Shot peening (SP) is recognized for its capacity to enhance surface strength and induce compressive residual stresses (CRS). Nevertheless, quantifying the mechanical property improvements in thin shot peened layers remains challenging with traditional methods. In this study, CNT/Al-Cu-Mg composites were subjected to shot peening. The microstructure evolution of the peened layers along the layer depth direction was investigated by XRD and TEM. Meanwhile, the changes in the mechanical properties of the shot peened layers and the release rules of CRS during tensile cycling at different numbers loads were measured by an in-situ X-ray stress analyzer and a micro-tensile device in conjunction with the Von Mises stress criterion. The results showed that SP generated the nano-gradient deformation layer with nanograins size of 50–100 nm near the surface. The yield strength of the surface layer was increased from 352 MPa before SP to 435 MPa, an increase of 23.6 %. Moreover, the observation of fracture morphology indicated that SP reduced the material plasticit moderately and the agglomeration of the Al2Cu. In addition, in the case of a certain CRS on the initial surface, the relaxation of CRS was correlated with the magnitude of applied loads and the number of cycles and couldn't occur when the applied loads is below a specific value.
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