Optical Parametric Oscillator Signal Research Articles

Watt-level single-frequency optical parametric oscillator around 2 µm

A single-frequency optical parametric oscillator (OPO) operating in the wavelength range around 2 µm is reported. The OPO comprises a periodically poled LiNbO3 (PPLN) crystal for quasi-phase matching and a four-mirror ring-cavity resonant to the signal. The OPO signal and idler are tuned from 1.89 to 2.05 µm and from 2.21 to 2.42 µm, respectively, by changing the crystal temperature. Output powers in excess of 2 W are demonstrated at a pump power of 9 W for both the signal and idler over all of the respective tuning ranges. A detailed characterization of the intensity and frequency noise is presented. The OPO exhibits an integrated intensity noise below 0.1% and a linewidth of ∼58 kHz for an observation time of 1 ms. The reported performance makes this source an ideal candidate for the generation of squeezed light around 2 µm via cascaded second-harmonic generation (SHG) and parametric downconversion (PDC).

KTA-OPO for 1742 nm laser generation driven by a composite Nd:YVO4-based self-Raman laser

In this work, a double-end diffusion bonded Nd:YVO4 self-Raman laser was designed to drive an intracavity, noncritically-phase-matched KTiOAsO4 (KTA) optical parametric oscillator (OPO). Both conversion efficiency and output power at 1.7 µm (the wavelength of the OPO signal field) were improved by effectively reducing the thermal lens effect and increasing the effective length of self-Raman medium. At an incident pump power of 15.4 W, the output power for 1742 nm output laser reached 2.16 W with a conversion efficiency of 14%, and the output having a pulse width of 10.5 ns and a pulse repetition frequency of 90 kHz. The competition between the OPO and cascaded Raman laser was observed when the incident pump power was above 12.4 W. The results highlight that in order to improve output power at 1742 nm, it is critical that both the cascaded, second-Stokes field at 1313 nm and the signal field generated at 1534 nm from the 1064 nm field driving the KTA-OPO be minimized, if not completely suppressed. This laser system combining the processes of stimulated Raman scattering and optical parametric oscillation for the generation of laser emission at 1742 nm may find significant application across a broad range of fields including biological engineering, laser therapy, optical coherence tomography and for the generation of mid-infrared laser wavelengths.

Dual-comb optical parametric oscillator in the mid-infrared based on a single free-running cavity.

We demonstrate a free-running single-cavity dual-comb optical parametric oscillator (OPO) pumped by a single-cavity dual-comb solid-state laser. The OPO ring cavity contains a single periodically-poled MgO-doped LiNbO3 (PPLN) crystal. Each idler beam has more than 245-mW average power at 3550 nm and 3579 nm center wavelengths (bandwidth 130 nm). The signal beams are simultaneously outcoupled with more than 220 mW per beam at 1499 nm and 1496 nm center wavelength. The nominal repetition rate is 80 MHz, while the repetition rate difference is tunable and set to 34 Hz. To evaluate the feasibility of using this type of source for dual-comb applications, we characterize the noise and coherence properties of the OPO signal beams. We find ultra-low relative intensity noise (RIN) below -158 dBc/Hz at offset frequencies above 1 MHz. A heterodyne beat note measurement with a continuous wave (cw) laser is performed to determine the linewidth of a radio-frequency (RF) comb line. We find a full-width half-maximum (FWHM) linewidth of around 400 Hz. Moreover, the interferometric measurement between the two signal beams reveals a surprising property: the center of the corresponding RF spectrum is always near zero frequency, even when tuning the pump repetition rate difference or the OPO cavity length. We explain this effect theoretically and discuss its implications for generating stable low-noise idler combs suitable for high-sensitivity mid-infrared dual-comb spectroscopy (DCS).

A 45-μJ, 10-kHz, burst-mode picosecond optical parametric oscillator synchronously pumped at a second harmonic cavity

A novel high-energy picosecond optical parametric oscillator (OPO) was realized by placing an OPO in a second-harmonic (SH) cavity. In a proof-of-principle experiment, we demonstrated excellent burst energy of 45 μJ for the OPO signal at 900 nm that operates at a pulse repetition rate of 10 kHz and a pulse width of 46.8 ps. The beam quality was measured as and in the orthogonal directions, corresponding to an average beam factor M 2 = 1.42. So far, this study is the first to investigate high-energy ps OPO synchronously pumped in a second-harmonic cavity.

CH and NO planar laser-induced fluorescence and Rayleigh-scattering in turbulent flames using a multimode optical parametric oscillator.

An optical parametric oscillator (OPO) is developed and characterized for the simultaneous generation of ultraviolet (UV) and near-UV nanosecond laser pulses for the single-shot Rayleigh scattering and planar laser-induced-fluorescence (PLIF) imaging of methylidyne (CH) and nitric oxide (NO) in turbulent flames. The OPO is pumped by a multichannel, 8-pulse Nd:YAG laser cluster that produces up to 225 mJ/pulse at 355 nm with pulse spacing of 100 µs. The pulsed OPO has a conversion efficiency of 9.6% to the signal wavelength of ∼430nm when pumped by the multimode laser. Second harmonic conversion of the signal, with 3.8% efficiency, is used for the electronic excitation of the A-X (1,0) band of NO at ∼215nm, while the residual signal at 430 nm is used for direct excitation of the A-X (0,0) band of the CH radical and elastic Rayleigh scattering. The section of the OPO signal wavelength for simultaneous CH and NO PLIF imaging is performed with consideration of the pulse energy, interference from the reactant and product species, and the fluorescence signal intensity. The excitation wavelengths of 430.7 nm and 215.35 nm are studied in a laminar, premixed CH4-H2-NH3-air flame. Single-shot CH and NO PLIF and Rayleigh scatter imaging is demonstrated in a turbulent CH4-H2-NH3 diffusion flame using a high-speed intensified CMOS camera. Analysis of the complementary Rayleigh scattering and CH and NO PLIF enables identification and quantification of the high-temperature flame layers, the combustion product zones, and the fuel-jet core. Considerations for extension to simultaneous, 10-kHz-rate acquisition are discussed.

Stimulated Raman scattering microscopy with long wavelengths for improved imaging depth

AbstractStimulated Raman scattering (SRS) imaging is a fast, label‐free, and sensitive technique to map the distribution of a vibrational species in a microscopy setting. It has great potential for applications in many fields, such as lipid imaging in biomedicine. However, depth penetration of the light into the sample is an issue with any light‐based technique, especially with multiphoton techniques such as SRS. Using longer wavelengths allows deeper penetration into densely scattering materials, but applying wavelengths above 1,500 nm is challenging technically. We have built a flexible SRS microscope system capable of imaging with a combination of 1,064 nm and wavelengths over 1,500 nm, using the idler output of an optical parametric oscillator (OPO). For comparison, the same system was also operated in the more common configuration, using 1,064 nm in combination with the OPO signal output around 800 nm. With the long‐wavelength settings, we show improved depth penetration in polyethylene plastic material and in a silicone phantom with embedded polymer microbeads, and we report images of lipid structure in biological tissue. These results demonstrate the technical feasibility of using these long wavelengths for SRS imaging. Disadvantages such as poorer spatial resolution and lower signal strength are also discussed. The application of this new approach to SRS microscopy can allow greater insight into deep‐lying structures in a non‐invasive way.

Precision saturated absorption spectroscopy of H3.

In our previous work on the Lamb-dips of the ν2 fundamental band transitions of H3+, the saturated absorption spectrum was obtained by third-derivative spectroscopy using frequency modulation with an optical parametric oscillator (OPO). However, frequency modulation also caused errors in the absolute frequency determination. To solve this problem, we built a tunable offset locking system to lock the pump frequency of the OPO to an iodine-stabilized Nd:YAG laser. With this improvement, we were able to scan the OPO idler frequency precisely and obtain the saturated absorption profile using intensity modulation. Furthermore, ion concentration modulation was employed to subtract the background noise and increase the signal-to-noise ratio. To determine the absolute frequency of the idler wave, the OPO signal frequency was locked to an optical frequency comb. The absolute frequency accuracy of our spectrometer was better than 7 kHz, demonstrated by measuring the wavelength standard transition of methane at 3.39 μm. Finally, we measured 16 transitions of H3+ and our results agree very well with other precision measurements. This work successfully resolved the discrepancies between our previous measurements and other precision measurements.

Potassium titanyl arsenate based cascaded optical parametric oscillator emit at 2.5 µm derived by neodymium-doped yttrium lithium fluoride laser

We reported a potassium titanyl arsenate (KTA) based cascaded optical parametric oscillator (OPO). The secondary OPO signal light at 2.5 µm was obtained with two OPO processes in one non-critical phase matching cut KTA crystal. This cascaded OPO was driven by a Q-switched neodymium-doped yttrium lithium fluoride (Nd:YLF) laser at 1047 nm. Making full use of the negative thermal lens effect and long upper level fluorescence lifetime of Nd:YLF, signal power of 605 mW at 2503 nm was achieved with a pulse repetition frequency of 15 kHz and an incident diode pump power of 9.7 W. Therefore, the cascaded OPO derived by Q-switched Nd:YLF laser could provide high peak power pulsed laser emission in mid-infrared band.

Intracavity difference-frequency mixing of optical parametric oscillator signal and idler pulses in BaGa4Se7.

An overall quantum conversion efficiency of 7.8% is achieved by intracavity mixing the signal and idler of a 1.064 μm pumped Rb:PPKTP optical parametric oscillator in BaGa4Se7. In this way, a pulse energy of ∼0.71 mJ is generated at ∼7 μm for a repetition rate of 100 Hz. Tuning of the mid-IR radiation is demonstrated by heating of the Rb:PPKTP crystal.

A novel frequency stabilization method for the seed laser of the pulse optical parametric oscillator in differential absorption lidar

A novel frequency stabilization method for the seed laser of the pulse optical parametric oscillator (OPO) in differential absorption lidar (DIAL) is proposed in this paper. The operating principle and the experimental setups are introduced in detail, and the accuracy of the frequency stabilization method and influence factors are also analyzed. The frequency of the seed laser is locked to an absorption line of water vapor (935.6849 nm) in the experiment, and the measured standard deviation of the frequency jitter is less than 8 MHz. The frequency of the seeded OPO signal is recorded thereafter. The standard deviation less than 28.7 MHz with the same frequency according to the seed laser is achieved, which is well applicable to DIAL.

Ignition and formation dynamics of a polariton condensate on a semiconductor microcavity pillar

We present an experimental study on the ignition and decay of a polariton optical parametric oscillator (OPO) in a semiconductor microcavity pillar. The combination of a continuous-wave laser pump, under quasi-phase-matching conditions, and a nonresonant, 2-ps-long pulse probe allows us to obtain the full dynamics of the system. The arrival of the probe induces a blueshift in the polariton emission, bringing the OPO process into resonance with the pump, which triggers the OPO process. We time-resolve the polariton OPO signal emission for more than 1 ns in both real space and momentum space. We fully characterize the emission of the OPO signal with spectral tomography techniques. Our interpretations are backed up by theoretical simulations based on the two-dimensional coupled Gross-Pitaevskii equation for excitons and photons.

Frequency comb generation by a continuous-wave-pumped optical parametric oscillator based on cascading quadratic nonlinearities

We report optical frequency comb generation by a continuous-wave pumped optical parametric oscillator (OPO) without any active modulation. The OPO is configured as singly resonant with an additional nonlinear crystal (periodically poled MgO:LiNbO3) placed inside the OPO for phase mismatched second harmonic generation (SHG) of the resonating signal beam. The phase mismatched SHG causes cascading χ(2) nonlinearities, which can substantially increase the effective χ(3) nonlinearity in MgO:LiNbO3, leading to spectral broadening of the OPO signal beam via self-phase modulation. The OPO generates a stable 4 THz wide (-30 dB) frequency comb centered at 1.56 μm.

Influence of output coupling on the performance of a passively Q-switched Nd:YAG laser with intracavity optical parametric oscillator

A singly-resonant intracavity optical parametric oscillator (OPO), pumped by a passively Q-switched Nd:YAG laser, is systematically investigated by means of a series of the output mirrors with various reflectivities for the fundamental wavelength at 1064 nm. Experimental results reveal that the output mirror with partial reflectivity instead of high reflection at 1064 nm not only is practicable to avoid the optical coatings damaged, but also enhances the dual-wavelength output efficiency for the OPO signal and fundamental laser waves. The overall optical-to-optical conversion efficiency is enhanced from 6.4% to 8.2% for the reflectivity decreasing from 99.8% to 90%.

Large-scale multipartite entanglement in the quantum optical frequency comb

We show theoretically that multipartite entanglement is generated on a massive scale in the spectrum, or optical frequency comb, of a single optical parametric oscillator (OPO) emitting well above threshold. In this system, the quantum dynamics of the strongly depleted pump field are responsible for the onset of the entanglement by correlating the two-mode squeezed, bipartite-entangled pairs of OPO signal fields. (Such pairs are independent of one another in the undepleted, classical pump approximation.) We verify the multipartite nature of the entanglement by evaluating the van Loock-Furusawa criterion for a particular set of entanglement witnesses deduced from physical considerations.

Role of supercurrents on vortices formation in polariton condensates

Observation of quantized vortices in non-equilibrium polariton condensates has been reported either by spontaneous formation and pinning in the presence of disorder or by imprinting them onto the signal or idler of an optical parametric oscillator (OPO). Here, we report a detailed analysis of the creation and annihilation of polariton vortex-antivortex pairs in the signal state of a polariton OPO by means of a short optical Gaussian pulse at a certain finite pump wave-vector. A time-resolved, interferometric analysis of the emission allows us to extract the phase of the perturbed condensate and to reveal the dynamics of the supercurrents created by the pulsed probe. This flow is responsible for the appearance of the topological defects when counter-propagating to the underlying currents of the OPO signal.

Eye-safe, 243-mJ, rapidly tuned by injection-seeding, near-infrared, optical, parametric, oscillator-based differential-absorption light detection and ranging transmitter

Here, we demonstrate and characterize a high-energy, eye-safe, spectrally narrow, and frequency-agile near-IR optical parametric oscillator (OPO). The injection-seeded, noncritical phase-matched (NCPM) potassium titanyle arsenate (KTA) and ring-cavity OPO was pumped in single longitudinal mode (SLM) at 7 ns full width at half maximum FWHM and 30 Hz, neodymium-doped yttrium aluminum garnet (Nd:YAG), generating 243 mJ per pulse OPO signal output with a conversion efficiency of 27%, spectral linewidth of 157 MHz, and approximately M2 of 29. Also, we demonstrate a nonmechanical method to switch the frequency of the OPO at a rate of 2 Hz from 1535.036 to 1535.195 nm, which represents the on/off resonances of carbon dioxide, respectively. However, the switching rate can be extended into the MHz range and is limited by the electronics driving the diode laser. Given the performance results of our frequency-agile OPO, this transmitter has great potential as a source in DIAL applications.

Development of Optical Parametric Oscillator Tunable in the Range 970-1460 nm

Optical parametric oscillator (OPO) tunable in the range 970-1460 nm has been developed using bet barium borate (BBO) crystal as the gain medium and second harmonic of Nd:YAG laser as pump source. Two sets of resonators were used to cover the range; first was nearly degenerate (970-1180 nm) and the second was nondegenerate (1240-1460 nm). The measured threshold pump pulse energy was nearly 8 mJ. Maximum signal pulse energy of about 14 mJ was obtained for pump pulse energy of nearly 31 mJ. Power scaling efficiency was about 70 per cent. The signal pulse width was ~5 ns corresponding to the pump pulse width of ~ 9 ns. OPO signal beam quality was Gaussian although the pump beam was top-hat multimode. Defence Science Journal, 2011, 61(4), pp.377-382 , DOI:http://dx.doi.org/10.14429/dsj.61.562

Efficient 18 μmKTiOPO_4 optical parametric oscillator pumped within an Nd:YAG/SrWO_4 Raman laser

A 1.8 μm optical parametric oscillator (OPO) based on a noncritically phase-matched KTiOPO4 crystal is demonstrated. OPO and stimulated Raman scattering techniques are successfully combined in an acousto-optically Q-switched Nd:YAG/SrWO4 Raman laser. The device efficiently realizes three steps of conversion: from a laser diode wavelength of 808 nm to the fundamental wavelength of 1064 nm; next, to the Stokes wavelength of 1180 nm; and finally to the OPO signal wavelength of 1810 nm. With an incident diode power of 7.2 W and a pulse repetition rate of 15 kHz, an average signal power of 485 mW is obtained with a diode-to-signal conversion efficiency of 6.75%. The beam quality factors (M2) of the signal wave in both horizontal and vertical directions are measured to be 1.7±0.2. The numerical output power results of the system, the thermal lensing, and the stability parameter of the cavity are also discussed.

Intracavity wavelength modulation of an optical parametric oscillator for coherent Raman microscopy

We present a novel intracavity frequency modulation scheme in a tunable, picosecond optical parametric oscillator (OPO). The OPO signal wavelength can be modulated with a depth of more than 10 nm at a rate of 38 MHz (one half its repetition rate). We discuss the design and construction of the light source and its application to the recently-developed frequency modulation coherent anti-Stokes Raman scattering (FM-CARS) and stimulated Raman scattering (SRS) techniques. The new light source allows for real time subtraction of the interfering background signal in coherent Raman imaging, yielding images with purely chemical contrast.

High‐resolution narrowband CARS spectroscopy in the spectral fingerprint region

AbstractCoherent anti‐Stokes Raman scattering (CARS) spectroscopy is an important technique for spectroscopy and chemically selective microscopy, but wider implementation requires dedicated versatile tunable sources. We describe an optical parametric oscillator (OPO) based on a magnesium oxide‐doped periodically poled lithium niobate crystal, with a novel variable output coupler, used as a tunable coherent light source. The OPO's signal wavelength ranges from 880 to 1040 nm and its idler wavelength from 1090 to 1350 nm.We use this OPO to demonstrate high‐resolution narrowband CARS spectroscopy on bulk polystyrene from 900 to 3600 cm−1, covering a large part of the molecular fingerprint region. Recording vibrational spectra using narrowband CARS spectroscopy has several advantages over spontaneous Raman spectroscopy, which we discuss. We isolate the resonant part of the CARS spectrum and compare it to the spontaneous Raman spectrum of polystyrene using the maximum entropy method of phase retrieval; we find them to be in extremely good agreement. Copyright © 2009 John Wiley & Sons, Ltd.