AbstractWhistler‐mode waves can modulate the electron distributions through wave‐particle interactions in the Earth's inner magnetosphere. In this paper, we have investigated the effects of the whistler waves on the electron distributions by a combination of electron magnetohydrodynamics and test‐particle simulations. Our simulations show a parallel whistler wave becomes gradually oblique during its propagation from the magnetic equator to higher latitudes. Such a whistler wave causes distinct flux increases of tens of keV electrons at large pitch angles to form electron butterfly distributions. This whistler wave traps numerous resonant electrons and transports them from lower latitudes to higher latitudes through nonlinear Landau trapping. Meanwhile, these trapped electrons are efficiently accelerated to higher energies contributing to the rapid formation of electron butterfly distributions at higher latitudes. Our study suggests nonlinear Landau trapping is a potential formation mechanism of the electron butterfly distributions observed in the Earth's inner magnetosphere.