Prague Asterix Laser System Research Articles

Characterization of hot electrons generated by laser–plasma interaction at shock ignition intensities

In an experiment carried out at the Prague Asterix Laser System at laser intensities relevant to shock ignition conditions (I > 1016 W/cm2), the heating and transport of hot electrons were studied by using several complementary diagnostics, i.e., Kα time-resolved imaging, hard x-ray filtering (a bremsstrahlung cannon), and electron spectroscopy. Ablators with differing composition from low Z (parylene N) to high Z (nickel) were used in multilayer planar targets to produce plasmas with different coronal temperature and collisionality and modify the conditions of hot-electron generation. The variety of available diagnostics allowed full characterization of the population of hot electrons, retrieving their conversion efficiency, time generation and duration, temperature, and angular divergence. The obtained results are shown to be consistent with those from detailed simulations and similar inertial confinement fusion experiments. Based on the measured data, the advantages, reliability, and complementarity of the experimental diagnostics are discussed.

Strongly magnetized plasma produced by interaction of nanosecond kJ-class laser with snail targets

Magnetized plasma studies are necessary for many applied studies, including laser-driven inertial fusion, modeling astrophysically relevant phenomena, and innovative industrial and medical applications. An interesting method of generating highly magnetized plasma can be based on the interaction of a laser with spiral-shaped cavity (snail-like) targets. A target shaped in this way can represent the central area of a spherical pellet that is not irradiated radially, but rather through an entrance hole allowing the laser beam to almost impact its inner surface tangentially (Pisarczyk et al 2018 Sci. Rep. 8 17 895). In the reported experiment, snail targets of various diameters were irradiated by linearly or circularly polarized radiation of a Prague asterix laser system (PALS) iodine laser delivering ∼500 J, 350 ps and 1.315 μm pulses on targets. Three-frame complex interferometry demonstrated that plasma is generated on the entire inside and outside surfaces of the snail target, starting from the very beginning of the laser–target interaction. The time-resolved records of the magnetic field and the electron density distribution inside and outside the snail target characterize the changes in the structure of the magnetized plasma. Inside the target, the magnetic field survives long after the termination of the laser–matter interaction, namely longer than 10 ns. Compared to a circularly polarized laser pulse, the irradiation of targets with a p-polarized beam increases both the emission of hot electrons (HEs) and the intensity of the magnetic field. The emission of HEs is not isotropic, and their energy distribution cannot be characterized by a single temperature.

Hot electron and x-ray generation by sub-ns kJ-class laser-produced tantalum plasma

This paper presents experimental investigation of temperature scaling and threshold of instability in hot electron and bremsstrahlung radiation from the interaction of sub-nanosecond and kilo-joule class laser pulses with a tantalum foil target at Prague Asterix Laser System. The laser intensity was varied between and W · cm−2 at the target focus. The energy distribution functions of electrons were measured by an angular array of magnetic spectrometers indicating the electron temperature in the range between 30 keV and 70 keV. The bremsstrahlung spectrum was characterized using a scintillator-based calorimeter. In particular, we show the laser-energy scaling of the total flux of hot electrons in the forward and backward directions with respect to the laser vector, the conversion efficiency of the laser energy to the energy carried by hot electrons, and the temperature of hot electrons as well as the unfolded bremsstrahlung temperature using a Monte Carlo code consistent with signals of the scintillator detector. The scaling shows that the electron flux increases discontinuously with increasing laser intensity from W · cm−2 with consequent instability in the production of hot electrons and bremsstrahlung radiation.

Morphology of Meteorite Surfaces Ablated by High-Power Lasers: Review and Applications

Under controlled laboratory conditions, lasers represent a source of energy with well-defined parameters suitable for mimicking phenomena such as ablation, disintegration, and plasma formation processes that take place during the hypervelocity atmospheric entry of meteoroids. Furthermore, lasers have also been proposed for employment in future space exploration and planetary defense in a wide range of potential applications. This highlights the importance of an experimental investigation of lasers’ interaction with real samples of interplanetary matter: meteorite specimens. We summarize the results of numerous meteorite laser ablation experiments performed by several laser sources—a femtosecond Ti:Sapphire laser, the multislab ceramic Yb:YAG Bivoj laser, and the iodine laser known as PALS (Prague Asterix Laser System). The differences in the ablation spots’ morphology and their dependence on the laser parameters are examined via optical microscopy, scanning electron microscopy, and profilometry in the context of the meteorite properties and the physical characteristics of laser-induced plasma.

2D MHD simulation of spontaneous magnetic fields generated during interaction of 1315.2-nm laser radiation with copper slabs at 1016 W/cm2

Multidimensional modeling of phenomena and processes occurring during the expansion of the laser-produced plasma for different irradiation conditions related to both the laser beam parameters and the target constructions is a very complex issue, especially when modeling requires consideration of kinetic processes associated with the development of various types of microscopic instability. Multidimensional PIC codes create such a possibility, but their use is limited to modeling phenomena even in a very narrow timescale due to the limited computational capabilities of current supercomputers. For this reason, the paper attempts to interpret the results of the spontaneous magnetic field (SMF) measurements obtained during the PALS (Prague Asterix Laser System) experiment [Pisarczyk et al., AIP Adv. 10, 115201 (2020); Pisarczyk et al., Phys. Plasmas 22, 102706 (2015)] based on the 2D magneto-hydrodynamic (MHD) model [Jach et al., Computer Modeling of Dynamic Interaction of Bodies by Free Point Method (PWN, Warsaw, 2011)]. The MHD equations were used with included arbitrary (i) current of hot electrons treating it as an additional external current and (ii) ion-sound instability responsible for the increase in anomalous resistance in areas with high temperature and low-density plasma. The spatial distribution of magnetic fields and current density obtained from 2D modeling are in acceptable agreement with the experimental results [Pisarczyk et al., Plasma Phys. Controlled Fusion 62, 115020 (2020); Zaraś-Szydłowska et al., AIP Adv. 10, 115201 (2020); Pisarczyk et al., Phys. Plasmas 22, 102706 (2015)]. The inclusion of temporal changes in anomalous resistance in modeling allowed us to explain the persistence of high SMF amplitude at the level of several megagauss after the laser pulse ended due to the effect of magnetic field freezing.

Measurement of strong electromagnetic pulses generated from solid targets at sub-ns kJ-class PALS laser facility

Measurements had been performed of strong electromagnetic pulses (EMPs) generated as a result of laser–target interaction at the sub-ns kJ-class Prague Asterix Laser System facility. Two conductive Prodyn FD5C D-dot pencil probes were used. Measurements were performed inside the experimental chamber and outside the chamber in a large chamber window 40 cm in diameter in a setup that guaranteed 6 GHz bandwidth. A very good signal-to-noise ratio (17:1) was obtained after some steps were taken to ensure proper EMP shielding of the data collection setup. The EMP signal in the time domain was found to have the form of a sharp initial spike followed by gradually decaying oscillations interspersed with some secondary spikes. The values of the vertical component of the electric field strength were estimated. The highest value recorded in this experiment was kV m−1 at a distance of 40 cm from the target. It was observed that plastic targets—particularly the 100s of µm thick plastic foils—tend to generate stronger EMP fields than Cu and Au targets. A time-frequency analysis was performed for a typical shot, clearly showing some spectral features that appear only sometime after the start of the signal and hence indicate EMP generation from secondary sources. Electrons ejected from the target were recorded with the energies exceeding 1.5 MeV, which indicates that highly energetic processes are triggered as a result of the laser–target interaction.

Design of modular multi-channel electron spectrometers for application in laser matter interaction experiments at Prague Asterix Laser System

This paper describes design, development, and implementation of a multi-channel magnetic electron spectrometer for the application in laser-plasma interaction experiments carried out at the Prague Asterix Laser System. Modular design of the spectrometer allows the setup in variable configurations to evaluate the angular distribution of hot electron emission. The angular array configuration of the electron spectrometers consists of 16 channels mounted around the target. The modules incorporate a plastic electron collimator designed to suppress the secondary radiation by absorbing the wide angle scattered electrons and photons inside the collimator. The compact model of the spectrometer measures electron energies in the range from 50keV to 1.5MeV using ferrite magnets and from 250keV to 5MeV using stronger neodymium magnets. An extended model of the spectrometer increases the measured energy range up to 21MeV or 35MeV using ferrite or neodymium magnets, respectively. Position to energy calibration was obtained using the particle tracking simulations. The experimental results show the measured angularly resolved electron energy distribution functions from interaction with solid targets. The angular distribution of hot electron temperature, the total flux, and the maximum electron energy show a directional dependence. The measured values of these quantities increase toward the target normal. For a copper target, the average amount of measured electron flux is 1.36 × 1011, which corresponds to the total charge of about 21nC.

Implementation of amplitude–phase analysis of complex interferograms for measurement of spontaneous magnetic fields in laser generated plasma

Generation of spontaneous magnetic fields (SMFs) is one of the most interesting phenomena accompanying an intense laser–matter interaction. One method of credible SMFs measurements is based on the magneto-optical Faraday effect, which requires simultaneous measurements of an angle of polarization plane rotation of a probe wave and plasma electron density. In classical polaro-interferometry, these values are provided independently by polarimetric and interferometric images. Complex interferometry is an innovative approach in SMF measurement, obtaining information on SMF directly from a phase–amplitude analysis of an image called a complex interferogram. Although the theoretical basis of complex interferometry has been well known for many years, this approach has not been effectively employed in laser plasma research until recently; this approach has been successfully implemented in SMF measurement at the Prague Asterix Laser System (PALS). In this paper, proprietary construction solutions of polaro-interferometers are presented; they allow us to register high-quality complex interferograms in practical experiments, which undergo quantitative analysis (with an original software) to obtain information on the electron density and SMFs distributions in an examined plasma. The theoretical foundations of polaro-interferometric measurement, in particular, complex-interferometry, are presented. The main part of the paper details the methodology of the amplitude–phase analysis of complex interferograms. This includes software testing and examples of the electron density and SMF distribution of a laser ablative plasma generated by irradiating Cu thick planar targets with an iodine PALS laser at an intensity above about 1016 W/cm2.

Effect of expanding plasma on propagation of electromagnetic pulses by laser-plasma interaction

Experiments were performed using the Prague Asterix Laser System to study the effect of expanding plasma on electromagnetic pulse propagation (EMP) in the interaction chamber in an intensity regime of 1016 W cm−2. Similar to the interaction that occurs between radio waves and the ionosphere, the expansion of laser-produced plasma causes the vacuum chamber to be gradually filled with inhomogeneous plasma that interacts with the emitted EMP. Combining the space-time analysis of a plasma density inside the interaction chamber and the fast Fourier transform filtering of antenna signals, we have resolved the influence of the expanding plasma on space-time characteristics of EMP.

Laser-driven strong shocks with infrared lasers at intensity of 1016 W/cm2

We present the results of an experiment on laser-driven shock waves performed at the Prague Asterix Laser system (PALS), where the fundamental frequency of the laser (1315 nm) is used to launch a strong shock in planar geometry. The experiment aims to characterize both shock waves and hot electrons generated at intensities of ≃1016 W/cm2. It is shown that, in these interaction conditions, hydrodynamics is strongly impacted by noncollisional mechanisms, and the role of the hot electrons, generated by parametric instabilities, is essential in determining shock dynamics.

Elaboration of 3-frame complex interferometry for optimization studies of capacitor-coil optical magnetic field generators

Recently developed three-frame complex-interferometry system driven by a Ti:Sa laser with 40 fs pulse has been installed at the PALS (Prague Asterix Laser System) laser facility. This unique diagnostic allows for the first time to perform simultaneous measurements of B-field in the coil region of the capacitor-coil targets (CCT) and the self-generated B-field (SMF) of the diode plasma in between the CCT-plates. CCT were irradiated by the PALS iodine laser (λ = 1315 nm) with energy in the range 250–500 J and pulse duration of 350 ps at full width at half maximum. The operation of this diagnostic system and methodologies for quantitative data analysis are presented in this study, including: (i) obtaining information about the induction of the magnetic field in the CCT coil based on measurements of the Faraday effect in the TGG (Terbium Gallium Garnet) paramagnetic crystal at the coil vicinity and (ii) determining magnetic field and current density distributions in the capacitor region of the CCT by analysis of the complex interferograms. The preliminary measurements confirmed the high potential of the reported setup for optimization studies of CCT targets.

Main spectral features of meteors studied using a terawatt-class high-power laser

Context. Meteor spectra are commonly interpreted using data from databases and tables. Several studies have demonstrated very sophisticated calculations of elemental compositions of meteoroid bodies based on the computation of synthetic meteor spectra or on the spectral analysis of airglow plasma containing evaporated, atomized, and ionized meteoroid matter. However, considering accuracy, reliability of computations, lack of laboratory experimental data in this field, as well as the complicated physical structure of meteor plasma, such qualitative assignment or quantitative calculations are still extensively discussed in the scientific community. Even on the laboratory level, many studies have shown the high complexity of the acquisition and interpretation of the data that are recorded with techniques of emission spectroscopy that are in fashion and philosophy similar to the spectral analysis of meteor plasma, that is, detection and quantification of the elements that are ablated from complicated multicomponent matrices. Aims. The current study is focused on the application of terawatt-class laser-induced breakdown spectroscopy (TC-LIBS) of real samples of chondritic meteorites. We recorded emission spectra with high resolution and high precision that contain spectral lines that are typical for real meteoric spectra. Experimental data were compiled in a form that is convenient for the meteoric spectra interpretation and calibration. Methods. TC-LIBS was carried out by a high-power terawatt-class laser facility, the Prague Asterix Laser System (PALS). The spectra were simultaneously recorded by an echelle high-resolution spectrograph in the UV/VIS spectral ranges and by a low-resolution spectrograph that was used for real observation of meteor spectra. We also present calculated synthetic spectra based on data from the NIST atomic spectra database. Results. We assembled etalon qualitative tables of major meteoric spectral features that can be used both for the spectral wavelength calibration of low-resolution observational instruments and for the exact interpretation of meteor spectra. The data are compared with real meteor spectra.

Prebiotic synthesis initiated in formaldehyde by laser plasma simulating high-velocity impacts

Context. It is well known that hydrogen cyanide and formamide can universally be considered as key molecules in prebiotic synthesis. Despite the fact that formamide has been detected in interplanetary and interstellar environments, other prebiotic species are far more abundant, including, for example, formaldehyde. However, several results indicate that formamide can play the role of important intermediate as well as that of a feedstock molecule in chemical abiogenesis. Diverse recently proposed scenarios of the origins of the first biopolymers show that liquid formamide environments could have been crucial for the formation of nucleobases, nucleosides, and for phosphorylation reactions, which lead to nucleotides.Aims.Here we report on a wide exploration of the formaldehyde reaction network under plasma conditions mimicking an asteroid descent in an Earth-like atmosphere and its impact.Methods.Dielectric breakdown using a high-power kJ-class laser system (PALS – Prague Asterix Laser System) along with quantum mechanical, ab initio molecular dynamics, and enhanced sampling simulations have been employed in order to mimic an asteroid impact plasma.Results.Being more abundant than formamide both in interstellar and interplanetary environments, during the era of early and late heavy bombardment of Earth and other planets, formaldehyde might have been delivered on asteroids to young planets. In the presence of nitrogen-bearing species, this molecule has been reprocessed under plasma conditions mimicking the local environment of an impacting body. We show that plasma reprocessing of formaldehyde leads to the formation of several radical and molecular species along with formamide.Conclusion. All the canonical nucleobases, the simplest amino acid (i.e., glycine), and the sugar ribose, have been detected after treatment of formaldehyde and nitrogen gas with dielectric breakdown. Our results, supported by quantum mechanical and enhanced sampling simulations, show that formaldehyde – by producing inter alia formamide – may have had the role of starting substance in prebiotic synthesis.

Time evolution of stimulated Raman scattering and two-plasmon decay at laser intensities relevant for shock ignition in a hot plasma

Laser–plasma interaction (LPI) at intensities $10^{15}{-}10^{16}~\text{W}\cdot \text{cm}^{-2}$ is dominated by parametric instabilities which can be responsible for a significant amount of non-collisional absorption and generate large fluxes of high-energy nonthermal electrons. Such a regime is of paramount importance for inertial confinement fusion (ICF) and in particular for the shock ignition scheme. In this paper we report on an experiment carried out at the Prague Asterix Laser System (PALS) facility to investigate the extent and time history of stimulated Raman scattering (SRS) and two-plasmon decay (TPD) instabilities, driven by the interaction of an infrared laser pulse at an intensity ${\sim}1.2\times 10^{16}~\text{W}\cdot \text{cm}^{-2}$ with a ${\sim}100~\unicode[STIX]{x03BC}\text{m}$ scalelength plasma produced from irradiation of a flat plastic target. The laser pulse duration (300 ps) and the high value of plasma temperature ( ${\sim}4~\text{keV}$ ) expected from hydrodynamic simulations make these results interesting for a deeper understanding of LPI in shock ignition conditions. Experimental results show that absolute TPD/SRS, driven at a quarter of the critical density, and convective SRS, driven at lower plasma densities, are well separated in time, with absolute instabilities driven at early times of interaction and convective backward SRS emerging at the laser peak and persisting all over the tail of the pulse. Side-scattering SRS, driven at low plasma densities, is also clearly observed. Experimental results are compared to fully kinetic large-scale, two-dimensional simulations. Particle-in-cell results, beyond reproducing the framework delineated by the experimental measurements, reveal the importance of filamentation instability in ruling the onset of SRS and stimulated Brillouin scattering instabilities and confirm the crucial role of collisionless absorption in the LPI energy balance.

Production of relativistic electrons, MeV deuterons and protons by sub-nanosecond terawatt laser

By the use of various experimental techniques, it is shown that the relativistic electrons, MeV protons, and deuterons are emitted from a 500-μm thick (CD2)n target exposed to Iλ2 ≈ 5 × 1016 W cm–2 μm2, which is delivered by the iodine photodissociation laser Prague Asterix Laser System. A parameter reflecting the laser-power efficiency of the proton acceleration is used for comparison of the observed maximum proton energy with data from other experiments. The number of protons and deuterons constituting the backward and forward jets is estimated. Values of maximum proton energies and electron temperatures indicate that the laser intensity should reach a relativistic level through the laser beam self-focusing. The occurrence of electron bunches in front of the irradiated target surface was identified by time resolved femtosecond interferometry. Energy distribution functions of electrons emitted in the both backward and forward directions are analysed and compared.

On the enhancement of p-11B fusion reaction rate in laser-driven plasma by α → p collisional energy transfer

The possibility of triggering an avalanche reaction in laser-driven p-11B fusion by the effect of collisional energy transfer from α particles to protons has recently been debated, especially in connection to the high yield of α particles (4 × 108 per laser shot) achieved on engineered targets at the Prague Asterix Laser System (PALS), with a pulse of 500 J, 0.3 ns FWHM. We elucidate this controversial subject within the framework of a simple two-population model for protons, based on the binary collision theory in a plasma. We find an avalanche characteristic time of almost 1 μs for the 675 keV fusion cross section resonance in typical PALS plasma, upon idealized confinement conditions. This avalanche time is one order of magnitude higher than previously reported, meaning that no such process can substantially develop in plasma at the PALS on the 675 keV resonance, not even in the most optimistic confinement scenarios. Nevertheless, we put forward for further investigation that more realistic conditions for setting up the avalanche regime could rather be attained by suitably targeting the narrow 163 keV resonance in the fusion cross section, also in connection to recently proposed laser-driven magnetic trapping techniques.

Measurements of parametric instabilities at laser intensities relevant to strong shock generation

Parametric instabilities at laser intensities in the range (2–6) × 1015 W/cm2 (438 nm, 250 ps, 100–300 J) have been investigated in planar geometry at the Prague Asterix Laser System facility via calorimetry and spectroscopy. The density scalelength of the plasma was varied by using an auxiliary pulse to form a preplasma before the arrival of the main laser beam and by changing the delay between the two pulses. Experimental data show that Stimulated Brillouin Scattering (SBS) is more effective than Stimulated Raman Scattering (SRS) in degrading laser-plasma coupling, therefore reducing the energy available for the generation of the shock wave. The level of the SBS backscatter and laser reflection is found to be in the range between 3% and 15% of the incident laser energy, while Backward SRS (BRS) reflectivity ranges between 0.02% and 0.2%, depending on the delay between the pulses. Half-integer harmonic emission is observed and provides a signature of Two Plasmon Decay (TPD) occurring around the quarter of the critical density. Data analysis suggests that SRS is driven in beam speckles with high local intensity and occurs in bursts, particularly at higher laser intensities, due to the presence of kinetic mechanisms saturating the SRS growth in the speckles. Time-resolved measurements also show that BRS occurs in the trailing part of the laser pulse, when the plasma has a longer density scalelength. Our measurements also indicate that hot electrons are predominantly produced by SRS rather than TPD.

Electromagnetic pulse (EMP) radiation by laser interaction with a solid H2 ribbon

The electromagnetic pulses (EMPs) generated during the interaction of a focused 1.315-μm sub-nanosecond laser pulse with a solid hydrogen ribbon were measured. The strength and temporal characteristics of EMPs were found to be dependent on the target density. If a low density target is ionized during the interaction with the laser, and the plasma does not physically touch the target holder, the EMP is weaker in strength and shorter in time duration. It is shown that during the H2 target experiment, the EMP does not strongly affect the response of fast electronic devices. The measurements of the EMP were carried out by Rohde&Schwarz B-Probes, particularly sensitive in the frequency range from 30 MHz and 1 GHz. Numerical simulations of resonant frequencies of the target chamber used in the experiment at the Prague Asterix Laser System kJ-class laser facility elucidate the peaked structure of EMP frequency spectra in the GHz domain.

Triple nuclear reactions (d, n) in laser-generated plasma from deuterated targets

Measurements performed at Prague Asterix Laser System laboratory have permitted to study nuclear reactions in plasma produced by high intensity laser pulses (1016 W/cm2) accelerating high energetic ions. In particular, the laser irradiation of deuterated polyethylene (CD2) primary target, as thin foils, has produced the ion acceleration of C and D ions, and the presence of a thick LiD secondary target has produced nuclear reaction events due to the deuteron-deuteron, deuterons-lithium, and deuteron-carbon interactions. Fast and slow neutrons have been obtained mainly from the nuclear reactions 7Li(d, n)8Be, 2H(d, n)3He, and 12C(d, n)13N. Plasma monitoring and measurements of kinetic energies of produced particles in different directions were obtained using many detectors. The analyses were based on a semiconductor time-of-flight technique, an electric and magnetic ion deflection in a Thomson spectrometer, and ion track detectors. The maximum yields of neutrons produced in the used experimental conditions were evaluated to be about 4 × 108 and 3 × 108 neutrons/laser shot at energies of 14 MeV and 2.4 MeV, from the D-Li and D-D reactions, respectively, while the production of low energy neutrons from the third D-C reaction was negligible.

Experimental study of the interaction of two laser-driven radiative shocks at the PALS laser

Radiative shocks (RS) are complex phenomena which are ubiquitous in astrophysical environments. The study of such hypersonic shocks in the laboratory, under controlled conditions, is of primary interest to understand the physics at play and also to check the ability of numerical simulations to reproduce the experimental results.In this context, we conducted, at the Prague Asterix Laser System facility (PALS), the first experiments dedicated to the study of two counter-propagating radiative shocks propagating at non-equal speeds up to 25–50 km/s in noble gases at pressures ranging between 0.1 and 0.6 bar. These experiments highlighted the interaction between the two radiative precursors. This interaction is qualitatively but not quantitatively described by 1D simulations. Preliminary results obtained with XUV spectroscopy leading to the estimation of shock temperature and ion charge of the plasma are also presented.