Presence Of Strong Electric Field Research Articles

Keldysh crossover in one-dimensional Mott insulators

Recent advancements in pulse laser technology have facilitated the exploration of nonequilibrium spectroscopy of electronic states in the presence of strong electric fields across a broad range of photon energies. The Keldysh crossover serves as an indicator that distinguishes between excitations resulting from photon absorption triggered by near-infrared multicycle pulses and those arising from quantum tunneling induced by terahertz pulses. Using a time-dependent density-matrix renormalization group, we investigate the emergence of the Keldysh crossover in a one-dimensional (1D) Mott insulator. We find that the Drude weight is proportional to photo-doped doublon density when a pump pulse induces photon absorption. In contrast, the Drude weight is suppressed when a terahertz pulse introduces doublons and holons via quantum tunneling. The suppressed Drude weight accompanies glassy dynamics with suppressed diffusion, which is a consequence of strong correlations and exhibits finite polarization decaying slowly after pulse irradiation. In the quantum tunneling region, entanglement entropy slowly grows logarithmically. These contrasting behaviors between the photon-absorption and quantum tunneling regions are a manifestation of the Keldysh crossover in 1D Mott insulators and provide a novel methodology for designing the localization and symmetry of electronic states called subcycle-pulse engineering.

Electric charging effects on insulating surfaces in cryogenic liquids.

This paper presents a new technique to study the adsorption and desorption of ions and electrons on insulating surfaces in the presence of strong electric fields in cryoliquids. The experimental design consists of a compact cryostat coupled with a sensitive electro-optical Kerr device to monitor the stability of the electric fields. The behavior of nitrogen and helium ions on a poly(methyl methacrylate) (PMMA) surface was compared to a PMMA surface coated with a mixture of deuterated polystyrene and deuterated polybutadiene. Ion accumulation and removal on these surfaces were unambiguously observed. Within the precision of the data, both surfaces behave similarly for the physisorbed ions. The setup was also used to measure the (quasi-)static dielectric constant of PMMA at T ≈ 70K. The impact of the ion adsorption on the search for a neutron permanent electric dipole moment in a cryogenic environment, such as the nEDM@SNS experiment, is discussed.

Self-consistent multi-component simulation of plasma turbulence and neutrals in detached conditions

Simulations of high-density deuterium plasmas in a lower single-null magnetic configuration based on a TCV discharge are presented. We evolve the dynamics of three charged species (electrons, and ), interacting with two neutrals species ( and ) through ionization, charge-exchange, recombination and molecular dissociation processes. The plasma is modelled by using the drift-reduced fluid Braginskii equations, while the neutral dynamics is described by a kinetic model. To control the divertor conditions, a puffing is used and the effect of increasing the puffing strength is investigated. The increase in fuelling leads to an increase of density in the scrape-off layer and a decrease of the plasma temperature. At the same time, the particle and heat fluxes to the divertor target decrease and the detachment of the inner target is observed. The analysis of particle and transport balance in the divertor volume shows that the decrease of the particle flux is caused by a decrease of the local neutral ionization together with a decrease of the parallel velocity, caused by the lower plasma temperature and the increase in momentum losses. The relative importance of the different collision terms is assessed, showing the crucial role of molecular interactions, as they are responsible for increasing the atomic neutral density and temperature, since most of the neutrals are produced by molecular activated recombination and dissociation. The presence of strong electric fields in high-density plasmas is also shown, revealing the role of the E × B drift in setting the asymmetry between the divertor targets. Simulation results are in agreement with experimental observations of increased density decay length, attributed to a decrease of parallel transport, together with an increase of plasma blob size and radial velocity.

Pair production as a probe for the dynamics of nuclear fission and α decay

Electron-positron pairs can be produced via the Schwinger mechanism in the presence of strong electric fields. In particular, the fields involved in $\alpha$ decay and nuclear fission are strong enough to produce them. The energy of the $e^+e^-$ pair is related to the relative distance and velocity of the daughter nuclei. Thus, the energy distribution of the produced pairs can give information about the dynamics of the fission and $\alpha$ decay processes. A neck model of nuclear fission is used to illustrate how the pairs can be used as a probe of the dynamics.

Study of the Roberge-Weiss phase caused by external uniform classical electric field using lattice QCD approach

The effect of an external electric field on the quark matter is an important question due to the presence of strong electric fields in heavy ion collisions. In the lattice QCD approach, the case of a real electric field suffers from the ‘sign problem’, and a classical electric field is often used similar as the case of chemical potential. Interestingly, in axial gauge a uniform classical electric field actually can correspond to an inhomogeneous imaginary chemical potential that varies with coordinate. On the other hand, with imaginary chemical potential, Roberge-Weiss (R-W) phase transition occurs. In this work, the case of a uniform classical electric field is studied by using lattice QCD approach, with the emphasis on the properties of the R-W phase. Novel phenomena show up at high temperatures. It is found that, the chiral condensation oscillates with z at high temperatures, and so is the absolute value of the Polyakov loop. It is verified that the charge density also oscillates with z at high temperatures. The Polyakov loop can be described by an ansatz Ap + Σq=u,dCq exp (LτQqiazeEz), where Ap is a complex number and Cd> 0, Cu ≥ 0 are real numbers that are fitted for different temperatures and electric field strengths. As a consequence, the behavior of the phase of Polyakov loop is different depending on whether the Polyakov loop encloses the origin, which implies a possible phase transition.

Determining atmospheric electric fields using MGMR3D

Cosmic-ray particles impinging on the atmosphere induce high-energy particle cascades in air, an extensive air shower (EAS), emitting coherent radio emission. This emission is affected by the presence of strong electric fields during thunderstorm conditions. To reconstruct the atmospheric electric field from the measured radio footprint of the EAS we use an analytic model for the calculation of the radio emission, MGMR3D. In this work we make an extensive comparison between the results of a microscopic model for radio emission, CoREAS, to obtain an improved parametrization for MGMR3D in the presence of atmospheric electric fields, as well as confidence intervals. The approach to extract the electric field structure is applied successfully to an event with a complicated radio footprint measured by LOFAR during thunderstorm conditions. This shows that, with the improved parametrization, MGMR3D can be used to extract the structure of the atmospheric electric field.

Circularly polarized light-induced potentials and the demise of excited states.

In the presence of strong electric fields, the excited states of single-electron molecules and molecules with large transient dipoles become unstable because of anti-alignment, the rotation of the molecular axis perpendicular to the field vector, where bond hardening is not possible. We show how to overcome this problem by using circularly polarized electromagnetic fields. Using a full quantum description of the electronic, vibrational, and rotational degrees of freedom, we characterize the excited electronic state dressed by the field and analyze its dependence on the bond length and angle and the stability of its vibro-rotational eigenstates. Although the dynamics is metastable, most of the population remains trapped in this excited state for hundreds of femtoseconds, allowing quantum control. Contrary to what happens with linearly polarized fields, the photodissociation occurs along the initial molecular axis, not perpendicular to it.

Possible Limitations of the Particle Image Velocimetry Method in the Presence of Strong Electric Fields

While examining the airflow generated between the asymmetrical electrodes connected to high voltage, the authors investigated the possible limitations of the particle image velocimetry (PIV) method in the presence of strong electric fields. The tracer particles used in the PIV method in these conditions are affected by electromagnetic forces; therefore, it is necessary to determine whether these forces have any non-negligible negative influence on the measurement results. For this purpose, the authors theoretically analyzed all the possible forces and measured the generated airflow using PIV and constant temperature anemometry methods. The experimental and theoretical results clearly show the viability of the PIV measurement method even in these very specific conditions.

The Initial Stage of Cloud Lightning Imaged in High‐Resolution

AbstractWith LOFAR we have been able to image the development of lightning flashes with meter‐scale accuracy and unprecedented detail. We discuss the primary steps behind our most recent lightning imaging method. To demonstrate the capabilities of our technique we show and interpret images of the first few milliseconds of two intracloud flashes. In all our flashes, the negative leaders propagate in the charge layer below the main negative charge. Among several interesting features we show that in about 2 ms after initiation the primary initial leader triggers the formation of a multitude (>10) negative leaders in a rather confined area of the atmosphere. From these only one or two continue to propagate after about 30 ms to extend over kilometers horizontally while another may propagate back to the initiation point. We also show that normal negative leaders can transition into an initial leader like state, potentially in the presence of strong electric fields. In addition, we show some initial breakdown pulses that occurred during the primary initial leader, and even during two “secondary” initial leaders that developed out of stepped leaders.

Acoustic Gain in Solids due to Piezoelectricity, Flexoelectricity, and Electrostriction

AbstractA quantitative discussion of the combined influence of three electromechanical effects: piezoelectricity, flexoelectricity, and electrostriction in solids is provided for acoustic absorption and gain. While piezoelectricity occurs in non‐centrosymmetric materials only, flexoelectricity and electrostriction exist in all materials. Two important new results are demonstrated: 1) the possibility to realize acoustic gain in all materials (centrosymmetric and non‐centrosymmetric) when the acoustic Cherenkov condition is fulfilled, and 2) realization of acoustic gain in the presence of a strong dc electric field, even when the Cherenkov condition is not fulfilled, in the case of strong cross‐coupling between piezoelectricity, flexoelectricity, and electrostriction. A simple analytical expression for the acoustic dispersion relation is derived for the combined effect of piezoelectricity, flexoelectricity, and electrostriction. At lower frequencies, the piezoelectric effect dominates for inversion‐asymmetric materials. At high frequencies (≈>1 MHz) flexoelectricity becomes increasingly important and eventually provides a major mechanism for gain and absorption in barium titanate (BaTiO3). In the presence of strong electric fields (≈>1 MV m−1), electrostriction provides a dominant isolated contribution to absorption/gain in BaTiO3. Strong coupling between the three electromechanical contributions determines the total absorption/gain coefficient.

Growth mechanism for nanotips in high electric fields

In this work we show using atomistic simulations that the biased diffusion in high electric field gradients creates a mechanism whereby nanotips may start growing from small surface asperities. It has long been known that atoms on a metallic surface have biased diffusion if electric fields are applied and that microscopic tips may be sharpened using fields, but the exact mechanisms have not been well understood. Our Kinetic Monte Carlo simulation model uses a recently developed theory for how the migration barriers are affected by the presence of an electric field. All parameters of the model are physically motivated and no fitting parameters are used. The model has been validated by reproducing characteristic faceting patterns of tungsten surfaces that have in previous experiments been observed to only appear in the presence of strong electric fields. The growth effect is found to be enhanced by increasing fields and temperatures.

Particle Imaging Velocimetry Measurement of Air Flow Between High Voltage Asymmetrical Electrodes

This paper deals with the airflow generation phenomenon occurring on a system of strongly asymmetrical electrodes connected to high DC voltage. The main focus was to measure the airflow directly between the electrodes using Particle Image Velocimetry. The authors are well aware of the many difficulties presented by the task of measuring in the presence of strong electric fields and the paper also describes the means used to overcome these issues. The results of performed measurements are presented, their agreement with theoretical description of given phenomenon is discussed and several possible practical applications are proposed.

Ab initio Calculation of the Dipole Moment Function of the OH Radical Ground State

Recently it has been theoretically predicted and experimentally confirmed that at altitudes of 80–110 km from the Earth’s surface the signals of the global navigation satellite systems (GNSS) are delayed as a result of a multiple resonance scattering by the Rydberg complexes. The attenuation of GNSS signals occurs mainly in the lower atmosphere layers, where the greatest effect is achieved through interaction with charged aerosol layers. A thunderstorm conditions are of particular interest whereby the presence of strong electric fields and hydration of aerosols can lead to the detachment of OH radicals from water clusters. Since the spectrum of radiation and absorption of these radicals for rotational transitions is part of the microwave range, they are expected to make an additional resonance contribution to the delay of radio signals thus necessitating a detailed study of the electronic structure of the OH radical. This paper offers the ab initio calculations of the dipole moment function for the ground X2Π state of the OH molecule using the dipole length approach and the finite-field method. The comparison with the experiment shows that in extended model spaces the approximation of the dipole length leads to more accurate values of the dipole moment than the finite-field method.

Effect of Ion Streaming on Diffusion of Dust Grains in Dissipative System

The presence of strong electric fields in the sheath region of laboratory complex plasma induces an ion drift and perturbs the field around dust grains. The downstream focusing of ions leads to the formation of oscillatory kind of attractive wake potential which superimpose with the normal Debye-Huckel (DH) potential. The structural properties of complex plasma and diffusion coefficient of dust grains in the presence of such a wake potential have been investigated using Langevin dynamics simulation in the subsonic regime of ion flow. The study reveals that the diffusion of dust grains is strongly affected by the ion flow, so that the diffusion changes its character in the wake potential to the DH potential dominant regimes. The dependence of the diffusion coefficient on the parameters, such as the neutral pressure, dust grain size, ion flow velocity, and Coulomb coupling parameter, have been calculated for the subsonic regime by using the Green-Kubo expression, which is based on the integrated velocity autocorrelation function. It is found that the diffusion and the structural property of the system is intimately connected with the interaction potential and significantly get affected in the presence of ion flow in the subsonic regime.

(Invited) Beyond Electrostatic Effects at Oxide Hetero-Interfaces: Electrochemical Phase Change, Strong Electric Fields, and Elastic Strain

Transition metal oxide hetero-interfaces are interesting due to the distinctly different properties that can arise from their interfaces, such as memristive behavior, superconductivity, high catalytic activity and magnetism. These interfaces are the source for local heterogeneities in composition, atomic structure and electronic structure. Classically, defect redistribution is quantified at the continuum level by concurrent solution of Poisson’s equation for the electrostatic potential and the steady-state equilibrium drift-diffusion equation for each defect. It is possible to inform this level of modeling with first principles calculations of band off-sets, and defect formation and segregation energies at thermodynamically relevant conditions. This approach had numerous successful implementations, including the quantification of charge transport properties at surfaces and grain boundaries. In this talk, I will discuss three phenomena that also need to be considered in a broader framework of defect structures and distributions at oxide hetero-interfaces. 1) Presence of strong electric fields that can cause polarization of defective systems and affect the defect abundance and structure. We have assessed this effect on neutral oxygen vacancies in simple binary oxides from first principles calculations. 2) Phase change under the effect of local electrostatic potential because of a change in the electrochemical potential of oxygen. We have assessed the ability to trigger phase change electrochemically in two classes of oxides, SrCoOx and VOx, and have quantified the phases and the corresponding distinctly different electronic properties by combining in operando x-ray diffraction and x-ray photoelectron and absorption spectroscopy. The results have implications both for oxide hetero-interfaces and for oxide electronic devices that aim to control properties electrically. 3) Elastic strain, that affect the stability and mobility of defects. In this recent work, we have focused on the stability of electronic defects, specifically the electron polarons versus free electrons SrTiO3, as a function of temperature and hydrostatic stress, by combining first principles calculations and quasi harmonic approximation. Our results demonstrate that it is possible to control the type of electronic defect, and so the transport properties, by means of electro-chemo-mechanics.

Nonlinear ionic transport through microstructured solid electrolytes: homogenization estimates

We consider the transport of multiple ionic species by diffusion and migration through microstructured solid electrolytes in the presence of strong electric fields. The assumed constitutive relations for the constituent phases follow from convex energy and dissipation potentials which guarantee thermodynamic consistency. The effective response is heuristically deduced from a multi-scale convergence analysis of the relevant field equations. The resulting homogenized response involves an effective dissipation potential per species. Each potential is mathematically akin to that of a standard nonlinear heterogeneous conductor. A ‘linear-comparison’ homogenization technique is then used to generate estimates for these nonlinear potentials in terms of available estimates for corresponding linear conductors. By way of example, use is made of the Maxwell-Garnett and effective-medium linear approximations to generate estimates for two-phase systems with power-law dissipation. Explicit formulas are given for some limiting cases. In the case of threshold-type behavior, the estimates exhibit non-analytical dilute limits and seem to be consistent with fields localized in low energy paths.

The LTCC device for miniature plasma generators characterization

Purpose The purpose of this paper is a presentation of a miniature vertical dielectric barrier discharge (DBD) plasma generators. The presented devices, with sub- and superstrate, were made using low temperature co-fired ceramics (LTCC). Such construction allowed to measure discharge spectra and device temperature easily. Design/methodology/approach The generators were made in the Du Pont 951 system with silver vertical metallizations and PdAg contacts. The devices had electrodes with different width and height. Also, the distance between them could be established. They were placed on substrate with buried temperature sensor and covered with a ceramic lid. The lid had opening to measure emitted light. Different configurations of vertical DBD were tested. Findings Geometry of vertical metallizations influences on spectra, as well as distance between them. Signal-to-noise ratio had a maximum for certain generators and can be measured by the intensity of highest peak. Research limitations/implications Height of vertical metallizations is limited by the difference in shrinkage of LTCC tape and via paste. Parameters of temperature sensors vary between measurements, according to rapid changes of temperature and presence of strong electric field. Practical implications The generators can be used for creating discharge for optical emission spectrometry. It is a convenient method to determine the amount of selected gas compounds. Originality/value This paper shows fabrication and performance of the novel vertical DBD generators with ceramic additions for convenient spectra measurement and monitoring temperature of the device during work.

Determining internal screening electric field of working polymer light emitting diodes

This study provides a method of determining the internal electric field of polymer light emitting diodes (LEDs) in the working condition. The method employs Stark signals induced by triangular shaped pulse biases and enables estimates of the internal field in a broad voltage region. The internal field under forward bias is shown to be determined by the screening effect caused by injected carriers. Spatial distribution calculated for the LED suggests the presence of strong electric field formed by accumulated carriers near the electrodes. The proposed method is applicable to a variety of devices and can promote understanding of veiled roles of internal fields on device operation.

Activation energies of colloidal particle aggregation: towards a quantitative characterization of specific ion effects

A quantitative description of specific ion effects is an essential and focused topic in colloidal and biological science. In this work, the dynamic light scattering technique was employed to study the aggregation kinetics of colloidal particles in the various alkali ion solutions with a wide range of concentrations. It indicated that the activation energies could be used to quantitatively characterize specific ion effects, which was supported by the results of effective hydrodynamic diameters, aggregation rates and critical coagulation concentrations. At a given concentration of 25 mmol L(-1), the activation energies for Li(+) are 1.2, 5.7, 28, and 126 times as much for Na(+), K(+), Rb(+), and Cs(+), respectively. Most importantly, the activation energy differences between two alkali cation species increase sharply with decrease of electrolyte concentrations, implying the more pronounced specific ion effects at lower concentrations. The dominant role of electrolyte cations during the aggregation of negatively charged colloidal particles was confirmed by alternative anions. Among the various theories, only the polarization effect can give a rational interpretation of the above specific ion effects, and this is substantially supported by the presence of strong electric fields from montmorillonite surfaces and its association mainly with electrolyte cations and montmorillonite particles. The classical induction theory, although with inclusion of electric field, requires significant corrections because it predicts an opposite trend to the experimentally observed specific ion effects.

A Robust C-Band Hydrometeor Identification Algorithm and Application to a Long-Term Polarimetric Radar Dataset

AbstractA new 10-category, polarimetric-based hydrometeor identification algorithm (HID) for C band is developed from theoretical scattering simulations including wet snow, hail, and big drops/melting hail. The HID is applied to data from seven wet seasons in Darwin, Australia, using the polarimetric C-band (C-POL) radar, to investigate microphysical differences between monsoon and break periods. Scattering simulations reveal significant Mie effects with large hail (diameter > 1.5 cm), with reduced reflectivity and enhanced differential reflectivity Zdr and specific differential phase Kdp relative to those associated with S band. Wet snow is found to be associated with greatly depreciated correlation coefficient ρhv and moderate values of Zdr. It is noted that large oblate liquid drops can produce the same electromagnetic signatures at C band as melting hail falling quasi stably, resulting in some ambiguity in the HID retrievals. Application of the new HID to seven seasons of C-POL data reveals that hail and big drops/melting hail occur much more frequently during break periods than during monsoon periods. Break periods have a high frequency of vertically aligned ice above 12 km, suggesting the presence of strong electric fields. Reflectivity and mean drop diameter D0 statistics demonstrate that convective areas in both monsoon and break periods may have robust coalescence or melting precipitation ice processes, leading to enhanced reflectivity and broader distributions of D0. Conversely, for stratiform regions in both regimes, mean reflectivity decreases below the melting level, indicative of evaporative processes. Break periods also have larger ice water path fractions, indicating substantial mixed-phase precipitation generation as compared with monsoonal periods. In monsoon periods, a larger percentage of precipitation is produced through warm-rain processes.