Region Of Octupole Deformation Research Articles

Octupole deformation in 143,145,146Ba

Gamma rays emitted by fission fragments of 252Cf and measured using the Gammasphere array continue to give insight into neutron rich nuclei. Using our high statistics data, we have reexamined high-spin states and linking transitions associated with octupole correlations in 143,145,146Ba. This has been a region of interest, when it was proposed that near 145Ba there was a region of octupole deformation. In an even-A system, it is possible that rotational band structures are explainable by simplex quantum numbers, s=+1 and s=−1. The previous bands including octupole bands in 143,145,146Ba have been extended. The new s=i octupole bands in 145Ba and new s=−1 octupole bands in 146Ba have been identified. In addition, collective model analysis of energy displacement, rotational frequency and B(E1)/B(E2) ratios have been carried out. Evidence of the rotational consequences of octupole deformation in even-even and even-odd isotopes is given. These nuclei have trends as rotation stabilizes the vibrational degrees of freedom. The experimental results are in agreement with theoretical calculations using the interacting boson and boson-fermion models that are based on a universal nuclear energy density functional.

Octupole deformation in neutron-rich actinides and superheavy nuclei and the role of nodal structure of single-particle wavefunctions in extremely deformed structures of light nuclei

Octupole deformed shapes in neutron-rich actinides and superheavy nuclei as well as extremely deformed shapes of the light nuclei have been investigated within the framework of covariant density functional theory. We confirmed the presence of new region of octupole deformation in neutron-rich actinides with the center around but our calculations do not predict octupole deformation in the ground states of superheavy nuclei. As exemplified by the study of 36Ar, the nodal structure of the wavefunction of occupied single-particle orbitals in extremely deformed structures allows to understand the formation of the α-clusters in very light nuclei, the suppression of the α-clusterization with the increase of mass number, the formation of ellipsoidal mean-field type structures and nuclear molecules.

New insights from studies of spontaneous fission with large detector arrays

The new insights into a) the rapidly varying structures of neutron-rich nuclei up to spins as high as 20 + and 19 −, b) the spontaneous fission process itself, and c) modes of cluster radioactivity that have come out of studies of spontaneous fission of 242Pu, 248Cm and 252Cf with large detector arrays are presented. The studies include γ-γ-γ coincidences with the second generation (14–20 Compton-suppressed Ge arrays) and new, third generation (35–45 Compton-suppressed Ge arrays, Gammasphere and Eurogam) gamma-ray detector arrays. The neutron-rich nuclei observed span the full range from superdeformed ( β 2 ≥ 0.4) double-magic ground states to spherical double-magic nuclei and competing shapes in between. New structure insights include the following: New regions of identical ground state bands to spins of 10 + to 16 + were discovered; one at the sudden onset of large deformation at N=60,62 in both even- and odd-A 98–101Sr, one at midshell N = 64,66 in 108,110Ru, one for N = 88–90 144,146Ba, one for N = 92–94 152,154Nd, and at high spin in 156Nd and also in excited bands in these regions. New shape coexisting structures in both even- and odd-A for A = 96–102 Sr and Zr nuclei are found. Evidence is found in both even-even and odd-A nuclei for a new region of octupole deformation around Z = 56 and N = 86–88. Rapid changes in moments of inertia are observed with changes in Z and N of two units with sudden changes in the moments of inertia associated with band crossings. The levels in many neutron-rich nuclei are observed for the first time. Earlier, plunger studies yielded lifetimes of low spin states and recently the Doppler Shift Line Shape Analysis yielded lifetimes of high spin states. For the first time, direct measurements of yields and neutron multiplicities have been made for five correlated pairs of fission fragments of SrNd, ZrCe, MoBa, RuXe and PdTe nuclei. Neutron multiplicities from 0–10 v emission (10v for the first time) were observed in MoBa correlated pairs with the 0 and 7–10 neutron-emission yields enhanced compared to gross yields for all fragments. The MoBa data provide evidence for two different fission modes. By unfolding the observed MoBa yields, the masses and excitation energies and mass distributions at scission were extracted. These data revealed a new mode involving the high neutron multiplicities that occurs essentially through one pair, 108Mo 144Ba, 107Mo 145Ba, or 106Mo 146Ba or some combination where the 144Ba, 145Ba and/or 146Ba at scission are hyperdeformed with a long-to-short axis ratio of 3:1. The zero-neutron emission channels provide new examples of the cold rearrangements of nucleons in a new type of cluster radioactivity. The cluster radioactivity model predicted the observed enhancements of the zero-neutron channels for odd-A-odd-A nuclei as well as the observed fine structure, that is, the spin distributions of the two fragments. The measurements of intensities and γ-γ-γ coincidences in SF with large detector arrays open a new era in the determination of previously inaccessible properties of neutron-rich nuclei and the fission process.