the limit of such methods, we designed a beyond-classical readout error mitigation protocol based on quantum state tomography (QST), which estimates the density matrix of a quantum system, and quantum detector tomography (QDT), which characterizes the measurement procedure. By treating readout error mitigation in the context of state tomography the method becomes largely readout mode-, architecture-, noise source-, and quantum state-independent. We implement this method on a superconducting qubit and evaluate the increase in reconstruction fidelity for QST. We characterize the performance of the method by varying important noise sources, such as suboptimal readout signal amplification, insufficient resonator photon population, off-resonant qubit drive, and effectively shortened T1 and T2 coherence. As a result, we identified noise sources for which readout error mitigation worked well, and observed decreases in readout infidelity by a factor of up to 30.

(Invited) Fundamentals of Plasmon-Induced Charge Transfer in Semiconducting Materials: Showcasing OER Catalysis

Using Localized Surface Plasmon Resonance Effect for Enhancing Electrochemical reactions has been reported earlier both in terms of direct electron injection/transfer (DET) in outer-sphere reductive processes as well as charge injection into semiconductors via plasmon-induced resonant electron transfer processes (PIRE). While the former (DET) is mainly influenced by the lifetimes of the ejected hot electrons and their rapid cooling at the interface. For inner sphere reductive processes via the LSPR phenomenon, direct charge injection into the LUMO states of the adsorbed species is required. In this regard, it is imperative to distinguish between the inter-band charge transfer of the adsorbed species because of exposure to photons.In contrast to these charge injections into semiconductors via plasmon-induced resonant electron transfer processes (PIRE), they must be more understood and complex. In this presentation, we will use the well-known endothermic anodic oxygen evolution reaction (OER) in alkaline pH to showcase the fundamental aspects of charge injection and its effect on the hole-driven OER mechanism. For this well-known OER catalyst, layered double hydroxides of Ni with Fe and Co dopants will be used. The electrochemical enhancement of OER will be explained based on detailed structural motifs of the semiconductors, its band structure, and the resonance effect of Au induced by the LSPR effect. Direct and indirect bandgaps will be discussed in the context of three possible mechanisms: (i) Charge carriers are directly injected into the semiconductor via LSPR. The semiconductor's conduction band is usually (-0.1 to 0.0 eV vs. NHE), and the valence band is between (2.00 and 3.5 eV), corresponding to electron energy between -2.00 to 3.5 eV vs. NHE. For LSPR nanoparticles, SPR energy is between 1.0 and 4.0 eV. Also, the Fermi energy of LSPR is usually 0.0 vs. NHE. Hence, LSPR only enables energetic electrons to be transferred from metals to semiconductors. It is the interface between LSPR and the semiconductor which is important. Charge injection is more prevalent when metal LSPR is of lower energy than the semiconductor—direct electron transfer (DET). (ii) Transfer does not involve direct electron injection but via (a) near-field electromagnetic and (b) resonant photon scattering mechanism. This has been shown to work by adding a thin dielectric material between the LSPR and the semiconductor. This would be most likely in the case of OER, where surface-localized plasmons will be the most important determinant instead of recombination events in the bulk of the semiconductor. This is most important for OER as it depends on the surface hole concentration. It should be noted that larger nanoparticles (>50 nm) have increased resonant photon scattering. Such a mechanism is more prevalent when we overlap metal LSPR and semiconductor bands, leading to plasmon-induced resonant electron transfer (PIRET). (iii) When metal LSPR is in direct contact with the semiconductor, all three phenomena could be active.

Efficient single-photon directional transfer between waveguides via two giant atoms

We investigate the single-photon transport properties in a double-waveguide quantum electrodynamic system. We force the energy degeneracy of the collective states by adjusting the direct coupling strength between the two giant atoms. Our results indicate that resonant photons can be completely transferred between the two waveguides owing to the scattering interference of eigenstates, which also results in the directional propagation of resonant photons in the output waveguide. Perfect transfer occurs when the two scattering states degenerate in the energy and decay rates. We further propose a simple scheme to realize the efficient photon transfer with directional control. This study has potential applications in quantum networks and integrated photonic circuits.

Temporal coupled-mode theory in nonlinear resonant photonics: From basic principles to contemporary systems with 2D materials, dispersion, loss, and gain

Temporal coupled-mode theory (CMT) is an acclaimed and widely used theoretical framework for modeling the continuous-wave response and temporal dynamics of any integrated or free-space photonic resonant structure. It was initially employed to understand how energy is coupled into and out of a cavity and how it is exchanged between different resonant modes. In the 30 years that followed its establishment, CMT has been expanded to describe a broad range of nonlinear interactions as well (self- and cross-phase modulation, saturable absorption, frequency generation, gain, etc.). In this Tutorial, we thoroughly present the basic principles and the evolution of CMT throughout the years, showcasing its immense capabilities for the analysis and design of linear and nonlinear resonant photonic systems. Importantly, we focus on the examples of modern, open nanophotonic resonators incorporating contemporary bulk or sheet (2D) materials that may be lossy and dispersive. For each linear/nonlinear effect under study, we follow a meticulous, step-by-step approach, starting from an accurate model of the physical phenomenon and proceeding to its introduction in the CMT framework all the way to the efficient solution of the resulting system of equations. Our work highlights the merits of CMT as an efficient, accurate, and versatile theoretical tool. We envision that it can serve both as an introductory reference for any reader and as a comprehensive handbook on how to incorporate a broad range of linear and nonlinear effects in the CMT framework.

Design and performance simulation of a silica microdisk cavity optical pressure sensor

The opto-mechanical system of optical whispering-gallery mode (WGM) microcavities confines resonant photons in micro-scale resonators for a long time, which can strongly enhance the interaction between light and matter, making it an ideal platform for various sensors. To measure the slim optical pressure in the interaction between the laser and matter, a silica microdisk cavity sensor with metal film is designed in this paper. In this study, the finite element method was employed to investigate the opto-mechanical coupling mechanism in a microdisk cavity. From the aspects of optics and mechanics, the structural parameters of the sensor were optimized and the performance was simulated. The simulation results show that at 1550 nm, the sensor’s optical quality factor (Q) can reach ∼104, the free spectral range is ∼5.3nm, the sensing sensitivity is 5.32mPa/Hz1/2, and the optical force resolution is 6.61×10−12N, which is better than the thin-film interferometry and optical lever method.

Resonant photoemission studies on Fe-Ni alloys

This paper investigates the electronic structure of Fe1−xNix (x = 0.32, 0.36, 0.4, 0.5) alloys employing high resolution photoelectron spectroscopy using synchrotron radiation. The valence bands and the core levels have been recorded at various on-resonance and off-resonance photon energies of Fe and Ni. An anti-resonance dip observed in the valence bands taken at Fe 3p → 3d resonance lies closer to the Fermi level compared to that observed at Ni 3p → 3d resonance, indicating larger density of itinerant Fe 3d electrons. Whereas, Ni 3d states are comparatively less itinerant in these alloys. The hybridization effects increase with increase of Fe content in the alloy system. The intensity of Ni L3M4,5M4,5 Coster-Cronig Auger transition observed with 853 eV (Ni 2p → 3d resonance) photon energy, drops down drastically for the Invar alloy (Fe0.64Ni0.36) as compared to other Fe-Ni alloys due to the existence of Ni in more than one local chemical surroundings as expected for Invar alloy. The electron-electron interaction energy (Udd) of Ni 3d shell is found to decrease with the decrease of Ni concentration. The 3p and 3s core levels of Fe and Ni recorded at 707 eV (Fe 2p → 3d resonance) are overwhelmed by various intense resonant Auger features such as Fe L3M2,3M2,3, Fe L3M2,3M4,5 and Fe L3M1M4,5. The 1S state of Fe L3M2,3M2,3 is greatly enhanced in the Invar alloy as compared to other alloys. The microscopic compositional in-homogeneity present in Invar alloy plays a crucial role in the screening of holes in Ni sites but does not contribute in screening the holes in Fe sites.

Ultrafast Resonant Photon Emission from a Molecule Driven by a Strong Coherent Field in Terms of Complex Spectral Analysis

In this study, we investigate the time–frequency-resolved resonant photon emission from a molecular vibrational oscillator driven by a monochromatic coherent external field. Using the complex spectral analysis of the Liouvillian, which integrates irreversible dissipative phenomena into quantum theory, we elucidate the fundamental processes of photon emission. Indeed, our analytical approach successfully decomposes the emission spectrum into two intrinsic contributions: one from a resonance eigenmode and another from continuous eigenmodes. These components are responsible for incoherent luminescence and coherent scattering photon emission processes, respectively. Our results show that while spontaneous emission dominates in the early stages of the emission process, coherent scattering gradually becomes more pronounced with time. Furthermore, destructive quantum interference between the two components plays a key role in determining the overall shape of the emission spectrum.

Controllable single-photon transport mediated by a time-modulated Jaynes–Cummings model

Controllable single-photon scattering in a one-dimensional waveguide coupled to a Jaynes–Cummings structure containing a time-modulated two-level atom interacting with a single-mode cavity is investigated. The photon transmission and reflection amplitudes are calculated by using an effective Floquet Hamiltonian in real space. The results show that the coupling between the atom and the cavity mode can dynamically be tuned via periodically modulating the atomic transition frequency. As a consequence, the scattering behaviors of the waveguide photons can be actively manipulated, and a controllable single-photon switch with high on-off ratio could be realized. More interestingly, the switch works well within a wide frequency region, i.e., the transmission of both resonant and off-resonant waveguide photons can be effectively switched on or off with appropriate system parameters. Furthermore, the proposed dynamically tunable switching scheme is robust against atomic dissipation associated with the help of atom-cavity coupling mismatch. Such single-photon device can be used as an elementary unit for various quantum information processing.

High-efficiency upconversion luminescence in UCNPs/CsPbBr3 nanocomposites enhanced by silver nanoparticles.

Upconversion nanocomposites with multiple light-emitting centers have attracted great attention as functional materials, but their low efficiency limits their further applications. Herein, a novel, to the best of our knowledge, system for nanocomposites consisting of upconversion nanoparticles (UCNPs) and perovskite quantum dots (PeQDs) assembled with Ag nanoparticles (NPs) is proposed. Upconversion luminescence (UCL) operation from PeQDs is triggered by near-infrared (NIR) sensitization through Förster resonance energy transfer (FRET) and photon reabsorption (PR). Especially, the photoluminescence (PL) emission efficiency is found to be significantly enhanced due to the increased energy transfer efficiency and radiative decay rate in the UCNPs/CsPbBr3 nanocomposites. The results offer new opportunities to improve the UCL properties of perovskites and open new development in the fields of LED lighting, solar cells, biomedicine, and so on.

Electrical manipulation of dissipation in microwave photon–magnon hybrid system through the spin Hall effect

Hybrid dynamic systems combine advantages from different subsystems for realizing information processing tasks in both classical and quantum domains. However, the lack of controlling knobs in tuning system parameters becomes a severe challenge in developing scalable, versatile hybrid systems for useful applications. Here, we report an on-chip microwave photon–magnon hybrid system where the dissipation rates and the coupling cooperativity can be electrically influenced by the spin Hall effect. Through magnon–photon coupling, the linewidths of the resonator photon mode and the hybridized magnon polariton modes are effectively changed by the spin injection into the magnetic wires from an applied direct current, which exhibit different trends in samples with low and high coupling strengths. Moreover, the linewidth modification by the spin Hall effect shows strong dependence on the detuning of the two subsystems, in contrast to the classical behavior of a standalone magnonic device. Our results point to a direction of realizing tunable, on-chip, scalable magnon-based hybrid dynamic systems, where spintronic effects provide useful control mechanisms.

Plasmon Resonance in a System of Bi Nanoparticles Embedded into (Al,Ga)As Matrix.

We reveal the feasibility of the localized surface plasmon resonance in a system of Bi nanoparticles embedded into an AlxGa1-xAs semiconductor matrix. With an ab initio determined dielectric function for bismuth and well-known dielectric properties of AlxGa1-xAs solid solution, we performed calculations of the optical extinction spectra for such metamaterial using Mie's theory. The calculations demonstrate a strong band of the optical extinction using the localized surface plasmons near a photon energy of 2.5 eV. For the semiconducting matrices with a high aluminum content x>0.7, the extinction by plasmonic nanoparticles plays the dominant role in the optical properties of the medium near the resonance photon energy.

Multiple-Photon Resonance Enabled Quantum Interference in Emission Spectroscopy of N2+

Quantum interference occurs frequently in the interaction of laser radiation with materials, leading to a series of fascinating effects such as lasing without inversion, electromagnetically induced transparency, Fano resonance, etc. Such quantum interference effects are mostly enabled by single-photon resonance with transitions in the matter, regardless of how many optical frequencies are involved. Here, we report on quantum interference driven by multiple photons in the emission spectroscopy of nitrogen ions that are resonantly pumped by ultrafast infrared laser pulses. In the spectral domain, Fano resonance is observed in the emission spectrum, where a laser-assisted dynamic Stark effect creates the continuum. In the time domain, the fast-evolving emission is measured, revealing the nature of free-induction decay arising from quantum radiation and molecular cooperativity. These findings clarify the mechanism of coherent emission of nitrogen ions pumped with mid-infrared pump laser and are found to be universal. The present work opens a route to explore the important role of quantum interference during the interaction of intense laser pulses with materials near multiple photon resonance.

Optical Microcavities Empowered Biochemical Sensing: Status and Prospects

Optical microcavities are compact structures that confine resonant photons in microscale dimensions for long periods of time, greatly enhancing light–matter interactions. Plentiful and profound physical mechanisms within these microcavities or functional microcavities have been extensively explored, including mode shift/splitting/broadening, lasing and gain enhancements, surface plasmon resonance, fluorescence resonance energy transferring, optical frequency comb spectroscopy, optomechanical interaction, and exceptional point. The versatility in design and the diverse range of materials, particularly composites involving metals and 2-dimensional materials, have paved a way for innovative approaches and improved performance in biochemical sensing applications. Leveraging the advantages ranging from miniaturization, high sensitivity, rapid response, and inherent stability, optical microcavity-based biochemical sensors have emerged to address the growing and increasingly complex demands of biochemical detection. This review commences with an exploration of fundamental mechanisms and structures and then delves into typical applications in recent advancements, covering the detection of biomacromolecules, cells, solid particles, liquid ions, and gas molecules. This review also culminates with a forward-looking perspective, highlighting future development trends and crucial research directions.

Terahertz Cavity Magnon Polaritons

AbstractHybrid light–matter coupled states, or polaritons, in magnetic materials have attracted significant attention due to their potential for enabling novel applications in spintronics and quantum information processing. However, most magnon‐polariton studies in the strong coupling regime to date have been carried out for ferromagnetic materials with magnon excitations at gigahertz frequencies. Here, strong resonant photon–magnon coupling at frequencies above 1 terahertz is investigated for the first time in a prototypical room‐temperature antiferromagnetic insulator, NiO, inside a Fabry–Pérot cavity. The cavity is formed by the crystal itself with a thickness adjusted to an optimal value. Terahertz time‐domain spectroscopy measurements in magnetic fields up to 25 T reveal the evolution of the magnon frequency through Fabry–Pérot cavity modes with photon–magnon anticrossing behavior, demonstrating clear vacuum Rabi splittings exceeding the polariton linewidths. These results show that NiO is a promising platform for exploring antiferromagnetic spintronics and cavity magnonics in the terahertz frequency range.

How to build an optical filter with an atomic vapor cell

The nature of atomic vapors, their natural alignment with interatomic transitions, and their ease of use make them highly suited for spectrally narrow-banded optical filters. Atomic filters come in two flavors: a filter based on the absorption of light by the Doppler broadened atomic vapor, i.e. a notch filter, and a bandpass filter based on the transmission of resonant light caused by the Faraday effect. The notch filter uses the absorption of resonant photons to filter out a small spectral band around the atomic transition. The off-resonant part of the spectrum is fully transmitted. Atomic vapors based on the Faraday effect allow for suppression of the detuned spectral fraction. Transmission of light originates from the magnetically induced rotation of linear polarized light close to an atomic resonance. This filter constellation allows selective acceptance of specific light frequencies. In this manuscript, we discuss these two types of filters and elucidate the specialties of atomic line filters. We also present a practical guide on building such filter setups from scratch and discuss an approach to achieve an almost perfect atomic spectrum backed by theoretical calculations.

Anomalous Loss Reduction Below Two‐Level System Saturation in Aluminum Superconducting Resonators

AbstractSuperconducting resonators are widely used in many applications such as qubit readout for quantum computing, and kinetic inductance detectors. These resonators are susceptible to numerous loss and noise mechanisms, especially the dissipation due to two‐level systems (TLS) which become the dominant source of loss in the few‐photon and low temperature regime. In this study, capacitively‐coupled aluminum half‐wavelength coplanar waveguide resonators are investigated. Surprisingly, the loss of the resonators is observed to decrease with a lowering temperature at low excitation powers and temperatures below the TLS saturation. This behavior is attributed to the reduction of the TLS resonant response bandwidth with decreasing temperature and power to below the detuning between the TLS and the resonant photon frequency in a discrete ensemble of TLS. When response bandwidths of TLS are smaller than their detunings from the resonance, the resonant response and thus the loss is reduced. At higher excitation powers, the loss follows a logarithmic power dependence, consistent with predictions from the generalized tunneling model (GTM). A model combining the discrete TLS ensemble with the GTM is proposed and matches the temperature and power dependence of the measured internal loss of the resonator with reasonable parameters.