Traditional sonic crystals (SCs) are based on scatterers or resonators distributed periodically that attenuate sound waves in different bands of frequencies. Recently, we adopted an improved design of SC, namely, the gradient-based sonic crystal (GBSC), designed with a gradient in the geometric parameters using nonuniform resonators and lattices. The finite element (FE) study on the GBSCs indicated that the gradient induces better attenuation than the traditional periodic SCs. This work is an extension of our previous work with experimental and new FE studies on different parameters of the GBSC in an attempt to improve the attenuation of the GBSCs. It was found that the gradient of the geometry enhances the Bragg scattering and resonance in the array, creating a large number of band frequencies. When designed properly by manipulating their gradient, GBSCs were found to target particular frequency bands over other GBSCs of identical filling ratios by coupling the resonant frequencies or the resonant and Bragg frequencies. It was also found that the thickness of the GBSC can be reduced by removing some specific columns from the array without significantly affecting the attenuation by the GBSC. Similarly, it was also found that the relative position of the resonator columns in a GBSC affects the band frequencies, and swapping the columns may also improve the attenuation by the GBSC.