Quantized Spin Hall Conductance Research Articles

Rational design of quantum spin Hall phase in type-III van der Waals heterostructures

Van der Waals heterostructures (vdWHs) are effective platforms for exploring various attractive topological phases. Here, based on the low-energy effective k·p model, we propose that the type-III vdWHs, which were previously considered as only belonging to trivial metallic phases, can realize the nontrivial quantum spin Hall (QSH) effect. We reveal that the band inversion of such a QSH phase is attributed to the band alignment of momentum space matching, i.e., the conduction band minimum and valence band maximum located at the same point in momentum space near the Fermi level. Moreover, using first-principles calculations, we show that the Mg(OH)2/Ga2O2 heterobilayer, a typical type-III vdWH with high thermodynamic stability, is an ideal candidate for achieving our strategy. We further calculate the helical gapless edge states and quantized spin Hall conductance, which are visible inside the global bandgap, thus facilitating the experimental observation. Our work offers a promising pathway for realizing the QSH phase in natural materials.

Switchable large-gap quantum spin Hall state in the two-dimensional MSi2Z4 class of materials

Quantum spin Hall (QSH) insulators exhibit spin-polarized conducting edge states that are topologically protected from backscattering and offer unique opportunities for addressing fundamental science questions and device applications. Finding viable materials that host such topological states, however, remains a challenge. Here by using in-depth first-principles theoretical modeling, we predict large bandgap QSH insulators in recently bottom-up synthesized two-dimensional (2D) MSi$_2$Z$_4$ (M = Mo or W and Z = P or As) materials family with $1T^\prime$ structure. A structural distortion in the $2H$ phase drives a band inversion between the metal (Mo/W) $d$ and $p$ states of P/As to realize spinless Dirac cone states without spin-orbit coupling. When spin-orbit coupling is included, a hybridization gap as large as $\sim 204$ meV opens up at the band crossing points, realizing spin-polarized conducting edge states with nearly quantized spin Hall conductivity. We also show that the inverted band gap is tunable with a vertical electric field which drives a topological phase transition from the QSH to a trivial insulator with Rashba-like edge states. Our study identifies 2D MSi$_2$Z$_4$ materials family with $1T^\prime$ structure as large bandgap, tunable QSH insulators with protected spin-polarized edge states and large spin-Hall conductivity.

Quantized spin Hall conductance in a magnetically doped two dimensional topological insulator

Soon after the discovery of the quantum spin Hall effect, it has been predicted that a magnetic impurity in the presence of strong Coulomb interactions will destroy the quantum spin Hall effect. However, the fate of the quantum spin Hall effect in the presence of magnetic impurities has not yet been experimentally investigated. Here, we report the successful experimental demonstration of a quantized spin Hall resistance in HgTe quantum wells dilutely alloyed with magnetic Mn atoms. These quantum wells exhibit an inverted band structure that is very similar to that of the undoped material. Micron sized devices of (Hg,Mn)Te quantum well (in the topological phase) show a quantized spin Hall resistance of h/2e2 at low temperatures and zero magnetic field. At finite temperatures, we observe signatures of the Kondo effect due to interaction between the helical edge channels and magnetic impurities. Our work lays the foundation for future investigations of magnetically doped quantum spin Hall materials towards the realization of chiral Majorana fermions.

Doping the chiral spin liquid: Topological superconductor or chiral metal

We point out that there are two different chiral spin liquid states on the triangular lattice and discuss the conducting states that are expected on doping them. These states labeled CS1 and CS2 are associated with two distinct topological orders with different edge states, although they both spontaneously break time reversal symmetry and exhibit the same quantized spin Hall conductance. While CSL1 is related to the Kalmeyer-Laughlin state, CSL2 is the $\nu =4$ member of Kitaev's 16 fold way classification. Both states are described within the Abrikosov fermion representation of spins, and the effect of doping can be accessed by introducing charged holons. On doping CSL2, condensation of charged holons leads to a topological d+id superconductor. However on doping CSL1 , in sharp contrast , two different scenarios can arise: first, if holons condense, a chiral metal with doubled unit cell and finite Hall conductivity is obtained. However, in a second novel scenario, the internal magnetic flux adjusts with doping and holons form a bosonic integer quantum Hall (BIQH) state. Remarkably, the latter phase is identical to a $d+id$ superconductor. In this case the Mott insulator to superconductor transition is associated with a bosonic variant of the integer quantum Hall plateau transition for the holon. We connect the above two scenarios to two recent numerical studies of doped chiral spin liquids on triangular lattice. Our work clarifies the complex relation between topological superconductors, chiral spin liquids and quantum criticality .

Spin Chain Network Construction of Chiral Spin Liquids.

We show that a honeycomb lattice of Heisenberg spin-1/2 chains with three-spin junction interactions allows for controlled analytical studies of chiral spin liquids (CSLs). Tuning these interactions to a chiral fixed point, we find a Kalmeyer-Laughlin CSL phase which here is connected to the critical point of a boundary conformal field theory. Our construction directly yields a quantized spin Hall conductance and localized spinons with semionic statistics as elementary excitations. We also outline the phase diagram away from the chiral point where spinons may condense. Generalizations of our approach can provide microscopic realizations for many other CSLs.

High Mobility HgTe Microstructures for Quantum Spin Hall Studies.

The topic of two-dimensional topological insulators has blossomed after the first observation of the quantum spin Hall (QSH) effect in HgTe quantum wells. However, studies have been hindered by the relative fragility of the edge states. Their stability has been a subject of both theoretical and experimental investigation in the past decade. Here, we present a new generation of high quality (Cd,Hg)Te/HgTe-structures based on a new chemical etching method. From magnetotransport measurements on macro- and microscopic Hall bars, we extract electron mobilities μ up to about 400 × 103 cm2/(V s), and the mean free path λmfp becomes comparable to the sample dimensions. The Hall bars show quantized spin Hall conductance, which is remarkably stable up to 15 K. The clean and robust edge states allow us to fabricate high quality side-contacted Josephson junctions, which are significant in the context of topological superconductivity. Our results open up new avenues for fundamental research on QSH effect as well as potential applications in spintronics and topological quantum computation.

Topological Insulators from Electronic Superstructures

The possibility of realizing topological insulators by spontaneous formation of electronic superstructure is theoretically investigated in a minimal two-orbital model including both the spin-orbit coupling and electron correlations on a triangular lattice. Using the mean-field approximation, we show that the model exhibits several different types of charge ordered insulators, where the charge disproportionation forms a honeycomb or kagome superstructure. We find that the charge ordered insulators in the presence of strong spin-orbit coupling can be topological insulators showing quantized spin Hall conductivity. Their band gap is dependent on electron correlations as well as the spin-orbit coupling, and even vanishes with showing the massless Dirac dispersion at the transition to a trivial charge ordered insulator. Our results suggest a new route to realize and control topological states of quantum matter by the interplay between the spin-orbit coupling and electron correlations.

Topological quantum phase transition in Kane-Mele-Kondo lattice model

We systematically explore the ground-state phase diagram of the Kane-Mele-Kondo lattice model on the honeycomb lattice, in particular, we focus on its magnetic properties which has not been studied in the previous publication[Feng, Dai, Chung, and Si, Phys. Rev. Lett. \textbf{111}, 016402 (2013)]. Beside the Kondo insulator found in that paper, two kinds of antiferromagnetic spin-density-wave phases are identified. One is the normal antiferromagnetic spin-density-wave state and the other is a nontrivial topological antiferromagnetic spin-density-wave state with a quantized spin Hall conductance and a helical edge-state. The quantum spin Hall insulator is found to be absent since it is always unstable to antiferromagnetic spin-density-wave states at least at the mean-field level in our model. Furthermore, the transition between the two spin-density-wave phases are topological quantum phase transition described by the three-dimensional quantum electrodynamics, in which conduction electrons contribute to the low-energy Dirac fermions while the spin-wave fluctuation of local spins gives rise to an effective dynamic U(1) gauge-field. Such nontrivial transition shows radical critical thermodynamic, transport and single-particle behaviors, which provide a fingerprint for this transition. Additionally, the transition of antiferromagnetic spin-density-wave states to the Kondo insulator is found to be first-order. The introduction of two novel magnetic phases and their topological quantum phase transition show rich and intrinsic physics involving in the Kane-Mele-Kondo lattice model.

Symmetry-Protected Quantum Spin Hall Phases in Two Dimensions

Symmetry-protected topological (SPT) states are short-range entangled states with symmetry. Nontrivial SPT states have symmetry-protected gapless edge excitations. In 2 dimension (2D), there are an infinite number of nontrivial SPT phases with SU(2) or SO(3) symmetry. These phases can be described by SU(2) or SO(3) nonlinear-sigma models with a quantized topological θ term. At an open boundary, the θ term becomes the Wess-Zumino-Witten term and consequently the boundary excitations are decoupled gapless left movers and right movers. Only the left movers (if θ>0) carry the SU(2) or SO(3) quantum numbers. As a result, the SU(2) SPT phases have a half-integer quantized spin Hall conductance and the SO(3) SPT phases have an even-integer quantized spin Hall conductance. Both the SU(2) and SO(3) SPT phases are symmetric under their U(1) subgroup and can be viewed as U(1) SPT phases with even-integer quantized Hall conductance.

Fermionic Magnons, Non-Abelian Spinons, and the Spin Quantum Hall Effect from an Exactly Solvable Spin-1/2Kitaev Model with SU(2) Symmetry

We introduce an exactly solvable SU(2)-invariant spin-1/2 model with exotic spin excitations. With time reversal symmetry (TRS), the ground state is a spin liquid with gapless or gapped spin-1 but fermionic excitations. When TRS is broken, the resulting spin liquid exhibits deconfined vortex excitations which carry spin-1/2 and obey non-Abelian statistics. We show that this SU(2) invariant non-Abelian spin liquid exhibits the spin quantum Hall effect with quantized spin Hall conductivity σ(xy)(s)=ℏ/2π, and that the spin response is effectively described by the SO(3) level-1 Chern-Simons theory at low energy. We further propose that a SU(2) level-2 Chern-Simons theory is the effective field theory describing the topological structure of the non-Abelian SU(2) invariant spin liquid.

Magnetic Response in Quantized Spin Hall Phase of Correlated Electrons

We investigate the magnetic response in the quantized spin Hall (SH) phase of layered-honeycomb lattice system with intrinsic spin-orbit coupling lambda_SO and on-site Hubbard U. The response is characterized by a parameter g= 4 U a^2 d / 3, where a and d are the lattice constant and interlayer distance, respectively. When g< (sigma_{xy}^{s2} mu)^{-1}, where sigma_{xy}^{s} is the quantized spin Hall conductivity and mu is the magnetic permeability, the magnetic field inside the sample oscillates spatially. The oscillation vanishes in the non-interacting limit U -> 0. When g > (sigma_{xy}^{s2} mu)^{-1}, the system shows perfect diamagnetism, i.e., the Meissner effect occurs. We find that superlattice structure with large lattice constant is favorable to see these phenomena. We also point out that, as a result of Zeeman coupling, the topologically-protected helical edge states shows weak diamagnetism which is independent of the parameter g.

Inverse quantum spin Hall effect generated by spin pumping from precessing magnetization into a graphene-based two-dimensional topological insulator

We present a multiterminal nanostructure for electrical probing of the quantum spin Hall effect (QSHE) in two-dimensional (2D) topological insulators (TIs). The device consists of a ferromagnetic (FM) island with precessing magnetization that pumps (in the absence of any bias voltage) pure spin current symmetrically into the left and right adjacent 2D TIs modeled as graphene nanoribbons with the intrinsic spin-orbit (SO) coupling. In the reference frame rotating with magnetization, the device is mapped onto a dc circuit with twice as many terminals whose effectively half-metallic ferromagnetic electrodes are biased by the frequency $\ensuremath{\hbar}\ensuremath{\omega}/e$ of the microwave radiation driving the magnetization precession at the ferromagnetic resonance conditions. The QSH regime of the six-terminal $\text{TI}|\text{FM}|\text{TI}$ nanodevice, attached to two longitudinal and four transverse normal metal electrodes, is characterized by the SO-coupling-induced energy gap, chiral spin-filtered edge states within finite length TI regions, and quantized spin Hall conductance when longitudinal bias voltage is applied, despite the presence of the FM island. The same unbiased device, but with precessing magnetization of the central FM island, blocks completely pumping of total spin and charge currents into the longitudinal electrodes while generating dc transverse charge Hall currents. Although these transverse charge currents are not quantized, their induction together with zero longitudinal charge current is a unique electrical response of TIs to pumped pure spin current that cannot be mimicked by SO coupled but topologically trivial systems. In the corresponding two-terminal inhomogeneous $\text{TI}|\text{FM}|\text{TI}$ nanostructures, we image spatial profiles of local spin and charge currents within TIs which illustrate transport confined to chiral spin-filtered edges states while revealing concomitantly the existence of interfacial spin and charge currents flowing around $\text{TI}\ensuremath{\mid}\text{FM}$ interfaces and penetrating into the bulk of TIs over some short distance.

Integer spin Hall effect in ballistic quantum wires

We investigate the ballistic electron transport in a two dimensional Quantum Wire under the action of an electric field ($E_y$). We demonstrate how the presence of a Spin Orbit coupling, due to the uniform electric confinement field gives a non-commutative effect as in the presence of a transverse magnetic field. We discuss how the non commutation implies an edge localization of the currents depending on the electron spins also giving a semi-classical spin dependent Hall current. We also discuss how it is possible obtain a quantized Spin Hall conductance in the ballistic transport regime by developing the Landauer formalism and show the coupling between the spin magnetic momentum and the orbital one due to the presence of a circulating current.

Nondissipative Spin Hall Effect via Quantized Edge Transport

The spin Hall effect in a two-dimensional electron system on honeycomb lattice with both intrinsic and Rashba spin-orbit couplings is studied numerically. Integer quantized spin Hall conductance is obtained at the zero Rashba coupling limit when electron Fermi energy lies in the energy gap created by the intrinsic spin-orbit coupling, in agreement with recent theoretical prediction. While nonzero Rashba coupling destroys electron spin conservation, the spin Hall conductance is found to remain near the quantized value, being insensitive to disorder scattering, until the energy gap collapses with increasing the Rashba coupling. We further show that the charge transport through counterpropagating spin-polarized edge channels is well quantized, which is associated with a topological invariant of the system.

Spin quantum Hall effect in unconventional superconductors

We study the properties of the "spin quantum Hall fluid" - a novel spin phase with quantized spin Hall conductance that is potentially realizable in superconducting systems with unconventional pairing symmetry. A simple realization is provided by a $d_{x^2-y^2} + id_{xy}$ superconductor which we argue has a dimensionless spin Hall conductance equal to two. A theory of the edge states of the $d_{x^2-y^2}+id_{xy}$ superconductor is developed. The properties of the transition to a phase with vanishing spin Hall conductance induced by disorder are considered. We construct a description of this transition in terms of a supersymmetric spin chain, and use it to numerically determine universal properties of the transition. We discuss various possible experimental probes of this quantum Hall physics.