Interactions between particle and particle layers are fundamental in modeling deposition processes. The complex mechanical behaviors of these layers pose significant challenges in precisely predicting the rebound characteristics of incident particle, especially at the micron and nanoscale. Very few related experimental studies have been reported in this area. To better control the structure of particle layers and offer a path to more systematic research, this study introduces the particle self-assembly method, combined with high-speed imaging technology, to investigate the influence of particle monolayer, their diameters, and impact velocity on critical capture velocity (vcr), normal coefficient of restitution (COR), and angle deflection of incident particles. Results indicate that self-assembled particle layers remain stable within an impact velocity range and experimental data within this stable range exhibit good repeatability. These layers significantly enhance kinetic energy dissipation. A semi-logarithmic plot revealed a negative linear relationship between vcr and particle size ratio. The effect of particle layer on COR depends on particle layer diameter and impact velocity. Specifically, the dissipation of particle layer diminishes and approaches zero for smaller layer particles (0.5 μm), but increases and stabilizes for larger particles (2 μm). Moreover, statistical results indicate that angle deflection decreases as particle size ratio increases, aligning with a power-law relationship predicted by Monte Carlo simulations. Overall, this study presents a novel method for understanding micro and nano particle layers' influence on incident particle dynamics.
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