Post-irradiation Examination Research Articles

Small punch test size reduction to enable high flux irradiation

Screening and qualification of new nuclear materials with superior irradiation resistance requires expensive irradiation exposure and post-irradiation examination before consideration into industrial nuclear structural components. The development of miniaturized test methods is needed for enhanced cost/time efficient testing, while enabling comparative and robust material property estimation in a timely and high throughput manner. The Small Punch Test (SPT) is drawing much interest, especially since the publication of an European standard. Motivated by this standard, a new SP test sample geometry is proposed in order to reduce the material volume to be tested, hences increasing the number of samples that can be introduced in an irradiation rig is proposed. The modified sample diameter has been reduced from 8 to 5.35 mm. The qualification of this new design is described here together with a detailed description of the SPT setup modification as compared to the reference setup of the EN standard. Finite element analyses and a series of experiments have been conducted using both standard and reduced size SP samples to demonstrate that the modified test gives estimates of the basic mechanical properties with the same magnitude of error and validates the modified sample geometry for usage in irradiated material testing.

Post-irradiation examination of UN-Mo-W fuels for space nuclear propulsion

The National Aeronautics and Space Administration's return to space nuclear propulsion stems from the need for a more efficient method of space travel. Nuclear thermal propulsion systems have been shown to be two times more efficient than chemical propulsion. NASA's Sirius program was created to fabricate and test fuels for space nuclear propulsion, specifically to determine their performance under prototypical startup conditions. The Sirius project featured 4 test capsules, Sirius-1 featured uranium nitride fuel dispersed in a matrix of tungsten and rhenium, while Sirius-2A, -2B, and -3 featured uranium nitride-molybdenum-tungsten fuel (UN-Mo-W). This study discusses the Sirius-2A and -2B irradiation experiments at the Idaho National Laboratory, specifically their performance under irradiation at the Transient Reactor Test Facility. It was found that the fuel samples overall did not exhibit significant cracking, though the Sirius-2A fuel did have one large crack on the surface of the fuel. There was minimal hydrogen absorption in the samples, though it is unknown if the absorption occurred during irradiation or during fabrication. Mechanical testing indicated that the UN fuel demonstrated ceramic behavior as expected, and the Mo/W matrix demonstrated linear elastic behavior to failure.

Performance Analysis of U3Si2-Al Fuel with Density of 2.96 gU/cm3 and Burnup of 56%

Post-irradiation examination (PIE) of a low-enriched-uranium silicide fuel plate, irradiated in the Indonesian Reaktor Serba Guna–Gerrit Augustinus Siwabessy (RSG-GAS) multipurpose reactor, was successfully conducted. The objective of the PIE project was to evaluate the performance and integrity of the fuel under radiation exposure and, furthermore, to explore the potential for increasing the burnup level, enhancing its efficiency and effectiveness. The targeted fuel plate, identified as IDA0045, was extracted from the experimental silicide fuel element RI-SIE2, which had a burnup level of approximately 56% loss of 235U. A scanning electron microscope combined with energy dispersive X-ray spectroscopy microstructural examination and a Vickers microhardness test were conducted for the top, middle, and bottom sections of the fuel. The PIE results indicated minimal occurrence of fuel swelling and good fuel integrity under irradiation, suggesting the possibility of increasing the burnup level.

Thermal Model of the AGR-5/6/7 Experiment with Offset Gas Gaps

Because of their high impact on calculated temperatures, the offset gas gaps between the graphite holder and capsule wall are evaluated for the thermal model of the Advanced Gas Reactor 5/6/7 (AGR-5/6/7) irradiation experiment. Fuel compact temperatures are a crucial factor in assessing the irradiation performance of tristructural isotropic (TRISO)-coated-particle fuel for use in high-temperature gas-cooled reactors. TRISO fuel irradiation performance is a core tenet of the U.S. Department of Energy’s Advanced Gas Reactor Fuel Development and Qualification Program, conducted in the Advanced Test Reactor at Idaho National Laboratory. Specifically, the irradiation experiments were intended to provide irradiation performance data to support fuel process development, qualify fuel for normal operating conditions, support the development of fuel performance models and codes, and provide irradiated fuel and materials for postirradiation examination and safety testing. The thermal model used to predict the fuel compact temperatures was a three-dimensional finite element model that was subject to uncertainty. The most dominant factor in the uncertainty pertaining to calculated fuel temperatures is the gas gap uncertainty, which is caused by the graphite holder nub-to-capsule wall clearance. In AGR-5/6/7 capsules, the graphite holders can be shifted away from being perfectly centered inside the stainless steel capsule walls. This is due to irradiation-induced graphite shrinkage or to insufficient nubs on the graphite holder leading to azimuthally varying gas gaps during irradiation. A method was developed to find the best offset magnitude and direction at the top and bottom of the graphite holders in Capsules 1 and 2, which experienced higher temperatures than originally predicted among the five AGR-5/6/7 axially dispersed capsules irradiated between 2018 and 2020. The differences between the calculated and the measured temperatures of thermocouples (TCs) placed in the graphite holder near the fuel compacts were used as the basis for the holder offset determination. The best-fit offset assumes that the root-mean-square error between the measured and calculated TC temperatures is a minimum value. Typical offsets in the range of 0.002 to 0.004 in. increase the fuel compact temperatures in the range of 100°C to 200°C when compared to the zero offset for Capsules 1 and 2. Additionally, because of irradiation-induced changes in the capsule geometries, the holder offsets change throughout the irradiation period.

Advanced interpretation of the SPHERE irradiation experiment with neutronics and fuel performance codes

The SPHERE experiment aimed at studying the behaviour of Minor Actinide-bearing Driver Fuel (U,Pu,Am)O2-x by comparing sphere-packed and pelletized fuels. The irradiation experiment was performed in the High Flux Reactor at Petten from August 2013 to April 2015, and was followed by post-irradiation examinations up to mid-2017. The present work consists in a new analysis of the SPHERE experiment, focusing on the pelletized fuel, by the means of both neutronics and fuel performance codes. This study is performed in the frame of the European Project PATRICIA. The adopted methodology and the main results achieved, assessed in particular against inert gas-related experimental data, are presented in the paper.

Microstructural and micromechanical characterization of Cr diffusion barrier in ATR irradiated U-10Zr metallic fuel

Chromium (Cr) has been recognized as a promising diffusion barrier candidate to mitigate the Fuel Cladding Chemical Interaction (FCCI) failure in metallic fuels for sodium-cooled fast reactor. This paper, for the first time, conducted an in-depth post-irradiation examination of the microstructure and composition evolution, and micromechanics of the Cr diffusion barrier in U-10Zr fuel/HT9 cladding irradiated in the Advanced Test Reactor (ATR) to 8.7% burnup at an averaged Peak Inner Cladding Temperature of 540–550 °C. Transmission Electron Microscope (TEM) characterization confirmed the preferential intergranular diffusion of Zr and U in the Cr diffusion barrier, suggesting that grain boundaries served as fast path for the diffusion of Zr and U into the Cr diffusion barrier. The interaction zone is dominated by nano crystalline α-ZrCr2 Laves phase. Despite the interaction, there is no microcracks being observed in the preserved Cr diffusion barrier and HT9 cladding, serving as a good barrier to mitigate FCCI under the studied in-reactor irradiation conditions. High density cavities in uniform distribution are observed inside Cr grains, nano particles contains Cr, Mn, and O are confirmed by Electron Energy Loss Spectroscopy (EELS) analysis. However, it is unclear whether the cavities will become an issue to the barrier integrity at higher burnup. In-situ Scanning Electron Microscopy (SEM) micro-tensile testing uncovered mechanical softening in the HT9 cladding nearing the Cr diffusion barrier, possibly due to the coarsening of lath structure and carbides precipitates.

Transmission electron microscopy characterization of Fuel Cladding Chemical Interaction (FCCI) in ATR-irradiated HT9 clad U-10M (10M = 5Mo-4.3Ti-0.7Zr wt%) metallic fuel

The pseudo-binary metallic fuel alloy, U-10M (wt%, M is the optimal combination of Mo, Ti, and Zr), has the potential to increase fuel solidus temperature, reduce the onset temperature of body-centered cubic phase, and increase the fuel's chemical stability compared with the conventional U-10Zr (wt%) metallic fuel. Post Irradiation Examination (PIE) confirmed excellent fuel performance for the U-10M (10M=5Mo-4.3Ti-0.7Zr wt%) fuel irradiated in the Advanced Test Reactor (ATR) to 2.2 at% burnup at Peak Inner Cladding Temperature (PICT) of 650 °C, an upper bound temperature for metallic fuel. But previous PIE study also observed Fuel Cladding Chemical Interaction (FCCI) on the cladding side, which is known as a fuel performance limiting issue but has not been fully understood yet. As an effort to improve the understanding of FCCI phenomenon, this study performed Scanning Electron Microscopy (SEM) and in-depth Transmission Electron Microscopy (TEM) characterization on a FCCI region. The examined FCCI region is dominated by (U, Zr)(Fe, Cr)2, suggesting that U-Fe interdiffusion reaction played a key role in inducing FCCI. Additionally, the FCCI boundary into the cladding consists of four distinctive phases, (U, Zr)(Fe, Cr)2, fcc-Cr, tetragonal UCr0.1Fe9.9Si2, intermetallic σ-FeCr, and lanthanide fission products at concentration up to ∼5.5 at%. Another goal of this study is to verify the involvement of Ti and Mo in FCCI formation on the cladding side. Observable Ti is found halfway of the thickness in the examined FCCI region, while 0.3–5 at% Mo is detected across the entire thickness of the examined FCCI region. Neither Ti nor Mo reacted with HT9 cladding constituents despite their diffusion footmark. Therefore, alloying Ti and Mo into the U-Zr fuel should not complicate the interdiffusion reaction on the HT9 cladding side.

Fission accelerated steady-state post irradiation examinations - Part II

The Advanced Fuels Campaign's Fission Accelerated Steady State Testing (FAST) approach at Idaho National Laboratory creates a benchmark for evaluating accelerated irradiation via control rodlets and advanced metal fuel alloys for sodium-cooled fast reactors (SFRs). FAST experiments have been developed to generate prototypic temperature conditions during steady state irradiations of scaled geometric fuel pins. This approach helps to attain higher burn ups at a much faster rate than previous irradiation tests. For this study, the results from profilometry, fission gas release, and metallography of a FAST experiment are presented. Profilometry determined 0 % effective strain in the rodlets. The fission gas release fraction was measured from puncture/collection analysis. Constituent redistribution was observed in two specimens despite the peak fuel temperatures being below the normal ranges in which redistribution is expected. Metallography of the two higher temperature specimens showed typical swelling with the solid pin closing the fuel-cladding gap and the annular specimen having a fully closed annulus. Additionally, metallography indicated no swelling, no redistribution, and a homogenous microstructure for specimens with lower irradiation temperature. Post irradiation examination of FAST rodlets generally showed the expected representative behavior of metallic fuels within SFRs.

Assessing the PLEIADES/GERMINAL V3 fuel performance code against transmutation experiments in sodium fast reactors

We present the results of a first assessment of the multiphysics PLEIADES/GERMINAL V3 fuel performance code against integral irradiation experiments of americium-bearing MOX fuel pins irradiated in sodium fast reactors. The pins considered in this work cover a range of americium contents from 2 to 5 weight %, being representative for the homogeneous transmutation path. The code predictions are compared to several post-irradiation examination results on integral (e.g., fission gas release) and local quantities (e.g., actinides redistribution in the fuel pellet), and demonstrate a satisfactory agreement with experimental data. The deviations between calculated and experimental quantities shed some light on modeling developments needed to better calculate the behavior of americium-bearing mixed-oxides fuel pins under irradiation.

Materials Science Analysis of RCCA Structural Materials and Calculations for Lifetime Extension

The paper considers the possibility of lifetime extending of the rod control cluster assemblies in operation by determining their residual lifetime using an approach that takes into account the actual position of the rod control cluster assembly in the core. Excessive conservatism was introduced by assuming that the immersion of the 10th working group in the core during all fuel campaigns is 70 %, while the actual position is 85-90 %. Taking into account the actual position of the rod control cluster assemblies indicates much less irradiation of the lower, most loaded part of control rod cladding and much less burnup of the 10B compared to 70 % immersion of the rod control cluster assemblies, since they are in the area of lower neutron flux density.
 The results of a comprehensive analysis of available studies and test results to determine the phenomena that can potentially approach the achievement of the boundary state of the structural components or limit the lifetime of control rods and rod control cluster assemblies in general are presented. Such phenomena include general corrosion of structural materials (42CrNiMo, Cr18Ni10Ti) (decrease in wall thickness, increased transfer of radioactive corrosion products the coolant); radiation resistance (degradation of mechanical characteristics) of control rod cladding materials (42CrNiMo) and other structural components of the rod control cluster assemblies (42CrNiMo, CrKh18Ni10Ti); radiation resistance of neutron-absorbing materials (B4C, Dy2O3∙TiO2); compatibility of absorbing materials with the control rod cladding.
 Based on the results of post-irradiation examinations of control rods tested in research reactors as dummy rods or rod control cluster assembly rods operated in the VVER-1000 core, the following boundary values were established that can be used as criteria for maintaining the integrity of the control rod cladding: maximum fast neutron fluence in the lower, most loaded part of the control rod cladding (in the weld area of the lower end plug and the cladding) should not exceed 34×1021 n/cm2; maximum burnup of the 10B isotope should not exceed 45 %. If these two criteria are met, the possibility of other potentially damaging phenomena is too low.
 According to the calculations that use the schedule of changes in the position of the rod control cluster assemblies of the control group and the power of one of the power units during one fuel cycle, one can preliminary conclude that the proposed approach will extend the lifetime of almost all rod control cluster assemblies from 25500 to 38000 hours in the automatic control group and from 75600 to 113500 hours in the shutdown group. The residual lifetime should be assessed for a particular power unit and each rod control cluster assembly separately, since each rod control cluster assembly has its own operating history.

HICU PIE results of neutron-irradiated lithium metatitanate pebbles

Lithium metatitanate (Li2TiO3) pebbles were irradiated with neutrons within the HICU (High neutron fluence Irradiation of pebble staCks for fUsion) experiment to investigate their material properties and tritium release behaviour in a post-irradiation examination (PIE). The irradiation temperature is the most significant influence on the material. Besides a higher irradiation temperature, a higher initial Li–6 content tends to lead to an increased tritium generation resulting in the formation of the secondary lithium depleted phase Li4Ti5O12. A pre-compaction of the pebble bed does not have an apparent influence on the material properties. Tritium is released as semi-tritiated water and semi-tritiated hydrogen (HTO and HT) and its release is enhanced at elevated irradiation temperatures.

Post-irradiation examination of commercial tantalum alloys following neutron irradiation

Post irradiation examination of two commercial tantalum alloys (based on Ta-8 %W) revealed significant irradiation hardening following neutron irradiation in the High Flux Isotope Reactor at Oak Ridge National Laboratory. Tensile samples of commercial Ta alloys T-111 and ASTAR-811C were irradiated to a total neutron fluence (E > 0.1 MeV) in the range (2–4)x1021 n/cm2 (0.39–0.75 dpa) at an irradiation temperature near 900 °C. Tensile testing conducted at room temperature and at 800 °C revealed significant irradiation hardening under all test conditions. Samples that were tensile tested at room temperature exhibited brittle failure, whereas ductility was maintained for elevated temperature testing. The irradiation hardening and embrittlement noted for both alloys was attributed to irradiation-induced dislocation loop formation as confirmed through scanning transmission electron microscopy analysis. Corresponding energy dispersive x-ray spectroscopy revealed radiation-induced segregation of Hf in these loop populations. This Hf enrichment is shown to result in eventual co-precipitation of elongated (Hf,O)-rich precipitates along the dislocation loops. These results show that irradiation hardening is enhanced via irradiation-enhanced precipitation at elevated irradiation temperatures. Consequently, the minimum recommended operating temperature window for Ta alloys should be increased to account for observed hardening/embrittlement at irradiation temperatures as high as 900 °C (1,173 K).

Materials qualification through the Nuclear Science User Facilities (NSUF): a case study on irradiated PM-HIP structural alloys

This article presents neutron irradiation and post-irradiation examination (PIE) capabilities available to the nuclear materials research community through the US Department of Energy’s Nuclear Science User Facilities (NSUF). The pressing need to deploy advanced nuclear reactors to combat climate change requires qualification of new fuels and materials. Among advanced manufacturing processes, powder metallurgy with hot isostatic pressing (PM-HIP) is nearest to becoming qualified for nuclear applications. This article provides examples from a recent irradiation and PIE program on a series of structural alloys fabricated by PM-HIP to illustrate how NSUF capabilities can be used to generate qualification data. The neutron irradiation experiments are described, and a sampling of results from tensile testing, nanoindentation, transmission electron microscopy, and atom probe tomography are presented, showing the favorable performance of PM-HIP alloys compared to their cast or forged counterparts under irradiation. This article provides a perspective on leveraging NSUF for future nuclear fuels and materials testing and qualification.

High-temperature steam oxidation study of irradiated FeCrAl defueled specimens

Post irradiation examinations (PIE) were performed on irradiated iron-chromium-aluminum (FeCrAl) specimens. These FeCrAl specimens were fabricated at the US Department of Energy's Oak Ridge National Laboratory (ORNL). The experimental setup involved subjecting FeCrAl cladding, along with UO2 pellets, to irradiation in the Idaho National Laboratory Advanced Test Reactor (ATR). In parallel, the FeCrAl alloy tubing without UO2 pellets was irradiated at ORNL's High Flux Isotope Reactor (HFIR). After irradiation, the ATR-irradiated rodlet was transported to an ORNL hot cell, where it was sectioned into multiple samples for the PIE and severe-accident testing. The sectioning process revealed that the fuel was not bonded to the cladding and could be easily detached from sectioned cladding slices. Microstructural analysis of the fuel cross sections demonstrated no significant interaction between the fuel and the cladding. Additionally, high-temperature steam oxidation tests on defueled cladding segments showed minimal oxygen uptake even at 1200 °C. The ATR-irradiated specimens began to exhibit signs of enhanced oxidation upon reaching a temperature of 1300 °C. Furthermore, enhanced oxidation was observed on the inner surface of the ATR-irradiated FeCrAl specimen, which had been subjected to 1300 °C for a duration of 1 min. By contrast, high-temperature steam oxidation experiments indicated that the HFIR-irradiated FeCrAl cladding provided good thermal stability when exposed to 1300 °C for up to 4 h. Comparative analysis encompassing the oxidation behavior of the ATR-irradiated fueled FeCrAl, HFIR-irradiated unfueled FeCrAl, and unirradiated FeCrAl suggests that the fuel–cladding interaction, although not visible via standard microscale electron microscopy measurements, may accelerate the deterioration of FeCrAl cladding in beyond-design-basis accident scenarios.

The UO2 Power-to-Melt Experiment Performed in the High Burnup Chemistry International Program

In this work, a detailed reevaluation of a past power-to-melt experiment performed within the so-called High Burnup Chemistry project is provided. A pressurized water reactor–type UO2 fuel rod was base irradiated in Belgian Reactor 3 up to a peak pellet burnup of 60 MWd/kgU. After base irradiation, the rod experienced a power ramp experiment in Belgian Reactor 2, reaching a ramp terminal level of 70 kW/m (later adjusted to 66 kW/m). Extensive post-irradiation examination was performed after both the base irradiation and the power ramp experiment. After the power ramp experiment, rod cladding failure and local fuel melting were observed. Fuel melting was observed in an 85-mm region around the peak power pellet with a normalized molten fuel radius in the range r/r0 = 0.20 to 0.27. The threshold power for melting derived from this experiment was 63.0 ± 4.4 kW/m.

Determination of the Gas Plenum Temperature of the P2M Instrumented Fuel Rodlets on the Basis of a Thermal-Hydraulic Study of the Belgian Reactor 2 Pressurized Water Capsule

To refine knowledge about pressurized water reactor fuel melting, the Power to Melt and Maneuverability (P2M) project in the Framework for Irradiation Experiments II (FIDES-II) managed by the Nuclear Energy Agency of the Organisation for Economic Co-operation and Development aims to perform two irradiation tests to reach fuel centerline partial melting using instrumented experimental fuel rodlets irradiated in a pressurized water capsule (PWC) of the Belgian Reactor 2 (BR2) [Studiecentrum voor Kernenergie (SCK CEN), Belgium]. Prior to these experiments, two preliminary tests will be performed in the PWC for qualification purpose toward safety. The experimental rodlets will be instrumented with a fuel centerline thermocouple in the lower part of the fuel and a pressure sensor (PS) in the upper part. An objective of the P2M experiments is to determine the amount of fission gas released from the fuel thanks to the PS measurement. The plenum pressure evolution is known from the measurement, and knowledge of the gas plenum temperature is required to determine the amount of fission gas released from the fuel to the plenum. The gas plenum temperature will depend on natural convection of the PWC coolant, and no temperature measurement will be possible within this gap during the test. This paper describes the setting up of a model of the BR2 PWC equipped with the P2M rodlets based on the coupled NEPTUNE_CFD (multiphase fluid calculation code) and SYRTHES (solid thermal module) simulation tools. Simulations performed thanks to this model allow assessment of the thermal-hydraulic (TH) behavior of the pressurized water in the capsule and the thermal behavior of the rodlet, in particular, regarding the temperature of the gas located in the plenum. For consistency of the results, computations presented in this paper were performed using a single and consistent set of TH models. A mesh sensitivity analysis was carried out for all the studied cases. Simulation results related to the water capsule behavior were found to be in good agreement with the available experimental data. The gas plenum temperature results obtained from this study will be used to assess the fission gas release during the test from the plenum pressure measurements. Overall experimental validation of fission gas release during the test will be possible after the transient test in BR2 based on the postirradiation examination program foreseen on the rodlets at the LECA-STAR facility [Commissariat à l’énergie atomique et aux énergies alternatives (CEA) Cadarache, France].

Fuel Performance Analysis of Fast Flux Test Facility MFF-3 and -5 Fuel Pins Using BISON with Post Irradiation Examination Data

Using the BISON fuel-performance code, simulations were conducted of an automated process to read initial and operating conditions from the Pacific Northwest National Laboratory (PNNL) database and reports, which contain metallic-fuel data from the Fast Flux Test Facility (FFTF) MFF Experiments. This work builds on previous modeling efforts involving 1977 EBR-II metallic fuel pins from experiments. Coupling the FFTF PNNL reports to BISON allowed for all 338 pins from MFF-3 and MFF-5 campaigns to be simulated. Each BISON simulation contains unique power and flux histories, axial power and flux profiles, and coolant-channel flow rates. Fission-gas release (FGR), fuel axial swelling, cladding profilometry, and burnup were all simulated in BISON and compared to available post-irradiation examination (PIE) data. Cladding profilometry, FGR, and fuel axial swelling simulation results for full-length MFF metallic pins were found to be in agreement with PIE measurements using FFTF physics and models used previously for EBR-II simulations. The main two peaks observed within the cladding profilometry were able to be simulated, with fuel-cladding mechanical interaction (FCMI), fuel-cladding chemical interaction (FCCI), and thermal and irradiation-induced creep being the cause. A U-Pu-Zr hot-pressing model was included in this work to allow pore collapse within the fuel matrix. This allowed better agreement between BISON-simulated cladding profilometry and PIE measurements for the peak caused by FCMI. This work shows that metallic fuel models used to accurately represent fuel performance for smaller EBR-II pins may be used for full-length metallic fuel, such as FFTF MFF assemblies and the Versatile Test Reactor (VTR). As new material models and PIE measurements become available, FFTF MFF assessment cases will be reassessed to further BISON model development.

Extending TRANSURANUS burnup model for AGR-like FHR fuel design

This study summarises the work performed to introduce a novel methodology to derive the radial form factor in the TRANSURANUS burnup model (TUBRNP) using data from simulations. Previous work used experimental data from post-irradiation examinations to obtain the radial form factor in TUBRNP for a conventional LWR. It was updated to include coefficients suitable for a HWR. The aim of this work is the creation of a reactor-dependent methodology using data from a Monte Carlo code when experimental data are missing, but that is still in line with the previous work. This new TUBRNP model, together with recently implemented correlations for Hastelloy-N to be used as cladding and FliBe as coolant, provide an updated TRANSURANUS fuel rod performance code that can be used in ongoing investigations for AGR-like molten salt cooled reactors. The proposed methodology can also be applied to advanced technology fuels in various SMRs.

Presentation of the xM3 Test Case of the P2M Simulation Exercise and Modeling with the Fuel Performance Code ALCYONE

This paper presents simulations of the xM3 power ramp with the fuel performance code ALCYONE performed during an international simulation exercise organized within the Organisation for Economic Co-operation and Development/Nuclear Energy Agency Power to Melt and Maneuverability project. The xM3 test involved a large-grain UO2 fuel from Mitsubishi Heavy Industries cladded with Zirlo and pre-irradiated in a Spanish pressurized water reactor up to an average burnup of 27 GWd/tU−1. It was then submitted to a staircase ramp protocol in the R2 reactor at Studsvik (Sweden) with 10 successive steps of 5 kW·m−1 up to a ramp terminal level of 70 kW·m−1. The fuel rodlet did not fail, and detailed post irradiation examinations performed during the Studsvik Cladding Integrity Project II evidenced recrystallization of the pellet center around a central hole, interpreted as signs of fuel melting. In this paper, simulations with ALCYONE of the xM3 power ramp, including an advanced model for fuel melting based on thermodynamic equilibrium calculations, are detailed. The model relies on the determination of the liquid fuel fraction evolution with temperature that is used to obtain a continuous description of the material properties during phase change. In consequence of the incorporation of rare earths and actinides in the bulk of the fuel, distinct solidus and liquidus temperatures are estimated. It is shown that the observed central hole and recrystallized central part of the pellet could be the consequence of totally melted fuel (liquidus is reached), partially melted fuel (solidus is reached), or pore migration only.

Multi-parameter optimization of gamma emission tomography instruments for irradiated nuclear fuel examination

Material test reactors have an extended use in irradiation testing of novel nuclear fuel materials and the fuel behavior in off-normal conditions. The performance of the nuclear fuel is examined in in-pile and out-of-pile post-irradiation examinations (PIEs), e.g., using Gamma Emission Tomography (GET). GET is a nondestructive assay that images the internal spatial distribution of gamma-emitting nuclides built up in the fuel due to irradiation. Since GET can be performed close to the reactor and without intrusion in the fuel object, it can potentially speed up the data generation from PIE in irradiation testing.The performance metrics of GET devices can be identified regarding time requirements, noise in the reconstructed image, signal-to-background ratio, and spatial resolution. However, these are complicated to determine, partly due to inherent trade-offs between the metrics themselves, partly because they depend on the fuel activity and its spectrum (i.e., object dependent), and, finally, on the GET setup and its configuration.This work proposes a structured methodology for optimizing the collimator design for a new generation of GET tomography setups, intending to improve spatial resolution by one order of magnitude: from the millimeter scale to the hundred-micron scale. The conflicting performance metrics are determined based on the controllable parameters of the GET setup and the uncontrollable parameters of an anticipated fuel object, able to provide a signal-to-background ratio above a customized limit, chosen based on the specific application. The trade-off between the performance remaining metrics is then visualized by a Pareto approach, where dominated solutions are rejected. Finally, constraints on noise level and measurement time are used to find the optimal spatial resolution, without applying noise suppression filters.Two GET setups are presented using the outlined method. Firstly, to upgrade the tomography test bench BETTAN at Uppsala University, a new segmented HPGe detector is planned to be used with low-activity fuel rod mock-ups. Secondly, a GET system for investigating high-activity nuclear fuel rods of representative burnup. For a nuclear fuel inspection, the results showed that a spatial resolution of about 300 μm is possible with reasonable noise and measurement time constraints.