Quantum Side Research Articles

Organic Two-Photon-Absorbing Photosensitizers Can Overcome Competing Light Absorption in Organic Photocatalysis.

Conventional organic photocatalysis typically relies on ultraviolet and short-wavelength visible photons as the energy source. However, this approach often suffers from competing light absorption by reactants, products, intermediates, and co-catalysts, leading to reduced quantum efficiency and side reactions. To address this issue, we developed novel organic two-photon-absorbing (TPA) photosensitizers capable of functioning under deep red and near-infrared light irradiation. Three model reactions including cyclization, Sonogashira Csp2-Csp cross-coupling, and Csp2-N cross-coupling reactions were selected to compare the performance of the new photosensitizers under both blue (427 nm) and deep red (660 nm) light irradiation. The obtained results unambiguously prove that for reactions involving blue light-absorbing reactants, products, and/or co-catalysts, deep red light source resulted in better performance than blue light when utilizing our TPA photosensitizers. This work highlights the potential of our metal-free TPA photosensitizers as a sustainable and effective solution to mitigate the competing light absorption issue in photocatalysis, not only expanding the scope of organic photocatalysts but also reducing reliance on expensive Ru/Ir/Os-based photosensitizers.

Correlated source coding with quantum side information at two decoders

Correlated source coding with quantum side information at two decoders

Reducing Entanglement with Physically Inspired Fermion-To-Qubit Mappings

In electronic structure simulations, fermion-to-qubit mappings represent the initial encoding step from the problem of fermions into a problem of qubits. This work introduces a physically inspired method for constructing mappings that significantly simplify entanglement requirements when one is simulating states of interest. The presence of electronic excitations drives the construction of our mappings, reducing correlations for target states in the qubit space. To benchmark our method, we simulate ground-states of small molecules and observe an enhanced performance when compared with classical and quantum variational approaches from prior research using conventional mappings. In particular, on the quantum side, our mappings require a reduced number of entangling layers to achieve accuracy for LiH, H2, (H2)2, H4≠ stretching, and benzene’s π system using the RY hardware-efficient ansatz. In addition, our mappings also provide an enhanced ground-state simulation performance in the density matrix renormalization group algorithm for the N2 molecule. Published by the American Physical Society 2024

Adversarial guesswork with quantum side information

The guesswork of a classical-quantum channel quantifies the cost incurred in guessing the state transmitted by the channel when only one state can be queried at a time, maximized over any classical pre-processing and minimized over any quantum post-processing. For arbitrary-dimensional covariant classical-quantum channels, we prove the invariance of the optimal pre-processing and the covariance of the optimal ost-processing. In the qubit case, we compute the optimal guesswork for the class of so-called highly symmetric informationally complete classical-quantum channels.

Experimental Guesswork with Quantum Side Information Using Twisted Light.

Guesswork is an information-theoretic quantity which can be seen as an alternate security criterion to entropy. Recent work has established the theoretical framework for guesswork in the presence of quantum side information, which we extend both theoretically and experimentally. We consider guesswork when the side information consists of the BB84 states and their higher-dimensional generalizations. With this side information, we compute the guesswork for two different scenarios for each dimension. We then performed a proof-of-principle experiment using Laguerre-Gauss modes to experimentally compute the guesswork for higher-dimensional generalizations of the BB84 states. We find that our experimental results agree closely with our theoretical predictions. This work shows that guesswork can be a viable security criterion in cryptographic tasks and is experimentally accessible in a number of optical setups.

Source coding with quantum side information at several decoders

Source coding with quantum side information at several decoders

Ke Li’s Lemma for Quantum Hypothesis Testing in General Von Neumann Algebras

A lemma stated by Li (Ann Statist 42:171-189, 2014) has been used in, for example, Nilanjana et al. (J Math Phys 57:062207, 2016), Kaur et al. (Phys Rev A 96:062318, 2017), Rouzé, Datta (IEEE Trans Inform Theory 64:593–612, 2018), Tomamichel, Tan (Comm Math Phys 338:103-137, 2015) and Wilde et al. (IEEE Trans Inform Theory 63:1792-1817, 2017) for various tasks in quantum hypothesis testing, data compression with quantum side information or quantum key distribution. This lemma was originally proven in finite dimension, with a direct extension to type I von Neumann algebras. Here, we show that the use of modular theory allows to give more transparent meaning to the objects constructed by the lemma, and to prove it for general von Neumann algebras. This yields a new proof of quantum Stein’s lemma with slightly weaker assumption, as well as immediate generalizations of its second-order asymptotics, for example the main results in Nilanjana et al. (J Math Phys 57:062207, 2016) and Li (Ann Statist 42:171-189, 2014).

100-Gbit/s Integrated Quantum Random Number Generator Based on Vacuum Fluctuations

Emerging communication and cryptography applications call for reliable fast unpredictable random number generators. Quantum random number generation allows for the creation of truly unpredictable numbers due to the inherent randomness available in quantum mechanics. A popular approach is to use the quantum vacuum state to generate random numbers. While convenient, this approach has been generally limited in speed compared to other schemes. Here, through custom codesign of optoelectronic integrated circuits and side-information reduction by digital filtering, we experimentally demonstrate an ultrafast generation rate of 100 Gbit/s, setting a new record for vacuum-based quantum random number generation by one order of magnitude. Furthermore, our experimental demonstrations are well supported by an upgraded device-dependent framework that is secure against both classical and quantum side information and that also properly considers the nonlinearity in the digitization process. This ultrafast secure random number generator in the chip-scale platform holds promise for next-generation communication and cryptography applications.1 MoreReceived 14 November 2022Accepted 3 February 2023DOI:https://doi.org/10.1103/PRXQuantum.4.010330Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasQuantum communicationQuantum cryptographyQuantum information processing with continuous variablesQuantum information theoryQuantum Information

Tight Exponential Analysis for Smoothing the Max-Relative Entropy and for Quantum Privacy Amplification

The max-relative entropy together with its smoothed version is a basic tool in quantum information theory. In this paper, we derive the exact exponent for the asymptotic decay of the small modification of the quantum state in smoothing the max-relative entropy based on purified distance. We then apply this result to the problem of privacy amplification against quantum side information, and we obtain an upper bound for the exponent of the asymptotic decreasing of the insecurity, measured using either purified distance or relative entropy. Our upper bound complements the earlier lower bound established by Hayashi, and the two bounds match when the rate of randomness extraction is above a critical value. Thus, for the case of high rate, we have determined the exact security exponent. Following this, we give examples and show that in the low-rate case, neither the upper bound nor the lower bound is tight in general. This exhibits a picture similar to that of the error exponent in channel coding. Lastly, we investigate the asymptotics of equivocation and its exponent under the security measure using the sandwiched Rényi divergence of order <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$s\in (1,2]$ </tex-math></inline-formula> , which has not been addressed previously in the quantum setting.

Provably-secure quantum randomness expansion with uncharacterised homodyne detection

Quantum random number generators (QRNGs) are able to generate numbers that are certifiably random, even to an agent who holds some side information. Such systems typically require that the elements being used are precisely calibrated and validly certified for a credible security analysis. However, this can be experimentally challenging and result in potential side-channels which could compromise the security of the QRNG. In this work, we propose, design and experimentally demonstrate a QRNG protocol that completely removes the calibration requirement for the measurement device. Moreover, our protocol is secure against quantum side information. We also take into account the finite-size effects and remove the independent and identically distributed requirement for the measurement side. More importantly, our QRNG scheme features a simple implementation which uses only standard optical components and are readily implementable on integrated-photonic platforms. To validate the feasibility and practicability of the protocol, we set up a fibre-optical experimental system with a home-made homodyne detector with an effective efficiency of 91.7% at 1550 nm. The system works at a rate of 2.5 MHz, and obtains a net randomness expansion rate of 4.98 kbits/s at 1010 rounds. Our results pave the way for an integrated QRNG with self-testing feature and provable security.

Duality Between Source Coding With Quantum Side Information and Classical-Quantum Channel Coding

In this paper, we establish an interesting duality between two different quantum information-processing tasks, namely, classical source coding with quantum side information, and channel coding over classical-quantum channels. The duality relates the optimal error exponents of these two tasks, generalizing the classical results of Ahlswede and Dueck [ <italic xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">IEEE Trans. Inf. Theory</i> , 28(3):430–443, 1982]. We establish duality both at the operational level and at the level of the entropic quantities characterizing these exponents. For the latter, the duality is given by an exact relation, whereas for the former, duality manifests itself in the following sense: an optimal coding strategy for one task can be used to construct an optimal coding strategy for the other task. Along the way, we derive a bound on the error exponent for classical-quantum channel coding with constant composition codes which might be of independent interest. Finally, we consider the task of variable-length classical compression with quantum side information, and a duality relation between this task and classical-quantum channel coding can also be established correspondingly. Furthermore, we study the strong converse of this task, and show that the strong converse property does not hold even in the i.i.d. scenario.

Simple and practical DIQKD security analysis via BB84-type uncertainty relations and Pauli correlation constraints

According to the entropy accumulation theorem, proving the unconditional security of a device-independent quantum key distribution protocol reduces to deriving tradeoff functions, i.e., bounds on the single-round von Neumann entropy of the raw key as a function of Bell linear functionals, conditioned on an eavesdropper&amp;apos;s quantum side information. In this work, we describe how the conditional entropy can be bounded in the 2-input/2-output setting, where the analysis can be reduced to qubit systems, by combining entropy bounds for variants of the well-known BB84 protocol with quantum constraints on qubit operators on the bipartite system shared by Alice and Bob. The approach gives analytic bounds on the entropy, or semi-analytic ones in reasonable computation time, which are typically close to optimal. We illustrate the approach on a variant of the device-independent CHSH QKD protocol where both bases are used to generate the key as well as on a more refined analysis of the original single-basis variant with respect to losses. We obtain in particular a detection efficiency threshold slightly below 80.26%, within reach of current experimental capabilities.

Eight-port homodyne detector: The effect of imperfections on quantum random-number generation and on detection of quadratures

The eight-port homodyne detector is an optical circuit designed to perform the monitoring of two quadratures of an optical field, the signal. By using quantum Bose fields and quantum stochastic calculus, we give a complete quantum description of this apparatus, when used as quadrature detector in continuous time. We can treat either the travelling waves in the optical circuit, either the observables involved in the detection part: two couples of photodiodes, postprocessing of the output currents. The analysis includes imperfections, such as not perfectly balanced beam splitters, detector efficiency, electronic noise, phase and intensity noise in the laser acting as local oscillator; this last noise is modelled by using mixtures of field coherent states as statistical operator of the laser component. Due to the monitoring in continuous time, the output is a stochastic process and its full probability distribution is obtained. When the output process is sampled at discrete times, the quantum description can be reduced to discrete mode operators, but at the price of having random operators, which contain also the noise of the local oscillator. Consequently, the local oscillator noise has a very different effect on the detection results with respect to an additive noise, such as the noise in the electronic components. As an application, the problem of secure random number generation is considered, based on the local oscillator shot noise. The rate of random bits that can be generated is quantified by the min-entropy; the possibility of classical and quantum side information is taken into account by suitable conditional min-entropies. The final rate depends on which parts of the apparatus are considered to be secure and on which ones are considered to be exposed to the intervention of an intruder. In some experimentally realistic situations, the entropy losses are computed.

Introduction and Analysis of Typical Quantum Hall Effect

Through reading and organizing a large amount of literature, we have gained a certain understanding of the Hall Effect. Meanwhile, we have selected the Hall Effect at the macroscopic level, and the Quantum Hall Effect, Quantum Anomalous Hall Effect, and Quantum Spin Hall Effect at the quantum side as the research content of this paper. We first explain the principles of these four phenomena, then we summarize their discovery history and the latest research progress, introduce their applications, and finally, based on our comprehension and generalization of the literature, we give a summary and outlook. This paper is helpful for the in-depth study of phenomena such as Quantum Hall Effect and Quantum Anomalous Hall Effect from Hall Effect.

One-Shot Hybrid State Redistribution

We consider state redistribution of a "hybrid" information source that has both classical and quantum components. The sender transmits classical and quantum information at the same time to the receiver, in the presence of classical and quantum side information both at the sender and at the decoder. The available resources are shared entanglement, and noiseless classical and quantum communication channels. We derive one-shot direct and converse bounds for these three resources, represented in terms of the smooth conditional entropies of the source state. Various coding theorems for two-party source coding problems are systematically obtained by reduction from our results, including the ones that have not been addressed in previous literature.

Private Classical Communication Over Quantum Multiple-Access Channels

We study private classical communication over quantum multiple-access channels. For an arbitrary number of transmitters, we derive a regularized expression of the capacity region. In the case of degradable channels, we establish a single-letter expression for the best achievable sum-rate and prove that this quantity also corresponds to the best achievable sum-rate for quantum communication over degradable quantum multiple-access channels. In our achievability result, we decouple the reliability and privacy constraints, which are handled via source coding with quantum side information and universal hashing, respectively. Hence, we also establish that the multi-user coding problem under consideration can be handled solely via point-to-point coding techniques. As a by-product of independent interest, we derive a distributed leftover hash lemma against quantum side information that ensures privacy in our achievability result.

Properties of Noncommutative Rényi and Augustin Information

R\'enyi and Augustin information are generalizations of mutual information defined via the R\'enyi divergence, playing a significant role in evaluating the performance of information processing tasks by virtue of its connection to the error exponent analysis. In quantum information theory, there are three generalizations of the classical R\'enyi divergence -- the Petz's, sandwiched, and log-Euclidean versions, that possess meaningful operational interpretation. However, the associated quantum R\'enyi and Augustin information are much less explored compared with their classical counterpart, and lacking crucial properties hinders applications of these quantities to error exponent analysis in the quantum regime. The goal of this paper is to analyze fundamental properties of the R\'enyi and Augustin information from a noncommutative measure-theoretic perspective. Firstly, we prove the uniform equicontinuity for all three quantum versions of R\'enyi and Augustin information, and it hence yields the joint continuity of these quantities in order and prior input distributions. Secondly, we establish the concavity of the scaled R\'enyi and Augustin information in the region of $s\in(-1,0)$ for both Petz's and the sandwiched versions. This completes the open questions raised by Holevo [IEEE Trans.~Inf.~Theory, 46(6):2256--2261, 2000], and Mosonyi and Ogawa [Commun.~Math.~Phys., 355(1):373--426, 2017]. For the applications, we show that the strong converse exponent in classical-quantum channel coding satisfies a minimax identity, which means that the strong converse exponent can be attained by the best constant composition code. The established concavity is further employed to prove an entropic duality between classical data compression with quantum side information and classical-quantum channel coding, and a Fenchel duality in joint source-channel coding with quantum side information.

Multi-User Distillation of Common Randomness and Entanglement From Quantum States

We construct new protocols for the tasks of converting noisy multipartite quantum correlations into noiseless classical and quantum ones using local operations and classical communication (LOCC). The former task is known as common randomness (CR) distillation, and it requires offsetting the amount of classical communication against the randomness created. We obtain a new lower bound on the “distillable common randomness,” an operational measure of the total genuine (classical) correlations in a quantum state. Our proof relies on a generalization of communication for omniscience (CO) [Csiszár and Narayan, IEEE Trans. Inf. Theory 50:3047-3061, 2004], and our contribution here is a novel simultaneous decoder for the compression of correlated classical sources by random binning with quantum side information at the decoder. For the latter task, we derive two lower bounds on the rate at which Greenberger-Horne-Zeilinger (GHZ) states can be asymptotically distilled from any given pure state under LOCC. Our approach consists in “making coherent” the proposed CR distillation protocols and recycling of resources [Devetak <italic xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">et al.</i> IEEE Trans. Inf. Theory 54(10):4587-4618, 2008]. The first lower bound is identical to a recent result by Vrana and Christandl [IEEE Trans. Inf. Theory 65(9):5945-5958, 2019], which is based on a combinatorial method to achieve the same rate. Our second lower bound generalises and improves upon this result, and unifies a number of other known lower bounds on GHZ distillation.

Equivalence of Three Classical Algorithms With Quantum Side Information: Privacy Amplification, Error Correction, and Data Compression

Privacy amplification (PA) is an indispensable component in classical and quantum cryptography. Error correction (EC) and data compression (DC) algorithms are also indispensable in classical and quantum information theory. We here study these three algorithms (PA, EC, and DC) in the presence of quantum side information, and show that they all become equivalent in the one-shot scenario. As an application of this equivalence, we take previously known security bounds of PA, and translate them into coding theorems for EC and DC which have not been obtained previously. Further, we apply these results to simplify and improve our previous result that the two prevalent approaches to the security proof of quantum key distribution (QKD) are equivalent. We also propose a new method to simplify the security proof of QKD.

Some Recent Progress in Learning Theory: The Quantum Side

Some Recent Progress in Learning Theory: The Quantum Side