New Degree Of Freedom Research Articles

Electric‐Field‐ and Stacking‐Tuned Antiferromagnetic FeClF Bilayer: The Coexistence of Bipolar Magnetic Semiconductor and Anomalous Valley Hall Effect

AbstractValley polarization from broken inversion symmetry provides a new degree of freedom for carriers, bipolar magnetic semiconductor (BMS) generates a purely spin‐polarized current under a gate voltage, but few systems possess the coexistence of valley polarization and BMS. Based on the recent experimental FeCl2 flakes, reversible electric‐field effect on the valley‐ and spin‐polarized Janus FeClF bilayer with different stackings are investigated herein. Janus FeClF bilayers in all three stacks possess interlayer antiferromagnetic (AFM) and intralayer ferromagnetic (FM) couplings. The most stable A (Cl‐Fe‐F‐Cl‐Fe‐F) stack possesses concurrent and spontaneous BMS nature and valley polarization with perpendicular magnetic anisotropy (PMA), while B (Cl‐Fe‐F‐F‐Fe‐Cl) and C (F‐Fe‐Cl‐Cl‐Fe‐F) stacks exhibit AFM semiconductor characters without valley polarization. Electric‐field achieves a transition of BMS and AFM semiconductor. Large ferrovalley (≈108 meV) exists and is mainly contributed by Fe‐dxy and orbitals. With the out‐of‐plane to in‐plane to out‐of‐plane transition of the easy axis, anomalous valley Hall effect (AVHE) can be manipulated to presence and disappearance by perpendicular electric‐field, indicating the valley switch effect (VSE). The coexisting BMS feature, PMA, AVHE and VSE make Janus FeClF bilayer a promising candidate for multifunctional valleytronic and spintronic applications, favoring broad explorations for the low‐dimensional Janus family.

Chirality-controlled second-order nonlinear frequency conversion in lithium niobate film metasurfaces.

The high-quality factor resonant metasurfaces have extensive applications in enhancing nonlinear frequency conversion efficiency at the subwavelength scale. However, methods for actively modulating the frequency conversion process are limited. We design a chiral lithium niobate film metasurface and investigate the photonic spin as a new degree of freedom to dynamically control the second-order nonlinear frequency conversion, without reconfiguring the structure by using external stimuli. The chiral resonance with circular dichroism (CD) of 0.62 gives rise to a high nonlinear CD of 0.84 in second-harmonic generation efficiency. Interestingly, combining the chiral resonance and an achiral quasi-bound state in the continuum enables us to investigate the photonic-spin-controlled sum-frequency generation and the photon pair generation from the spontaneous parametric downconversion process. Owing to the ultrahigh quality factor exceeding 103 both for two resonances, the second-order nonlinear frequency conversion occurs at a wavelength region of 0.2 nm, suggesting good monochromaticity. Our work opens new, to our knowledge, avenues for practical implementation of dynamically controlled nonlinear optical devices and will find utility in holography, switchable light sources, and information processing.

Relaxation of first-class constraints and the quantization of gauge theories: From “matter without matter” to the reappearance of time in quantum gravity

We make a conceptual overview of a particular approach to the initial-value problem in canonical gauge theories. We stress how the first-class phase-space constraints may be relaxed if we interpret them as fixing the values of new degrees of freedom. This idea goes back to Fock and Stueckelberg, leading to restrictions of the gauge symmetry of a theory, and it corresponds, in certain cases, to promoting constants of Nature to physical fields. Recently, different versions of this formulation have gained considerable attention in the literature, with several independent iterations, particularly in classical and quantum descriptions of gravity, cosmology, and electromagnetism. In particular, in the case of canonical quantum gravity, the Fock–Stueckelberg approach is relevant to the so-called problem of time. Our overview recalls and generalizes the work of Fock and Stueckelberg and its physical interpretation with the aim of conceptually unifying the different iterations of the idea that appear in the literature and of motivating further research.

Optimal Capacitance Design for IRS Aided Wireless Power Transfer for Sustainable IoT Communication

ABSTRACTIntelligent reflecting surface (IRS) is a cutting‐edge technique that can significantly improve wireless propagation. It can efficiently utilize wireless power transfer to enable sustainable Internet‐of‐Things (IoT) transmission by reconfiguring the incident signal from the active transmitter. However, the flexibility of capacitance tuning in the IRS system, which controls underlying reflections, is often overlooked. The effective capacitance design in the IRS system can provide a new degree of freedom in the IoT communication system, which can enable additional performance gain in the received power. To achieve this, a novel IRS circuital optimization model is proposed in this work. It incorporates various electrical parameters of the meta‐surface unit cell for improved IoT‐enabled communication. The proposed optimization model provides an optimal capacitance as a function of phase shift (PS), which is controlled by IRS, incident frequency, and other IRS electrical parameters. This optimal capacitance is then used to define the received power. The convexity of the optimization problem is proved, and the global optimal capacitance is obtained for received power maximization. Our simulations show that the proposed optimization model outperforms the existing constructive interference‐based optimal PS method, for which the capacitance is first calculated. Finally, the analytical results are numerically validated with several optimal design insights.

Constraint Realization‐Based Hamel Field Integrator for Geometrically Exact Planar Euler–Bernoulli Beam Dynamics

ABSTRACTIn this article, we first introduce a Hamel field integrator designed for a geometrically exact Euler–Bernoulli beam with infinite‐dimensional holonomic constraints, constructed using a Lagrange multiplier. This method addresses the complexities introduced by constraints, but the additional multiplier introduces a new degree of freedom and hence results in a system with mixed‐type partial differential equations. To address this issue, we further propose a constraint realization method based on perturbation theory for infinite‐dimensional mechanical systems within the framework of Hamel's formalism. This method circumvents the use of additional Lagrange multiplier, significantly reducing the computational complexity of modeling problems. Building on this, we construct a perturbed Hamel field integrator optimized for parallel computing and incorporate artificial viscosity to accelerate constraint convergence. While applicable to three dimensions, our method is demonstrated in a simplified context using planar Euler–Bernoulli beam examples to illustrate the effectiveness of the unified mathematical framework.

Anomalous wavefront control of Lamb wave with metasurfaces via superposed prism resonance

As a special branch of metamaterials characterized by phase discontinuity, elastic metasurfaces have presented extraordinary capacity for elastic wave manipulation. This class of metamaterials has received extensive attention in recent years. In this paper, a subwavelength elastic metasurface with locally resonant prisms is employed to steer the propagation of the A0 Lamb wave. Based on the dispersion curve and transmission ratio, we establish that the resonant feature of prisms is influenced by the diagonal ratio of cross section. By gradually tuning the diagonal ratio of prism cross section, the pattern of resonance modes and the mechanism of resonance superposition are clarified. In this regard, two different resonant modes can be superimposed at a certain frequency. A complete 2 π phase shift that is crucial for redirecting wave propagation can therefore be realized. To have a broader working frequency range, the influence of prism height on the resonance superposed frequency and the effect of plate thickness on the incident flexural wave are explored. Based on the generalized Snell’s law, negative refraction is verified numerically through a metasurface assembled from unit cells with constant phase change. In addition, other wavefront modulations such as eccentric focusing, nonparaxial propagation are also demonstrated. This novel design introduces new degrees of freedom in many engineering applications such as seismic wave protection, structural health monitoring and energy harvesting.

Emergent Behavior of a Photoswitchable Solute in a Biphasic Solvent System.

Due to thermal E/Z isomerization, hydrazones in solution typically exist in thermodynamic equilibria between their isomers. Irradiation of such solutions leads to photostationary states that may differ from the equilibrium distribution. Operating such switchable hydrazones in a biphasic system of two immiscible solvents introduces three new degrees of freedom: the E/Z equilibrium in the second solvent and two equilibria for distribution of each of the isomers between the solvents. Irradiation of such a system can be performed in three different ways - the first solvent only, the second solvent only, and both solvents at once - all yielding distinct outcomes. Depending on the choice of materials and the mode of irradiation, such setup may lead to different emergent behaviors that are not immediately intuitive, including net cyclic transport or the accumulation of one photoswitched product in one of the phases, beyond what is reachable by irradiating a simple solution of the same photoswitch.

Dissimilar soliton molecule formed by dissipative pulses in a single-mode mode-locked fiber laser

Soliton molecules, or also known as optical bound states, are the most representative example of solitons’ particle nature and have given birth to diverse light-matter analogies. Despite detailed research on regular bound states, the soliton molecule synthesis of dissimilar pulses has rarely been reported. Here, soliton molecules formed by dissimilar dissipative solitons are demonstrated in a single-mode mode-locked fiber laser, with an in-depth analysis of their evolution dynamics. This novel bound state features pulse trapping between two ultrafast vector pulses with distinct pulse properties including energy, duration, and chirp, leading to unique temporal and spectral profiles. This laser provides an optimal platform for studying complex interactions between different types of dissipative solitons. The findings here can provide new degrees of freedom for the generation of optical soliton molecules and can fuel applications in optical information processing, metrology, and spectroscopy.

Strain-oxygen vacancies coupling in topotactic (La,Sr)CoO3-δ thin films

Oxygen defect engineering is a widely used approach for tuning physical properties in oxides. Multivalent transition metal oxide La0.7Sr0.3CoO3-δ (LSCO) shows oxygen vacancy-driven metal-to-insulator transition (MIT) due to topotactic phase transition and its high oxygen vacancy tolerance. Here, we introduce strain as a new degree of freedom to study the strain-oxygen vacancy coupling effects and elucidate its impact on the electronic property in oxygen-deficient LSCO epitaxial thin films grown on SrTiO3 (100) single crystal. By combining the experimental results with density functional theory plus U (DFT+U) calculations, we reveal that 2.1 % in-plane tensile strain can stabilize the insulating state of LSCO with a surprisingly low concentration of oxygen vacancies, <0.5 %. This study reveals that the MIT in LSCO is governed by the combination of oxygen vacancies and strain, offering the potential for additional tuning knob of the material's electronic properties.

Realization of Time-Reversal Invariant Photonic Topological Anderson Insulators.

Disorder, which is ubiquitous in nature, has been extensively explored in photonics for understanding the fundamental principles of light diffusion and localization, as well as for applications in functional resonators and random lasers. Recently, the investigation of disorder in topological photonics has led to the realization of topological Anderson insulators characterized by an unexpected disorder-induced phase transition. However, the observed photonic topological Anderson insulators so far are limited to the time-reversal symmetry breaking systems. Here, we propose and realize a photonic quantum spin Hall topological Anderson insulator without breaking time-reversal symmetry. The disorder-induced topological phase transition is comprehensively confirmed through the theoretical effective Dirac Hamiltonian, numerical analysis of bulk transmission, and experimental examination of bulk and edge transmissions. We present convincing evidence for the unidirectional propagation and robust transport of helical edge modes, which are the key features of nontrivial time-reversal invariant topological Anderson insulators. Furthermore, we demonstrate disorder-induced beam steering, highlighting the potential of disorder as a new degree of freedom to manipulate light propagation in magnetic-free systems. Our work not only paves the way for observing unique topological photonic phases but also suggests potential device applications through the utilization of disorder.

Inherent Temporal Metamaterials with Unique Time-Varying Stiffness and Damping.

Time-varying metamaterials offer new degrees of freedom for wave manipulation and enable applications unattainable with conventional materials. In these metamaterials, the pattern of temporal inhomogeneity is crucial for effective wave control. However, existing studies have only demonstrated abrupt changes in properties within a limited range or time modulation following simple patterns. This study presents the design, construction, and characterization of a novel temporal elastic metamaterial with complex time-varying constitutive parameters induced by self-reconfigurable virtual resonators (VRs). These VRs, achieved by simulating the resonating behavior of mechanical resonators in digital space, function as virtualized meta-atoms. The autonomously time-varying VRs cause significant temporal variations in both the stiffness and loss factor of the metamaterial. By programming the time-domain behavior of the VRs, the metamaterial's constitutive parameters can be modulated according to desired periodic or aperiodic patterns. The proposed time-varying metamaterial has demonstrated capabilities in shaping the amplitudes and frequency spectra of waves in the time domain. This work not only facilitates the development of materials with sophisticated time-varying properties but also opens new avenues for low-frequency signal processing in future communication systems.

Rolling Motion of Rigid Skyrmion Crystallites Induced by Chiral Lattice Torque.

Magnetic skyrmions are topologically protected spin textures with emergent particle-like behaviors. Their dynamics under external stimuli is of great interest and importance for topological physics and spintronics applications alike. So far, skyrmions are only found to move linearly in response to a linear drive, following the conventional model treating them as isolated quasiparticles. Here, by performing time and spatially resolved resonant elastic X-ray scattering of the insulating chiral magnet Cu2OSeO3, we show that for finite-sized skyrmion crystallites, a purely linear temperature gradient not only propels the skyrmions but also induces continuous rotational motion through a chiral lattice torque. Consequently, a skyrmion crystallite undergoes a rolling motion under a small gradient, while both the rolling speed and the rotational sense can be controlled. Our findings offer a new degree of freedom for manipulating these quasiparticles toward device applications and underscore the fundamental phase difference between the condensed skyrmion lattice and isolated skyrmions.

Effects of thickness, temperature and substrate on phonon anisotropy in layered Ta2NiSe5

Anisotropy in crystal structure has provided a new degree of freedom to tune the physical and photoelectric properties of low-symmetrical materials, enabling the anisotropic band structure and polarization-resolved applications. Thus, the identification and control on the anisotropy is of great importance for the development of polarization-integrated devices. In this work, we introduce a promising two-dimensional (2D) dimetal chalcogenide Ta2NiSe5 with strong in-plane anisotropic structure and explore the effects of thickness, temperature and substrate on its in-plane anisotropy via an angle-resolved polarized Raman spectra. It is shown that the Raman mode softens with increasing temperature, revealing the anharmonic phonon properties of the Ta2NiSe5 flakes. We found that the anisotropy of phonon vibration is strongly related with the thickness, temperature and used substrate, which is more obvious at thinner samples, higher temperature and opaque silicon substrate compared to sapphire and suspended conditions. This work first reveals the influence factor on the anisotropy of phonon mode, which will guide the fundamental research of anisotropic physics and experimental design for the angle-resolved electronics.

Transverse Spin-Orbit Interaction of Light.

Light carries both longitudinal and transverse spin angular momentum. The spin can couple with its orbital counterpart, known as the spin-orbit interaction (SOI) of light. Complementary to the longitudinal SOI known previously, here we show that transverse SOI of light is inherent in the Helmholtz equation when transverse spinning light propagates in curved paths. It lifts the degeneracy of dispersion relations of light for opposite transverse spin states, analogous to the Dresselhaus effect. Transverse SOI is ubiquitous in nanophotonic systems where transverse spin and optical path bending are inevitable. It can explain anomalous effects like the dispersion relation of surface plasmon polaritons on curved paths and the energy level of whispering gallery modes. Our results reveal the analogies of spin photonics and spintronics and offer a new degree of freedom for integrated photonics, spin photonics, and astrophysics.

Polarization-Controlled Exciton-Polaritons in WS2 Strongly Coupled with Low-Symmetry Photonic Crystal Nanostructures.

Atomically thin transition metal dichalcogenides (TMDs) with ambient stable exciton resonances have emerged as an ideal material platform for exciton-polaritons. In particular, the strong coupling between excitons in TMDs and optical resonances in anisotropic photonic nanostructures can form exciton-polaritons with polarization selectivity, which offers a new degree of freedom for the manipulation of the light-matter interaction. In this work, we present the experimental demonstration of polarization-controlled exciton-polaritons in tungsten disulfide (WS2) strongly coupled with polarization singularities in the momentum space of low-symmetry photonic crystal (PhC) nanostructures. The utilization of polarization singularities can not only effectively modulate the polarization states of exciton-polaritons in the momentum space but also facilitate or suppress their far field coupling capabilities by tuning the in-plane momentum. Our results provide new strategies for creating polarization-selective exciton-polaritons.

Chiral Twist Interface Modulation Enhances Thermoelectric Properties of Tellurium Crystal.

Manipulating the grain boundary and chiral structure of enantiomorphic inorganic thermoelectric materials facilitates a new degree of freedom for enhancing thermoelectric energy conversion. Chiral twist mechanisms evolve by the screw dislocation phenomenon in the nanostructures; however, contributions of such chiral transport have been neglected for bulk crystals. Tellurium (Te) has a chiral trigonal crystal structure, high band degeneracy, and lattice anharmonicity for high thermoelectric performance. Here, Sb-doped Te crystals are grown to minimize the severe grain boundary effects on carrier transport and investigate the interface of chiral Te matrix and embedded achiral Sb2Te3 precipitates, which induce unusual lattice twists. The low grain boundary scattering and conformational grain restructuring provide electrical-favorable semicoherent interfaces. This maintains high electrical conductivity leading to a twofold increase in power factor compared to polycrystal samples. The embedded Sb2Te3 precipitates concurrently enable moderate phonon scattering leading to a remarkable decrease in lattice thermal conductivity and a high dimensionless figure of merit(zT)of 1.1 at 623 K. The crystal growth and chiral atomic reorientation unravel the emerging benefits of interface engineering as a crucial contributor to effectively enhancing carrier transport and minimizing phonon propagation in thermoelectric materials.

The interlayer twist effectively regulates interlayer excitons in InSe/Sb van der Waals heterostructure

The interlayer twist angle endows a new degree of freedom to manipulate the spatially separated interlayer excitons in van der Waals (vdWs) heterostructures. Herein, we find that the band-edge Γ-Γ interlayer excitation directly forms interlayer exciton in InSe/Sb heterostructure, different from that of transition metal dichalcogenides (TMDs) heterostructures in two-step processes by intralayer excitation and transfer. By tuning the interlayer coupling and breathing vibrational modes associated with the Γ-Γ photoexcitation, the interlayer twist can significantly adjust the excitation peak position and lifetime of recombination. The interlayer excitation peak in InSe/Sb heterostructure can shift ~400 meV, and the interlayer exciton lifetime varies in hundreds of nanoseconds as a periodic function of the twist angle (0°–60°). This work enriches the understanding of interlayer exciton formation and facilitates the artificial excitonic engineering of vdWs heterostructures.

Linear Bloch-Siegert phase-encoded low-field MRI: RF coils, pulse sequence, and image reconstruction.

Conventional gradient systems have several weaknesses including high cost and bulk. As a step towards addressing these while providing new degrees of freedom for spatial encoding and system design in Magnetic Resonance Imaging (MRI), a radio frequency (RF) gradient encoding system and pulse sequence for phase encoding using the Bloch-Siegert (BS) shift were developed. Optimized BS spatial encoding coils with bucking windings (counter-wound loops) were designed and constructed, along with compatible homogeneous imaging coils for excitation and signal reception. Two coil systems were developed: one for phantom imaging and a second for human wrist imaging. BS phase-encoded imaging and BS RF pulse simulations were performed. Pulse sequences were designed for linear stepping in k-space and implemented on a 47.5-mT scanner to image resolution phantoms in both coil setups. Reconstructions were performed using both the full -based encoding fields for each BS pulse amplitude and using inverse discrete Fourier transforms. A gradient was used for frequency encoding during signal readout, and the third axis was projected. Specific absorption ratio (SAR) calculations were performed for the wrist coil to determine the safety of BS-based RF encoding for fields in the low field MRI regime. The optimized RF spatial encoding coils resulted in higher linearity ( and 0.9921 in the phantom and wrist coils, respectively) than coils used in previous work. The phantom and wrist imaging coils were validated in simulations and experimentally to produce a peak G and 0.8 G with 12-W input power, respectively, in the field-of-view (length = 11 cm) used for imaging. Nominal imaging resolutions of 5.22 and 7.21 mm were, respectively, achieved by the two-coil systems in the RF phase-encoded dimension. Coil systems, pulse sequences, and image reconstructions were developed for linear RF phase encoding using the BS shift and validated using a 47.5-mT open low field scanner, establishing a key component required for gradient-free imaging at low field strengths.

Non-Abelian Holonomy in Degenerate Non-Hermitian Systems.

Non-Abelian holonomy, a noncommutative process that measures the parallel transport of non-Abelian gauge fields, has so far been realized in degenerate Hermitian systems with degenerate eigenstates or nondegenerate non-Hermitian systems with exceptional points. Here, we introduce non-Abelian holonomy into degenerate non-Hermitian systems possessing degenerate exceptional points and degenerate energy topologies. The interplay between energy degeneracy and energy topology around exceptional points leads to a non-Abelian holonomy with multiple energy levels and multiple degenerate levels simultaneously, going beyond that in degenerate Hermitian systems with a single energy level, or in nondegenerate non-Hermitian systems with a single degenerate level. We exploit an on-chip photonic platform to experimentally demonstrate the holonomy induced non-Abelian phenomenon, including the switching of eigenstates associated with different degenerate exceptional points and sequence-dependent holonomic outcomes. Our work shifts the paradigm of non-Abelian holonomy and adds new degrees of freedom for non-Abelian applications.

Extending the operational range of Francis turbines: A case study of a 200 MW prototype

Francis turbines are now widely used to support the integration of renewable and intermittent energy sources such as solar and wind power. Consequently, these turbines often operate away from their best efficiency point (BEP). Such operations cause detrimental pressure fluctuations in the runner and draft tube, leading to early fatigue failures. To address these harmful flow conditions and extend the operating range of Francis turbines, a mitigation system was developed and tested on a large-scale, high-head 200 MW Francis turbine. The system consists of four circular rods placed in the draft tube with variable radial protrusion lengths, adjustable using linear actuators. Pressure, accelerometer, and vibration sensors installed on the turbine allowed quantification of the rod system performance. The results demonstrate the system’s capability to reduce pressure pulsations by up to 80 % in terms of maximum pressure amplitude and 100 % in terms of fatigue cycle in both low and high-frequency ranges, up to ten times the runner frequency, based on pressure analysis. The optimal rod protrusion ranges from 5 to 20 % of the runner outlet diameter function of the operating load. The impact of the rods’ protrusion on the turbine structure appears negligible from the accelerometer measurements performed on the draft tube and spiral casing. The hydraulic efficiency is reduced by up to 1 %. These findings are significant across a wide range of part-load operations, from 40 % to 60 % load, indicating the potential to extend the operational range of existing Francis turbines. The research presented here is a novel attempt to enhance the existing Francis turbines with a new degree of freedom using protruding rods.