Powerful Ultrashort Laser Pulses Research Articles

Wavelength-Tunable Chirped Pulse Amplification System (1720 nm–1800 nm) Based on Thulium-Doped Fiber

Chirped pulse amplification (CPA) has been a commonly used methodology to obtain powerful ultrashort laser pulses ever since its first demonstration. However, wavelength-tunable CPA systems are much less common. Wavelength-tunable ultrashort and intense laser pulses are desirable in various fields such as nonlinear spectroscopy and optical parametric amplification. In this work, we report a 1720 nm–1800 nm tunable CPA system based on Tm-doped fiber. The tunable CPA system contains a seed laser, a pulse stretcher, two cascaded amplifiers and a pulse compressor. The dispersion-managed seed laser cavity emits wavelength-tunable laser pulses with pulse durations of several ps and spectral widths from 25 nm to 34 nm. After being stretched temporally to tens of ps, the laser pulses are then amplified in two-stage amplifiers and compressed in a Treacy-type compressor. At 1720 nm, the maximum average power of 126 mW is obtained with a pulse duration of 507 fs; at 1800 nm, the maximum average power of 264 mW is obtained with a pulse duration of 294 fs. The pulse repetition rates are around 22.7 MHz. We perform an analysis of the system design based on numerical simulations and go on to suggest further steps for improvement. To the best of our knowledge, this is the first demonstration of a tunable CPA system beyond 1.1 μm. Considering the specific wavelength range, this wavelength-tunable CPA system is highly desirable for biomedical imaging, sensing, and parametric amplifiers.

Graphene nano-sieves by femtosecond laser irradiation

The formation of nano-pores in graphene crystal structure is alternative way to engineer its electronic properties, chemical reactivity, and surface interactions, enabling applications in technological fields such as sensing, energy and separation. The past few years, nano-perforation of graphene sheets has been accomplished by a variety of different methods suffering mainly from poor scalability and cost efficiency issues. In this work, we introduce an experimental protocol to engineer nanometer scale pores in CVD graphene membranes under ambient conditions, using low power ultra-short laser pulses and overcoming the drawbacks of other perforation techniques. Using Atomic Force Microscopy (AFM) and Scanning Electron Microscopy (SEM) we visualized and quantified the nanopore network while Raman spectroscopy is utilized to correlate the nano-perforated area with the nanotopographic imaging. We suggest that Raman imaging provides the identification of nanoporous area and, in combination with AFM, we provide solid evidence for the reproducibility of the method, since under these experimental conditions, nanopores of a certain size distribution are formed.

Multiscale model for ultrashort pulsed parallel laser structuring—part II. The macroscale model

The increasing pixel density in displays demands high quality in the production of fine metal masks (FMMs). The production process of FMMs boils down to structuring tiny holes in thin metal sheets or foils. The manufacturing requirements of FMMs are high precision in terms of the hole geometry to let enough light escape from each diode and high productivity to produce the required amount. To achieve both objectives, high power ultrashort pulse (USP) lasers can be utilized. Because USP lasers fall short of the productivity requirements, they are combined with multibeam scanners. During production, the multibeam scanners deposit a lot of heat in the metal foil, which can ultimately yield temperature-induced distortions. To understand and finally avoid such distortions, a process simulation is sought. In a preceding study, the structuring of a single hole (the microscale) was investigated, but due to the large differences in the time and spatial scales involved, it was not feasible to simulate the production of the whole part (the macroscale). Within this treatise, a multiscale approach that takes into account the necessary information from the microscale to describe temperature-induced distortions on the macroscale is described. This approach targets laser ablation processes with pulse durations ranging from picoseconds up to nanoseconds provided the ablation is not melt-driven. First, a representative volume element (RVE) is generated from the results of the microscale model. Then, this RVE is utilized in the thermo-elastic structural mechanics simulation on the macroscale. The multiscale model is validated numerically against a hole-resolved computation, which shows good agreement. Naturally, the simulation is highly dependent on the microscale model, which in turn depends on the material properties. To handle material changes well, an experimental calibration has to be performed. This calibration is not part of this treatise, but it will be described in a future publication. In addition to the calibration process, the validation with experiments will be conducted in future research. Additionally, the authors envision the automation of the whole process, resulting in a first-time-right approach for the development of FMMs. Finally, the procedure might be extended to the requirements of other filtration purposes.

Multi-pass cells for post-compression of ultrashort laser pulses

Ultrafast lasers reaching extremely high powers within short fractions of time enable a plethora of applications. They grant advanced material processing capabilities, are effective drivers for secondary photon and particle sources, and reveal extreme light-matter interactions. They also supply platforms for compact accelerator technologies, with great application prospects for tumor therapy or medical diagnostics. Many of these scientific cases benefit from sources with higher average and peak powers. Following mode-locked dye and titanium-doped sapphire lasers, broadband optical parametric amplifiers have emerged as high peak- and average power ultrashort pulse lasers. A much more power-efficient alternative is provided by direct post-compression of high-power diode-pumped ytterbium lasers—a route that advanced to another level with the invention of a novel spectral broadening approach, the multi-pass cell technique. The method has enabled benchmark results yielding sub-50-fs pules at average powers exceeding 1 kW, has facilitated femtosecond post-compression at pulse energies above 100 mJ with large compression ratios, and supports picosecond to few-cycle pulses with compact setups. The striking progress of the technique in the past five years puts light sources with tens to hundreds of TW peak and multiple kW of average power in sight—an entirely new parameter regime for ultrafast lasers. In this review, we introduce the underlying concepts and give brief guidelines for multi-pass cell design and implementation. We then present an overview of the achieved performances with both bulk and gas-filled multi-pass cells. Moreover, we discuss prospective advances enabled by this method, in particular including opportunities for applications demanding ultrahigh peak-power, high repetition rate lasers such as plasma accelerators and laser-driven extreme ultraviolet sources.

Thermal imaging of high power ultrashort pulse laser ablation of alumina towards temperature optimized micro machining strategies

The application of pulsed laser systems with pulse durations in the pico- and femtosecond regime for material processing is commonly associated with a cold ablation. Due to the minimized interaction-time between the ultrashort laser pulses and the material, this statement is almost valid as long as no heat accumulation effect appears. With the increasing demand of high productivity processes, the average power of ultrashort pulsed laser systems increases above 100 W, which leads, however, to increased thermal effects during laser processing. This is especially important for laser processing of technical ceramics like alumina. Large temperatures gradients, which locally occur during laser processing using high average power could lead to thermal modifications and cracks in the material. In this study, we present a process-optimization method for high power laser ablation of alumina based on thermal imaging. The use of a 2D IR camera enables the estimation of the temperature distribution during the laser processing. We investigate the influence of laser power up to 80 W, pulse duration between 900 fs and 10 ps and processing duration on the resulting material temperature. Beside the material temperature we evaluate the material removal rate and the resulting surface quality.

Exotic silicon phases synthesized through ultrashort laser-induced microexplosion: Characterization with Raman microspectroscopy

Confined microexplosions induced in silicon by powerful ultrashort laser pulses can lead to new Si phases. Some of these have not previously been observed via near-equilibrium compression of silicon. In this study, confocal Raman micro-spectroscopy and Raman imaging of arrays of microexplosions have been conducted to search for Raman signatures of these novel allotropes of silicon. A microexplosion is generated at the interface between a thick silicon dioxide confinement layer and underlying silicon. It is characterised by a void at the interface above a region of compressed silicon. Raman data show a rich assembly of silicon phases within the modified silicon. Residual stresses up to 4.5 GPa in the modifications have been determined from the shift in the main diamond-cubic Si Raman peak. The computed Raman spectra for a number of Si allotropes show reasonable agreement with the experimental spectra. Two structurally similar tetragonal phases of silicon (the rhombohedral r8 and the body-centred bc8) phases as well as recently identified bt8-Si are all highly likely to be contained in Raman spectra from many laser-modified sites. Although the st12-Si phase, previously observed in our electron diffraction studies of the highly compressively stressed laser-modified regions, was not reliably identified from Raman data, we suggest this could be due to the possible difference in residual stress level in the sites analysed by the electron diffraction and Raman spectra. Several other unidentified Raman peaks were observed, suggesting the presence of other unknown silicon phases. All of these silicon phases are expected to have attractive semiconducting properties including narrow band gap that open up novel applications.

Picosecond laser machining of tungsten carbide

Hard materials such as tungsten carbide (WC) are extensively used in cutting tools in high-value manufacturing, and the machining of these materials with sufficient speed and quality is essential to exploit their full potential. Over the last two decades, short (nanosecond (ns)) and ultra-short (picosecond (ps); femtosecond (fs)) pulse laser machining has been evaluated by various researchers and proposed as an alternative to the current state-of-the-art machining techniques for advanced materials like WC, which include mechanical grinding and electrical discharge machining. However, most of the established/existing research on this topic is based on low power lasers, which may not be adopted in industrial production environments due to its low material removal rate. This paper presents the results of a fundamental study, on using a 300 W picosecond laser for the deep machining of tungsten carbide. The influence of various laser parameters on the geometric precision and quality (surface and sub-surface) of the ablated area was analysed, and the ablation mechanism is discussed in detail. Laser pulse frequency and scanning speed have minimal effect on ablation rate at high power levels. The surface roughness of the ablated area increases with the ablation depth. At optimal conditions, no significant thermal defects such as a recast layer, micro crack or heat affected zone were observed, even at a high average power of 300 W. The material removal rate (MRR) seems to be proportional to the average power of the laser, and a removal rate of around 45 mm3 per minute can be achieved at 300 W power level. Edge wall taper appears to be a significant issue that needs to be resolved to enable industrial exploitation of high power ultra-short pulse lasers.

Antireflective coatings with high damage threshold prepared by laser ablation

Latest developments in the field of high power ultra-short pulse lasers have led to intensive studies dedicated to the fabrication possibility of new antireflective coatings which exhibit high damage threshold. Therefore, this study is focused on the deposition and characterization of metal oxide heterostructures followed by laser-induced damage threshold tests which evidence their application in high power laser optics. Al2O3, SiO2, and HfO2 layers are combined to obtain different heterostructures, i.e. HfO2/Al2O3/HfO2/Al2O3/HfO2 and HfO2/SiO2/HfO2/SiO2/HfO2. The metal oxide heterostructures are deposited in a controllable oxygen atmosphere, either at room temperature or high temperatures (600 °C) by pulsed laser deposition (PLD). The morphological, structural and optical properties of the as-deposited heterostructures are first investigated. Atomic force microscopy and spectroscopic ellipsometry investigations reveal a lower roughness of the heterostructures based on HfO2/Al2O3 layers grown at 600 °C as compared to those grown at room temperature. Furthermore, following the laser-induced damage threshold (LIDT) tests carried out with a Ti–Sapphire laser, higher LIDT values are obtained for the HfO2/Al2O3-based heterostructures than for the HfO2/SiO2-based heterostructures. The ability to control the morphological and structural properties of the antireflective coatings by modifying the deposition parameters of the metal oxide heterostructures demonstrates that PLD is a suitable technique for the manufacturing of antireflective coatings for high power ultra-short laser systems.

Uniform long focal depth with centimeter-scale range produced by an aspherical mirror

An aspherical mirror used to produce light fields with uniform long focal depth is first proposed by the energy conservation equation and the principle of equal optical path. The focusing characteristics of the novel mirror are studied in detail by numerical simulations based on scalar diffraction theory. Compared with parabolic mirror with similar parameters, the largest difference of surface profile is only at the micron level and the length of focal depth is stretched about 100 times. By using the apodization function, the oscillation of the axial intensity can be eliminated effectively and the axial inhomogeneity can be less than 0.5%. The effect of pulse shape on the focusing properties is also discussed and it is found that the pulse shape must be flat-top to obtain uniform long focal depth for a picosecond pulse. The novel mirror presented in this paper can be used for focusing high power ultrashort pulse laser with pulse width of picoseconds or femtoseconds, and there are many potential applications in physics of strong field.

Investigation of heat accumulation effects during deep hole percussion drilling by high power ultrashort pulsed laser radiation

In the last few years, commercially available ultrashort pulsed (usp) laser systems have reached average powers of several 100 W, which makes them also interesting for enhancing traditional applications. For example, laser drilling, a conventionally melt-dominated process, would benefit from the advantages of an usp ablation process. Due to the small processing area in laser drilling, substantial heat accumulates already at a few Watts of average power. This heat accumulation creates melt but also increases the mean ablation rate at least 1 order of magnitude and could lead to a productive drilling process. In this study, the increase of the mean ablation rate in percussion drilling due to heat accumulation is examined for various metals and sample thicknesses for high average powers of up to 300 W and a pulse energy in the milliJoule range. Those investigations have not yet been performed in such detail. It is shown that by doubling the pulse energy the drilling time can be decreased by 2 orders of magnitude due to heat accumulation. This behavior is valid for various metals like steel or aluminum, despite their varying material parameters. By analyzing the influence of different repetition rates and focal diameters, it is shown that the predominant parameter to characterize the heat accumulation is the average power. No significant difference is observed if the average power starting from 20 W is set up by a high pulse energy or repetition rate. Stainless steel has a different behavior compared to the other investigated metals when the pulse duration is changed from 2 to 20 ps, which is caused by a modified plasma generation. For stainless steel, the drilling time is found to be describable with one empirical formula for the entire range of examined average power and sample thickness.

Time dependent spatial entanglement in atom-field interaction

By using stochastic ensembles of walkers in physical and in one-body Hilbert spaces the recently proposed time-dependent quantum Monte Carlo (TDQMC) method offers the unique capability to calculate one-body density matrices at fully correlated level, without referencing the many-body quantum state. Here TDQMC is applied to study entanglement of simple systems such as Moshinsky atom (oscillator potentials) and atoms with Coulomb potentials in one spatial dimension. Our findings indicate that the dynamic entanglement of atoms exposed to powerful ultrashort laser pulse can be easily manipulated by introducing an appropriate phase modulation where the negative chirp enhances the entanglement while the positive one suppresses it. These findings can be used to explore the correlation properties of different constituents of complex quantum systems subjected to appropriately shaped laser radiation.

Self-phase modulation and spectral broadening in millimeter long self-written polymer waveguide integrated with single mode fibers

Polymer waveguide bridges up to 1.2 mm in length were optically written between two single-mode optical fibres. Optical Nonlinearity of polymer waveguide was measured by coupling a high power ultra-short pulsed laser. Before waveguide fabrication fiber ends were treated by adhesion promoter which covalently bond to both the silica fibre and the photopolymer, also photopolymerization was conducted from both fibres. The new techniques improve both the mechanical properties and optical transmission of polymer bridges. The optical insertion loss was 1.1 dB for the longest waveguides. A considerably long interaction length of polymer waveguide allows spectral broadening and self-phase modulation features to occur in response to the high power laser propagation through the polymer bridges. The spectral broadening in polymer waveguide was much broader than that of 1.5 m plain fibre. The ultrafast nonlinearity of the polymer waveguides was determined to be of the order of 103 times the nonlinearity of silica.

Design and experimental study on high quality beam and high stability power of laser

High-performance lasers with high-quality beam laser and high-stability power are widely used for laser machining, laser precision measuring, etc. Reflection curved mirrors are widely used in lasers to provide several small intracavity focal spots and reduce the dispersion and volume of the laser. The primary disadvantage of using reflection curved mirrors in folded resonators is that relatively large angles of incidence deform the circular transverse pattern of the output beam and limit laser performance. In addition, in high power lasers or ultra short pulse lasers, the gain medium thermal lens focal length fluctuation is the primary cause of the instability of laser output power. This paper focuses on beam quality and power stability of laser, and an effective method of solving the two problems, i.e., astigmatism and instability power of laser, is presented. The laser resonator with high-quality laser beam and high-stability power is very easy and intuitive to design by this method, in which the resonator transform circle graphic theory is used and the thermal lens and astigmatism compensation is taken into account. The theoretical investigation shows that the astigmatism in two terminal arms of the folded laser resonator can be successfully eliminated by using this method, and the experimental measurements of the pattern of the laser output beam show that the deformations of spot intensity profiles in the two terminal arms can be simultaneously compensated for completely in the cavity, which is in good agreement with the analytical prediction. When the focal length of the laser crystal thermal lens varies, the variations of radii of spots not only at some key position, but also at all locations of the laser resonance designed by this method, are overtly smaller than the variation of the normal resonant cavity. The stability of the output laser power of the laser is better than that of a universal laser resonator under the same external conditions.

Femtosecond laser-induced damage threshold in snow micro-structured targets

Enhanced acceleration of protons to high energy by relatively modest high power ultra-short laser pulses, interacting with snow micro-structured targets was recently proposed. A notably increased proton energy was attributed to a combination of several mechanisms such as localized enhancement of the laser field intensity near the tip of $1~\unicode[STIX]{x03BC}\text{m}$ size whisker and increase in the hot electron concentration near the tip. Moreover, the use of mass-limited target prevents undesirable spread of absorbed laser energy out of the interaction zone. With increasing laser intensity a Coulomb explosion of the positively charged whisker will occur. All these mechanisms are functions of the local density profile and strongly depend on the laser pre-pulse structure. To clarify the effect of the pre-pulse on the state of the snow micro-structured target at the time of interaction with the main pulse, we measured the optical damage threshold (ODT) of the snow targets. ODT of $0.4~\text{J}/\text{cm}^{2}$ was measured by irradiating snow micro-structured targets with 50 fs duration pulses of Ti:Sapphire laser.

Measurement of resonant bend loss in anti-resonant hollow core optical fiber.

We present the results of measurements of resonant spectral bend loss using a novel apparatus in a series of hollow core anti-resonant optical fibers, important for their applications in the delivery of industrial power ultra-short laser pulses. The measured bend losses exhibit clear wavelength-bend diameter resonances. We demonstrate, in good agreement with theoretical analysis, that the sensitivity to bend diameter (in terms of minimum bend radii) is dependent on the ratio between cladding and core structure size. By decreasing the cladding capillary diameter: core diameter ratio from 0.70 to 0.43 the minimum bend diameter is decreased from >160 mm to ~15 mm at a wavelength of 800 nm. Furthermore it is demonstrated that the exact position of the loss bands is highly dependent on the orientation of the fiber structure with the bend plane.

Lasers in analysis: Potential and prospects for the development of ultrashort pulsed lasers

The main achievements in the analytical application of lasers, their potential applications, and prospects for further development of this field were described. The role of laser generation conditions and modes, especially of pulse duration, on laser applicability in analysis was discussed. The propagation of powerful ultrashort laser pulses (USPs) in transparent samples and the positive role of chirping and filamentation were considered. New methods of laser-induced breakdown spectroscopy based on ultrashort pulses, chirping, and filamentation were discussed.

Study of terahertz generation via the interaction of two-color ultra-short laser pulses with water vapor plasmas

In this work, using a two dimensional particle in cell-Monte Carlo collision simulation scheme, the Terahertz (THz) generation process via the interaction of a two-color ultra-short laser pulses with the water vapor gas (H2O) is examined. The background gas pressure and various laser parameters, e.g., its pulse shape, duration, and waist, are varied, and their effects on the temporal variation of the generated current density, THz electric field, and THz spectral intensity are studied. It is shown that the best pulse shape generating the THz signal radiation with the highest intensity is a trapezoidal pulse. Moreover, the intensity of generated THz radiation is increased at the higher pulse durations and waists. In addition, at the higher water vapor gas pressures, the time to peak of the generated current density is shifted to the earlier moments. Finally, it is observed that, for the laser pulses with the intensities of about 8 × 1013 W/cm2, the water vapor triatomic molecules are a proper source for the THz radiation generation under the illumination of high power ultra-short two-color laser pulses.

High-throughput machining using a high-average power ultrashort pulse laser and high-speed polygon scanner

High-throughput ultrashort pulse laser machining is investigated on various industrial grade metals (aluminum, copper, and stainless steel) and Al2O3 ceramic at unprecedented processing speeds. This is achieved by using a high-average power picosecond laser in conjunction with a unique, in-house developed polygon mirror-based biaxial scanning system. Therefore, different concepts of polygon scanners are engineered and tested to find the best architecture for high-speed and precision laser beam scanning. In order to identify the optimum conditions for efficient processing when using high-average laser powers, the depths of cavities made in the samples by varying the processing parameter settings are analyzed and, from the results obtained, the characteristic removal values are specified. For overlapping pulses of optimum fluence, the removal rate is as high as 27.8 mm3/min for aluminum, 21.4 mm3/min for copper, 15.3 mm3/min for stainless steel, and 129.1 mm3/min for Al2O3, when a laser beam of 187 W average laser powers irradiates. On stainless steel, it is demonstrated that the removal rate increases to 23.3 mm3/min when the laser beam is very fast moving. This is thanks to the low pulse overlap as achieved with 800 m/s beam deflection speed; thus, laser beam shielding can be avoided even when irradiating high-repetitive 20-MHz pulses.

Hollow-core fibers for high power pulse delivery.

We investigate hollow-core fibers for fiber delivery of high power ultrashort laser pulses. We use numerical techniques to design an anti-resonant hollow-core fiber having one layer of non-touching tubes to determine which structures offer the best optical properties for the delivery of high power picosecond pulses. A novel fiber with 7 tubes and a core of 30µm was fabricated and it is here described and characterized, showing remarkable low loss, low bend loss, and good mode quality. Its optical properties are compared to both a 10µm and a 18µm core diameter photonic band gap hollow-core fiber. The three fibers are characterized experimentally for the delivery of 22 picosecond pulses at 1032nm. We demonstrate flexible, diffraction limited beam delivery with output average powers in excess of 70W.

The Application of Cryogenic Laser Physics to the Development of High Average Power Ultra-Short Pulse Lasers

Ultrafast laser physics continues to advance at a rapid pace, driven primarily by the development of more powerful and sophisticated diode-pumping sources, the development of new laser materials, and new laser and amplification approaches such as optical parametric chirped-pulse amplification. The rapid development of high average power cryogenic laser sources seems likely to play a crucial role in realizing the long-sought goal of powerful ultrafast sources that offer concomitant high peak and average powers. In this paper, we review the optical, thermal, thermo-optic and laser parameters important to cryogenic laser technology, recently achieved laser and laser materials progress, the progression of cryogenic laser technology, discuss the importance of cryogenic laser technology in ultrafast laser science, and what advances are likely to be achieved in the near-future.