Quantum Frequency Conversion Research Articles

Noise analysis of a quasi-phase-matched quantum frequency converter and higher-order counter-propagating SPDC

Quantum frequency conversion (QFC) will be an indispensable ingredient in future quantum technologies. For example, large-scale fibre-based quantum networks will require QFC to interconnect heterogeneous building blocks like emitters, channels, memories, and detectors. The performance of existing QFC devices – typically realized in periodically poled nonlinear crystals – is often severely limited by parasitic noise that arises when the pump wavelength lies between the inter-converted wavelengths. Here we comprehensively investigate the noise spectrum of a QFC device pumped by a CW 1064 nm laser. The converter was realized as a bulk periodically poled potassium titanyl phosphate (ppKTP) crystal quasi-phase-matched for conversion between 637 nm and 1587 nm, which was also polished and coated to resonantly enhance the pump field by a factor of 50. While Raman scattering dominates the noise background from 1140 nm to 1330 nm, at larger energy shifts (beyond 60 THz), parasitic spontaneous parametric down-conversion (SPDC) is the strongest noise source. Further, the noise spectrum was contaminated by a regular succession of narrow-band peaks, which we attribute to a heretofore unidentified higher-order counter-propagating SPDC processes – with quasi-phase-matching orders up to 44 evident in our measurements. This work provides a comprehensive overview of the limiting noise sources in QFC devices that use quasi-phase-matched crystals and will prove an invaluable resource in guiding their future development.

Qubit teleportation between a memory-compatible photonic time-bin qubit and a solid-state quantum network node

We report on a quantum interface linking a diamond NV center quantum network node and 795nm photonic time-bin qubits compatible with Thulium and Rubidium quantum memories. The interface makes use of two-stage low-noise quantum frequency conversion and waveform shaping to match temporal and spectral photon profiles. Two-photon quantum interference shows high indistinguishability between converted 795nm photons and the native NV center photons. We use the interface to demonstrate quantum teleportation including real-time feedforward from an unbiased set of 795nm photonic qubit input states to the NV center spin qubit, achieving a teleportation fidelity well above the classical bound. This proof-of-concept experiment shows the feasibility of interconnecting different quantum network hardware.

Metropolitan-scale heralded entanglement of solid-state qubits.

A key challenge toward future quantum internet technology is connecting quantum processors at metropolitan scale. Here, we report on heralded entanglement between two independently operated quantum network nodes separated by 10 kilometers. The two nodes hosting diamond spin qubits are linked with a midpoint station via 25 kilometers of deployed optical fiber. We minimize the effects of fiber photon loss by quantum frequency conversion of the qubit-native photons to the telecom L-band and by embedding the link in an extensible phase-stabilized architecture enabling the use of the loss-resilient single-click entangling protocol. By capitalizing on the full heralding capabilities of the network link in combination with real-time feedback logic on the long-lived qubits, we demonstrate the delivery of a predefined entangled state on the nodes irrespective of the heralding detection pattern. Addressing key scaling challenges and being compatible with different qubit systems, our architecture establishes a generic platform for exploring metropolitan-scale quantum networks.

Frequency tuning of a squeezed vacuum state using interferometric enhanced acousto-optic effect

Quantum frequency conversion is one of the important tools for quantum information processing. So far, the frequency conversion of continuous variable quantum state in radio frequency range has not been demonstrated yet. Here, we experimentally demonstrate the optical frequency fine tuning of a squeezed vacuum state by using an acousto-optic modulator based bi-frequency interferometer. The systematic efficiency of the frequency tuning device is 91%, which is only confined by the optical transmission efficiency of the acousto-optic modulators. The amount of frequency tuning is 80 MHz, which is orders of magnitude larger than the line-width of the laser used to generate the squeezed state and can, in principle, be further extended. A squeezed vacuum state with −3.47 ± 0.02 dB squeezing level is sent to the frequency tuning device, and a squeezing level of −1.98 ± 0.02 dB is directly measured by a fiber coupled homodyne detector after the frequency tuning. Our scheme can also be applied to a variety of other quantum optical states as well and will serve as a handy tool for quantum networks.

Measurement of dispersion properties in a short optical fiber for an efficient quantum frequency converter

Measurement of dispersion properties in a short optical fiber for an efficient quantum frequency converter

Multiplexed quantum frequency conversion.

We study multiplexed quantum frequency conversion (m-QFC) on a single waveguide, where a single pump beam simultaneously converts multiple signal beams at distinct wavelengths. Using a three-peak periodically poled lithium niobate (PPLN) waveguide, we demonstrate the multiplexed upconversion in the telecom band with internal efficiencies up to 73.6%. Tested with a multichannel photon-pair source, the quantum correlation is preserved well after the conversion, with coincidence-to-accidental ratio reaching 767. These results highlight a viable device approach to multiplexed quantum key distribution, quantum sensing, and quantum computing.

Efficient and widely tunable mid-infrared sources using GaAs and AlGaAs integrated platforms for second-order frequency conversion

Integrated coherent mid-infrared (mid-IR) sources are crucial for spectroscopy and quantum frequency conversion (QFC) to facilitate scalable fiber-based application of single photons. Direct mid-IR emission with broad tunability poses fundamental challenges from the gain media and mirror components. This paper presents a characterization of a second-order nonlinear platform. It showcases a mid-IR parametric coherent source with a continuous tuning range exceeding 230 nm centered around 2425 nm, achieved through difference-frequency generation (DFG). The nonlinear coefficient d14 of gallium arsenide (GaAs) and aluminum gallium arsenide (AlGaAs) on insulator is experimentally determined via second-harmonic generation (SHG) in waveguides of various lengths, and the tolerance of the process is investigated. These materials are explored for their high conversion efficiency, utilizing monolithic epitaxial quantum dots and integrated waveguides for QFC. The results demonstrate efficient and tunable mid-IR emission suitable for compact, scalable quantum emitters, with applications in environmental and health monitoring.

Demonstration of quantum network protocols over a 14-km urban fiber link

We report on the implementation of quantum entanglement distribution and quantum state teleportation over a 14.4 km urban dark-fiber link, which is partially underground, partially overhead, and patched in several stations. We characterize the link for its use as a quantum channel and realize its active polarization stabilization. Using a type-II cavity-enhanced SPDC photon pair source, a 40Ca+ single-ion quantum memory, and quantum frequency conversion to the telecom C-band, we demonstrate photon-photon entanglement, ion-photon entanglement, and teleportation of a qubit state from the ion onto a remote telecom photon, all realized over the urban fiber link.

Generation of squeezed high-order harmonics

For decades, most research of high harmonic generation (HHG) considered matter as quantum but light as classical. Recently, HHG driven by quantum states of light such as bright squeezed vacuum was predicted to reach beyond the classical HHG cutoff. Moreover, in squeezed coherent illumination, it was shown that the underlying dynamics are significantly modified by the photon statistics effective force. Here we show that HHG driven by quantum light results in quantum high harmonics. We derive a formula for the quantum state of the high harmonics, when driven by arbitrary quantum light states, and then explore specific cases of experimental relevance. Specifically, for a moderately squeezed pump, HHG driven by squeezed coherent light results in squeezed high harmonics. Harmonic squeezing is optimized by syncing ionization times with the pump's squeezing phase. Beyond this regime, as pump squeezing is increased, the harmonics initially acquire squeezed thermal photon statistics, and then occupy an intricate quantum state which strongly depends on the semiclassical nonlinear response function of the interacting system. Our results pave the way for generation of squeezed extreme-ultraviolet ultrashort pulses, and more generally, quantum frequency conversion into previously inaccessible spectral ranges, which may enable ultrasensitive attosecond metrology. Published by the American Physical Society 2024

Calibration-independent bound on the unitarity of a quantum channel with application to a frequency converter

We report on a method to certify a unitary operation with the help of source and measurement apparatuses whose calibration throughout the certification process needs not be trusted. As in the device-independent paradigm our certification method relies on a Bell test and requires no assumption on the underlying Hilbert space dimension, but it removes the need for high detection efficiencies by including the single additional assumption that non-detected events are independent of the measurement settings. The relevance of the proposed method is demonstrated experimentally by bounding the unitarity of a quantum frequency converter. The experiment starts with the heralded creation of a maximally entangled two-qubit state between a single 40Ca+ ion and a 854 nm photon. Entanglement preserving frequency conversion to the telecom band is then realized with a non-linear waveguide embedded in a Sagnac interferometer. The resulting ion-telecom photon entangled state is assessed by means of a Bell-CHSH test from which the quality of the frequency conversion is quantified. We demonstrate frequency conversion with an average certified fidelity of ≥84% and an efficiency ≥3.1 × 10−6 at a confidence level of 99%. This ensures the suitability of the converter for integration in quantum networks from a trustful characterization procedure.

Low-noise short-wavelength pumped frequency downconversion for quantum frequency converters

We present a highly efficient low-noise quantum frequency converter from the visible range to telecom wavelengths, combining a pump laser at intermediate frequency resonantly enhanced in an actively stabilized cavity with a monocrystalline bulk crystal. A demonstrator for photons emitted by nitrogen-vacancy-center qubits achieves 43% external efficiency with a noise photon rate per wavelength (frequency) band of 2 s−1/pm(17 s−1/GHz) – reducing the noise by two orders of magnitude compared with current devices based on periodically poled crystals with waveguides. With its tunable output wavelength, this device enables the generation of indistinguishable telecom photons from different network nodes and is, as such, a crucial component for a future quantum internet based on optical fiber.

Entanglement of nanophotonic quantum memory nodes in a telecom network

A key challenge in realizing practical quantum networks for long-distance quantum communication involves robust entanglement between quantum memory nodes connected by fibre optical infrastructure1–3. Here we demonstrate a two-node quantum network composed of multi-qubit registers based on silicon-vacancy (SiV) centres in nanophotonic diamond cavities integrated with a telecommunication fibre network. Remote entanglement is generated by the cavity-enhanced interactions between the electron spin qubits of the SiVs and optical photons. Serial, heralded spin-photon entangling gate operations with time-bin qubits are used for robust entanglement of separated nodes. Long-lived nuclear spin qubits are used to provide second-long entanglement storage and integrated error detection. By integrating efficient bidirectional quantum frequency conversion of photonic communication qubits to telecommunication frequencies (1,350 nm), we demonstrate the entanglement of two nuclear spin memories through 40 km spools of low-loss fibre and a 35-km long fibre loop deployed in the Boston area urban environment, representing an enabling step towards practical quantum repeaters and large-scale quantum networks.

Nanocavity-Mediated Purcell Enhancement of Er in TiO2 Thin Films Grown via Atomic Layer Deposition.

The use of trivalent erbium (Er3+), typically embedded as an atomic defect in the solid-state, has widespread adoption as a dopant in telecommunication devices and shows promise as a spin-based quantum memory for quantum communication. In particular, its natural telecom C-band optical transition and spin-photon interface make it an ideal candidate for integration into existing optical fiber networks without the need for quantum frequency conversion. However, successful scaling requires a host material with few intrinsic nuclear spins, compatibility with semiconductor foundry processes, and straightforward integration with silicon photonics. Here, we present Er-doped titanium dioxide (TiO2) thin film growth on silicon substrates using a foundry-scalable atomic layer deposition process with a wide range of doping controls over the Er concentration. Even though the as-grown films are amorphous after oxygen annealing, they exhibit relatively large crystalline grains, and the embedded Er ions exhibit the characteristic optical emission spectrum from anatase TiO2. Critically, this growth and annealing process maintains the low surface roughness required for nanophotonic integration. Finally, we interface Er ensembles with high quality factor Si nanophotonic cavities via evanescent coupling and demonstrate a large Purcell enhancement (≈300) of their optical lifetime. Our findings demonstrate a low-temperature, nondestructive, and substrate-independent process for integrating Er-doped materials with silicon photonics. At high doping densities this platform can enable integrated photonic components such as on-chip amplifiers and lasers, while dilute concentrations can realize single ion quantum memories.

Storage of telecom wavelength heralded single photons in a fiber cavity quantum memory

We demonstrate the storage and retrieval of heralded single photons in a fiber-based cavity quantum memory. The photons are stored, and retrieved, from the memory using quantum frequency conversion which switches the photon into, and out of, resonance with the cavity. The photons, generated in the telecom O-band with a bandwidth of 81 GHz, are retrieved from the memory with a 1/e lifetime of 1.64 µs, or 32.8 cavity round trips. We show that non-classical photon statistics remain for 70 round trips. The internal memory efficiency after 0.5 µs of storage is 10.9 ± 0.5%; a coupling efficiency of 60% into the memory cavity yields a total efficiency of 6.0 ± 0.3%. These results mark a crucial step forward in the development of fiber-based quantum memories, and high-bandwidth memories operating at telecom wavelengths, with applications to photon source multiplexing and fiber-based quantum networking.

Frequency conversion to the telecom O-band using pressurized hydrogen.

Large-scale quantum networks rely on optical fiber networks and photons as so-called flying qubits for information transport. While dispersion and absorption of optical fibers are minimum at the infrared telecom wavelengths, most atomic and solid state platforms operate at visible or near-infrared wavelengths. Quantum frequency conversion is required to bridge these two wavelength regimes, and nonlinear crystals are currently employed for this process. Here, we report a novel approach of frequency conversion to the telecom band. This interaction is based on coherent Stokes Raman scattering (CSRS), a four-wave mixing process resonantly enhanced in a dense molecular hydrogen gas. We show the conversion of photons from 863 nm to the telecom O-band and demonstrate that the input polarization state is preserved. This process is intrinsically broadband and can be adapted to any other wavelength.

Telecom Networking with a Diamond Quantum Memory

Practical quantum networks require interfacing quantum memories with existing channels and systems that operate in the telecom band. Here we demonstrate low-noise, bidirectional quantum frequency conversion that enables a solid-state quantum memory to directly interface with telecom-band systems. In particular, we demonstrate conversion of visible-band single photons emitted from a silicon-vacancy (SiV) center in diamond to the telecom O band, maintaining low noise (g2(0)<0.1) and high indistinguishability (V=89±8%). We further demonstrate the utility of this system for quantum networking by converting telecom-band time-bin pulses, sent across a lossy and noisy 50-km deployed fiber link, to the visible band and entangling them with a diamond quantum memory with fidelity F≥87±2.5%. These results demonstrate the viability of SiV quantum memories integrated with telecom-band systems for scalable quantum networking applications. Published by the American Physical Society 2024

Telecom-band quantum dot technologies for long-distance quantum networks.

A future quantum internet is expected to generate, distribute, store and process quantum bits (qubits) over the world by linking different quantum nodes via quantum states of light. To facilitate long-haul operations, quantum repeaters must operate at telecom wavelengths to take advantage of both the low-loss optical fibre network and the established technologies of modern optical communications. Semiconductor quantum dots have thus far shown exceptional performance as key elements for quantum repeaters, such as quantum light sources and spin-photon interfaces, but only in the near-infrared regime. Therefore, the development of high-performance telecom-band quantum dot devices is highly desirable for a future solid-state quantum internet based on fibre networks. In this Review, we present the physics and technological developments towards epitaxial quantum dot devices emitting in the telecom O- and C-bands for quantum networks, considering both advanced epitaxial growth for direct telecom emission and quantum frequency conversion for telecom-band down-conversion of near-infrared quantum dot devices. We also discuss the challenges and opportunities for future realization of telecom quantum dot devices with improved performance and expanded functionality through hybrid integration.

Low-noise quantum frequency conversion in a monolithic cavity with bulk periodically poled potassium titanyl phosphate

Low-noise quantum frequency conversion in a monolithic cavity with bulk periodically poled potassium titanyl phosphate

Two‐Stage, Low Noise Quantum Frequency Conversion of Single Photons from Silicon‐Vacancy Centers in Diamond to the Telecom C‐Band

AbstractThe silicon‐vacancy center in diamond holds great promise as a qubit for quantum communication networks. However, since the optical transitions are located within the visible red spectral region, quantum frequency conversion to low‐loss telecommunication wavelengths becomes a necessity for its use in long‐range, fiber‐linked networks. This work presents a highly efficient, low‐noise quantum frequency conversion device for photons emitted by a silicon‐vacancy (SiV) center in diamond to the telecom C‐band. By using a two‐stage difference‐frequency mixing scheme, spontaneous parametric down‐conversion (SPDC) noise is circumvented and Raman noise is minimized, resulting in a very low noise rate of 10.4 ± 0.7 photons per second as well as an overall device efficiency of 35.6%. By converting single photons from SiV centers, it demonstrates the preservation of photon statistics upon conversion.

Compact all-fiber quantum-inspired LiDAR with over 100 dB noise rejection and single photon sensitivity

Entanglement and correlation of quantum light can enhance LiDAR sensitivity in the presence of strong background noise. However, the power of such quantum sources is fundamentally limited to a stream of single photons and cannot compete with the detection range of high-power classical LiDAR transmitters. To circumvent this, we develop and demonstrate a quantum-inspired LiDAR prototype based on coherent measurement of classical time-frequency correlation. This system uses a high-power classical source and maintains the high noise rejection advantage of quantum LiDARs. In particular, we show that it can achieve over 100dB rejection (with 100ms integration time) of indistinguishable (with statistically identical properties in every degree of freedom) in-band noise while still being sensitive to single photon signals. In addition to the LiDAR demonstration, we also discuss the potential of the proposed LiDAR receiver for quantum information applications. In particular, we propose the chaotic quantum frequency conversion technique for coherent manipulation of high dimensional quantum states of light. It is shown that this technique can provide improved performance in terms of selectivity and efficiency as compared to pulse-based quantum frequency conversion.