Neutron Detector Research Articles

A SiC Microstructured Neutron Detector Based on Deep Trench Etching Process

A SiC Microstructured Neutron Detector Based on Deep Trench Etching Process

A Chlorine based detector (LaCl3(Ce)) for 2.5 MeV neutron spectroscopy in deuterium nuclear fusion plasmas with enhanced particle discrimination algorithm

Abstract Neutron Emission Spectroscopy is an effective nuclear fusion plasma diagnostics technique for diagnosing the fuel ion populations on fusion plasma experiments. The state of the art 2.5 MeV neutron spectrometer for deuterium plasmas is based on the time of flight (TOF) technique, which however requires the development of large scale instruments. In the last years, compact detectors made with Chlorine based scintillators have been explored. In these instruments, neutron detection is based on the 35Cl(n,p)35S nuclear reaction, which results in a Gaussian peak in the recorded neutron energy spectrum. In this context, one option is offered by CLYC scintillators, which have the drawback of a limited counting rate capability (a few tens of kHz). Another option is offered by the LaCl3:(Ce) scintillators, which combine a comparable energy resolution and, most importantly, a faster signal (<1 μs) enabling measurements at higher counting rates. On the other hand, LaCl3 has a more challenging particle discrimination. The standard method based on pulse shape analysis provides a limited particle identification and poses restrictions in the counting rate capability of the instruments. An innovative particle identification algorithm based on Fourier Transforms has been developed providing higher accuracy and effectiveness. In this paper, we present the performance of a 2.5 MeV neutron spectrometer based on a LaCl3 scintillator in terms of pulse shape discrimination and energy resolution. Results are used to discuss their use for neutron spectroscopy applications in tokamak plasmas.

Solid, structured composite neutron detectors with high dynamic range capability

Neutron detectors are essential across disciplines such as fundamental science, nuclear security, safeguards, and civilian applications. While 3He-filled gas proportional counters have long been revered for their efficacy in detecting thermal neutrons and praised for their efficiency, neutron/gamma discrimination, and stability, the scarcity of 3He has spurred a search for alternatives. Here, we explore a solid structured scintillating particle composite (SPC) consisting of 6Li-containing scintillating glass particles within an acrylic matrix as a neutron detector for high dynamic range applications. We show for the first time that an SPC neutron detector can boast an intrinsic detection efficiency of 0.261% for pure 252Cf fission neutrons and an overall neutron detection efficiency of (0.546 ± 0.003)% at the Neutron Free-in-Air facility while being able to function in an intense gamma-ray environment. We also show that the SPC neutron detector supports fast neutron capture times and enables a dual-readout scheme that extends the detector dynamic range to high incident neutron fluxes. A scalable fabrication process allows for tailoring the SPC detector properties to the requirements of specific applications. Good agreement is found between the experimental results taken with a National Institute of Standards and Technology traceable 252Cf source and the coupled MCNP6 and optical-ray-tracing simulations.

Development of an online neutron beam monitoring system for accelerator-based boron neutron capture therapy in a hospital.

Boron neutron capture therapy (BNCT) is a next-generation radiotherapy, utilizing both an external neutron beam and a -containing pharmaceutical. A compact accelerator for a high intensity neutron source was installed to conduct BNCT in a hospital. The dose administered to a patient was evaluated by measuring the proton beamcurrent. Neutron intensity should be monitored in real-time by measuring the neutrons emitted from the target during BNCT irradiation. This is crucial due to potential neutron target degradation. Online neutron beam monitoring systems are required for reliable measurements of the administered neutron dose. An online neutron beam monitoring system was developed to monitor neutron intensity irradiating on the patient at the National Cancer Center Hospital (NCCH). The neutron detector comprised a back-illuminated thin Si diode of 40- thickness and an ultrathin natural LiF neutron converter of 0.05- thickness. The neutron detector was installed on the neutron target unit, regardless of whether a patient was present, without any additional modifications to the setup. The response functions for high photon dose rates of upto 100 Gy/h were measured. The pulse heights were measured using the neutron beam monitor during BNCT neutron irradiation. Neutron temporal response measured using the online beam monitor was acquired and compared with the proton beam current and the measurements at a patient position. From this measurement at the patient position, the neutron fluence rate irradiating on a patient wasobtained. The neutron events were separated from the photon events. The neutron counting rates increased rapidly with the starting of proton beam irradiation and dropped to zero upon its termination. During intermittent drops and recoveries in the proton beam, the neutron beam monitor for counting rates responded quickly, synchronizing with the beam current. A scatter plot of the neutron counting rate and proton beam current indicated a good linear correlation. A direct relationship between the online neutron beam monitor's neutron counting rates and those of the patient neutron detector showed a good correlation coefficient of 0.84. A ratio of the both neutron counting rates showed a standard deviation of 6%. The correlation coefficient and standard deviation were improved to 0.94 and 1.5%, by re-binning the neutron temporal response with longer acquisition period than 1 s. Using the online neutron beam monitor, the neutron fluence rate was obtained from the direct relationship within 1.5%. Therefore, real-time monitoring of neutron intensity was achieved within the acceptable level as per the International Commission on Radiation Units and Measurementsreport. The online neutron beam monitoring system was developed to monitor the BNCT neutron beam intensity at NCCH. The temporal response of the neutron beam monitor was synchronized with the neutron counting rate at the patient position. Using the online neutron beam monitor, the neutron fluence rate irradiating on the patient can be monitored from the direct relationship. Fluctuation of the neutron beam intensity through BNCT irradiation and the degradation of the lithium target through the lifespan of the neutron target could be monitored using the neutron beammonitor.

Stoichiometric effect on the defect states and optical properties of LiInSe2 single crystals

LiInSe2 crystals are promising semiconductor materials for neutron detectors due to the large neutron capture cross-sectional area of the specific isotopes (6Li) and high charge transport properties. However, the optoelectronic performance fails to reach the expected level due to the difficulty of controlling the crystal defects. Herein, we modulate the stoichiometric ratio to control the type of defects in single LiInSe2 crystals grown by the vertical Bridgman method. The UV‒vis–NIR transmission results indicate that the band gap of the yellow colored Li1.01In1Se2 sample is close to ~ 2.83 eV at room temperature, and this value is consistent with the theoretical band gap of LiInSe2 (~ 2.86 eV). Photoluminescence (PL) spectroscopy was used to analyze the defect concentration. The results indicate that the defect types in the yellow Li1.01In1Se2 single crystal are VSe+ and LiIn2−; these result from the introduction of excess Li and the suppression of the adverse defects in InLi2+ and VLi−. These results demonstrate a feasible route for obtaining high-quality yellow 6LiInSe2 crystals and promote the application of 6LiInSe2 neutron detectors.

Transient Current Analysis of GaN Neutron Detector Based on the SRIM and TCAD Methods

Utilizing Technology Computer Aided Design (TCAD) software, this study determines the optimal thickness and doping concentration for the intrinsic gallium nitride (GaN) layer in a p-i-n GaN diode to improve detection efficiency and reliability. The study examines energy loss and the transient current response induced by alpha and 3H particles within the GaN p-i-n diode. Additionally, TCAD elucidates the transient current behavior arising from electron-hole pair generation, utilizing the Stopping and Range of Ions in Matter SRIM-2013 linear energy transfer distribution as a guide. The simulations disclose that the tailing effect in the transient current response results from radiation-induced hole accumulation. Elevated applied bias results in increased transient current pulse amplitude, attributed to an extended depletion region that boosts carrier collection. These insights are expected to drive advancements in GaN-based neutron detector technology, essential for advancing nuclear and space science applications in the next generation.

Development of a multi-layer high-efficiency GEM-based neutron detector for spallation sources

Neutron detection is nowadays mostly based on 3He gas detectors, but its shortage and the continuous upgrades of the neutron facilities require new devices to perform experiments with maximum performances. This work presents a new detector based on the Gas Electron Multiplier (GEM) combined with several boron layers. This detector combines the features of GEM technology with the properties of boron as a neutron converter and the device is produced to sustain high neutron fluxes with high detection efficiency. The detector has been characterised at the ISIS Pulsed Neutron and Muon Source (UK). Based on the analysis of our results, the detector has shown a good response to thermal and epithermal neutrons reaching a detection efficiency of 16% at 1.8 Å (25 meV). The good detection efficiency (even increasable with the addition of further boron GEM foils) and the good time resolution, make the detector a unique device for the neutron techniques. In particular, its use can easily be envisaged in techniques involving neutron transmission measurements, that require high fluxes impinging on the detectors, with the added bonus of a 2D-resolved capability due to the padded anode.

Isotopically Enriched Lithium Fluoride Crystals for Detection of Neutrons with the Fluorescent Track Technique.

In this work, the properties of LiF crystals grown using Li of different isotopic compositions are described from the standpoint of their application as fluorescent nuclear track detectors used in measurements in the neutron radiation fields. The crystals were grown using two techniques: the Czochralski method and the micro-pulling-down method. Three isotopic compositions of Li were studied: natural, highly enriched in 6Li, and highly enriched in 7Li. It was found that 6LiF detectors are about six times more sensitive to thermal (low energy) neutrons than natural LiF, which significantly decreases the lower detection limit. 7LiF detectors are insensitive to thermal neutrons, which makes it easier to detect tracks due to other radiation modalities, such as energetic ions or nuclei recoiled in collisions with high-energy neutrons. Besides the response to neutron radiation, no other significant differences in the crystal properties were identified, irrespective of the isotopic composition and crystal growth method employed.

Measurement of tritium production in the helium cooled pebble bed test blanket module mock-up at JET during DTE2

Quite often, detectors for measuring nuclear performance and radiation quantities of relevance in fusion experiments are requested to withstand harsh working conditions due to intense neutron and gamma radiation fields. High temperature constitutes a further harsh element in some locations of the machine, where it is necessary to perform some on-line measurements, as expected in the breeding blanket. This is an essential component in future fusion power plants to provide tritium self-sufficiency and its performance must be continuously monitored. Some Test Blanket Modules (TBMs) will be installed in ITER to provide the first experimental data to validate the predictions on tritium production and recovery. In the meantime, within EUROfusion program, the mock-up of the Helium Cooled Pebble Bed Test Blanket Module (HCPB TBM), previously used for the TBM experiment at the Frascati Neutron Generator (FNG), had been installed at JET to test some detectors and for benchmarking numerical codes used for breeding blanket assessment during DTE2 campaign. A diamond detector, calibrated to measure the tritium production through neutron detection inside the HCPB TBM mock-up, was tested during some plasma pulses of the DTE2 campaign at JET. The main outcome is that, as far as neutron emission rate is below 1015 s−1, neutrons are properly detected along the plasma discharge evolution by TBM diamond detector, consistently with the JET neutron monitor KN1. Moreover, the amount of tritium measured (E) is 1.40 × 10–12 tritons per source neutron and the comparison with MCNP radiation transport simulation (C) gives a ratio C/E = 0.77. Such measurements, considered promising, and their comparison with calculations are discussed in the present work. Criticalities emerged are analyzed and some improvements proposed with the main purpose of speeding up signal processing to make the system capable of working at higher plasma neutron emission rates.

Characterization of new silicon carbide neutron detectors with thermal and fast neutrons

The aim of this work is to present a characterization of a new silicon carbide (SiC) neutron detector fabricated at the Institute of Microelectronics of Barcelona (IMB-CNM-CSIC). The device is based on a 50μm thick p-n diode built in a 4H-SiC wafer. Performance studies were carried out under different neutron energy spectra, including thermal and quasi-monoenergetic fast neutrons at the CNA HiSPANoS facility. We implemented a method for the fabrication of enriched LiF conversion layers to use for the detection of thermal neutrons. The detector was proven to be capable of being used for thermal neutron detection with conversion layers of 10B and LiF. A detection efficiency of 6 ± 1% was achieved with a 25μm thick LiF conversion layer. It was also confirmed that the device can be employed for the detection of recoil nuclei and protons produced by fast neutrons. The spectra obtained experimentally were compared with PHITS simulations. This work represents the first step towards the design and fabrication of new SiC neutron detectors in the IMB-CNM-CSIC clean room with potential applications in various scientific and technological fields.

Comparison of Rhodium, Vanadium, Cobalt, Inconel & Silver Emitter Self-Powered Neutron Detectors: Literature Review Article

Self-Powered Neutron Detectors (SPNDs) are in use as in-core Neutron Fluence Detectors in Nuclear Power Plants. Though the detectors are simple in design and have a common structure for the same application, there are various types of emitters (neutron-sensitive electrodes) that make SPNDs categorized into different types. There are various SPNDs in application at different types of nuclear power reactors. SPND emitters are chosen based on their characteristics/behavior in the neutron & gamma flux environment in the reactor core. A detailed Literature Review was done on five different types of SPNDs. This paper focuses on the physics behind the operation, characteristics, and review of Vanadium, Rhodium, Inconel, and Cobalt & Silver emitter-based SPNDs. A comparison study was done by a literature review on these detectors.

Performance of large-scale [formula omitted]Li-doped pulse-shape discriminating plastic scintillators

A 6Li-doped plastic scintillator with pulse-shape discrimination capabilities, commercially identified as EJ-299-50, has been developed and produced at the kilogram-scale. A total of 44 kg-scale bars of dimensions 5.5 cm x 5.5 cm x 50 cm of this material have been characterized. Optical properties like light output and effective attenuation length have been found to be comparable to 6Li-doped liquid scintillators. The scintillator EJ-299-50 shows good neutron detection capabilities with an effective efficiency for capture on 6Li of approximately 85%. Stability tests performed on two formulation variations showed no intrinsic degradation in the material or optical properties during several months of observations.

A novel embedded spherical semiconductor neutron detector efficiency estimation using GEANT4 simulation methodology

The present research work explores on the estimation of thermal neutron detection efficiency for the novel embedded spherical configuration design using GEANT4 toolkit. Initially, single and multiple layer of embedded spherical configurations were designed in geometry category class of GEANT4 toolkit using Boron (10B) converter material followed by, estimation of simulated thermal neutron detection efficiency at different radii which varies between 0.05 μm to 5 μm for both single and multiple layer embedded spherical detector configuration. The maximum thermal neutron detection efficiency obtained for the single layer embedded spherical detector configuration is ∼ 5.1% at an optimum (critical) radius of ∼ 4.55 μm. It was noticed that with the rise in the number of layers of embedded spherical detector configuration the thermal neutron detection efficiency was also increasing. Furthermore, investigation of the effect of varying level of Low Level Discriminator and different enrichment level of 10B on the efficiency was also studied. Finally, the histoplot was investigated for a typical 10 layers of embedded spherical detector configuration at typical lower (200 nm) and higher (3 μm) radius.

The effect of Sb2O3 on optical, scintillation and service performance of Ce3+-ion doped gadolinium aluminosilicate glasses

Ce3+-doped gadolinium aluminosilicate glass has great potential as a scintillator in neutron detection and high-energy physics. Ce3+-doped gadolinium aluminosilicate glasses with different concentrations of clarifier Sb2O3 were prepared by high temperature feeding method, combined with crucible interlocking technology. Ce4+ ions were reduced to be Ce3+ ions by CO atmosphere in an interlocking crucible. The properties of glass with 0.7 mol% content of Sb2O3 are the best. The glass has a high density (>6.0 g/cm3) and high refractive index (nd > 1.74). Compared with the sample without clarifier Sb2O3, the light yield of the glass increased to about 2 times. From XPS results, it is concluded that the proportion of bridge and non-bridge oxygen in the glass is 58.83 % and 41.67 % respectively. The composition of bridge oxygen in the glass is high, so there are many silicon-oxygen polyhedrons, and the structure in the glass system is stable, which is beneficial to the light yield. It can be seen from the Ce3d spectrum that there is no third characteristic peak of Ce4+ at ∼916 eV, indicating that the content of Ce3+ is more than that of Ce4+. The presence of Ce3+ in the glass is excellent for scintillation properties.

Neutron spectrum measurements inside a self-shielded cyclotron during 18F production using a single-cylindrical neutron spectrometer with gold and indium activation foils

The Single-Cylindrical Neutron Spectrometer (SCNS) is a single moderated spectrometer in the form of a cylinder with a diameter of 8 cm and a length of 16 cm. Seven Au activation foil type neutron detectors are installed on the moderator axis with varying distances. This spectrometer is used to measure the neutron spectrum in self-shielded cyclotron during 18F production using a proton of 11 MeV and a beam current of 25 µA for 70 min. The detector response was calculated using MCNPX 2.7. The measurement results obtained activity of 198Au and 116mIn and were validated with simulation using MCNPX. With the detector response values and detector activity from the measurements, a neutron spectrum was obtained using the unfolding technique using the UMG program. The neutron spectrum from measurements using SCNS with Au and In activation foil detectors has a difference of 8 %. Meanwhile, with the MCNPX calculation results, the measurement results using the Au foil are 1 % while with the In foil it is 10 %.

All Inorganic Scintillating Fiber for Thermal Neutron Detection

AbstractThermal neutron detection with scintillating fibers has excellent scientific and technological potential for remote and spatially resolved detection. However, most fibers are polymers, and developing all‐inorganic scintillating fibers remains a significant challenge. Herein, all‐inorganic scintillating fibers and prototype neutron detection devices are successfully constructed for neutron detection. The scintillating fibers with a perfect waveguide configuration and tunable size have been fabricated through the melt‐in‐tube method. The interactions between the thermal neutron and scintillating fiber have been theoretically analyzed. The dependence of the neutron absorption ability on the core diameter, cladding thickness, and 6Li abundance has been investigated. Guided by the above experimental and theoretical results, the configuration of the scintillating fiber and the corresponding neutron detection prototype device has been built. Its practical application for neutron detection has been demonstrated, and importantly, the single thermal neutron event can be successfully monitored. The device shows great promise for neutron detection applications in special scenarios such as tiny space and electromagnetic interference environments.

Demonstration of shape analysis of neutron resonance transmission spectrum measured with a laser-driven neutron source

Laser-driven neutron sources (LDNSs) can generate strong short-pulse neutron beams, which are valuable for scientific studies and engineering applications. Neutron resonance transmission analysis (NRTA) is a nondestructive technique used for determining the areal density of each nuclide in a material sample using pulsed thermal and epithermal neutrons. Herein, we report the first successful NRTA performed using an LDNS driven by the Laser for Fast Ignition Experiment at the Institute of Laser Engineering, Osaka University. The key challenge was achieving a well-resolved resonance transmission spectrum for material analysis using an LDNS with a limited number of laser shots in the presence of strong background noise. We addressed this by employing a time-gated 6Li\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$^{6}{\ extrm{Li}}$$\\end{document}-glass scintillation neutron detector to measure the transmission spectra, reducing the impact of electromagnetic noise and neutron and gamma-ray flashes. Output waveforms were recorded for each laser shot and analyzed offline using a counting method. This approach yielded a spectrum with distinct resonances, which were attributed to 115In\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$^{115}\\,{\ extrm{In}}$$\\end{document} and 109Ag\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$^{109}{\ extrm{Ag}}$$\\end{document}, as confirmed through neutron transmission simulation. The spectrum was analyzed using the least-square nuclear-resonance fitting program, REFIT, demonstrating the possibility of using an LDNS for nondestructive areal-density material characterization.

Analysis of neutron time-of-flight spectra with a Bayesian unfolding methodology

We have developed an innovative methodology for obtaining the neutron energy distribution from a time-of-flight (TOF) measurement based on the iterative Bayesian unfolding method and accurate Monte Carlo simulations. This methodology has been validated through the analysis of a realistic virtual β-decay experiment, including the most relevant systematic effects in a real experiment. The proposed methodology allowed for obtaining accurate results over the energy range above the neutron detection threshold.

Organic electronic-based neutron detectors

In recent decades organic electronics has entered the mainstream of consumer electronics, driven by innovations in scalability and low power applications, and low-cost fabrication methods. The potential for using organic semiconductor electronic devices as radiation detectors, and in particular for neutron detection is reported. We report results of laboratory tests using α particles as well as the response to thermal and fast neutrons covering the energy range 0.025 eV to 16.5 MeV. GEANT4 simulations are used to provide a detailed understanding of the performance and potential of this emerging technology for radiation detection.

Fabrication and Characterization of Ce3+-Doped Lithium Alumino-Silicate Scintillating Glass-Ceramic and Fiber.

Ce3+-doped lithium alumino-silicate (Li-Al-Si) scintillating glass was prepared using a melting method and crystallized via heat treatment. X-ray diffraction and transmission electron microscopy confirmed the presence of nanocrystals in the materials. Radioluminescence spectra, obtained by X-ray excitation, and luminescence spectra, obtained by 338 nm excitation, showed that the luminescence intensity increased after crystallization. The glass was combined with pure silica as the inner cladding to fabricate a hybrid fiber core using a melt-in-tube technique. The composition of the fiber core was examined using an electron probe microanalyzer. The glass fiber produced strong blue luminescence under UV excitation. After a micro-crystallizing heat treatment of the hybrid fiber at 850 °C in a reducing atmosphere, a Ce3+-doped lithium alumino-silicate glass-ceramic scintillating hybrid fiber was obtained. The nanocrystal structure of the fiber core was examined using micro-Raman spectroscopy. Excitation and luminescence spectra of the hybrid fiber before and after micro-crystallization were measured using microspectrofluorimetry. The results demonstrated that the fiber remained luminous after micro-crystallization. Hence, this work provides a new way to prepare scintillating glass-ceramic hybrid fibers for neutron detection.