Periodically-poled Crystal Research Articles

Scaling narrowband THz generation to large apertures in LiNbO3 and KTP.

Millijoule-scale pulses of multicycle terahertz radiation (MC-THz) are increasingly being pursued as drivers for applications requiring high-fields and high spectral brightness. An attractive approach for generating high peak-power MC-THz pulses is nonlinear optical down-conversion of laser pulses in periodically-poled crystals. A principal limitation to the yield, however, is the small (sub-centimeter) apertures of commercially-available crystals which restrict the amount of laser energy that can be used. Here, we explore MC-THz generation by down conversion in two types of large-aperture media for which periodic poling has been achieved in different ways: (1) extension of traditional, voltage-based poling of bulk material to larger (centimeter) scales; and (2) manual poling by assembly of large aperture sub-millimeter thick wafers in alternating orientations. We explore the dependence of efficiency on laser peak fluence and crystal length for both types of media and extend upon previous work with the wafer approach by increasing the number of wafers in the stack, implementing cryogenic cooling and testing an alternate material: potassium titanyl phosphate (KTP). Driving with up to 0.2 J, half-picosecond laser pulses centered at 1,030 nm, we obtain conversion efficiencies of up to 0.14%, resulting in ∼1% bandwidth MC-THz pulses of up to 207 μJ.

基于单块周期极化晶体的级联三倍频蓝光输出技术的研究

基于单块周期极化晶体的级联三倍频蓝光输出技术的研究

Tunable diffraction-free array in nonlinear photonic crystal

Diffraction-free beams have attracted increasing research interests because of their unique performances and broad applications in various fields. Although many methods have been developed to produce such beams, it is still challenging to realize a tunable non-diffracting beam. Here, we report the generation of a tunable diffraction-free array through second-harmonic generation in a nonlinear photonic crystal, i.e., a 2D periodically-poled LiTaO3 crystal. In such a crystal, the second-harmonic wave is engineered by properly designing the domain structure based on the Huygens-Fresnel principle. The characteristics of the generated diffraction-free array including its period, propagation length, and wavelength can be tuned by simply changing the input wavelength. Our observation not only enriches the diffraction-free optics, but also has potential applications for photolithography and imaging.

Frequency up-conversion of quantum images

We develop the theory of frequency up-conversion of an arbitrary spatially-broadband quantum state (quantum image), deriving the analytical solutions for the cases of plane-wave pump and short crystal with arbitrary pump. By using an example of the quantum image imposed by the orbital angular momentum of the pump beam in spontaneous parametric down-conversion, we show that 99%-fidelity up-conversion of quantum images from an infrared wavelength to the visible wavelength can be obtained in periodically-poled lithium-niobate crystals at reasonable pump intensities well below the crystal damage threshold.

Observation of spontaneous polarization misalignments in periodically poled crystals using second-harmonic generation microscopy

Periodically poled crystal (PPC) is a key component for nonlinear optical applications. Its poling quality relies largely on successful domain inversion and the alignment of spontaneous polarization (SP) vectors in each domain. Here we report the unexpected observation of bulk second harmonic generation (SHG) in PPC when excitation propagating along its optical axis. Based on its tensorial nature, SHG is highly sensitive to the orientation of SP, and therefore the misalignment of SP in each domain of PPC can be revealed noninvasively by SHG microscopy. This nonlinear imaging modality provides optical sectioning capability with 3D sub-micrometer resolution, so it will be useful for in situ investigation of poling quality in PPC.

Three-photon states in nonlinear crystal superlattices

It has been a longstanding goal in quantum optics to realize controllable sources generating joint multiphoton states, particularly, photon triplet with arbitrary spectral characteristics. We demonstrate that such sources can be realized via cascaded parametric down-conversion (PDC) in superlattice structures of nonlinear and linear segments. We consider scheme that involves two parametric processes: $\omega_{0}\rightarrow\omega_{1}+\omega_{2}$, $\omega_{2}\rightarrow\omega_{1}+\omega_{1}$ under pulsed pump and investigate spontaneous creation of photon triplet as well as generation of high-intensity mode in intracavity three-photon splitting. We show preparation of Greenberger-Horne-Zeilinger polarization entangled states in cascaded type-II and type-I PDC in framework of consideration dual-grid structure that involves two periodically-poled crystals. We demonstrate the method of compensation of the dispersive effects in non-linear segments by appropriately chosen linear dispersive segments of superlattice for preparation heralded joint states of two polarized photons. In the case of intracavity three-photon splitting, we concentrate on investigation of photon-number distributions, third-order photon-number correlation function as well as the Wigner functions. These quantities are observed both for short interaction time intervals and in over transient regime, when dissipative effects are essential.

Intense ultra-broadband down-conversion from randomly poled nonlinear crystals

Randomly poled nonlinear crystals are shown to be able to emit intense ultra-broadband photon-pair fields with properties comparable to those coming from chirped periodically-poled crystals. Their intensities scale linearly with the number of domains. Also photon pairs extending over intervals with durations comparable to one optical cycle can be generated in these crystals.

Cavity-enhanced generation of 6 W cw second-harmonic power at 532 nm in periodically-poled MgO:LiTaO_3

We report on efficient cw high-power second harmonic generation in a periodically poled LiTaO3 crystal placed in a resonant enhancement cavity. We tested three configurations, differing in the coupling mirror reflectivity, and a maximum conversion efficiency of about 76%, corresponding to 6.1 W of green light with 8.0 W of fundamental power, was achieved. This is, to the best of our knowledge, the highest cw power ever reported using a periodically-poled crystal in an external cavity. We observed photo-thermal effect induced by photon absorption at the mirrors and in the crystal, which however does not affect stable operation of the cavity. A further effect arises for two out of the three configurations, at higher values of the input power, which degrades the performance of the locked cavity. We suggest this effect is due to the onset of competing nonlinearities in the same crystal.

RECENT PROGRESS ON PARAMETRIC GENERATION OF MONOCHROMATIC THz PULSES

We review our recent progress on power scaling of THz pulses generated from several nonlinear-optical crystals. By using a high-resistivity GaP crystal, we have significally increased the output peak power to as high as 722 W. By stacking three GaP wafers, we have further increased the highest output peak power to 2.36 kW. On the other hand, by using CO2 laser pulses, we have obtained the average output power of 260 μW. We have also used these laser pulses to scale up the output power for the THz pulses to 29.8 μW by stacking GaAs wafers. Indeed, by stacking up to ten wafers, we have increased the output power by a factor of 160. Finally, by using ultrafast laser pulses, we have achieved record-high output powers for the THz pulses generated from multi-period periodically-poled LiNbO3 crystals based on a backward configuration. The highest output power measured by us so far is 10.7 μW.

Efficient ultrafast ultraviolet generation based on frequency doubling in short-period periodically-poled KTiOPO4 crystal

We efficiently generated ultrafast coherent ultraviolet radiation based on secondharmonic generation in periodically-poled KTiOPO 4 with the shortest period of 2.55 µm. The highest output power was measured to be 20.1 mW at 377.1 nm.

Field-induced light deflection in lithium niobate and lithium tantalate: the possible configurations

Field-induced light deflection by ferroelectric domain walls in lithium niobate (LN) and lithium tantalate (LT) is theoretically studied. The phenomenon can occur not only when both the incident wave vector k and the electric field E are parallel to the z-axis—as demonstrated by experiments made so far—but also when E and/or k are perpendicular to z. In particular, for E parallel to x and k parallel to y, the deflection phenomenon is predicted to have the same characteristics as in triclinic or monoclinic ferroelastics: the large deflection angle is related to the natural birefringence, whereas the deflection amplitude is proportional to the small tilt angle of the neutral lines, which is here induced by the electric field. In periodic domain structures, interference between deflected waves occurs, and the deflected intensity is expected to be largely enhanced when the Bragg condition is satisfied. This transverse configuration is thus specially attractive to characterize periodically-poled crystals.

Properties of entangled photon pairs generated in periodically poled nonlinear crystals

Using a rigorous quantum model a comprehensive study of physical properties of entangled photon pairs generated in spontaneous parametric down-conversion in chirped periodically-poled crystals is presented. Spectral, temporal, as well as spatial characteristics of photon pairs are analyzed. Spectral bandwidths, photon-pair flux, and entanglement area can be effectively controlled by chirping. Quantification of entanglement between photons in a pair is given. Splitting of entanglement area in the transverse plane accompanied by spectral splitting has been revealed. Using the model temperature dependencies of the experimental intensity profiles reported in literature have been explained.

Non-collinear quasi phase matching and annular profiles in difference frequency generation with focused Gaussian beams

We present and experimentally test a simple model for difference frequency generation (DFG) in periodically-poled crystals with gaussian pumping beams. Focusing of input beams originates several non-collinear quasi-phase-matching configurations of the interacting wavevectors, which contribute to the idler output field. In this picture, we accurately describe a number of effects, such as the occurrence of annular idler intensity profiles and the asymmetric trend of DFG power vs temperature. Finally, we quantitatively test the model by means of an indirect measurement of the crystal poling period.

Optical characterization of periodically-poled KTiOPO_4

We demonstrate how the Maker fringes that are observable in spontaneous parametric down-conversion (SPDC) give a direct visualization of the poling quality of a periodically-poled crystal. Identical Maker fringes are observed in the optical spectrum of collinear SPDC and the temperature dependence of second harmonic generation. We analyze these Maker fringes via a unified treatment of the tuning curve in crystals with small and slowly-varying deformations of the poling structure. Our theoretical model, based on a Fourier analysis of the poling deformations, distinguishes between duty-cycle variations and variations of the poling phase. The analysis indicates that the poling phase is approximately fixed, while the duty-cycle typically varies between 36% and 64%.

Optimizing single-photon-source heralding efficiency and detection efficiency metrology at 1550 nm using periodically poled lithium niobate

We explore the feasibility of using high conversion-efficiency periodically-poled crystals to produce photon pairs for photon-counting detector calibrations at 1550 nm. The goal is the development of an appropriate parametric down-conversion (PDC) source at telecom wavelengths meeting the requirements of high-efficiency pair production and collection in single spectral and spatial modes (single-mode fibres). We propose a protocol to optimize the photon collection, noise levels and the uncertainty evaluation. This study ties together the results of our efforts to model the single-mode heralding efficiency of a two-photon PDC source and to estimate the heralding uncertainty of such a source.

Characterization of optical and nonlinear properties of periodically-poled RbTiOAsO4 in the mid-infrared range via difference-frequency generation

Tunable mid-infrared coherent radiation (3.25- 3.7 μm) is generated by quasi-phase-matched difference frequency generation in a multi-grating periodically-poled RbTiOAsO4 crystal. The spontaneous polarization and coercive field of flux-grown RbTiOAsO4 are determined by polarization switching measurements. The nonlinear interaction enables us to explore the optical and nonlinear properties of this material in the mid-infrared range, where data is scarce. The measurements are used to derive a mid- infrared corrected dispersion equation for nz in RbTiOAsO4. This equation is in excellent agreement with previously published measurements of nonlinear interactions in periodically-poled RbTiOAsO4. The measured wavelength and temperature bandwidths are ≈48 nm cm and ≈29 °C cm, respectively. A relatively high temperature tuning slope of the phase-matched idler wavelength, -1.27 nm/°C, is measured. This may be useful for realizing temperature-tuned nonlinear devices.

Visible and infrared dispersion of the refractive indices in periodically poled and single domain Nd:Mg:LiNbO3 crystals

crystals are measured in the transparency region (with the accuracy ±0.0002) and for the upper phonon polariton branch (with the accuracy ±0.003–±0.05), from 0.44 μm up to 10.5 μm. The method of spontaneous parametric light scattering is used for measurement of the ordinary refractive index dispersion in the mid-infrared region and for determination of the domain grating period d=5.6±0.2 μm in the periodically-poled crystal.