Nepal Climate Observatory-Pyramid Research Articles

Biogenic particles formed in the Himalaya as an important source of free tropospheric aerosols

Aerosols of biogenic and anthropogenic origin affect the total radiative forcing of global climate. Poor knowledge of the pre-industrial aerosol concentration and composition, in particular of particles formed directly in the atmosphere from gaseous precursors, constitutes a large uncertainty in the anthropogenic radiative forcing. Investigations of new particle formation at pre-industrial-like conditions can contribute to the reduction of this uncertainty. Here we present observations taken at the remote Nepal Climate Observatory Pyramid station at 5,079 m above sea level, a few kilometres from the summit of Everest. We show that up-valley winds funnel gaseous aerosol precursors to higher altitudes. During this transport, these are oxidized into compounds of very low volatility, which rapidly form a large number of aerosol particles. These are then transported into the free troposphere, which suggests that the whole Himalayan region may act as an ‘aerosol factory’ and contribute substantially to the free tropospheric aerosol population. Aerosol production in this region occurs mainly via organic precursors of biogenic origin with little evidence of the involvement of anthropogenic pollutants. This process is therefore likely to be essentially unchanged since the pre-industrial period, and may have been one of the major sources that contributes to the upper tropospheric aerosol population during that time. Newly formed biogenic particles in the Himalaya increase free-tropospheric background aerosol concentration by a factor of up to two.

Black Carbon and Ozone Variability at the Kathmandu Valley and at the Southern Himalayas: A Comparison between a “Hot Spot” and a Downwind High-Altitude Site

Several studies have reported the transport of short-lived climate forcers/pollutants (SLCF/P) from the highly polluted areas in southern Asia (e.g., the Indo-Gangetic Plain and the Himalayan foothills) to the Himalayas, with significant implications for the global and regional climate, crop yields, and human health. In this work, we perform a comparison of nearly three years (February 2013–October 2015) of simultaneous black carbon (BC) and surface ozone (O3) measurements at two sites in Nepal, viz., Paknajol (1380 m a.s.l.), in the Kathmandu Valley, and the WMO/GAW global station Nepal Climate Observatory-Pyramid (NCO-P, 5079 m a.s.l.), near the base camp of Mt. Everest. The two sites are only 150 km apart and are characterized by different situations: While the Kathmandu Valley is one of the regional urban “hot spots” for concerns related to air pollution, NCO-P is representative of the background conditions of the high Himalayas and the free troposphere. Therefore, the possible role played by emissions occurring in the planetary boundary layer (PBL) of the Kathmandu Valley in influencing the variability in SLCF/P at NCO-P was investigated. BC and O3 concentrations at NCO-P showed a linear correlation with the modeled PBL height over the Kathmandu urban area, providing evidence that the anthropogenic emissions occurring within the Kathmandu PBL could affect the variability in BC and O3 at NCO-P. Furthermore, when introducing an additional constraint into the analysis (viz., back-trajectories), we show that on days when air mass transport between the two measurement sites was observed (10% of the period), at least 22% and 16% of BC and O3 variability at NCO-P can be explained by concurrent variability in SLCF/P over the Kathmandu Valley.

STEFLUX, a tool for investigating stratospheric intrusions: application to two WMO/GAW global stations

Abstract. Stratospheric intrusion (SI) events are a topic of ongoing research, especially because of their ability to change the oxidation capacity of the troposphere and their contribution to tropospheric ozone levels. In this work, a novel tool called STEFLUX (Stratosphere-to-Troposphere Exchange Flux) is presented, discussed, and used to provide a first long-term investigation of SI over two global hot-spot regions for climate change and air pollution: the southern Himalayas and the central Mediterranean Basin. The main purpose of STEFLUX is to obtain a fast-computing and reliable identification of the SI events occurring at a specific location and during a specified time window. It relies on a compiled stratosphere-to-troposphere exchange (STE) climatology, which makes use of the ERA-Interim reanalysis dataset from the ECMWF, as well as a refined version of a well-established Lagrangian methodology. STEFLUX results are compared to the SI observations (SIO) at two high-mountain WMO/GAW global stations in these climate hot spots, i.e., the Nepal Climate Observatory-Pyramid (NCO-P, 5079 m a.s.l.) and Mt. Cimone (2165 m a.s.l.), which are often affected by SI events. Compared to the observational datasets at the two specific measurement sites, STEFLUX is able to detect SI events on a regional scale. Furthermore, it has the advantage of retaining additional information concerning the pathway of stratospheric-affected air masses, such as the location of tropopause crossing and other meteorological parameters along the trajectories. However, STEFLUX neglects mixing and dilution that air masses undergo along their transport within the troposphere. Therefore, the regional-scale STEFLUX events cannot be expected to perfectly reproduce the point measurements at NCO-P and Mt. Cimone, which are also affected by small-scale (orographic) circulations. Still, the seasonal variability in SI events according to SIO and STEFLUX agrees fairly well. By exploiting the fact that the ERA-Interim reanalysis extends back to 1979, the long-term climatology of SI events at NCO-P and Mt. Cimone is also assessed in this work. The analysis of the 35-year record at both stations denies the existence of any significant trend in the SI frequency, except for winter seasons at NCO-P. Furthermore, for the first time, by using the STEFLUX outputs, we investigate the potential impact of specific climate factors (i.e. ENSO, QBO, and solar activity) on SI frequency variability over the Mediterranean Basin and the Himalayas.

High Concentrations of Ozone Air Pollution on Mount Everest: Health Implications for Sherpa Communities and Mountaineers.

Surface ozone measurements were collected during ascending transects in the Mount Everest region of Nepal with passive nitrite-coated Ogawa filter samplers to obtain 8-hour personal exposures (2860-5364 m asl). In addition, the Nepal Climate Observatory-Pyramid, a GAW-WMO Global Station sited in the Khumbu Valley (5079 m asl), collected ozone mixing ratios with photometric gas analyzer. Surface ozone measurements increased with altitude with concentrations that exceed 100 ppb (8-hour exposure). Highest values were during the spring season and the result of diverse contributions: hemispheric background values, the descent of ozone-rich stratospheric air, and the transport of tropospheric pollutants occurring at different spatial scales. Multiple climate factors, including descending stratospheric ozone and imported anthropogenic air masses from the Indo-Gangetic Plain, contribute to ambient ozone exposure levels in the vicinity of Mount Everest that are similar to if not higher than those reported in industrialized cities.

Transport of short-lived climate forcers/pollutants (SLCF/P) to the Himalayas during the South Asian summer monsoon onset

Over the course of six years (2006–2011), equivalent black carbon (eqBC), coarse aerosol mass (PM1–10), and surface ozone (O3), observed during the monsoon onset period at the Nepal Climate Observatory–Pyramid WMO/GAW Global Station (NCO-P, 5079 m a.s.l.), were analyzed to investigate events characterized by a significant increase in these short-lived climate forcers/pollutants (SLCF/P). These events occurred during periods characterized by low (or nearly absent) rain precipitation in the central Himalayas, and they appeared to be related to weakening stages (or ‘breaking’) of the South Asian summer monsoon system. As revealed by the combined analysis of atmospheric circulation, air-mass three-dimensional back trajectories, and satellite measurements of atmospheric aerosol loading, surface open fire, and tropospheric NOx, the large amount of SLCF/P reaching the NCO-P appeared to be related to natural (mineral dust) and anthropogenic emissions occurring within the PBL of central Pakistan (i.e., Thar Desert), the Northwestern Indo-Gangetic plain, and the Himalayan foothills. The systematic occurrence of these events appeared to represent the most important source of SLCF/P inputs into the central Himalayas during the summer monsoon onset period, with possible important implications for the regional climate and for hydrological cycles.

Synoptic-scale dust transport events in the southern Himalaya

Abstract The variability of long-range dust transport events observed in the southern Himalaya and its relation with source areas have been studied thanks to five years’ continuous measurements which were carried out at the “Nepal Climate Observatory-Pyramid” (NCO-P, 27°57′N, 86°48′E), the highest Northern Hemisphere GAW-WMO global station sited at 5079 m a.s.l. in the high Khumbu valley (Nepal) on the southern Himalaya. During the period March 2006–February 2011, the analyses of the aerosol particle concentrations and LAGRANTO three-dimensional backward trajectories indicated the occurrence of 275 days affected by synoptic-scale dust transport, which account for 22.2% of the investigated period. The frequency of dust transport days (DTDs) showed a clear seasonal cycle, with the highest seasonal value observed during pre-monsoon season (33.5% of the pre-monsoon’s days are DTDs). Large enhancements in coarse aerosol number concentration N 1–10 (average: +689%) and mass PM 1–10 (average: +1086%) were observed during the dust transport events as compared to the days without dust (dust-free days, DFDs). In addition, the single scattering albedo (SSA) also showed higher values, ranging from 0.87 to 0.90, during DTDs with respect to DFDs (0.80–0.87). The predominant source of mineral dust reaching the measurement site was identified in the arid regions of the north-western Indian subcontinent (Thar desert), which accounted for 41.6% of the trajectories points associated with DTDs. Seasonal analysis also indicated that the winter season was significantly influenced by far western desert regions, such as North Africa and the Arabic Peninsula.

Influence of open vegetation fires on black carbon and ozone variability in the southern Himalayas (NCO-P, 5079 m a.s.l.)

We analysed the variability of equivalent black carbon (BC) and ozone (O3) at the global WMO/GAW station Nepal Climate Observatory-Pyramid (NCO-P, 5079 m a.s.l.) in the southern Himalayas, for evaluating the possible contribution of open vegetation fires to the variability of these short-lived climate forcers/pollutants (SLCF/SLCP) in the Himalayan region.We found that 162 days (9% of the data-set) were characterised by acute pollution events with enhanced BC and O3 in respect to the climatological values. By using satellite observations (MODIS fire products and the USGS Land Use Cover Characterization) and air mass back-trajectories, we deduced that 56% of these events were likely to be affected by emissions from open fires along the Himalayas foothills, the Indian Subcontinent and the Northern Indo-Gangetic Plain.These results suggest that open fire emissions are likely to play an important role in modulating seasonal and inter-annual BC and O3 variability over south Himalayas.

Black carbon aerosols over the Himalayas: direct and surface albedo forcing

Absorbing aerosols such as black carbon (BC) or dust over high-altitude Himalayan regions have potential implications on the regional climate and hydrological cycle over South Asia. Making use of extensive measurements of atmospheric BC from several Himalayan stations, an assessment of radiative forcing due to direct and snow-albedo darkening is examined. Generally, BC concentration in the atmosphere peaks during pre-monsoon season over the Himalayas and the climatological mean of atmospheric BC over Hanle (western Himalayas, 4.5 km msl) and Nepal Climate Observatory-Pyramid (central Himalayas, 5 km msl) are 106±27 ng m−3 and 190±95 ng m−3, respectively. Based on the optical and physical properties of composite aerosols measured at Hanle, clear sky direct radiative forcing (DRF) at the top of the atmosphere is estimated as 1.69 W m−2 over snow surface and −1.54 W m−2 over sandy surface during pre-monsoon season. The estimated amount of BC in the snow varied from 117 to 1.7 µg kg−1 for wide range of dry deposition velocities (0.01–0.054 cm s−1) of BC, snow depth (2–10 cm) and snow densities (195–512 kg m−3). Using a size-resolved wet scavenging parametrisation, the amount of BC on snow due to wet scavenging is estimated as 29 µg kg−1 for an accumulated snow depth of 27 cm. For the range of 10–200 µg kg−1 of BC in snow, the diurnally averaged forcing due to snow darkening has been found to vary from 0.87 to 10.2 W m−2 for fresh snow and from 2.6 to 28.1 W m−2 for the aged snow, which is significantly higher than the DRF. The direct and surface albedo radiative forcing could lead to significant warming over the Himalayas during pre-monsoon.

Transport of Stratospheric Air Masses to the Nepal Climate Observatory–Pyramid (Himalaya; 5079 m MSL): A Synoptic-Scale Investigation

AbstractThis work analyzes and classifies stratospheric airmass transport events (ST) detected at the Nepal Climate Observatory–Pyramid (NCO-P; 27°57′N, 86°48′E, 5079 m MSL) Global Atmospheric Watch–World Meteorological Organization station from March 2006 to February 2008. For this purpose, in situ ozone (O3), meteorological parameters (atmospheric pressure and relative humidity), and black carbon (BC) are analyzed. The paper describes the synoptic-scale meteorological scenarios that are able to favor the development of ST over the southern Himalaya, by analyzing the meteorological fields provided by the ECMWF model (geopotential height, wind speed, and potential vorticity), satellite Ozone Monitoring Instrument data (total column ozone), and three-dimensional back trajectories calculated with the Lagrangian Analysis Tool (LAGRANTO) model. The study, which represents the first “continuous” classification of ST in the southern Himalaya, permitted classification of 94% of ST days within four synoptic-scale scenarios: stratospheric potential vorticity structures (PVS), subtropical jet stream (SJS), quasi-stationary ridges (QSR), and monsoon depressions (MD). SJS and PVS were the most frequent scenarios (48% and 30% of occurrences, respectively), QSR occurred for 12% of the ST days, and MD were detected only during the monsoon season (3%). SJS and PVS scenarios presented a peak frequency during the nonmonsoon seasons, when the jet stream and westerly disturbances influence atmospheric circulation over the southern Himalaya. During the identified ST, significant variations of O3 (+24%) and BC (−56%) were recorded relative to the averaged 2-yr mean values. On average, PVS and SJS were the most effective synoptic-scale scenarios in modifying the O3 and BC levels at NCO-P from postmonsoon to premonsoon seasons, and ST is one of the leading processes in defining the “background” BC variability at NCO-P.

Seasonal variations of aerosol size distributions based on long-term measurements at the high altitude Himalayan site of Nepal Climate Observatory-Pyramid (5079 m), Nepal

Abstract. The present paper investigates the diurnal and seasonal variability of the aerosol total number concentration, number and volume size distribution between 10 nm and 10 μm, from a combination of a scanning mobility particle sizer (SMPS) and an optical counter (OPC), performed over a two-year period (January 2006–February 2008) at the Nepal Climate Observatory-Pyramid (NCO-P) research station, (5079 m a.s.l.). The annual average number concentration measured over the two-year period at the NCO-P is 860 cm−3. Total concentrations show a strong seasonality with maxima during pre-monsoon and post-monsoon seasons and minima during the dry and monsoon seasons. A diurnal variation is also clearly observed, with maxima between 09:00 and 12:00 UTC. The aerosol concentration maxima are mainly due to nucleation processes during the post-monsoon season, as witnessed by high nucleation mode integrated number concentrations, and to transport of high levels of pollution from the plains by valley breezes during the pre-monsoon season, as demonstrated by high accumulation mode integrated number concentrations. Night-time number concentration of particles (from 03:00 to 08:00 NST) are relatively low throughout the year (from 450 cm−3 during the monsoon season to 675 cm−3 during the pre-monsoon season), indicating the of high altitudes background level, as a result of downslope winds during this part of the day. However, it was found that these background concentrations are strongly influenced by the daytime concentrations, as they show the same seasonal variability. If nighttime concentrations were presumed to be representative of free troposphere (FT)/residual layer concentrations, they would be found to be two times higher than at other lower altitudes European sites, such as the Jungfraujoch. However, BL intrusions might contaminate the free troposphere/residual layer even at this altitude, especially during regional air masses influence. Night-time measurements were subsequently selected to study the FT composition according to different air masses, and the effect of long range transport to the station.

Aerosol mass and black carbon concentrations, a two year record at NCO-P (5079 m, Southern Himalayas)

Abstract. Aerosol mass and the absorbing fraction are important variables, needed to constrain the role of atmospheric particles in the Earth radiation budget, both directly and indirectly through CCN activation. In particular, their monitoring in remote areas and mountain sites is essential for determining source regions, elucidating the mechanisms of long range transport of anthropogenic pollutants, and validating regional and global models. Since March 2006, aerosol mass and black carbon concentration have been monitored at the Nepal Climate Observatory-Pyramid, a permanent high-altitude research station located in the Khumbu valley at 5079 m a.s.l. below Mt. Everest. The first two-year averages of PM1 and PM1−10 mass were 1.94 μg m−3 and 1.88 μg m−3, with standard deviations of 3.90 μg m−3 and 4.45 μg m−3, respectively, while the black carbon concentration average is 160.5 ng m−3, with a standard deviation of 296.1 ng m−3. Both aerosol mass and black carbon show well defined annual cycles, with a maximum during the pre-monsoon season and a minimum during the monsoon. They also display a typical diurnal cycle during all the seasons, with the lowest particle concentration recorded during the night, and a considerable increase during the afternoon, revealing the major role played by thermal winds in influencing the behaviour of atmospheric compounds over the high Himalayas. The aerosol concentration is subject to high variability: in fact, as well as frequent "background conditions" (55% of the time) when BC concentrations are mainly below 100 ng m−3, concentrations up to 5 μg m−3 are reached during some episodes (a few days every year) in the pre-monsoon seasons. The variability of PM and BC is the result of both short-term changes due to thermal wind development in the valley, and long-range transport/synoptic circulation. At NCO-P, higher concentrations of PM1 and BC are mostly associated with regional circulation and westerly air masses from the Middle East, while the strongest contributions of mineral dust arrive from the Middle East and regional circulation, with a special contribution from North Africa and South-West Arabian Peninsula in post-monsoon and winter season.

Atmospheric Brown Clouds in the Himalayas: first two years of continuous observations at the Nepal Climate Observatory-Pyramid (5079 m)

Abstract. This paper provides a detailed description of the atmospheric conditions characterizing the high Himalayas, thanks to continuous observations begun in March 2006 at the Nepal Climate Observatory-Pyramid (NCO-P) located at 5079 m a.s.l. on the southern foothills of Mt. Everest, in the framework of ABC-UNEP and SHARE-Ev-K2-CNR projects. The work presents a characterization of meteorological conditions and air-mass circulation at NCO-P during the first two years of activity. The mean values of atmospheric pressure, temperature and wind speed recorded at the site were: 551 hPa, −3.0 °C, 4.7 m s−1, respectively. The highest seasonal values of temperature (1.7 °C) and relative humidity (94%) were registered during the monsoon season, which was also characterized by thick clouds, present in about 80% of the afternoon hours, and by a frequency of cloud-free sky of less than 10%. The lowest temperature and relative humidity seasonal values were registered during winter, −6.3 °C and 22%, respectively, the season being characterised by mainly cloud-free sky conditions and rare thick clouds. The summer monsoon influenced rain precipitation (seasonal mean: 237 mm), while wind was dominated by flows from the bottom of the valley (S–SW) and upper mountain (N–NE). The atmospheric composition at NCO-P has been studied thanks to measurements of black carbon (BC), aerosol scattering coefficient, PM1, coarse particles and ozone. The annual behaviour of the measured parameters shows the highest seasonal values during the pre-monsoon (BC: 316.9 ng m−3, PM1: 3.9 μg m−3, scattering coefficient: 11.9 Mm−1, coarse particles: 0.37 cm−3 and O3: 60.9 ppbv), while the lowest concentrations occurred during the monsoon (BC: 49.6 ng m−3, PM1: 0.6 μg m−3, scattering coefficient: 2.2 Mm−1, and O3: 38.9 ppbv) and, for coarse particles, during the post-monsoon (0.07 cm−3. At NCO-P, the synoptic-scale circulation regimes present three principal contributions: Westerly, South-Westerly and Regional, as shown by the analysis of in-situ meteorological parameters and 5-day LAGRANTO back-trajectories. The influence of the brown cloud (AOD>0.4) extending over Indo–Gangetic Plains up to the Himalayan foothills has been evaluated by analysing the in-situ concentrations of the ABC constituents. This analysis revealed that brown cloud hot spots mainly influence the South Himalayas during the pre-monsoon, in the presence of very high levels of atmospheric compounds (BC: 1974.1 ng m−3, PM1: 23.5 μg m−3, scattering coefficient: 57.7 Mm−1, coarse particles: 0.64 cm−3, O3: 69.2 ppbv, respectively). During this season 20% of the days were characterised by a strong brown cloud influence during the afternoon, leading to a 5-fold increased in the BC and PM1 values, in comparison with seasonal means. Our investigations provide clear evidence that, especially during the pre-monsoon, the southern side of the high Himalayan valleys represent a "direct channel" able to transport brown cloud pollutants up to 5000 m a.s.l., where the pristine atmospheric composition can be strongly influenced.

Estimated impact of black carbon deposition during pre-monsoon season from Nepal Climate Observatory – Pyramid data and snow albedo changes over Himalayan glaciers

Abstract. The possible minimal range of reduction in snow surface albedo due to dry deposition of black carbon (BC) in the pre-monsoon period (March–May) was estimated as a lower bound together with the estimation of its accuracy, based on atmospheric observations at the Nepal Climate Observatory – Pyramid (NCO-P) sited at 5079 m a.s.l. in the Himalayan region. A total BC deposition rate was estimated as 2.89 μg m−2 day−1 providing a total deposition of 266 μg m−2 for March–May at the site, based on a calculation with a minimal deposition velocity of 1.0×10−4 m s−1 with atmospheric data of equivalent BC concentration. Main BC size at NCO-P site was determined as 103.1–669.8 nm by correlation analyses between equivalent BC concentration and particulate size distributions in the atmosphere. The BC deposition from the size distribution data was also estimated. It was found that 8.7% of the estimated dry deposition corresponds to the estimated BC deposition from equivalent BC concentration data. If all the BC is deposited uniformly on the top 2-cm pure snow, the corresponding BC concentration is 26.0–68.2 μg kg−1, assuming snow density variations of 195–512 kg m−3 of Yala Glacier close to NCO-P site. Such a concentration of BC in snow could result in 2.0–5.2% albedo reductions. By assuming these albedo reductions continue throughout the year, and then applying simple numerical experiments with a glacier mass balance model, we estimated reductions would lead to runoff increases of 70–204 mm of water. This runoff is the equivalent of 11.6–33.9% of the annual discharge of a typical Tibetan glacier. Our estimates of BC concentration in snow surface for pre-monsoon season is comparable to those at similar altitudes in the Himalayan region, where glaciers and perpetual snow regions begin, in the vicinity of NCO-P. Our estimates from only BC are likely to represent a lower bound for snow albedo reductions, because we used a fixed slower deposition velocity. In addition, we excluded the effects of atmospheric wind and turbulence, snow aging, dust deposition, and snow albedo feedbacks. This preliminary study represents the first investigation of BC deposition and related albedo on snow, using atmospheric aerosol data observed at the southern slope in the Himalayas.

Tropospheric ozone variations at the Nepal Climate Observatory-Pyramid (Himalayas, 5079 m a.s.l.) and influence of deep stratospheric intrusion events

Abstract. The paper presents the first 2 years of continuous surface ozone (O3) observations and systematic assessment of the influence of stratospheric intrusions (SI) at the Nepal Climate Observatory at Pyramid (NCO-P; 27°57' N, 86°48' E), located in the southern Himalayas at 5079 m a.s.l.. Continuous O3 monitoring has been carried out at this GAW-WMO station in the framework of the Ev-K2-CNR SHARE and UNEP ABC projects since March 2006. Over the period March 2006–February 2008, an average O3 value of 49±12 ppbv (±1δ) was recorded, with a large annual cycle characterized by a maximum during the pre-monsoon (61±9 ppbv) and a minimum during the monsoon (39±10 ppbv). In general, the average O3 diurnal cycles had different shapes in the different seasons, suggesting an important interaction between the synoptic-scale circulation and the local mountain wind regime. Short-term O3 behaviour in the middle/lower troposphere (e.g. at the altitude level of NCO-P) can be significantly affected by deep SI which, representing one of the most important natural input for tropospheric O3, can also influence the regional atmosphere radiative forcing. To identify days possibly influenced by SI at the NCO-P, a specially designed statistical methodology was applied to the time series of observed and modelled stratospheric tracers. On this basis, during the 2-year investigation, 14.1% of analysed days were found to be affected by SI. The SI frequency showed a clear seasonal cycle, with minimum during the summer monsoon (1.2%) and higher values during the rest of the year (21.5%). As suggested by back-trajectory analysis, the position of the subtropical jet stream could play an important role in determining the occurrence of deep SI transport on the southern Himalayas. We estimated the fraction of O3 due to SI at the NCO-P. This analysis led to the conclusion that during SI O3 significantly increased by 27.1% (+13 ppbv) with respect to periods not affected by such events. Moreover, the integral contribution of SI (O3S) to O3 at the NCO-P was also calculated, showing that up to 13.7% of O3 recorded at the measurement site could be possibly attributed to SI. On a seasonal basis, the lowest SI contributions were found during the summer monsoon (less than 0.1%), while the highest were found during the winter period (up to 24.2%). Even considering the rather large uncertainty associated with these estimates, the obtained results indicated that, during non-monsoon periods, high O3 levels could affect NCO-P during SI, thus influencing the variability of tropospheric O3 over the southern Himalayas.

Aerosol optical properties and radiative forcing in the high Himalaya based on measurements at the Nepal Climate Observatory-Pyramid site (5079 m a.s.l.)

Abstract. Intense anthropogenic emissions over the Indian sub-continent lead to the formation of layers of particulate pollution that can be transported to the high altitude regions of the Himalaya-Hindu-Kush (HKH). Aerosol particles contain a substantial fraction of strongly absorbing material, including black carbon (BC), organic compounds (OC), and dust all of which can contribute to atmospheric warming, in addition to greenhouse gases. Using a 3-year record of continuous measurements of aerosol optical properties, we present a time series of key climate relevant aerosol properties including the aerosol absorption (σap) and scattering (σsp) coefficients as well as the single-scattering albedo (w0). Results of this investigation show substantial seasonal variability of these properties, with long range transport during the pre- and post-monsoon seasons and efficient precipitation scavenging of aerosol particles during the monsoon season. The monthly averaged scattering coefficients range from 0.1 Mm−1 (monsoon) to 20 Mm−1 while the average absorption coefficients range from 0.5 Mm−1 to 3.5 Mm−1. Both have their maximum values during the pre-monsoon period (April) and reach a minimum during Monsoon (July–August). This leads to dry w0 values from 0.86 (pre-monsoon) to 0.79 (monsoon) seasons. Significant diurnal variability due to valley wind circulation is also reported. Using aerosol optical depth (AOD) measurements, we calculated the resulting direct local radiative forcing due to aerosols for selected air mass cases. We found that the presence of absorbing particulate material can locally induce an additional top of the atmosphere (TOA) forcing of 10 to 20 W m−2 for the first atmospheric layer (500 m above surface). The TOA positive forcing depends on the presence of snow at the surface, and takes place preferentially during episodes of regional pollution occurring on a very regular basis in the Himalayan valleys. Warming of the first atmospheric layer is paralleled by a substantial decrease of the amount of radiation reaching the surface. The surface forcing is estimated to range from −4 to −20 W m−2 for small-scale regional pollution events and large-scale pollution events, respectively. The calculated surface forcing is also very dependent on surface albedo, with maximum values occurring over a snow-covered surface. Overall, this work presents the first estimates of aerosol direct radiative forcing over the high Himalaya based on in-situ aerosol measurements, and results suggest a TOA forcing significantly greater than the IPCC reported values for green house gases.

Chemical composition of PM<sub>10</sub> and PM<sub>1</sub> at the high-altitude Himalayan station Nepal Climate Observatory-Pyramid (NCO-P) (5079 m a.s.l.)

Abstract. We report chemical composition data for PM10 and PM1 from the Nepal Climate Observatory-Pyramid (NCO-P), the world's highest aerosol observatory, located at 5079 m a.s.l. at the foothills of Mt. Everest. Despite its high altitude, the average PM10 mass apportioned by the chemical analyses is of the order of 6 μg m−3 (i.e., 10 μg/scm), with almost a half of this mass accounted for by organic matter, elemental carbon (EC) and inorganic ions, the rest being mineral dust. Organic matter, in particular, accounted for by 2.0 μg m−3 (i.e., 3.6 μg/scm) on a yearly basis, and it is by far the major PM10 component beside mineral oxides. Non-negligible concentrations of EC were also observed (0.36 μg/scm), confirming that light-absorbing aerosol produced from combustion sources can be efficiently transported up the altitudes of Himalayan glaciers. The concentrations of carbonaceous and ionic aerosols follow a common time trend with a maximum in the premonsoon season, a minimum during the monsoon and a slow recovery during the postmonsoon and dry seasons, which is the same phenomenology observed for other Nepalese Himalayan sites in previous studies. Such seasonal cycle can be explained by the seasonal variations of dry and moist convection and of wet scavenging processes characterizing the climate of north Indian subcontinent. We document the effect of orographic transport of carbonaceous and sulphate particles upslope the Himalayas, showing that the valley breeze circulation, which is almost permanently active during the out-of-monsoon season, greatly impacts the chemical composition of PM10 and PM1 in the high Himalayas and provides an efficient mechanism for bringing anthropogenic aerosols into the Asian upper troposphere (>5000 m a.s.l.). The concentrations of mineral dust are impacted to a smaller extent by valley breezes and follow a unique seasonal cycle which suggest multiple source areas in central and south-west Asia. Our findings, based on two years of observations of the aerosol chemical composition, provide clear evidence that the southern side of the high Himalayas is impacted by transport of anthropogenic aerosols which constitute the Asian brown cloud.

The ABC-Pyramid Atmospheric Research Observatory in Himalaya for aerosol, ozone and halocarbon measurements

In this work we present the new ABC-Pyramid Atmospheric Research Observatory (Nepal, 27.95 N, 86.82 E) located in the Himalayas, specifically in the Khumbu valley at 5079 m a.s.l. This measurement station has been set-up with the aim of investigating natural and human-induced environmental changes at different scales (local, regional and global). After an accurate instrumental set-up at ISAC-CNR in Bologna (Italy) in autumn 2005, the ABC-Pyramid Observatory for aerosol (physical, chemical and optical properties) and trace gas measurements (ozone and climate altering halocarbons) was installed in the high Khumbu valley in February 2006. Since March 2006, continuous measurements of aerosol particles (optical and physical properties), ozone (O 3) and meteorological parameters as well as weekly samplings of particulate matter (for chemical analyses) and grab air samples for the determination of 27 halocarbons, have been carried out. These measurements provide data on the typical atmospheric composition of the Himalayan area between India and China and make investigations of the principal differences and similarities between the monsoon and pre-monsoon seasons possible. The study is carried out within the framework of the Ev-K 2-CNR “SHARE-Asia” (Stations at High Altitude for Research on the Environment in Asia) and UNEP—“ABC” (Atmospheric Brown Clouds) projects. With the name of “Nepal Climate Observatory—Pyramid” the station is now part of the Observatory program of the ABC project.