Polarization Dependence Research Articles

Strongly enhanced shift current at exciton resonances in a noncentrosymmetric wide-gap semiconductor.

Excitons are fundamental quasiparticles that are ubiquitous in photoexcited semiconductors and insulators. Despite causing a sharp and strong photoabsorption near the interband absorption edge, charge-neutral excitons do not yield photocurrent in conventional photovoltaic processes unless dissociated into free charge carriers. Here, we experimentally demonstrate that excitons can directly contribute to photocurrent generation through a nonlinear light-matter interaction in a noncentrosymmetric semiconductor CuI. Epitaxial thin films of CuI exhibit a substantial enhancement of photocurrent at exciton resonance energies even below the bandgap. From the light polarization dependence, this photocurrent is identified to be shift current, a nonlinear photocurrent driven by the change in the geometric Berry phase of electron wave functions upon the optical transition. The shift current at the exciton resonance is much larger than that induced above the band gap by free electron-hole excitation, and their signs are opposite. First-principles calculations elucidate that the sign and magnitude of the exciton shift current are strongly dependent on the strain in the thin film. The present study reveals the crucial role of excitons in enhancing the shift current magnitude and its strain sensitivity, and will open an unprecedented route for efficient manipulation of nonlinear optical effects.

Probing the Dark Universe with Gravitational Waves

Gravitational waves (GWs) are expected to interact with dark energy and dark matter, affecting their propagation on cosmological scales. To model this interaction, we derive a gauge-invariant effective equation and action valid for all GW polarizations. This is achieved by encoding the effects of GW interactions at different orders of perturbation into a polarization-, frequency-, and time-dependent effective speed. The invariance of perturbations under time-dependent conformal transformations and the gauge invariance of GWs allow us to derive the unitary gauge effective action in any conformally related frame, thereby clarifying the relationship between the Einstein and Jordan frames. Tests of the polarization and frequency dependencies in the propagation time and luminosity distance of different GW polarizations allow us to probe the dark Universe, which acts as an effective medium, modeled by the GW effective speed.

Hyperon Production in Bi + Bi Collisions at the Nuclotron-Based Ion Collider Facility and Angular Dependence of Hyperon Spin Polarization

The strange baryon production in Bi + Bi collisions at sNN=9.0 GeV is studied using the PHSD transport model. Hyperon and anti-hyperon yields, transverse momentum spectra, and rapidity spectra are calculated, and their centrality dependence and the effect of rapidity and transverse momentum cuts are studied. The rapidity distributions for Λ¯, Ξ, Ξ¯ baryons are found to be systematically narrower than for Λs. The pT slope parameters for anti-hyperons vary more with centrality than those for hyperons. Restricting the accepted rapidity range to |y|<1 increases the slope parameters by 13–30 MeV, depending on the centrality class and the hyperon mass. Hydrodynamic velocity and vorticity fields are calculated, and the formation of two oppositely rotating vortex rings moving in opposite directions along the collision axis is found. The hyperon spin polarization induced by the medium vorticity within the thermodynamic approach is calculated, and the dependence of the polarization on the transverse momentum and rapidity cuts and on the centrality selection is analyzed. The cuts have stronger effect on the polarization of Λ and Ξ hyperons than on the corresponding anti-hyperons. The polarization signal is maximal for the centrality class, 60–70%. We show that, for the considered hyperon polarization mechanism, the structure of the vorticity field makes an imprint on the polarization signal as a function of the azimuthal angle in the transverse momentum plane, ϕH, cosϕH=px/pT. For particles with positive longitudinal momentum, pz>0, the polarization increases with cosϕH, while for particles with pz<0 it decreases.

Suppression of symmetry-breaking correlated insulators in a rhombohedral trilayer graphene superlattice.

Counterintuitive temperature dependence of isospin flavor polarization has recently been found in twisted bilayer graphene, where unpolarized electrons in a Fermi liquid become a spin-valley polarized insulator upon heating. So far, the effect has been limited to v = +/-1 (one electron/hole per superlattice cell), leaving open questions such as whether it is a general property of symmetry-breaking electronic phases. Here, by studying a rhombohedral trilayer graphene/boron nitride moiré superlattice, we report that at v = -3 a resistive peak emerges at elevated temperatures or in parallel magnetic fields. Concomitantly, the Hall carrier density tends to reset at the integer filling, signaling spin-valley flavor symmetry breaking. These phenomena can also be observed at v = -1 and -2 when the displacement field is large enough to suppress correlated insulators at low temperatures. Our results greatly expand the scope for observing the counterintuitive temperature dependence of flavor polarization, i.e., the regimes proximal to symmetry-breaking phases where the flavor polarization order strongly fluctuates, encouraging more experimental and theoretical exploration of isospin flavor polarization dynamics in flat-band moiré systems.

Experimental studies of in-medium modification of [formula omitted] meson mass through [formula omitted] decays

ϕ meson is an ideal probe to explore mass modification inside the nucleus due to partial restoration of chiral symmetry with its narrow width. The modification of ϕ mass is related to the strange-quark condensate 〈s̄s〉 in a finite density. J-PARC E88 has been proposed as an experiment to study the modification of ϕ mass inside nuclei in proton–nucleus collisions. Complementary to ϕ→e+e− decay measurements at J-PARC E16, E88 will measure high-statistics ϕ→K+K− decays of about 1 M in p+C, p+Cu, and p+Pb collisions by deploying kaon identification detectors at forward angles in the E16 spectrometer. Utilizing the high-statistics data, the momentum and polarization dependence of mass modification will be studied to evaluate the strange quark condensate in nucleons, and Lorentz-symmetry breaking effects. In this paper, we will discuss physics goals, the experimental design and feasibility, the performance of kaon identification detectors, and the timeline of the E88.

High-performance and scalable polarization splitter-rotator based on photonic crystal nanobeam reflection

The polarization splitter-rotator (PSR) is a key device for polarization processing in polarization diversity systems, which has wide applications in achieving polarization independence and mixed multiplexing. However, it remains a significant challenge to simultaneously achieve a better balance in bandwidth, crosstalk (CT), polarization extinction ratio (PER), and compact footprint of the PSR. In this article, a photonic crystal nanobeam (PCN) structure is introduced to PSR for large bandwidth and compact size, with a device length of only 104 µm. Additionally, to achieve lower CT, a bridge waveguide is introduced for primary filtering. Simulation results show that the insertion loss (IL) is less than 0.55 dB, CT less than -35 dB, and PER greater than 35 dB within a bandwidth exceeding 110 nm, while maintaining a large process tolerance. Furthermore, the proposed PSR design breaks through the limitations of traditional schemes by extending its functionality effectively. To further improve integration, a novel approach to PSR using mode hybridization followed by spatial beam splitting is proposed. By controlling the phase-matching condition of various modes in different waveguides, the designed spatial beam splitting achieves lower CT and better compactness. Simulation results verify that the IL of the improved scheme is less than 1 dB, CT less than -24 dB, and PER greater than 22 dB within an 85 nm bandwidth, while reducing the overall length to less than 20 µm.

Quarkonium polarization in medium from open quantum systems and chromomagnetic correlators

We study the spin-dependent in-medium dynamics of quarkonia by using the potential nonrelativistic QCD (pNRQCD) and the open quantum system framework. We consider the pNRQCD Lagrangian valid up to the order rM0=r and r0M=1M in the double power counting. By considering the Markovian condition and applying the Wigner transformation upon the diagonal spin components of the quarkonium density matrix with the semiclassical expansion, we systematically derive the Boltzmann transport equation for quarkonia with polarization dependence in the quantum optical limit. Unlike the spin-independent collision terms governed by certain chromoelectric field correlators, new gauge invariant correlators of chromomagnetic fields determine the recombination and dissociation terms with polarization dependence at the order we are working. We also derive a Lindblad equation describing the in-medium transitions between spin-singlet and spin-triplet heavy quark-antiquark pairs in the quantum Brownian motion limit. The Lindblad equation is governed by new transport coefficients defined in terms of the chromomagnetic field correlators. Our formalism is generic and valid for both weakly coupled and strongly coupled quark gluon plasmas. It can be further applied to study spin alignment of vector quarkonia in heavy ion collisions. Published by the American Physical Society 2024

Angle‐Resolved Polarized Raman Study of Layered Cr2Se3

ABSTRACTThe polarization‐resolved Raman spectra of two‐dimensional Cr2Se3 synthesized via chemical vapor deposition (CVD) and chemical vapor transport (CVT) techniques were investigated in detail. The samples were characterized using X‐ray diffraction (XRD), transmission electron microscopy (TEM), and energy‐dispersive X‐ray spectroscopy (EDS). A distinct polarization dependence was observed in the Raman intensity of all the Cr‐Cr, Cr‐Se, and Se‐Se modes in both samples. The observed angle‐dependent Raman intensities of each peak could be related to the crystal structure‐specific Raman tensor. XRD results of the bulk Cr2Se3 sample synthesized via CVT confirm its trigonal crystal structure, and the Raman peaks can be fitted using the Raman tensors for the 𝐴𝑔 and 𝐸𝑔 modes for both the parallel and crossed polarizations. However, for the Cr2Se3 samples directly grown on Si/SiO2 substrates by CVD, it was necessary to assume the triclinic crystal structure in order to explain the polarized Raman dependence of all the peaks in both parallel and crossed polarization directions. This is the first experimental result suggesting the existence of triclinic Cr2Se3 crystal structure, which has been theoretically predicted in the Materials Project database.

Phase transition investigation of ferroelectric and dielectric properties of (NH 2 CH 2 COOH)3 H2SO4 crystal using green function method and two sublattice PLCM model Hamiltonian

The Greens function technique and extended two sublattice pseudospin lattice coupled-mode (PLCM) model Hamiltonian have been applied to study the phase transition mechanism in (NH2CH2COOH)3H2SO4 compound. The two sublattice PLCM model Hamiltonian is modified by considering anharmonic phonon interactions, extra spin-lattice interactions, and an external applied electric field term. By using the double-time thermal-dependent Green function technique, the theoretical equations for the total shift, total width, normal mode frequency, transition temperature, relative permittivity, dielectric tangent loss, acoustic attenuation and spontaneous polarization are derived. By fitting the distinct model parameters in the theoretical equations, we calculated the temperature dependence of normal mode frequency, relative permittivity, tangent loss, acoustic attenuation and spontaneous polarization. The numerically obtained results are hold well and correlated with experimental data.

Modeling photomolecular effect using generalized boundary conditions for Maxwell equations

We recently demonstrated via experiments in hydrogels and at a single air-water interface the photomolecular effect: photons directly cleaving off water molecular clusters in the visible spectrum where bulk water has negligible absorption. To model single interface experiments, here we re-derive generalized boundary conditions for Maxwell equations by assuming a transition region of the electromagnetic fields across the interface, leading naturally to the Feibelman parameters used before to describe surface photoelectric and surface plasmon effects on metals. This generalization leads to modifications of the Fresnel coefficients and an expression for the surface absorptance that can reasonably explain trends in our single-interface experimental data on the angle and polarization dependence of the beam deflection. Our work provides further support for the existence of the photomolecular effect, suggests that surface absorption should exist in many materials, and lays a foundation for assessing the impacts of such surface absorption based on the Maxwell equations.

Demonstration of 4-quadrant analog in-memory matrix multiplication in a single modulation

Analog in-memory computing (AIMC) leverages the inherent physical characteristics of resistive memory devices to execute computational operations, notably matrix-vector multiplications (MVMs). However, executing MVMs using a single-phase reading scheme to reduce latency necessitates the simultaneous application of both positive and negative voltages across resistive memory devices. This degrades the accuracy of the computation due to the dependence of the device conductance on the voltage polarity. Here, we demonstrate the realization of a 4-quadrant MVM in a single modulation by developing analog and digital calibration procedures to mitigate the conductance polarity dependence, fully implemented on a multi-core AIMC chip based on phase-change memory. With this approach, we experimentally demonstrate accurate neural network inference and similarity search tasks using one or multiple cores of the chip, at 4 times higher MVM throughput and energy efficiency than the conventional four-phase reading scheme.

Spatial imaging of polarized deuterons at the Electron-Ion Collider

We study diffractive vector meson production at small-x in the collision of electrons and polarized deuterons e+d↑. We consider the polarization dependence of the nuclear wave function of the deuteron, which results in an azimuthal angular dependence of the produced vector meson when the deuteron is transversely polarized. The Fourier coefficients extracted from the azimuthal angular dependence of the vector meson differential cross-section exhibit notable differences between longitudinally and transversely polarized deuterons. The angular dependence of the extracted effective deuteron radius provides direct insight into the structure of the polarized deuteron wave function. Furthermore, we observe slightly increased gluon saturation effects when the deuteron is longitudinally polarized compared to the transversely polarized case. The small-x observables studied in this work will be accessible at the future Electron-Ion Collider.

Impact of polarization pulling on optimal spectrometer design for stimulated Brillouin scattering microscopy.

Brillouin spectroscopy has become an important tool for mapping the mechanical properties of biological samples. Recently, stimulated Brillouin scattering (SBS) measurements have emerged in this field as a promising technology for lower noise and higher speed measurements. However, further improvements are fundamentally limited by constraints on the optical power level that can be used in biological samples, which effectively caps the gain and signal-to-noise ratio (SNR) of SBS biological measurements. This limitation is compounded by practical limits on the optical probe power due to detector saturation thresholds. As a result, SBS-based measurements in biological samples have provided minimal improvements (in noise and imaging speed) compared with spontaneous Brillouin microscopy, despite the potential advantages of the nonlinear scattering process. Here, we consider how a SBS spectrometer can circumvent this fundamental trade-off in the low-gain regime by leveraging the polarization dependence of the SBS interaction to effectively filter the signal from the background light via the polarization pulling effect. We present an analytic model of the polarization pulling detection scheme and describe the trade-space unique to Brillouin microscopy applications. We show that an optimized receiver design could provide >25× improvement in SNR compared to a standard SBS receiver in most typical experimental conditions. We then experimentally validate this model using optical fiber as a simplified test bed. With our experimental parameters, we find that the polarization pulling scheme provides 100× higher SNR than a standard SBS receiver, enabling 100× faster measurements in the low-gain regime. Finally, we discuss the potential for this proposed spectrometer design to benefit low-gain spectroscopy applications such as Brillouin microscopy by enabling pixel dwell times as short as 10 μs.

Use of the 5P3/2→6P3/2 electric dipole forbidden transition in Rb as a non-perturbing probe of atom dynamics in an operating magneto-optical trap

Abstract Results of spectroscopy experiments using the $5P_{3/2} \to 6P_{3/2}$ electric dipole forbidden transition in cold rubidium atoms are presented. Production of this forbidden transition is detected by observing the emission of the $420 $ nm fluorescence photons that result from the decay of the $6P_{3/2} $ state into the ground state. The experiments are performed under the steady state operation conditions of a magneto-optical trap (MOT), and thus provide non-perturbing information on the atom-light system. The hyperfine structure of the $6P_{3/2}$ level is completely resolved, and the fluorescence peaks show the expected Autler-Townes (AT) splitting of the emission lines. This hyperfine structure is used to calibrate the frequency scale of all spectra recorded. A combination of this absolute frequency scale and an expression for the AT profile allows an absolute determination of the effective Rabi frequency and detuning of the MOT. The behavior of these AT doublets is studied as a function of frequency detuning and also as a function of the trapping light intensity.
The experiments also take full advantage of the strong polarization dependence of the relative intensities of the hyperfine fluorescence components.
This study results in a sensitive probe of the relative populations of the magnetic sublevel projections relative to the trapping magnetic field gradient.
An almost isotropic population distribution was found, but small deviations from isotropy could be determined with this electric dipole forbidden probe.

Changes in the longitude polarization dependence of Jupiter's moon Io as evidence of the long-term variability of its volcanic activity

The aim of the work was to investigate the longitude (orbital) dependence of the polarization of Jupiter's moon Io and compare results of our study with what is reported in the literature. We used our published observations and supplemented them with new measurements carried out with the polarimeters mounted on the 2.6 m Shajn telescope of the Crimean Astrophysical Observatory and the 2 m telescope of the Peak Terskol Observatory in the UBVRI bands at phase angles between 10° and 12° in August 2023 – February 2024. We have determined that amplitude of the orbital polarization in the V band does not exceed ≈0.1 %. It is the deepest −0.17 ± 0.03 % at L ≈ 270° and the shallowest −0.07 ± 0.03 % near L ≈ 130°. These parameters differ markedly from that obtained by Zellner and Gradie (1975), which found that the orbital polarization variations from 0.4 to 0.5 % for α > 10°, and the negative branch is the deepest near L = 160° and the shallowest near L = 300°. These differences may be a consequence of changes in the reflective properties of the local areas of Io's surface due to long-term changes in Io's local or global volcanic activity.

Tunneling Barrier Thickness Dependence of Spin Polarization of Ferromagnet in Magnetic Tunnel Junctions

Abstract For designing low-impedance magnetic tunnel junctions (MTJs), it has been found that tunneling magnetoresistance strongly correlates with the insulating barrier thickness, imposing a fundamental problem about the relationship between spin polarization of ferromagnet and the insulating barrier thickness in MTJs. Here, we investigate the influence of alumina barrier thickness on tunneling spin polarization (TSP) through a combination of theoretical calculations and experimental verification. Our simulating results reveal a significant impact of barrier thickness on TSP, exhibiting an oscillating decay of TSP with the barrier layer thinning. Experimental verification is realized on FeNi/AlO x /Al superconducting tunnel junctions to directly probe the spin polarization of FeNi ferromagnet using Zeeman-split tunneling spectroscopy technique. These findings provide valuable insights for designs of high-performance spintronic devices, particularly in applications such as magnetic random access memories, where precise control over the insulating barrier layer is crucial.

High-accuracy direction measurement and high-resolution computational spectral reconstruction based on photonic crystal array

Portable and wearable miniaturized spectrometers play a crucial role in various fields. In this paper, we present a method for simultaneously realizing high-accuracy direction measurement and high-resolution computational spectral reconstruction based on the angle sensitivity of conventional photonic crystals (PCs), wherein an optical filter array is composed of multiple one-dimensional PCs. The high-angle sensitivity of PCs results in angle-dependent optical spectra. When these spectra with different angles are used to reconstruct the target spectra in an unknown direction and the interval between adjacent angles is sufficiently small, the accurate direction of the target can be automatically identified. Moreover, the computational spectra still have high resolution over a wide range of incidences. The computational spectra under arbitrary polarizations can also be recognized based on the polarization dependence of the PCs at an oblique incidence. Our research results are significant for engineering a new miniaturized comprehensive computational spectrometer with target-direction perception and omnidirectional spectral reconstruction abilities.

Room‐Temperature Single‐Molecule Infrared Imaging and Spectroscopy through Bond‐Selective Fluorescence

Infrared (IR) spectroscopy stands as a workhorse for exploring bond vibrations, offering a wealth of chemical insights across diverse frontiers. With increasing focus on the regime of single molecules, obtaining IR‐sensitive information from individual molecules at room temperature would provide essential information about unknown molecular properties. Here, we leverage bond‐selective fluorescence microscopy, facilitated by narrowband picosecond mid‐IR and near‐IR double‐resonance excitation, for high‐throughput mid‐IR structural probing of single molecules. We robustly capture single‐molecule images and analyze the combined polarization dependence, vibrational peaks, linewidths, and lifetimes of probe molecules with representative scaffolds. From bulk to single molecules, we find that vibrational lifetimes remain consistent, while linewidths are narrowed by approximately twofold and anisotropy becomes more pronounced. Additionally, unexpected peak shifts from single molecules were observed, attributed to the generation of new modes due to previously unexplored dimerization, supported by quantum chemistry calculations. These findings underscore the importance of infrared analysis on individual single molecules in ambient environments, offering molecular information crucial for functional imaging and the investigation of the fundamental properties and utilities of luminescent molecules.

Room-Temperature Single-Molecule Infrared Imaging and Spectroscopy through Bond-Selective Fluorescence.

Infrared (IR) spectroscopy stands as a workhorse for exploring bond vibrations, offering a wealth of chemical insights across diverse frontiers. With increasing focus on the regime of single molecules, obtaining IR-sensitive information from individual molecules at room temperature would provide essential information about unknown molecular properties. Here, we leverage bond-selective fluorescence microscopy, facilitated by narrowband picosecond mid-IR and near-IR double-resonance excitation, for high-throughput mid-IR structural probing of single molecules. We robustly capture single-molecule images and analyze the combined polarization dependence, vibrational peaks, linewidths, and lifetimes of probe molecules with representative scaffolds. From bulk to single molecules, we find that vibrational lifetimes remain consistent, while linewidths are narrowed by approximately twofold and anisotropy becomes more pronounced. Additionally, unexpected peak shifts from single molecules were observed, attributed to the generation of new modes due to previously unexplored dimerization, supported by quantum chemistry calculations. These findings underscore the importance of infrared analysis on individual single molecules in ambient environments, offering molecular information crucial for functional imaging and the investigation of the fundamental properties and utilities of luminescent molecules.

Ultra-wideband solar absorber via vertically structured GDPT metamaterials

We explore a new solar absorber via vertically structured metamaterials integrating 2D graphene, dielectric layers of silica (SiO2), aluminum oxide (Al2O3), and phase-transition vanadium dioxide (VO2) graphene, dielectric, phase transition (GDPT), achieving broadband absorption and polarization independence. Applying the finite-difference time-domain (FDTD) method, the optical performance of the absorber is analyzed under the normal incidence of a plane wave spanning wavelengths from 250 to 4000 nm. Particularly, our investigation reveals a broad bandwidth exceeding 90 % absorption, spanning 3559 nm from 250 to 3809 nm, with an impressive average absorption efficiency of over 95.9 %. Significantly, the absorber demonstrates polarization independence and insensitivity to large angles of incidence, enhancing its practical capability. We illuminate the important role of Fabry-Perot resonance in absorption by precisely tuning layer thicknesses to induce interference effects. The integration of graphene, dielectric layers, and VO2, augmented by Fabry-Perot resonance, provides a vital foundation for high-performance solar energy conversion technology. This technology has important applications in efficient and broadband solar absorbers, and these absorbers can maintain high performance under different conditions. Our goal is to solve current technological challenges and contribute to the development of next-generation solar energy conversion for various photon technologies, such as energy harvesting, electromagnetic wave capture, and photovoltaic devices.