Precision Frequency Metrology Research Articles

Highly coherent phase-lock of an 8.1 μm quantum cascade laser to a turn-key mid-IR frequency comb

A continuous-wave Fabry–Pérot quantum cascade laser (QCL) emitting at 8.1 μm operating in the single mode regime has been coherently phase locked to a turn-key low-noise commercial mid-Infrared (mid-IR) optical frequency comb. The stability of the comb used as a reference is transferred to the QCL resulting in an integrated residual phase error of 0.4 rad. The laser linewidth is narrowed by more than two orders of magnitude reaching sub-kHz level at 1 ms observation time, limited by the spectral purity of the mid-IR comb. Our experiment is an important step toward the development of both powerful and metrology-grade QCLs and fully stabilized QCL frequency comb and opens perspectives for precision measurements and frequency metrology in the mid-IR.

Axion Wind Detection with the Homogeneous Precession Domain of Superfluid Helium-3

Axions and axionlike particles may couple to nuclear spins like a weak oscillating effective magnetic field, the "axion wind." Existing proposals for detecting the axion wind sourced by dark matter exploit analogies to nuclear magnetic resonance (NMR) and aim to detect the small transverse field generated when the axion wind resonantly tips the precessing spins in a polarized sample of material. We describe a new proposal using the homogeneous precession domain of superfluid ^{3}He as the detection medium, where the effect of the axion wind is a small shift in the precession frequency of a large-amplitude NMR signal. We argue that this setup can provide broadband detection of multiple axion masses simultaneously and has competitive sensitivity to other axion wind experiments such as CASPEr-Wind at masses below 10^{-7} eV by exploiting precision frequency metrology in the readout stage.

Magnonic Frequency Comb through Nonlinear Magnon-Skyrmion Scattering.

An optical frequency comb consists of a set of discrete and equally spaced frequencies and has found wide applications in the synthesis over a broad range of spectral frequencies of electromagnetic waves and precise optical frequency metrology. Despite the analogies between magnons and photons in many aspects, the analog of an optical frequency comb in magnonic systems has not been reported. Here, we theoretically study the magnon-skyrmion interaction and find that a magnonic frequency comb (MFC) can be generated above a threshold driving amplitude, where the nonlinear scattering process involving three magnons prevails. The mode spacing of the MFC is equal to the breathing-mode frequency of the skyrmion and is thus tunable by either electric or magnetic means. The theoretical prediction is verified by micromagnetic simulations, and the essential physics can be generalized to a large class of magnetic solitons. Our findings open a new pathway to observe frequency comb structures in magnonic devices that may inspire the study of fundamental nonlinear physics in spintronic platforms in the future.

Microscale whispering-gallery-mode light sources with lattice-confined atoms

Microlasers, relying on the strong coupling between active particles and optical microcavity, exhibit fundamental differences from conventional lasers, such as multi-threshold/thresholdless behavior and nonclassical photon emission. As light sources, microlasers possess extensive applications in precision measurement, quantum information processing, and biochemical sensing. Here we propose a whispering-gallery-mode microlaser scheme, where ultracold alkaline-earth metal atoms, i.e., gain medium, are tightly confined in a two-color evanescent lattice that is in the ring shape and formed around a microsphere. To suppress the influence of the lattice-induced ac Stark shift on the moderately-narrow-linewidth laser transition, the red-detuned trapping beams operate at a magic wavelength while the wavelength of the blue-detuned trapping beam is set close to the other magic wavelength. The tiny mode volume and high quality factor of the microsphere ensure the strong atom-microcavity coupling in the bad-cavity regime. As a result, both saturation photon and critical atom numbers, which characterize the laser performance, are substantially reduced below unity. We explore the lasing action of the coupled system by using the Monte Carlo approach. Our scheme may be potentially generalized to the microlasers based on the forbidden clock transitions, holding the prospect for microscale active optical clocks in precision measurement and frequency metrology.

Corrigendum to “Axion detection with precision frequency metrology” [Phys. Dark Universe 26 (2019) 100345

Corrigendum to “Axion detection with precision frequency metrology” [Phys. Dark Universe 26 (2019) 100345

Switching dynamics of dark-pulse Kerr frequency comb states in optical microresonators

Dissipative Kerr solitons are localized structures that exist in optical microresonators. They lead to the formation of microcombs --- chip-scale frequency combs that could facilitate precision frequency synthesis and metrology by capitalizing on advances in silicon photonics. Previous demonstrations have mainly focused on anomalous dispersion microresonators. Notwithstanding, localized structures also exist in the normal dispersion regime in the form of circulating dark pulses, but their physical dynamics is far from being understood. Here, we report the discovery of reversible switching between coherent dark-pulse Kerr combs, whereby distinct states can be accessed deterministically. Furthermore, we reveal that the formation of dark-pulse Kerr combs is associated with the appearance of a new resonance, a feature that has never been observed for dark-pulses and is ascribed to soliton behavior. These results contribute to understanding the nonlinear physics in few-mode microresonators and provide insight into the generation of microcombs with high conversion efficiency.

Ultraviolet to mid-infrared supercontinuum generation in single-crystalline aluminum nitride waveguides.

We demonstrate ultrabroadband supercontinuum generation from ultraviolet to mid-infrared wavelengths in single-crystalline aluminum nitride waveguides. Tunable dispersive waves are observed at the mid-infrared regime by precisely controlling the waveguide widths. In addition, ultraviolet light is generated through cascaded second-harmonic generation in the modal phase-matched waveguides. Numerical simulation indicates a high degree of coherence of the generated spectrum at around the telecom pump and two dispersive waves. Our results establish a reliable path for multiple octave supercontinuum comb generation in single-crystalline aluminum nitride to enable applications including precision frequency metrology and spectroscopy.

Tailoring the waveguide dispersion of nonlinear fibers for supercontinuum generation with superior intrapulse coherence

Spectral coherence is an important prerequisite for many applications of femtosecond supercontinua, including precision frequency metrology, attosecond science, and high-field physics. These applications often critically depend on measurement of the carrier-envelope phase via f − 2 f interferometry. As mode-locked laser sources cannot directly provide octave-spanning spectra, one typically resorts to spectral broadening in highly nonlinear optical fibers to generate the necessary spectral coverage. This process comes with a caveat, as coherence can be severely degraded in the broadening process. This degradation can be mitigated by suitable choice of a fiber dispersion profile. Here we numerically investigate prototypical fiber designs and analyze their susceptibility to coherence degradation. It is found that the generally favored soliton fission process provides the best broadening efficiency at the expense of rather scarce coherence conditions. Sufficient pulse energy provided, all-normally dispersive fiber designs fare far better in terms of spectral coherence. Finally, fiber designs with flattened normal dispersion provide the best compromise between efficiency and resulting spectral coherence. Our study indicates that the spectral width of a supercontinuum may be deceiving. Even when compressible into a short pulse, this does not automatically qualify for sufficient spectral coherence to conduct carrier-envelope-phase-sensitive experiments. The numerical simulations in this study provide a guideline for coherent spectral broadening. In turn, these guidelines may help to improve carrier-envelope phase stabilization and, in particular, to enable stabilization of laser oscillators that have previously proven difficult to stabilize.

Axion detection with precision frequency metrology

We investigate a new class of galactic halo axion detection techniques based on precision frequency and phase metrology. Employing equations of axion electrodynamics, it is demonstrated how a dual mode cavity exhibits linear mode-mode coupling mediated by the axion upconversion and axion downconversion processes. The approach demonstrates phase sensitivity with an ability to detect axion phase with respect to externally pumped signals. Axion signal to phase spectral density conversion is calculated for open and closed loop detection schemes. The fundamental limits of the proposed approach come from the precision of frequency and environment control electronics, rather than fundamental thermal fluctuations allowing for table-top experiments approaching state-of-the-art cryogenic axion searches in sensitivity. Practical realisations are considered, including a TE-TM mode pair in a cylindrical cavity resonator and two orthogonally polarised modes in a Fabry-P{\'e}rot cavity.

Octave-spanning supercontinuum generation in nanoscale lithium niobate waveguides.

We demonstrate octave-spanning supercontinuum generation in unpoled lithium niobate waveguides, which are engineered to possess anomalous dispersion and pumped by a turn-key femtosecond laser centered at 1560nm. Tunable dispersive waves and strong phase-matched second-harmonic generation are both observed by controlling the widths of the waveguides. The major features of the experimental spectra are reproduced by numerical modeling of the generalized nonlinear Schrödinger equation, which can be used to guide waveguide designs for tailoring the supercontinuum spectrum. Our results identify a path to a simple and integrable supercontinuum source in lithium niobate nanophotonic platform and will enable new capabilities in precision frequency metrology.

Generation of multiple near-visible comb lines in an AlN microring via χ(2) and χ(3) optical nonlinearities

On-chip frequency upconversion of a near-infrared (NIR) Kerr comb in a χ(2) and χ(3) system provides a convenient route to extending the comb spectra into the visible band. Yet to date, only limited visible or near-visible comb lines have been obtained using this scheme. In this work, we demonstrate the generation of multiple near-visible comb lines based on spectral translation from a broadband NIR Kerr comb. This physical process is implemented in an aluminum nitride (AlN)-on-sapphire microring, where we achieve a wideband frequency upconversion by incorporating the phase-mismatched fundamental and first-order near-visible modes. Upon tuning the pump into the resonance with sufficient power, we attain a broadband NIR Kerr comb and 153 corresponding near-visible comb lines in 720–840 nm with a reasonable efficiency over 4.1 × 10−5%. The wideband frequency upconversion can be adapted to on-chip frequency stabilization of self-referenced microcombs, as required for precision optical clocks and frequency metrology.

Relativistic and QED Effects in the Fundamental Vibration of T_{2}.

The hydrogen molecule has become a test ground for quantum electrodynamical calculations in molecules. Expanding beyond studies on stable hydrogenic species to the heavier radioactive tritium-bearing molecules, we report on a measurement of the fundamental T_{2} vibrational splitting (v=0→1) for J=0-5 rotational levels. Precision frequency metrology is performed with high-resolution coherent anti-Stokes Raman spectroscopy at an experimental uncertainty of 10-12MHz, where sub-Doppler saturation features are exploited for the strongest transition. The achieved accuracy corresponds to a 50-fold improvement over a previous measurement, and it allows for the extraction of relativistic and QED contributions to T_{2} transition energies.

Role of Intrapulse Coherence in Carrier-Envelope Phase Stabilization.

The concept of coherence is of fundamental importance for describing the physical characteristics of light and for evaluating the suitability for experimental application. In the case of pulsed laser sources, the pulse-to-pulse coherence is usually considered for a judgment of the compressibility of the pulse train. This type of coherence is often lost during propagation through a highly nonlinear medium, and pulses prove incompressible despite multioctave spectral coverage. Notwithstanding the apparent loss of interpulse coherence, however, supercontinua enable applications in precision frequency metrology that rely on coherence between different spectral components within a laser pulse. To judge the suitability of a light source for the latter application, we define an alternative criterion, which we term intrapulse coherence. This definition plays a limiting role in the carrier-envelope phase measurement and stabilization of ultrashort pulses. It is shown by numerical simulation and further corroborated by experimental data that filamentation-based supercontinuum generation may lead to a loss of intrapulse coherence despite near-perfect compressibility of the pulse train. This loss of coherence may severely limit active and passive carrier-envelope phase stabilization schemes and applications in optical high-field physics.

Excess carrier-envelope phase noise generation in saturable absorbers.

Attosecond spectroscopy and precision frequency metrology depend on the stabilization of the carrier-envelope phase (CEP) of mode-locked lasers. Unfortunately, the phase of only a few types of lasers can be stabilized to jitters in the few-hundred millirad range. In a comparative experimental study, we analyze a femtosecond Ti:sapphire laser and three mode-locked fiber lasers. We numerically demodulate recorded time series of the free-running carrier-envelope beat note. Our analysis indicates a correlation between amplitude and frequency fluctuations at low Fourier frequencies for essentially all lasers investigated. While this correlation typically rolls off at frequencies beyond 100kHz, we see clear indications for a broadband coupling mechanism in one of the fiber lasers. We suspect that the observed coupling mechanism acts to transfer intracavity power fluctuations into excess phase noise. This coupling mechanism is related to the mode-locking mechanism employed and not to the gain medium itself. We further verify this hypothesis by numerical simulations, which identify resonances of the saturable absorber mirror as a possible explanation for the coupling mechanism. Finally, we discuss how to avoid a detrimental influence of such resonances.

Precision measurement and frequency metrology with ultracold atoms

Abstract Precision measurement and frequency metrology have pushed many scientific and technological frontiers in the field of atomic, molecular and optical physics. In this article, we provide a brief review on the recent development of optical atomic clocks, with an emphasis placed on the important inter-dependence between measurement precision and systematic effects. After presenting a general discussion on the motivation and techniques behind the development of optical lattice clocks, where the use of many atoms greatly enhances the measurement precision, we present the JILA strontium optical lattice clock as the leading system of frequency metrology with the lowest total uncertainty, and we describe other related research activities. We discuss key ingredients that have enabled the optical lattice clocks with ultracold atoms to reach the 18th digit in both precision and accuracy. Furthermore, we discuss extending the power of precision clock spectroscopy to study quantum many-body physics and to provide control for atomic quantum materials. In addition, we explore future research directions that have the potential to achieve even greater precision.

Prospects for atomic clocks based on large ion crystals

We investigate the feasibility of precision frequency metrology with large ion crystals. For clock candidates with a negative differential static polarisability, we show that micromotion effects should not impede the performance of the clock. Using Lu+ as a specific example, we show that quadrupole shifts due to the electric fields from neighbouring ions do not significantly affect clock performance. We also show that effects from the tensor polarisability can be effectively managed with a compensation laser at least for a small number of ions (<1000). These results provide new possibilities for ion-based atomic clocks, allowing them to achieve stability levels comparable to neutral atoms in optical lattices and a viable path to greater levels of accuracy.

Design of the Ion Trap and Vacuum System for 171Yb-ion Optical Frequency Standard

We are developing a frequency standard based on the ultra-narrow electric octupole transition of the ytterbium-ion (171Yb+), which is in the optical wavelength region. In this article, we describe optimized design of our end-cap type Paul trap which will be used for trapping single ions for precision frequency metrology. Selection of the materials for fabricating different parts of the trap assembly is also described. Customized design of the ultra-high vacuum chamber, which houses the ion trap, oven producing ytterbium atomic beam, compensation electrodes and high numerical aperture fluorescence collection lens together with four pairs of optical viewports is lastly described.

Mode-resolved 10-GHz frequency comb from a femtosecond optical parametric oscillator.

We report a 10-GHz frequency comb generated by filtering a 333.3-MHz OPO frequency comb with a Fabry-Perot (FP) cavity, which was directly stabilized to the incident fundamental comb. This result is supported by a detailed analysis of the Vernier-effect-induced multiple peaks in the transmitted comb power as the FP cavity spacing is detuned. Modes of the generated 10-GHz comb were clearly resolved by a Fourier transform spectrometer with a spectral resolution of 830MHz, considerably better than the Nyquist sampling limit. The potentially broad tuning range of this mode-resolved OPO frequency comb opens unique opportunities for precise frequency metrology and high-precision spectroscopy.

Visible supercontinuum generation in large-core photonic crystal fiber with high air-filling fraction

We demonstrate new experimental results for visible supercontinuum generation in large-core photonic crystal fiber with high air-filling fraction. Supercontinuum is generated by picosecond pulses from a passively mode-locked Yb:KGW laser. A smooth supercontinuum generation near 800 nm is achieved using 4.5 m long large-core photonic crystal fiber even with 6 mW average coupled power. These results are of interest in high power white light sources and have potential applications in precise frequency metrology and spectroscopy. The data obtained could be used also in theoretical studies of nonlinear interaction in large-core photonics crystal fibers with high air-filling fraction.

On-chip frequency comb generation at visible wavelengths via simultaneous second- and third-order optical nonlinearities.

Microresonator-based frequency comb generation at or near visible wavelengths would enable applications in precise optical clocks, frequency metrology, and biomedical imaging. Comb generation in the visible has been limited by strong material dispersion and loss at short wavelengths, and only very narrowband comb generation has reached below 800 nm. We use the second-order optical nonlinearity in an integrated high-Q silicon nitride ring resonator cavity to convert a near-infrared frequency comb into the visible range. We simultaneously demonstrate parametric frequency comb generation in the near-infrared, second-harmonic generation, and sum-frequency generation. We measure 17 comb lines converted to visible wavelengths extending to 765 nm.