Picosecond Pulses Research Articles

Néel Vector Auto-Oscillations and Reorientations Induced by Spin-Polarized Electric Currents in Antiferromagnetic Mn2Au Nanolayer

The electrical excitation of spin dynamics in antiferromagnets is important for the development of high-speed spintronic devices with a low power consumption. Here, we present a theoretical study of the spin dynamics generated in the Ni/Cu/Mn2Au/Cu/Ni nanostructure by a perpendicular-to-plane electric current. Our investigation includes atomistic simulations of spin reorientations in a few monolayer antiferromagnetic Mn2Au film and numerical calculations of nonequilibrium spin accumulation in the nanostructure comprising ferromagnetic Ni polarizers with antiparallel magnetizations. This combined approach enables us to quantify the dynamics of Mn magnetic moments induced by the spin-transfer torque created by the spin-polarized charge flow. The calculations show that the direct electric current with the density exceeding some temperature-dependent threshold value gives rise to steady-state auto-oscillations of the Néel vector in the [Formula: see text]-oriented Mn2Au nanolayer. As the precession of Mn magnetic moments occurs around an out-of-plane direction strongly deflected from their initial in-plane orientations, the emergence of auto-oscillations should be regarded as the realization of a dynamic spin reorientation transition in the antiferromagnetic crystal. Remarkably, the precession frequency rises with increasing current density J and exceeds 1[Formula: see text]THz at [Formula: see text][Formula: see text]A[Formula: see text]m[Formula: see text], which makes the described antiferromagnetic spin transfer nano-oscillator attractive for device applications. Furthermore, our simulations demonstrate that a picosecond current pulse injected into the Ni/Cu/Mn2Au/Cu/Ni nanostructure can induce a precessional switching of the Néel vector. Depending on the current density and pulse duration, the Néel vector rotates by either 90° or 180° and attains stable orientation along the corresponding [Formula: see text] easy axis in the plane of the Mn2Au nanolayer. This feature shows that the Ni/Cu/Mn2Au/Cu/Ni nanostructure could be used as a nonvolatile memory cell with the electrical writing and readout.

Needle-Free Targeted Injections Using Bubble Laser Technology in Therapeutics.

This work explores bubble laser technology as an alternative to needles in injection systems for vaccination, cancer treatment, insulin delivery, and catheter hygiene. The technology leverages laser-induced microfiltration and bubble dynamics to create high-speed pneumatic jets that penetrate the skin without needles, addressing discomfort, infection risk, and needle-related concerns. The system's performance is analyzed based on laser wavelength, pulse duration, and Gaussian beam droplet size. The findings indicate a significant increase in spot size at 1064 nm compared with 400 nm, consistent with the diffraction theory. Induced bubble dynamics reveal bubble generation, jetting, and fluid interactions as the Weber number increases, as well as jet velocity and fluid inertia. For femtosecond pulses, increasing the pulse duration from 100 to 1500 fs reduces the bubble lifespan from 0.8 to 0.3 arbitrary units, and the collapse pressure decreases from 2.1 to 0.4 bar. For picosecond pulses, the bubble lifetime decreases from 0.9 to 0.5 arbitrary units, and the pressure drop decreases from 2.0 to 0.4 bar as the pulse length extends from 2000 to 8000 ps. Jet formation in laser jet injection systems is enhanced by short pulses in water that produce longer-lasting bubbles. Drug delivery based on the Rayleigh-Plesset equation is characterized by a low-pressure collapse and short bubble lifetime. Thus, this relationship suggests that bubble laser technology can provide a more controlled and safer method of needle-free procedures, increasing compliance and reducing tissue trauma.

Near-infrared-terahertz hyper-Raman spectroscopy of an excited silicon surface.

We recorded the hyper-Raman spectra resulting from the interaction of a near-infrared (near-IR) picosecond pulse and a terahertz (THz) ultrashort pulse at the surface of a (111) silicon sample. A simple model is proposed to analyze the evolution of the hyper-Raman spectra vs the time delay between the near-IR and THz pulses. It links the hyper-Raman spectra to the multi-phonon absorption in silicon. This approach makes it possible to demonstrate that, during carrier generation by the near-IR pulse, the two-phonon and three-phonon absorption bands are enhanced in modes involving optical phonons. This process results from the very rapid and strong population of the optical phonons induced by the photo-generated hot carriers. It occurs over a few hundreds of femtoseconds and lasts throughout the duration of the near-IR pulse.

Comparative analysis of microlens array formation in fused silica glass by laser: Femtosecond versus picosecond pulses

The growing demand for flexible, high-quality fabrication of free-form micro-optics drives the development of laser-based fabrication techniques for both the shape formation and surface polishing of optical elements. In this paper, we performed a thorough and systematic study on fused silica glass ablation using 10 ps and 320 fs duration pulses. Ablation processes for both pulse durations were optimized based on the measurements of the removed material layer thickness and surface roughness, and by analyzing the topographies of ablated cavities to remove material layers as thin as possible with minimum surface damage. Our findings demonstrate higher process resolution and surface quality for femtosecond pulses. Ablation of pre-roughened glass reduced the minimal removable glass layer thickness well below the 1 μm mark for both pulse durations, improving the process resolution. The minimal removable glass layer thickness was 14 times smaller for the femtosecond pulses, with up to 4.5 times lower surface roughness compared to samples processed with picosecond pulses. On the other hand, results revealed faster glass removal rates with picosecond pulses. In the end, arrays of microlenses were fabricated with both pulse durations and subsequently polished with a CO2 laser. Results revealed higher performance of microlenses fabricated with femtosecond pulses, providing better focusing capabilities and lesser beam scattering. Finally, this study demonstrated the successful fabrication of free-form optical elements with femtosecond and picosecond pulses, demonstrating the versatility and the potential of laser-based techniques.

Surface roughness metrology with a raster scanning single photon LiDAR

We explore a novel, to the best of our knowledge, approach to surface roughness metrology utilizing a single pixel, raster scanning single photon counting LiDAR system. It uses a collimated laser beam in picosecond pulses to probe a surface, capturing the changes of back-scattered photons from different points on the surface into a single mode fiber, and counting them using a single photon detector. These back-scattered photons carry speckle noise produced by the rough surface, and the variation in photon counts over different illumination points across the surface becomes a good measure of its roughness. By analyzing the variation frequency as the LiDAR scans over the surface using machine learning techniques, we demonstrate general measurements of surface roughness from 1.21 (1.27±4.51) to 102.01 (87.97±10.55) microns.

Industrial picosecond pulse laser welding of stainless-steel to quartz for optical applications

We report on the development of a robust picosecond laser welding process for the industrially relevant material combination of quartz and stainless steel. The process requires high numerical aperture focusing of a 6 ps 1030 nm laser through the transparent quartz onto the interface between the two materials. It is found that increased mechanical pressure applied during welding increases reliability and weld performance and with the correct choice of welding parameters parts will survive ISO standard thermal cycling and vibration testing demonstrating the suitability of the process for industrial application.

Optical Dynamics of Picosecond Pulse Trains in Aluminum and Zinc Tetracarboxy-Phthalocyanines

Optical Dynamics of Picosecond Pulse Trains in Aluminum and Zinc Tetracarboxy-Phthalocyanines

Pulse length effects in the nonresonant long-wave infrared nonlinear optical response of n-Ge, GaAs, and ZnSe

Nonlinear optical refraction and nonlinear absorption are characterized in important long-wave infrared optical materials with picosecond and femtosecond laser pulses. The effective nonlinear refractive indices are found to be constant across a range of pulse parameters. Nonlinear absorption far from resonance is observed at relatively low (∼1GW/cm2) intensities in these materials, and the onset intensity and fluence scale strongly with pulse length. A free carrier dominated nonlinear absorption mechanism is identified for picosecond pulses, whereas nonperturbative photoionization causes femtosecond absorption.

Experimental Proof of the Effect of Induced Optical Coalescence of Bubston Clusters at Water Breakdown Induced by Picosecond and Nanosecond Laser Pulses

Experimental Proof of the Effect of Induced Optical Coalescence of Bubston Clusters at Water Breakdown Induced by Picosecond and Nanosecond Laser Pulses

Silicon heterojunction back contact solar cells by laser patterning.

Back contact silicon solar cells, valued for their aesthetic appeal by removing grid lines on the sunny side, find applications in buildings, vehicles and aircrafts, enabling self-power generation without compromising appearance1-3. Patterning techniques arrange contacts on the shaded side of the silicon wafer, offering benefits for light incidence as well. However, the patterning process complicates production and causes power loss. Here we employ lasers to streamline back contact solar cell fabrication and enhance power conversion efficiency. Our approach produces the first silicon solar cell to exceed 27% efficiency. Hydrogenated amorphous silicon layers are deposited on the wafer for surface passivation and collection of light-generated carriers. A dense passivating contact, diverging from conventional technology practice, is developed. Pulsed picosecond lasers at different wavelengths are used to create back contact patterns. The developed approach is a streamlined process for producing high-performance back contact silicon solar cells, with a total effective processing time of about one-third that of emerging mainstream technology. To meet terawatt demand, we develop rare indium-less cells at 26.5% efficiency and precious silver-free cells at 26.2% efficiency. The integration of solar solutions in buildings and transportation is poised to expand with these technological advancements.

Efficient high-power 1.9 µm picosecond Raman laser in H2-filled hollow-core fiber without generation of rotational lines

In this paper, an efficient high-power 1.9 µm picosecond Raman laser through pure vibrational stimulated Raman scattering (SRS) in H2-filled hollow-core fiber (HCF) is demonstrated. The maximum Raman conversion efficiency of 34 % and the Raman power of 7.3 W (36.5 µJ) is achieved within a 130 cm length of our in-house fabricated fiber. By controlling the H2 pressure, the high-order Stokes and rotational Stokes/anti-Stokes will not be generated, thereby enhancing the efficacy of the 1st Stokes conversion. In addition, the vibrational anti-Stokes are produced inevitably, which can be explained by the phase-matching of higher-order modes. Our results show SRS in H2-filled HCF to be a promising method for generating high-power 1.9 µm picosecond pulses, which are valuable in spectroscopy, defense, and efficient nonlinear conversion.

Energy-efficient picosecond spin-orbit torque magnetization switching in ferro- and ferrimagnetic films.

Electrical current pulses can be used to manipulate magnetization efficiently via spin-orbit torques. Pulse durations as short as a few picoseconds have been used to switch the magnetization of ferromagnetic films, reaching the terahertz regime. However, little is known about the reversal mechanisms and energy requirements in the ultrafast switching regime. In this work we quantify the energy cost for magnetization reversal over seven orders of magnitude in pulse duration, in both ferromagnetic and ferrimagnetic samples, bridging quasi-static spintronics and femtomagnetism. To this end, we develop a method to stretch picosecond pulses generated by a photoconductive switch by an order of magnitude. Thereby we can create current pulses from picoseconds to durations approaching the pulse width available with commercial instruments. We show that the energy cost for spin-orbit torque switching decreases by more than an order of magnitude in all samples when the pulse duration enters the picosecond range. We project an energy cost of 9 fJ for a 100 × 100 nm2 ferrimagnetic device. Micromagnetic and macrospin simulations unveil a transition from a non-coherent to a coherent magnetization reversal with a strong modification of the magnetization dynamical trajectories as pulse duration is reduced. Our results show the potential for high-speed magnetic spin-orbit torque memories and highlight alternative magnetization reversal pathways at fast timescales.

Subnanosecond 1.3-μm laser for generating picosecond pulses in the long-wavelength infrared range

Subnanosecond 1.3-μm laser for generating picosecond pulses in the long-wavelength infrared range

Statistical features of the response of a superconducting hot-electron bolometer to extremely weak terahertz pulses of picosecond and nanosecond duration

We study the statistical distributions of the output signals of a superconducting hot-electron bolometer (HEB) detector exposed to weak photon pulses of 1 THz (terahertz) frequency. Pulses with variable photon numbers were generated through strongly non-degenerate parametric downconversion (PDC) in a LiNbO3 crystal at 4.8 K. Fundamental differences in histograms are found between two PDC pumping modes, with pulse widths of 28 ps and 10 ns. HEB response to a picosecond THz pulse was detected in the form of a single elementary electrical pulse (SEP), with the average amplitude proportional to radiation intensity and dispersion relative to the bolometer's dark current. HEB responses to extremely weak radiation intensities have been recorded using nanosecond pulsed illumination. We found that nanosecond histograms are asymmetrical and broaden as radiation intensity increases, indicating that the nanosecond response consists of several SEPs. Poisson–Gauss approximation of histograms indicates that not only the average number of SEPs increase but also the average amplitude of a SEP increases with increasing power of incident THz radiation.

Analysis of high-quality ultrashort pulse generation based on a dual-drive Mach-Zehnder modulator and chirp compensation

This study reports on high-quality picosecond pulse generation using a single-stage dual-drive Mach-Zehnder modulator (DDMZM) and chirp compensation. Sinusoidal microwave signals with different amplitudes are sent to two RF ports of the DDMZM to form a pulse train and pulse compression is achieved by compensating for the linear frequency chirp with a single-mode fiber (SMF). Three parameters encompassing the power difference between two RF signals, the power of RF signals, and the bias point of the DDMZM that affect the pulse formation have been numerically studied. The optimum length of SMF used for chirp compensation is obtained by simulating the temporal propagation and evolution of the pulse in SMF and 3.56-ps chirp-compensated ultrashort pulses are realized at 1.55 µm with a 25-GHz repetition rate experimentally. Modulator-based flexible ultrashort pulse generation can be achieved easily by tuning the RF generator and light source, and customized high-quality pulses according to practical applications can be expected.

Strong Spin-Motion Coupling in the Ultrafast Dynamics of Rydberg Atoms.

Rydberg atoms in optical lattices and tweezers is now a well-established platform for simulating quantum spin systems. However, the role of the atoms' spatial wave function has not been examined in detail experimentally. Here, we show a strong spin-motion coupling emerging from the large variation of the interaction potential over the wave function spread. We observe its clear signature on the ultrafast many-body nanosecond-dynamics of atoms excited to a Rydberg S state, using picosecond pulses, from an unity-filling atomic Mott-insulator. We also propose an approach to tune arbitrarily the strength of the spin-motion coupling relative to the motional energy scale set by trapping potentials. Our work provides a new direction for exploring the dynamics of strongly correlated quantum systems by adding the motional degree of freedom to the Rydberg simulation toolbox.

Generating tunable picosecond pulses at 900 nm directly from the all-fiber structured parametric oscillator

In this work, we present an all-fiber structured parametric oscillator capable of directly generating pulses within the 900 nm wavelength range. Leveraging the four-wave mixing effect within photonic crystal fibers, the oscillator converts the 1030 nm pump light into two distinct sidebands centered at 900 nm and 1250 nm. Employing time-dispersion-tuning techniques, we achieved a remarkable continuously tunable wavelength range spanning 60 nm, from 865 nm to 925 nm. These pulses exhibited a pulse width of 3.2 ps and a peak power of 500 W at 900 nm, with a repetition rate of 30.6 MHz.

High-power hollow-core fiber gas laser at 3.1 µm with a linear-cavity structure.

Mid-infrared hollow-core fiber (HCF) gas lasers based on a population inversion regime of gas molecules have made advanced development in recent years, but mostly with single-pass cavity-free structures. Here, we demonstrated a 3.1 µm high-power acetylene-filled HCF continuous wave (CW) laser and a self-Q-switched pulse laser with a linear-cavity structure. This configuration not only facilitates the transformation of amplified spontaneous emission into the laser output but also enhances the coherence of the light source and imparts distinct cavity mode characteristics. Harnessing a homemade high-power 1535 nm single-frequency fiber laser that served as the pump source, a CW laser output of 8.23 W at 3.1 µm was achieved, which is over three orders of magnitude higher than those in reported works so far. The corresponding slope efficiency of 31.8% and beam quality of Mx 2 = 1.18 and My 2 = 1.15 were characterized. When the gas pressure was up to 50 mbar, the laser generated a 3.1 µm self-Q-switched pulse with an output power of 1.98 W as well as a pulse width of 45 ns under the repetition rate of 4.59 MHz. To the best of our knowledge, this is the first time that an HCF gas laser achieves a self-Q-switched pulse. Future studies will aim to further optimize the experimental setup, potentially enabling the direct generation of picosecond pulses in the mid-infrared wavelength band.

Efficient multiphoton microscopy with picosecond laser pulses.

Multiphoton microscopes employ femtosecond lasers as light sources because the high peak power of the ultrashort pulse allows for multiphoton excitation of fluorescence in the examined sample. However, such short pulses are susceptible to broadening in a microscope's highly dispersive optical elements and require careful dispersion management, otherwise decreasing excitation efficiency. Here, we have developed a 10 nJ Yb:fiber picosecond laser with an integrated pulse picker unit and evaluated its performance in multiphoton microscopy. Our results show that performance comparable to femtosecond pulses can be obtained with picosecond pulses only by reducing the pulse repetition rate and that such pulses are significantly less prone to the effect of chromatic dispersion. These findings proved that the temporal pulse compression is not always efficient, and it can be omitted by using a smaller and easier-to-use all-fiber setup.

Modification of nanoparticles synthesized during ablation of metals in water using nanosecond, picosecond, and femtosecond pulses

We show that the pulse duration of laser radiation used for metal ablation in water affects the nanoparticle morphology over a two-month aging period. Aluminum, copper, indium, and zinc spherical nanoparticles evolved into the elliptical, triangular, seed-like, rod-like, and rectangular forms. The most effective transformation of spherical nanoparticles into nonspherical shapes occurred with picosecond pulse ablation. Spectral analysis of the aged nanoparticle suspensions revealed changes in both the visible and UV ranges. Our study showed the correlation between the suppression of the surface plasmon resonances of the suspensions of aged nanoparticles and modification of spherical structures toward the nonspherical nano- and microparticles.