The study investigated students’ perceptions regarding the use of an integrated set of five Google Tools (i.e., Google Classroom, Google Sites, Google Slides, Google Docs, and Google Forms) in creating a Computer-Mediated Communication (CMC) environment for self-regulated learning in an asynchronous course. Using a mixed-method convergent research design, a single online questionnaire comprising close- and open-ended questions was used to collect quantitative and qualitative data. Purposive sampling was employed, and two cohorts of undergraduate education majors were chosen. 114 participants completed the questionnaire. Quantitative data from Likert items were subjected to descriptive analysis and supplemented with students’ open-ended narratives, while specific qualitative data were examined with inductive thematic analysis. The quantitative findings revealed that students positively perceived the integrated set of Google Tools in terms of its usefulness, ease of use, confirmation, satisfaction, and continuance intention for supporting their self-regulated learning. The qualitative findings highlight students’ predominantly positive perception of Google Classroom as a Learning Management System (LMS) for self-regulated learning, stemming from its ease of use, efficient interface, and notification and reminder features. Minimal instances of other perceptions were also observed. The study proposes practical implications for educators to facilitate students’ online self-regulated learning by leveraging and integrating these five Google Tools in forming a CMC environment. Recommendations include allocating adjustment time and practice tasks to help students familiarize with the tools for smooth online learning.