Optical Information Technology Research Articles

A Dynamic H-Bonding Network Enables Stimuli-Responsive Color-Tunable Chiral Afterglow Polymer for 4D Encryption.

The development of stimuli-responsive and color-tunable chiral organic afterglow materials has attracted great attention but remains a daunting challenge. Here, a simple yet effective strategy through the construction of a dynamic H-bonding network is proposed to explore the multi-color stimuli-responsive chiral afterglow by doping a self-designed chiral phosphorescent chromophore into a polyvinyl alcohol matrix. A stimuli-responsive deep blue chiral afterglow system with a lifetime of up to 3.35 s, quantum yield of 25.0%, and luminescent dissymmetry factor of up to 0.05 is achieved through reversible formation and breakdown of the H-bonding network upon thermal-heating and water-fumigating. Moreover, multi-color stimuli-responsive chiral afterglow can be obtained by chiral and afterglow energy transfer, allowing the establishment of afterglow information displays and high-level 4D encryption. This work not only offers a facile platform to develop advanced stimuli-responsive materials but also opens a new avenue for developing next-generation optical information technology with enhanced functionality and responsiveness.

Unveiling photon–photon coupling induced transparency and absorption

Abstract This study presents the theoretical foundations of an analogous electromagnetically induced transparency (EIT) and absorption (EIA) which we are referring as coupling induced transparency (CIT) and absorption (CIA) respectively, along with an exploration of the transition between these phenomena. We provide a concise phenomenological description with analytical expressions for transmission spectra and dispersion elucidating how the interplay of coherent and dissipative interactions in a coupled system results in the emergence of level repulsion and attraction, corresponding to CIT and CIA, respectively. This theory comprehensively captures both the phenomena while modelling the microstripline loaded resonators and their couplings systematically. The model is validated through numerical simulations using a hybrid system comprising a split ring resonator (SRR) and electric inductive-capacitive (ELC) resonator in planar geometry. We analyse two cases while keeping ELC parameters constant; one involving a dynamic adjustment of the SRR size with a fixed split gap, and the other entailing a varying gap while maintaining a constant SRR size. Notably, in the first case, the dispersion profile of the transmission signal demonstrates level repulsion, while the second case results in level attraction, effectively showcasing CIT and CIA, respectively. These simulated findings not only align with the theoretical model but also underscore the versatility of our approach. Subsequently, we expand our model to a more general case, demonstrating that a controlled transition from CIT to CIA is achievable by manipulating the dissipation rate of individual modes within the hybrid system, leading to either coherent or dissipative interactions between the modes. The results provide a pathway for designing hybrid systems that can control the group velocity of light, offering potential applications in the fields of optical switching and quantum information technology.

Spin-related excited-state phenomena in photochemistry.

The spin of electrons plays a vital role in chemical reactions and processes, and the excited state generated by the absorption of photons shows abundant spin-related phenomena. However, the importance of electron spin in photochemistry studies has been rarely mentioned or summarized. In this review, we briefly introduce the concept of spin photochemistry based on the spin multiplicity of the excited state, which leads to the observation of various spin-related photophysical properties and photochemical reactivities. Then, we focus on the recent advances in terms of light-induced magnetic properties, excited-state magneto-optical effects and spin-dependent photochemical reactions. The review aims to provide a comprehensive overview to utilize the spin multiplicity of the excited state in manipulating the above photophysical and photochemical processes. Finally, we discuss the existing challenges in the emerging field of spin photochemistry and future opportunities such as smart magnetic materials, optical information technology and spin-enhanced photocatalysis.

Demonstrating long-term stable optical coupling between single-mode optical fibers and well-defined energy photons emitted from nitrogen impurity centers in GaAs flakes

A key challenge in realizing scalable optical quantum information technology is not only to obtain stable single photons coupled to single-mode fibers but also to match the emission energy between remote emitters. We have fabricated an energy-matching favorable and long-term stable structure by coupling a nitrogen impurity center with a well-defined emission energy to a single-mode optical fiber core. The nitrogen-doped GaAs microflakes sandwiched between the two FC (acronym for "ferrule connector" or "fiber channel") connectors yielded sharp emission peaks due to nitrogen isoelectronic traps. Although some emitters showed spectral diffusion, the unaffected emitters showed stable emission and were able to generate photons stably for over 20 h continuously without photodegradation. In addition, the photoluminescence spectrum does not change in shape and intensity after more than 3 years, indicating that the photon source with this structure is resistant to thermal cycling and positional drift and has excellent long-term stability.

Pushing photon-pair generation rate in microresonators by Q factor manipulation.

Photon pairs generated by employing spontaneous nonlinear effects in microresonators are critically essential for integrated optical quantum information technologies, such as quantum computation and quantum cryptography. Microresonators featuring high-quality (Q) factors can offer simple yet power-efficient means to generate photon pairs, thanks to the intracavity field enhancement. In microresonators, it is known that the photon-pair generation rate (PGR) is roughly proportional to the cubic power of the Q factor. However, the upper limit on PGR is also set by the Q factor: a higher Q factor brings a longer photon lifetime, which in turn leads to a lower repetition rate allowing for photon flow emitted from the microresonator, constrained by the Fourier-transform limit. Exceeding this limit will result in the overlap of photon wave packets in the time domain, thus degrading the quantum character of single-photon light beams. To push the limit of PGR in a single resonator, we propose a method by harnessing the resonance linewidth-manipulated microresonators to improve the maximum achievable photon repetition rate while keeping the power efficiency. The maximum achievable PGR and power efficiency are thus balanced by leveraging the combination of low and high-Q resonances.

Efficient two-dimensional Fraunhofer diffraction pattern via electron spin coherence

In this letter, we have discussed the two-dimensional diffraction pattern via electron spin coherence in a GaAs quantum dot. Impulsive stimulated Raman excitation utilizing coherent optical fields is employed for the purpose of regulating the electron spin coherence within a charged ensemble of GaAs quantum dots, by means of an intermediate charged exciton (trion) state. We show that for the coupling two-dimensional standing wave (SW) field in the x and y directions, the two-dimensional Fraunhofer pattern can be formed for a weak probe light. By using the experimental parameters and controlling the Rabi frequency of the SW field and relative phase between applied lights, the symmetry and asymmetry diffraction pattern are obtained for the weak probe light due to the four-wave mixing mechanism. Our proposed model may have potential applications in high-capacity optical communications and quantum information technologies.

Continuous-Spectrum-Polarization Recombinant Optical Encryption with a Dielectric Metasurface.

The Jones matrix, with eight degrees of freedom (DoFs), provides a general mathematical framework for the multifunctional design of metasurfaces. Theoretically, the maximum eight DoFs can be further extended in the spectrum dimension to endow unique encryption capabilities. However, the topology and intrinsic spectral responses of meta-atoms constrains the continuous engineering of polarization evolution over wavelength dimension. In this work, a forward evolution strategy to quickly establish the mapping relationships between the solutions of the dispersion Jones matrix and the spectral responses of meta-atoms is reported. Based on the eigenvector transformation method, arbitrary conjugate polarization channels over the continuous-spectrum dimension are successfully reconstructed. As a proof-of-concept, a silicon metadevice is demonstrated for optical information encryption transmission. Remarkably, the arbitrary combination forms of polarization and wavelength dimension increase the information capacity (210 ), and the measured polarization contrasts of the conjugate polarization conversion are >94% in the entire wavelength range (3-4µm). It is believed that the proposed approach will benefit secure optical and quantum information technologies.

Peculiarities of Electron Wave Packet Dynamics in Planar Nanostructures in the Presence of Magnetic and Electric Fields

Currently, spatially localized electron densities and currents are considered to be candidates for use in the encoding of quantum information. For this reason, the control of their temporal dynamics is an important task. In this work, the spatiotemporal evolution of an electron wave packet in planar nanostructure in the presence of transverse magnetic and lateral electric fields is investigated by direct analytical solution of the non-stationary Schrödinger equation. Methods to control and manage the dynamics of the spatially localized electron density distribution are developed. The production of photon-like quantum states of electrons opens up opportunities for applications similar to quantum optical and quantum information technologies but implemented with charge carriers. Quantum control of the trajectory of the electron wave packet, accompanied by dramatic suppression of its spreading, is demonstrated. This study discovered methods to manage spatially localized electron behavior in a nanostructure that allows a controllable charge quantum transfer and gives rise to new prospects for quantum nanoelectronics technology.

RGB Tricolor and Multimodal Dynamic Optical Information Encryption and Decoding for Anti-Counterfeiting Applications.

Conventional optical anti-counterfeiting strategies are based on the single-color emission, which are easily deciphered and thus greatly limited in the application of information security. Herein, a multimodal dynamic optical information coding with red, green, and blue (RGB) tricolors has been developed by photoluminescence (PL), persistent luminescence (PersL), thermally stimulated luminescence (TSL), and thermally stimulated persistent luminescence (TSPL). The BaSi2O2N2:Eu2+ phosphors with a blue emission peak at 494 nm were used as the crucial blue optical information coding material and exhibited the distinctive response properties to light, heat, and force stimuli with intrinsic trap depths of 0.674 and 0.82 eV. More importantly, by combining the red Sr2Si5N8:Eu2+,Dy3+ and green SrSi2O2N2:Eu2+,Dy3+ nitride phosphors, a RGB tricolor and multimodal strategy has been successfully developed for anti-counterfeiting applications. The "RGB tricolor flower" with RGB emissions is given as a typical example to achieve the dynamic display of optical information encryption and decoding through the various PL, PersL, TSL, and TSPL modes. Finally, the traditional quick response (QR) code mechanism has been integrated into the design of multi-information encrypted RGB tricolor anti-counterfeiting devices with different identifiabilities of the encrypted information in natural light, PL, PersL, TSL, and TSPL modes. The laminated layers of RGB QR code patterns containing different specific information, such as "DLPU" and "116034", can be effectively recognized in the corresponding modes. The design strategy of RGB tricolor and multimodal optical information encryption and decoding devices in this work greatly improves the security level of advanced optical information technologies and extends the potential applications in dynamic anti-counterfeiting fields.

High-dimensional orbital angular momentum comb

The article comments on a recently reported OAM comb. The proposed approach relies on a simple azimuthal binary phase modulation scheme to transform a Gaussian beam into a structured light beam containing multiple OAM components with equal spacing and uniform power. It provides a convenient way to simultaneously tailor multiple OAM channels, with the potential to impact many fields, including optical information technology.

Single-Photon Counting with Semiconductor Resonant Tunneling Devices.

Optical quantum information science and technologies require the capability to generate, control, and detect single or multiple quanta of light. The need to detect individual photons has motivated the development of a variety of novel and refined single-photon detectors (SPDs) with enhanced detector performance. Superconducting nanowire single-photon detectors (SNSPDs) and single-photon avalanche diodes (SPADs) are the top-performer in this field, but alternative promising and innovative devices are emerging. In this review article, we discuss the current state-of-the-art of one such alternative device capable of single-photon counting: the resonant tunneling diode (RTD) single-photon detector. Due to their peculiar photodetection mechanism and current-voltage characteristic with a region of negative differential conductance, RTD single-photon detectors provide, theoretically, several advantages over conventional SPDs, such as an inherently deadtime-free photon-number resolution at elevated temperatures, while offering low dark counts, a low timing jitter, and multiple photon detection modes. This review article brings together our previous studies and current experimental results. We focus on the current limitations of RTD-SPDs and provide detailed design and parameter variations to be potentially employed in next-generation RTD-SPD to improve the figure of merits of these alternative single-photon counting devices. The single-photon detection capability of RTDs without quantum dots is shown.

Review on Applications of Dendrimer-Chemical Compounds in Pharmaceutical and Industrial Fields

This review involved Dendrimer in pharmaceutical applications. Dendrimers are the most important medical nano-polymers in the fields of chemistry and pharmacology, which have been used in many pharmaceutical applications. Many technical applications of many biological elements such as proteins, viruses, or bacteria, including applications of chromatography, optical information technology, sensors, stimulation and drug delivery, require immobilization or immobilization of these biologicals. Here, carbon nanotubes, gold particles and synthetic polymers can be used for such purposes. Here we note that this immobilization process can be achieved mostly through adsorption or chemical bonding or to a lesser extent by incorporating these elements as guests in the host matrices. We also note that in the case of guest and host systems, an optimal method for immobilizing the bio-elements as well as incorporating them into a serial structure based on the nanoscale must be established to facilitate the interactions of the bio-nano-elements within their own environment. This is due to the large number of synthetic or natural polymers available and the advanced and developed methods for processing such systems for nanofibers, rods or tubes etc., this makes the polymers a good base for immobilizing different biomaterials.

High-Efficiency Fast-Radiative Blue-Emitting Perovskite Nanoplatelets and Their Formation Mechanisms.

High-efficiency blue perovskite emitters with fast fluorescence radiation are not only crucial to achieving high-quality displays but also highly desired for optical wireless communications and quantum information technologies. Here, we demonstrate the preparation of blue-emitting Eu3+-, Sb3+-, and Ba2+-induced CsPbBr3 nanoplatelets with narrow spectral widths. Among them, Sb3+-doped CsPbBr3 NPLs can reach a photoluminescence quantum yield of 95%, with a very short fluorescence lifetime of 1.48 ns and greatly reduced ligand dosage. Through nuclear magnetic resonance analysis and density functional theory calculations, we find that the dopant-ligand interaction and dopant-induced growth energy barrier decide the growth kinetics of doped nanoplatelets. These mechanisms offer a fresh route to controlling the dimension of nanoscale perovskite emitters and benefit the development of fast-radiative perovskite emitters.

非平衡光纤干涉仪的相位稳定方法研究

By using photons to carry quantum information, optical quantum information technology plays an essential role in quantum communication, quantum metrology, and linear optical quantum computing. In recent years, the unbalanced fiber interferometer has been widely applied in preparing, manipulating, and measuring photon qubits. However, the unbalanced fiber interferometer based on fiber devices is sensitive to the environment's thermal, mechanical, and acoustic noise. Thus, phase stabilization based on feedback control is essential in utilizing an unbalanced fiber interferometer. The existing phase stabilization methods typically employ a reference laser combined with optoelectronic detection, thus introducing additional noise to photon qubits. In this paper, we propose and demonstrate a feedback control method to stabilize a phase in an unbalanced fiber interferometer by combining weak coherent reference light and single photon counting. Using theoretical analysis, we realized the phase stabilization of an unbalanced fiber Michelson interferometer with an arm-length difference of about 1 m. The results showed that the jitter of the stabilized phase is less than 0.042 rad, while the visibility of single-photon interference fringes is higher than 99%.

Optical Mode Tuning of Monolayer Tungsten Diselenide (WSe2) by Integrating with One-Dimensional Photonic Crystal through Exciton-Photon Coupling.

Two-dimensional materials, such as transition metal dichalogenides (TMDs), are emerging materials for optoelectronic applications due to their exceptional light–matter interaction characteristics. At room temperature, the coupling of excitons in monolayer TMDs with light opens up promising possibilities for realistic electronics. Controlling light–matter interactions could open up new possibilities for a variety of applications, and it could become a primary focus for mainstream nanophotonics. In this paper, we show how coupling can be achieved between excitons in the tungsten diselenide (WSe2) monolayer with band-edge resonance of one-dimensional (1-D) photonic crystal at room temperature. We achieved a Rabi splitting of 25.0 meV for the coupled system, indicating that the excitons in WSe2 and photons in 1-D photonic crystal were coupled successfully. In addition to this, controlling circularly polarized (CP) states of light is also important for the development of various applications in displays, quantum communications, polarization-tunable photon source, etc. TMDs are excellent chiroptical materials for CP photon emitters because of their intrinsic circular polarized light emissions. In this paper, we also demonstrate that integration between the TMDs and photonic crystal could help to manipulate the circular dichroism and hence the CP light emissions by enhancing the light–mater interaction. The degree of polarization of WSe2 was significantly enhanced through the coupling between excitons in WSe2 and the PhC resonant cavity mode. This coupled system could be used as a platform for manipulating polarized light states, which might be useful in optical information technology, chip-scale biosensing and various opto-valleytronic devices based on 2-D materials.

Directional control of propagating graphene plasmons by strain engineering

Control of propagating surface plasmon on a scale beyond the diffraction limit is important for the development of integrated nanophotonic circuits and optical information technology. In this paper, a strain-based modulation mechanism for directional control of propagating graphene plasmons was proposed. We demonstrated numerically that the GPs can be directionally controlled by the implementation of strain on graphene. The topologies of GPs excited by a z-polarized optical emitter in unstrained and strained graphene were illustrated both in real space and momentum space. When imposing strain engineering to graphene in different directions with a different modulus, multi-dimensional control of GPs in any direction can be realized. The simulated propagation length ratio η of the GPs can reach 3.5 when the strain with a modulus of 0.20 is applied along or perpendicular to the zigzag direction of graphene. Besides, the effect of PDMS on GPs was investigated finally for the experiments to be carried out and we show that the PDMS does not affect the generation of directional GPs under strain engineering. Our proposed directional control of GPs not only has the advantages of wide operating wavelength but does not require additional coupling mechanisms, which is beneficial to the design of integrated photonic devices.

Tautomeric influence on the photoinduced birefringence of 4-substituted phthalimide 2-hydroxy Schiff bases in PMMA matrix.

The photoinduced birefringence of two 4-substituted phthalimide 2-hydroxy Schiff bases, containing salicylic (4) and 2-hydroxy-1-naphthyl (5) moieties has been investigated in PMMA matrix. Their optical behaviour as nanocomposite films was revealed by combined use of DFT quantum chemical calculations (in ground and excited state) and experimental optical spectroscopy (UV-Vis and fluorescence). The results have shown that solid-state reversible switching takes place by enol/keto tautomerization and Z/E isomerization. Birefringence study was performed in the PMMA nanocomposite films using pump lasers at λrec = 355nm and λrec = 442nm. Fast response time and high stability of anisotropy up to 58% for (4) and 95% for (5) after turning off the excitation laser, was observed, which makes these materials appropriate candidates for cutting-edge optical information technology materials. The possibility for multiple cycles of recording, reading and optical erasure of the photoinduced birefringence at λrec = 442nm in 5 has been demonstrated. The obtained results have shown that the maximum value of the measured birefringence is close to the anisotropic characteristics of the most frequently used azo materials.

Growth of high quality Si-based (Gd2Ce)(Fe4Ga)O12 thin film and prospects as a magnetic recording media

Ce3+-doped rare-earth iron garnet is a hot magneto-optical material in the field of optical communication and information technology. However, the integration of magneto-optical devices has encountered difficulties due to the poor-quality film deposited on Si. This paper focuses on high-quality Si-based (Gd2Ce)Fe5O12 and (Gd2Ce)(Fe4Ga)O12 thin films by using radio frequency magnetron sputtering method. It was found that the introduction of Ga3+ ions can protect Ce3+ from oxidation, stabilize the garnet phase, improve the optical transmittance, and reduce the lattice mismatch between the thin film and the Si substrate. And heating the substrate at 500 ℃ is conducive to grow high-quality Si-based films. The (Gd2Ce)(Fe4Ga)O12/Si thin film has the strong Kerr magneto-optical effect and the pretty high coercivity. Moreover, this film has the obvious out-of-plane magnetic anisotropy and its vertical matrix ratio close to 1, which indicates that it has the considerable prospects for high-density perpendicular magnetic recording.

Ultrabright Quantum Photon Sources on Chip.

Quantum photon sources of high rate, brightness, and purity are increasingly desirable as quantum information systems are quickly scaled up and applied to many fields. Using a periodically poled lithium niobate microresonator on chip, we demonstrate photon-pair generation at high rates of 8.5 and 36.3MHz using only 3.4 and 13.4 μW pump power, respectively, marking orders of magnitude improvement over the state of the art, across all material platforms. These results constitute the first direct measurement of the device's giant single photon nonlinearity. The measured coincidence to accidental ratio is well above 100 at those high rates and reaches 14682±4427 at a lower pump power. The same chip enables heralded single-photon generation at tens of megahertz rates, each with low autocorrelation g_{H}^{(2)}(0)=0.008 and 0.097 for the microwatt pumps, which marks a new milestone. Such distinct performance, facilitated by the chip device's noiseless and giant optical nonlinearity, will contribute to the forthcoming pervasive adoption of quantum optical information technologies.

Approbation of the Laser Doppler Anemometer Lad-08 on the Secondary Standard Test Rig for Air Flow Speed

In the field of fundamental metrology and ensuring the unity of measuring instruments, the role of optical information methods, systems and technologies of non-contact diagnostics of dynamic processes is extremely relevant. The profiles of the axial velocity component were measured in the working section of the secondary standard test rig for air flow speed. The flow kinematics inside the working section is studied using a laser Doppler anemometer (LDA) with an adaptive temporal selection of the velocity vector (LAD-08).