THz Pulses Research Articles

Enhanced inertial magnetization response driven by chirped terahertz field

We explore the spin dynamics process in ferromagnets driven by chirped THz fields, utilizing the spin dynamics model derived from the inertial Landau-Lifshitz-Gilbert equation. Our findings reveal a substantial enhancement in spin dynamics intensity, ranging from 15% to 20% when the sample is subjected to a chirped THz pulse. Additionally, it is observed that chirped THz fields have the capability to shift the peak of spin dynamics, with the variation dependent on the chirping time of the THz pulse. Furthermore, the underlying physical mechanisms responsible for such spin dynamics are well explained by the Zeeman torque and the time delay of different frequencies of the chirped THz fields within the framework of the inertial Landau-Lifshitz-Gilbert equation.

Formation of quasi unipolar pulses in nonequilibrium magnetized plasma channels

The possibility of controlling both the spectral and polarization properties of THz pulses propagating in strongly nonequilibrium extended magnetized plasma channels formed by intense UV femtosecond laser pulses in nitrogen (air) is analyzed. The formation of quasiunipolar pulses with a nonzero electric area and a specific state of polarization is discussed. The transformation of such pulses upon leaving the region of a static magnetic field is analyzed.

Significant Enhancement in THz Emission and Piezoelectricity in Atomically Thin Nb-Doped MoS2.

A significantly enhanced THz radiation generation from femtosecond photoexcited MoS2 layers due to Nb-doping is reported here. Different microscopic mechanisms involved in the THz photocurrent generation vary in their relative contributions in the two cases of photoexcitation, i.e., above and below the electronic bandgap of the layers. For a moderate Nb-doping level of just ∼0.05%, we have observed a multifold enhancement in the THz emission for the case of the above bandgap excitation, which is, though, nearly 1.5 times for the case of the below bandgap excitation of the monolayer MoS2. Alongside the difference in THz generation efficiency, the THz pulse polarity is also reversed at the above bandgap excitation of the Nb-doped layers, consequent to the reversed surface depletion field. Except for a slightly smaller difference in the THz enhancement factor, all the observations are reproducible in the bilayers as well to imply a weaker inversion symmetry and reduced screening of the surface depletion field due to Nb-doping. Furthermore, we employed pristine MoS2 and Nb-doped MoS2 monolayers to fabricate piezoelectric nanogenerator devices. Like enhancement in the ultrafast THz emission, the piezoelectric performance of the nanogenerator, fabricated with the Nb-doped MoS2 monolayer is also increased by a similar factor.

Optimized terahertz generation in BNA organic crystals with chirped Ti:sapphire laser pulses.

We report on the efficient generation of intense terahertz radiation from the organic crystal N-benzyl-2-methyl-4-nitroaniline pumped by chirped Ti:sapphire femtosecond laser pulses. The THz energy and spectrum as a function of the pump fluence and duration of the chirped laser pulses are studied systematically. For the appropriate positively chirped pump pulses, a significant boost in the THz generation efficiency by a factor of around 2.5 is achieved, and the enhancement of high-frequency components (>1 THz) shortens the THz pulse duration. Via complete characterization of THz properties and transmitted laser spectra, this nonlinear behavior is attributed to the extended effective interaction length for phase matching as a result of the self-phase modulation of the intense pump laser pulses. Numerical calculations well reproduce the experimental observation. Our results demonstrate a robust, efficient, strong-field (up to several MV/cm) THz source using the common sub-10 mJ and sub-100 fs Ti:sapphire laser systems without optical parametric amplifiers.

The development of a low-temperature terahertz scanning tunneling microscope based on a cryogen-free scheme.

We have developed a cryogen-free, low-temperature terahertz scanning tunneling microscope (THz-STM). This system utilizes a continuous-flow cryogen-free cooler to achieve low temperatures of ∼25K. Meanwhile, an ultra-small ultra-high vacuum chamber results in the reduction of the distance from sample to viewport to only 4cm. NA = 0.6 can be achieved while placing the entire optical component, including a large parabolic mirror, outside the vacuum chamber. Thus, the convenience of optical coupling is much improved without compromising the performance of STM. Based on this, we introduced THz pulses into the tunnel junction and constructed the THz-STM, achieving atomic-level spatial resolution in THz-driven current imaging and sub-picosecond (sub-ps) time resolution in autocorrelation signals during pump-probe measurements. Experimental data from various representative samples are presented to showcase the performance of the instrument, establishing it as an ideal platform for studying non-equilibrium dynamic processes at nanoscale.

Analytically controlling the laser-induced electron phase in sub-cycle motion

We develop an approach to directly control the phase of an electron's sub-cycle motion in an intense laser field. The method is established by tuning a low-frequency electric field applied on a centrosymmetric gaseous target during its interaction with a few-cycle infrared laser pulse. We find a universal analytical relation between the low-frequency electric field and its induced harmonic frequency shift, derived by the strong-field approximation. This simple relation and its universality are confirmed numerically by directly solving the time-dependent Schrödinger equation. Moreover, we demonstrate the benefits of the discovered relation in applications, including continuously and precisely tuning XUV waves and developing a method of comprehensively sampling the THz pulse. Published by the American Physical Society 2024

A Chirped Characteristic-Tunable Terahertz Source for Terahertz Sensing.

In broadband terahertz waves generated by femtosecond lasers, spatial chirp will be simultaneously produced with the introduction of angular dispersion. The chirp characteristics of the terahertz wave will directly affect the frequency response, bandwidth response, and intensity response of the terahertz sensor. To enhance the capability of terahertz sensors, it is necessary to control and improve the chirped characteristics of broadband terahertz sources. We generate a chirped terahertz wave via optical rectification in a LiNbO3 prism using the technique of pulse front tilt. The effect of the pump-beam spot size on THz generation is systematically studied. The pump's spot size is manipulated using a telescope system. With a pump spot diameter of 1.8 mm, the scanning spectrum of the THz pulse is narrower and is divided into multiple distinct peaks. In contrast, using a pump spot diameter of 3.7 mm leads to increased efficiency in the generation of THz pulses. Also, we investigate the underlying properties governing the generation of chirped terahertz pulses using varying pump pulse spot diameters.

Coherent control of rare earth 4f shell wavefunctions in the quantum spin liquid Tb2Ti2O7

The resonant excitation of electronic transitions with coherent laser sources creates quantum coherent superpositions of the involved electronic states. Most time-resolved studies have focused on gases or isolated subsystems embedded in insulating solids, aiming for applications in quantum information. Here, we focus on the coherent control of orbital wavefunctions in the correlated quantum material Tb2Ti2O7, which forms an interacting spin liquid ground state. We show that resonant excitation with a strong THz pulse creates a coherent superposition of the lowest energy Tb 4f states. The coherence manifests itself as a macroscopic oscillating magnetic dipole, which is detected by ultrafast resonant x-ray diffraction. We envision the coherent control of orbital wavefunctions demonstrated here to become a new tool for the ultrafast manipulation and investigation of quantum materials.

Generation of extremely strong accelerating electric field by focusing radially polarized THz pulses with a paraboloid ring

Efficient acceleration of electrically charged particles by focused electromagnetic pulses requires a strong accelerating electric field as well as a sufficiently large interaction region. Single-cycle terahertz pulses are promising candidates for such applications due to their advantageous wavelength and available peak electric field at the MV/cm level. We propose and characterize a focusing optics for a possible electron vacuum accelerator. This consists of a reflaxicon for beam shaping and a ring-like segment of an on-axis parabolic mirror for tight focusing of the radially polarized THz pulse in order to reach a strong accelerating electric field. The electric field distribution in the focal region was determined by the Stratton–Chu vector diffraction method. Semi-analytical and purely analytical formulae were also derived, simplifying the computation procedure. By focusing radially polarized single-cycle terahertz pulses with 3mJ pulse energy, calculations predict accelerating electric field component in the order of 100MV/cm, well suitable for particle acceleration.

Single-cycle, 643 mW average power terahertz source based on tilted pulse front in lithium niobate.

We present the highest, to the best of our knowledge, average power from a laser-driven single-cycle THz source demonstrated so far, using optical rectification in the tilted pulse front geometry in cryogenically cooled lithium niobate, pumped by a commercially available 500 W ultrafast thin-disk ytterbium (Yb) amplifier. We study repetition rate-dependent effects in our setup at 100 and 40 kHz at this high average power, revealing different optimal fluence conditions for efficient conversion. The demonstrated sources with multi-100 mW average power at these high repetition rates combine high THz pulse energies and high repetition rate and are thus ideally suited for nonlinear THz spectroscopy experiments with significantly reduced measurement times. The presented result is a first benchmark for high average power THz time-domain spectroscopy systems for nonlinear spectroscopy, driven by very high average power ultrafast Yb lasers.

Can specific THz fields induce collective base-flipping in DNA? A stochastic averaging and resonant enhancement investigation based on a new mesoscopic model.

We study the metastability, internal frequencies, activation mechanism, energy transfer, and the collective base-flipping in a mesoscopic DNA via resonance with specific electric fields. Our new mesoscopic DNA model takes into account not only the issues of helicity and the coupling of an electric field with the base dipole moments, but also includes environmental effects, such as fluid viscosity and thermal noise. Also, all the parameter values are chosen to best represent the typical values for the opening and closing dynamics of a DNA. Our study shows that while the mesoscopic DNA is metastable and robust to environmental effects, it is vulnerable to certain frequencies that could be targeted by specific THz fields for triggering its collective base-flipping dynamics and causing large amplitude separation of base pairs. Based on applying the Freidlin-Wentzell method of stochastic averaging and the newly developed theory of resonant enhancement to our mesoscopic DNA model, our semi-analytic estimates show that the required fields should be THz fields with frequencies around 0.28 THz and with amplitudes in the order of 450 kV/cm. These estimates compare well with the experimental data of Titova et al., which have demonstrated that they could affect the function of DNA in human skin tissues by THz pulses with frequencies around 0.5 THz and with a peak electric field at 220 kV/cm. Moreover, our estimates also conform to a number of other experimental results, which appeared in the last couple years.

Resonantly enhanced terahertz four-wave mixing in fluorides.

Converting a THz signal into the optical domain is of great interest for THz sensing and spectroscopy. Here intense broadband THz pulses with a central frequency of ΩTHz are mixed with an optical pump at ωp, and a signal is observed at a wavelength of ωs = 2(ωp - Δωp) - ΩTHz with the detuning ωp - Δωp being due to pump pulse spectral broadening. The observed THz-four-wave mixing (FWM) signal close to 400 nm is shown to result from a resonantly amplified four-wave mixing in CaF2, BaF2, and MgF2.

Short failure localization in advanced package using optoelectronic sampling terahertz time domain reflectometry and deconvolution method

Failure localization in advanced packaging is a challenging task. Optoelectronic sampling Terahertz time-domain reflectometry (OES THz TDR) employs ultrafast lasers to generate high-frequency THz pulse. The THz pulse is coupled into advanced package trace using radio frequency probe. When there is an open or short failure in the circuit, TDR signal could be captured. Deconvolution processing method was introduced to remove noise from multiple reflections of the remaining circuit. A short failure model with remaining circuit was studied. After deconvolution, the TDR localization accuracy improves from 573 μm to 12 μm, and the correlation coefficient improved from 99.612 % to 99.955 %. Advanced package sample including substrate, C4 bump, interposer, and micro bump was analyzed. By comparing the TDR waveform of short failure sample and references, the short failure is localized inside of the die. By destroying the failure sample and measuring the current-voltage curve, the short failure location is verified.

THz generation by AlGaAs/GaAs heterostructured p-i-n diode

The generation of terahertz radiation by heterostructure p-i-n AlxGa1−xAs/GaAs diodes excited by femtosecond optical pulses was studied experimentally and using the Monte Carlo method. It is shown that when the reverse bias varies, the terahertz generation mechanism changes. With a positive bias on the p-i-n diode, the THz generation mechanism is due to the reflection of the photoexcited electrons from the interface. With a large internal electric field, THz generation in the p-i-n diode occurs due to the acceleration of electrons at the ballistic stage of their movement in the electric field to velocities significantly exceeding the steady state velocity (“velocity overshoot”). The subsequent sharp decrease in velocity of electrons is associated with their inter-valley transitions from the Γ-valley to the L-valley of the conduction band. At electric fields less than 22 kV/cm, the effect of electric field screening by photoexcited carriers has a significant impact on the formation of photocurrent and, accordingly, on the THz generation mechanism. As the reverse bias decreases, this effect leads to a shift in the maximum of the THz pulse toward shorter times and it begins to dominate at electric fields less than 10 kV/cm.

Spatiotemporal walk-off and improved focusing of plasma THz sources

High-field THz sources with peak field strengths exceeding MV/cm are essential for nonlinear THz spectroscopy and coherent control of matter on ultrafast time scales. Two-color femtosecond laser plasma sources employing long filamentation have been reported as providing single-cycle, >MV/cm fields, with multi-decade spanning bandwidth and polarization control, making them promising sources for such experiments. In this work, we report the observation of spatiotemporal spreading of the THz pulse when standard off-axis parabolic mirrors are used for collection and focusing of long filament plasma-based THz pulses. This produces a flying focus for THz light, with the axial focal region propagating at a velocity of 1/3 the speed of light. The THz emission is then subsequently spread over a temporal width of ∼10 ps, approximately 100 times the THz pulse duration detected by electro-optic sampling at any single point along the focus. The consequences of this non-ideal focusing are a potential and drastic overestimation of the peak THz electric field based on energy measurements, as well as significant phase noise arising from beam pointing fluctuations. We show that this spatiotemporal spreading can be minimized using a simple axicon lens that perfectly collimates the extended filament source, resulting in improved spatial and temporal focusing of the THz pulse.

Pulsed THz radiation under ultrafast optical discharge of vacuum photodiode

In this paper, we first present an experimental demonstration of terahertz radiation pulse generation with energy up to 5 pJ under the electron emission during ultrafast optical discharge of a vacuum photodiode. We use a femtosecond optical excitation of metallic copper photocathode for the generation of ultrashort electron bunch and up to 45 kV/cm external electric field for the photo-emitted electron acceleration. Measurements of terahertz pulses energy as a function of emitted charge density, incidence angle of optical radiation and applied electric field have been provided. Spectral and polarization characteristics of generated terahertz pulses have also been studied. The proposed semi-analytical model and simulations in COMSOL Multiphysics prove the experimental data and allow for the optimization of experimental conditions aimed at flexible control of radiation parameters.Graphical

Numerical investigation of a THz-driven dielectric accelerator with a Bragg-reflector for accelerating sub-relativistic electron beams

Structure-based novel accelerators exhibit significant potential for substantial reduction in size and associated costs of future accelerators. Utilizing high-power THz sources in dielectric accelerator structures presents a favorable compromise for achieving elevated gradients and alleviating beam injection requirements. We conducted numerical investigations on an energy-efficient dielectric single grating structure accompanied by a Bragg-reflector, employing THz pulses to generate a phase-modified field for accelerating sub-relativistic electron beams. The structural parameters were optimized to enhance the strength of the acceleration field. The simulation results demonstrate that the side-coupling single grating structure, accompanied by a Bragg-reflector, designed for sub-relativistic electron beam acceleration, can increase the relative structural energy efficiency by more than 50% compared to a dual-grating accelerator structure. Moreover, it offers an available maximum acceleration gradient of up to 400 MeV m−1.

Reconfigurable Chiral Spintronic THz Emitters

AbstractCollective spin arrangements manifest diverse spin textures, encompassing ferromagnetism, antiferromagnetism, and chiral vortices. However, mapping these spin textures in ultrathin magnetic multilayers has remained elusive. A reconfigurable chiral spintronic terahertz emission method is introduced through investigations on a model system of synthetic antiferromagnet and the spin information of individual ferromagnet (FM) layers is extracted. Upon femtosecond photoexcitation of the synthetic antiferromagnet (FM1/Ru/FM2), the ferromagnets generate a pair of linearly polarized ultrafast spin currents, which, after relaxation at the FM/Ru interface, emit corresponding THz pulses. The Ruderman–Kittel–Kasuya–Yosida interactions between the two FMs give rise to magnetic‐field‐controlled spin textures causing a spin relaxation imbalance at the interfaces and induce a phase shift between the orthogonal components of the emitted terahertz fields, consequently reconfiguring the polarization of the emitted terahertz field from linear to circular. This approach offers a novel means of investigating electronic and magnetic states in ultrathin spintronic heterostructures, low‐dimensional quantum materials, topological insulators, and Weyl semimetals. Furthermore, it enables the exploration of spin textures, including skyrmions, merons, and solitons.

Active ballistic orbital transport in Ni/Pt heterostructure

Orbital current, defined as the orbital character of Bloch states in solids, can travel with larger coherence length through a broader range of materials than its spin counterpart, facilitating a robust, higher density and energy efficient information transmission. Hence, active control of orbital transport plays a pivotal role in the progress of the evolving field of quantum information technology. Unlike spin angular momentum, orbital angular momentum couples to phonon angular momentum efficiently via orbital-crystal momentum (L-k) coupling, allowing us to control orbital transport through crystal field potential mediated angular momentum transfer. Here, leveraging the orbital dependant efficient L-k coupling, we have experimentally demonstrated the active control of orbital current velocity in Ni/Pt heterostructure. We observe terahertz emission from Ni/Pt heterostructure via long-range ballistic orbital transport, as evidenced by the delay, and chirping in the emitted THz pulse correlating with increased Pt thickness. Additionally, we also have identified a critical energy density required to overcome collisions in orbital transport, enabling a swifter flow of orbital current. Femtosecond light driven active control of the ballistic orbital transport lays the foundation for the development of dynamic optorbitronics for transmitting information over extended distance.

Light-Field-Driven Non-Ohmic Current Generation by an Intense THz Pulse in a Weyl Semimetal

Light-Field-Driven Non-Ohmic Current Generation by an Intense THz Pulse in a Weyl Semimetal