Generation Of Nonclassical Light Research Articles

Quantum catalysis in cavity quantum electrodynamics

Catalysis plays a key role in many scientific areas, most notably in chemistry and biology. Here we present a catalytic process in a paradigmatic quantum optics setup, namely the Jaynes-Cummings model, where an atom interacts with an optical cavity. The atom plays the role of the catalyst, and it allows for the deterministic generation of nonclassical light in the cavity. Considering a cavity prepared in a “classical” coherent state, and choosing appropriately the atomic state and the interaction time, we obtain an evolution with the following properties. First, the state of the cavity has been modified, and it now features nonclassicality, as witnessed by sub-Poissonian statistics or Wigner negativity. Second, the process is catalytic in the sense that the atom is deterministically returned to its initial state exactly, and it can be reused multiple times. What is more, we also show that our findings are robust under dissipation and can be applied to scenarios featuring cavity loss and atomic decay. Finally, we investigate the mechanism of this catalytic process, in particular highlighting the key role of correlations and quantum coherence. Published by the American Physical Society 2024

Nonclassical light generation and control from laser-driven semiconductor intraband excitations

Nonclassical light generation and control from laser-driven semiconductor intraband excitations

Polarization-Selective Enhancement of Telecom Wavelength Quantum Dot Transitions in an Elliptical Bullseye Resonator.

Semiconductor quantum dots are promising candidates for the generation of nonclassical light. Coupling a quantum dot to a device capable of providing polarization-selective enhancement of optical transitions is highly beneficial for advanced functionalities, such as efficient resonant driving schemes or applications based on optical cyclicity. Here, we demonstrate broadband polarization-selective enhancement by coupling a quantum dot emitting in the telecom O-band to an elliptical bullseye resonator. We report bright single-photon emission with a degree of linear polarization of 96%, Purcell factor of 3.9 ± 0.6, and count rates up to 3 MHz. Furthermore, we present a measurement of two-photon interference without any external polarization filtering. Finally, we demonstrate compatibility with compact Stirling cryocoolers by operating the device at temperatures up to 40 K. These results represent an important step toward practical integration of optimal quantum dot photon sources in deployment-ready setups.

Decoherence of photon entanglement by transmission through brain tissue with Alzheimer's disease.

The generation, manipulation and quantification of non-classical light, such as quantum-entangled photon pairs, differs significantly from methods with classical light. Thus, quantum measures could be harnessed to give new information about the interaction of light with matter. In this study we investigate if quantum entanglement can be used to diagnose disease. In particular, we test whether brain tissue from subjects suffering from Alzheimer's disease can be distinguished from healthy tissue. We find that this is indeed the case. Polarization-entangled photons traveling through brain tissue lose their entanglement via a decohering scattering interaction that gradually renders the light in a maximally mixed state. We found that in thin tissue samples (between 120 and 600 micrometers) photons decohere to a distinguishable lesser degree in samples with Alzheimer's disease than in healthy-control ones. Thus, it seems feasible that quantum measures of entangled photons could be used as a means to identify brain samples with the neurodegenerative disease.

Nonlinear coupling of linearly uncoupled resonators through a Mach–Zehnder interferometer

Optical nonlinear processes in linearly uncoupled resonators are being actively studied as a convenient way to engineer and control the generation of non-classical light. In these structures, one can take advantage of the independent combs of resonances of two linearly uncoupled ring resonators for field enhancement, with the phase-matching condition being significantly relaxed compared to a single resonator. However, previous implementations of this approach have shown a limited operational bandwidth along with a significant reduction of the generation efficiency. Here, we experimentally demonstrate that a Mach–Zehnder interferometer can be used to effectively linearly uncouple two resonators and, at the same time, allows for their efficient nonlinear coupling. We demonstrate that this structure can lead to an unprecedented control over the rings' interaction and can operate over more than 160 nm, covering the S-, C-, and L-telecom bands. In addition, we show that the photon pair generation efficiency is increased by a factor of four with respect to previous implementations.

High-Performance Single-Photon Sources at Telecom Wavelength Based on Broadband Hybrid Circular Bragg Gratings

Semiconductor quantum dots embedded in hybrid circular Bragg gratings are a promising platform for the efficient generation of nonclassical light. The scalable fabrication of multiple devices with similar performance is highly desirable for their practical use as sources of single and entangled photons, while the ability to operate at telecom wavelength is essential for their integration with the existing fiber infrastructure. In this work we combine the promising properties of broadband hybrid circular Bragg gratings with a membrane-transfer process performed on 3" wafer scale. We develop and study single-photon sources based on InAs/GaAs quantum dots emitting in the telecom O-band, demonstrating bright single-photon emission with Purcell factor > 5 and count rates up to 10 MHz. Furthermore, we address the question of reproducibility by benchmarking the performance of 10 devices covering a wide spectral range of 50 nm within the O-band.

Generation and modulation of non-classical light in a strongly coupled photon–emitter system

Non-classical light, especially its single photon and squeezing properties, plays a fundamental role in on-chip quantum networks. The single photon property has been widely studied in photonic cavities including photonic crystals (PhCs), micropillar cavities, nanowires, and plasmonic cavities. However, the generation and modulation of squeezing light in nanophotonic cavities remain to be explored. Here, we theoretically demonstrate a strongly coupled PhC–plasmonic-emitter system enabling non-classical light generation and modulation. The hybridization of a PhC waveguide and an Ag nanoparticle forms a band-edge mode with a narrow linewidth and a strong confined field, which enables strong light–emitter interaction, further resulting in simultaneous generation of squeezing and single photon properties for on-chip applications. Non-classical light emission can be modulated with the detuning between the band-edge mode and the emitter. The emission is efficiently channeled by the PhC waveguide with a high coupling efficiency, accompanying unidirectional transmission under excitation by a circularly polarized emitter. The system provides a candidate for tunable and bifunctional on-chip non-classical light sources at the nanoscale and may offer more possibilities to build versatile quantum networks.

Plexcitonic Quantum Light Emission from Nanoparticle-on-Mirror Cavities.

We investigate the quantum-optical properties of the light emitted by a nanoparticle-on-mirror cavity filled with a single quantum emitter. Inspired by recent experiments, we model a dark-field setup and explore the photon statistics of the scattered light under grazing laser illumination. Exploiting analytical solutions to Maxwell’s equations, we quantize the nanophotonic cavity fields and describe the formation of plasmon–exciton polaritons (or plexcitons) in the system. This way, we reveal that the rich plasmonic spectrum of the nanocavity offers unexplored mechanisms for nonclassical light generation that are more efficient than the resonant interaction between the emitter natural transition and the brightest optical mode. Specifically, we find three different sample configurations in which strongly antibunched light is produced. Finally, we illustrate the power of our approach by showing that the introduction of a second emitter in the platform can enhance photon correlations further.

Optical Quality of InAs/InP Quantum Dots on Distributed Bragg Reflector Emitting at 3rd Telecom Window Grown by Molecular Beam Epitaxy.

We present an experimental study on the optical quality of InAs/InP quantum dots (QDs). Investigated structures have application relevance due to emission in the 3rd telecommunication window. The nanostructures are grown by ripening-assisted molecular beam epitaxy. This leads to their unique properties, i.e., low spatial density and in-plane shape symmetry. These are advantageous for non-classical light generation for quantum technologies applications. As a measure of the internal quantum efficiency, the discrepancy between calculated and experimentally determined photon extraction efficiency is used. The investigated nanostructures exhibit close to ideal emission efficiency proving their high structural quality. The thermal stability of emission is investigated by means of microphotoluminescence. This allows to determine the maximal operation temperature of the device and reveal the main emission quenching channels. Emission quenching is predominantly caused by the transition of holes and electrons to higher QD’s levels. Additionally, these carriers could further leave the confinement potential via the dense ladder of QD states. Single QD emission is observed up to temperatures of about 100 K, comparable to the best results obtained for epitaxial QDs in this spectral range. The fundamental limit for the emission rate is the excitation radiative lifetime, which spreads from below 0.5 to almost 1.9 ns (GHz operation) without any clear spectral dispersion. Furthermore, carrier dynamics is also determined using time-correlated single-photon counting.

Efficient harmonic generation in an adiabatic multimode submicron tapered optical fiber

Optical nanotapers fabricated by tapering optical fibers have attracted considerable interest as an ultimate platform for high-efficiency light-matter interactions. While previously demonstrated applications relied exclusively on the low-loss transmission of only the fundamental mode, the implementation of multimode tapers that adiabatically transmit several modes has remained very challenging, hindering their use in various emerging applications in multimode nonlinear optics and quantum optics. Here, we report the realization of multimode submicron tapers that permit the simultaneous adiabatic transmission of multiple higher-order modes including the LP02 mode, through introducing deep wet-etching of conventional fiber before fiber tapering. Furthermore, as a critical application, we demonstrate fundamental-to-fundamental all-fiber third-harmonic generation with high conversion efficiencies. Our work paves the way for ultrahigh-efficiency multimode nonlinear and quantum optics, facilitating nonclassical light generation in the multimode regime, multimode soliton interactions and photonic quantum gates, and manipulation of the evanescent-field-induced optical trapping potentials of atoms and nanoparticles.

Light-matter quantum dynamics of complex laser-driven systems.

We propose a novel general approximation to transform and simplify the description of a complex fully quantized system describing the interacting light and matter. The method has some similarities to the time-dependent Born-Oppenheimer approach: we consider a quantum description of light rather than of nuclei and follow a similar separation procedure. Our approximation allows us to obtain a decoupled system for the light-excited matter and "dressed" light connected parametrically. With these equations at hand, we study how intense light as a quantum state is affected due to the back-action of the interacting matter. We discuss and demonstrate the possibility of the light-mode entanglement and nonclassical light generation during the interaction.

Investigation of 1064-nm Pumped Type II SPDC in Potassium Niobate for Generation of High Spectral Purity Photon Pairs

The generation and detection of nonclassical light of about 2 μm has good potential in an emerging field of high-sensitivity metrology, especially gravitational wave detection, as well as free-space quantum communication. A pair of photons is generated through a spontaneous parametric down-conversion (SPDC) process in a nonlinear optic crystal, which can be properly entangled in a spatial region where two beams with each polarization overlap or in a Sagnac-loop interferometer configuration. We investigated theoretically and numerically Type II SPDC in a potassium niobate (KNbO3, KN) crystal, which is useful as a material platform for generating photon pairs of high spectral purity in the 2-μm range. The technique is based on the frequency degenerate SPDC under Type II extended phase matching (EPM). We described the EPM characteristics of KN and showed that it is practically feasible for a 1064-nm pumped SPDC under moderate temperature conditions. The effective nonlinear optic coefficient of KN is at least four-times larger than those of other crystals using the Type II EPM approach, which implies a significant improvement in SPDC efficiency. The joint spectral analysis showed that a pair of photons can be generated with a high purity of 0.995 through proper pump filtering.

Exploring entanglement in open cavity parametric oscillators: From triply to doubly resonant cavities

We use a versatile model to evaluate the multipartite entanglement and the nonclassical light generation in optical parametric oscillators, exploring the differences between doubly and triply resonant cavity configurations. We demonstrate the entanglement of the pump mode with converted fields in both situations, and the fundamental differences of oscillators using parametric down conversion and four wave mixing processes as the intracavity amplification technique. The strong correlations involving the sidebands of the pump and converted fields give the signatures of a rich dynamic of multipartite entanglement.

Photorefractive effect in LiNbO3-based integrated-optical circuits for continuous variable experiments.

We investigate the impact of the photorefractive effect on lithium niobate integrated quantum photonic circuits dedicated to continuous variable on-chip experiments. The circuit main building blocks, i.e. cavities, directional couplers, and periodically poled nonlinear waveguides, are studied. This work demonstrates that photorefractivity, even when its effect is weaker than spatial mode hopping, might compromise the success of on-chip quantum photonics experiments. We describe in detail the characterization methods leading to the identification of this possible issue. We also study to which extent device heating represents a viable solution to counter this effect. We focus on photorefractive effect induced by light at 775 nm, in the context of the generation of non-classical light at 1550 nm telecom wavelength.

Widely tunable ultra-narrow-linewidth dissipative soliton generation at the telecom band

Ultra-narrow-linewidth mode-locked lasers with wide wavelength tunability can be versatile light sources for a variety of newly emergent applications. However, it is very challenging to achieve the stable mode locking of substantially long, anomalously dispersive fiber laser cavities employing a narrowband spectral filter at the telecom band. Here, we show that a nearly dispersion-insensitive dissipative mode-locking regime can be accessed through a subtle counterbalance among significantly narrowband spectral filtering, sufficiently deep saturable absorption, and moderately strong in-fiber Kerr nonlinearity. This achieves ultra-narrow-linewidth (a few gigahertz) nearly transform-limited self-starting stable dissipative soliton generation at low repetition rates (a few megahertz) without cavity dispersion management over a broad tuning range of wavelengths covering the entire telecom C-band. This unique laser may have immediate application as an idealized pump source for high-efficiency nonlinear frequency conversion and nonclassical light generation in dispersion-engineered tightly light-confining microphotonic/nanophotonic systems.

Hybrid integration methods for on-chip quantum photonics

The goal of integrated quantum photonics is to combine components for the generation, manipulation, and detection of nonclassical light in a phase-stable and efficient platform. Solid-state quantum emitters have recently reached outstanding performance as single-photon sources. In parallel, photonic integrated circuits have been advanced to the point that thousands of components can be controlled on a chip with high efficiency and phase stability. Consequently, researchers are now beginning to combine these leading quantum emitters and photonic integrated circuit platforms to realize the best properties of each technology. In this paper, we review recent advances in integrated quantum photonics based on such hybrid systems. Although hybrid integration solves many limitations of individual platforms, it also introduces new challenges that arise from interfacing different materials. We review various issues in solid-state quantum emitters and photonic integrated circuits, the hybrid integration techniques that bridge these two systems, and methods for chip-based manipulation of photons and emitters. Finally, we discuss the remaining challenges and future prospects of on-chip quantum photonics with integrated quantum emitters.

Generation of non-classical light in a photon-number superposition

The ability to generate light in a pure quantum state is essential for advances in optical quantum technologies. However, obtaining quantum states with control in the photon-number has remained elusive. Optical light fields with zero and one photon can be produced by single atoms, but so far it has been limited to generating incoherent mixtures, or coherent superpositions with a very small one-photon term. Here, we report on the on-demand generation of quantum superpositions of zero, one, and even two photons, via pulsed coherent control of a single artificial atom. Driving the system up to full atomic inversion leads to the generation of quantum superpositions of vacuum and one photon, with their relative populations controlled by the driving laser intensity. A stronger driving of the system, with $2\pi$-pulses, results in a coherent superposition of vacuum, one and two photons, with the two-photon term exceeding the one-photon component, a state allowing phase super-resolving interferometry. Our results open new paths for optical quantum technologies with access to the photon-number degree-of-freedom.

Tunable Photon Statistics Exploiting the Fano Effect in a Waveguide.

A strong optical nonlinearity arises when coherent light is scattered by a semiconductor quantum dot coupled to a nanophotonic waveguide. We exploit the Fano effect in such a waveguide to control the phase of the quantum interference underpinning the nonlinearity, experimentally demonstrating a tunable quantum optical filter which converts a coherent input state into either a bunched or an antibunched nonclassical output state. We show theoretically that the generation of nonclassical light is predicated on the formation of a two-photon bound state due to the interaction of the input coherent state with the quantum dot. Our model demonstrates that the tunable photon statistics arise from the dependence of the sign of two-photon interference (either constructive or destructive) on the detuning of the input relative to the Fano resonance.

Quality of photon antibunching in two cavity-waveguide arrangements on a chip

A quantum emitter coupled to an optical bimodal cavity in the solid-state implementation has recently proven to be an excellent platform for coherent generation of nonclassical light on a chip. However, the impacts of the structural couplings between the photonic modes via different arrangements of optical cavity and waveguide are rarely considered. Here, we explore in detail the characteristics of the photon antibunching in bimodal cavity quantum electrodynamics (QED) via taking into account two different cavity-waveguide arrangements: (i) an inline geometry and (ii) a side-coupled geometry. In our scheme, both cavity modes are simultaneously coupled to a two-level emitter but are not directly coupled to each other, owing to their orthogonal polarizations. It is clearly shown that the quality of the photon antibunching in the bimodal cavity QED, namely, the smallness of the second-order intensity correlation function at zero time, is closely related to the cavity-waveguide arrangements. The optimal photon antibunching can be achieved in the side-coupled geometry and the antibunching quality is about two orders of magnitude lower than that in the inline geometry. This enhancement of the photon antibunching is ascribed to the combination of two kinds of quantum interference effects in the waveguide-cavity QED system. We also find that the side-coupled architecture can make the device robust against the frequency mismatch between the two cavity modes, as compared to the inline geometry. In addition, we find that this mismatch can be used to generate better antibunching. The realization of our proposal with existing cavity-waveguide QED architectures is also discussed.1 MoreReceived 15 September 2018DOI:https://doi.org/10.1103/PhysRevA.98.053801©2018 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasCavity quantum electrodynamicsQuantum description of light-matter interactionQuantum interference effectsTechniquesCavity resonatorsAtomic, Molecular & Optical

Electromagnetic control and improvement of nonclassicality in a strongly coupled single-atom cavity-QED system

We present a study of the electromagnetic control of nonclassicality of the outgoing light field in a single atom cavity QED system. By exploring the energy eigenvalues and eigenstates, we show that the eigenstates are similar to the Jaynes-Cummings ladder of eigenstates and can be optically controlled by an external control field. Tuning the control field frequency to the one photon resonance, we show the superbunching behavior in the outgoing light field can be observed at the frequency of one photon resonance. We also show that there exists a magic control field intensity at which two photon blockade phenomenon can be significantly improved. In particular, it is possible to adjust the nonclassicality of the outgoing field from quantum to classical by varying the control field intensity. The work presented here provides an optical method to control statistical features of the outgoing field and can be useful for the nonclassical light generation, quantum gate operation and exotic quantum state generation.