Abstract Angular differential neutron elastic scattering cross sections have been measured by using a 7 Li(p,n) quasi-monoenergetic neutron beam. The neutron beam whose peak energy is 134 MeV was incident upon a natural carbon sample, and the scattering neutrons were measured by liquid organic scintillators with the time-of-flight (TOF) technique. The results were compared with the existing experimental data measured by a recoil-proton telescope, and the evaluated nuclear data of JENDL/HE-2007 and ENDF/B-VII.0.