Negative Discharge Research Articles

Observational Evidence of Negative Leader Reactivation Processes Following a Negative Return Stroke in Lightning Discharges

AbstractHigh‐time‐resolved mapping results of two rare reactivation processes following a negative return stroke are discovered and analyzed. At first, the discharges prior to the reactivation process were dominated by positive discharges lasting for tens of milliseconds in a limited space in the vicinity of a decayed negative leader channel. The positive discharges produced no detectable electric field change. Then, negative discharges started and propagated along the decayed downward negative leader channels at a speed exceeding 106 m/s for a few microseconds and produced negative electric field changes. The analysis reveals that the processes are physically distinct from recoil leaders and side discharges in terms of propagation behaviors, electromagnetic characteristics, and time scale. The possible mechanisms of the processes are discussed. The observation suggests that the reactivation processes of the negative leaders may lead to subsequent return strokes.

Initiation of Downward Positive Leader Beneath the Negative Leader Channel

AbstractDue to the weak radiation generated by positive leaders, our understanding of how positive leaders are initiated and reach the ground remains limited. This study investigated positive cloud‐to‐ground (CG) lightning induced after the long intracloud lightning based on high‐speed video and fast antenna mapping results. Below the cloud base in the field of view, re‐breakdowns of decayed negative branches occurred consecutively beneath the horizontal negative channel in the form of bidirectional leaders. These bidirectional leaders advanced along the same channel, and eventually, the third reached the ground, generating a positive return stroke (RS) with a peak current of 157 kA. Following the RS, new negative discharges emerge adjacent to the vertical return stroke channel, persisting and propagating to form a continuing current (CC) lasting over 200 milliseconds.

Application End Evaluation of Electrostatic Precipitation for Control PM and NOx Emissions from Small-Scale Combustions

Electrostatic precipitators (ESPs) have shown promise in reducing particulate matter (PM) emissions, but their potential for simultaneous NOx reduction in small-scale combustion systems remains underexplored. This study focuses on using non-thermal plasma generated in a corona discharge to reduce PM and NOx emissions from small-scale combustion. ESP was specifically designed for a commercially available 15 kW boiler with wood pellet combustion and used with both positive and negative discharge polarity to control emissions without any chemical additives. ESP performance was evaluated across a range of specific input energies (SIE) in terms of particle mass and number concentrations and NOx concentrations obtained by continuous gas analysis. ESP ensured the reduction in PM concentrations from 48 mg/m3 to the magnitude of PM content in the ambient air. The highest precipitation efficiency was observed for particles in the 20–200 nm range. Concurrently, NOx emissions were reduced by up to 78%, from 178 mg/m3 to 39 mg/m3. These results were achieved at specific input energies of 36 for positive and 48 J/L for negative corona, which is significantly lower than those reported for many existing separate PM and NOx control systems. This study demonstrates the potential of ESPs as a compact, energy-efficient solution for simultaneous PM and NOx removal in small-scale combustion systems, offering promising implications for improving air pollution control technologies for small-scale combustion systems.

Effect of the negative-end discharge on the positive leader propagation in bidirectional leader discharges

Lightning strikes on aircraft are mainly due to self-triggered bidirectional leader discharges. Understanding the physical processes of lightning strikes is the basis for designing appropriate lightning protection measures. For this purpose, the development processes of bidirectional leaders triggered by a floating conductor were studied in a laboratory. In this paper, an experimental platform for the observation of bidirectional leader discharges is established through a reasonable gap arrangement. The discharge processes were recorded by a high-speed camera with up to 504 000 f/s. The effects of negative streamer discharges on the positive leader propagation speed as well as brightness during the bidirectional leader discharge at different electric field rise rates were mainly studied and quantitatively analyzed by introducing incremental coefficients. The experimental results show that the discharge development at the negative end of the floating conductor lags behind that at the positive end, and there is a coupling phenomenon between the positive and the negative discharge. At low electric field rise rates, when a negative streamer discharge occurs, it causes a positive corona burst, resulting in a sharp increase in brightness, while on the contrary the leader speed change is not as pronounced as the brightness change. As the rate of rise of the electric field increases, the effect of the discharge at the negative end on the positive end gradually decreases. This work could provide a theoretical basis for understanding the physical process of lightning strikes on aircraft.

The propagation of negative pulsed discharges facilitated by artificially injected gas bubble in water

Abstract The artificial injection of bubbles into the electrode gap can effectively enhance the performance of underwater pulsed spark discharge (UPSD). It is crucial to investigate the morphology and propagation characteristics of discharges for a comprehensive understanding of bubble-stimulated UPSD. This paper presented an extensive study of negative discharges facilitated by the injected large bubble (with a diameter of 3 mm) in UPSD. The bridging effect of the bubble and the morphology and propagation of discharges were observed through the shadowgraph images captured by a high-speed camera. A numerical model was built to analyse the influence of the bubble on the initial electric field distribution between the electrodes. The characteristics of discharges were notably influenced by bubble parameters and energization conditions. Not in all cases could the bubble play the bridging effect role. The effective range of the bubble was roughly confined to a small region near the HV electrode tip. The experimental results obtained in this paper have certain guiding significance for the practical application of UPSD.

Pedestal properties of negative triangularity discharges in ASDEX Upgrade

Abstract In this work, we explore the pedestal properties of negative triangularity discharges with upper triangularity of δ u ≈ − 0.35 and with both ion ∇ B drift directions. In all cases, the discharges undergo a transition to H-mode with accompanying edge-localized modes (ELMs) that are not explained by the peeling-ballooning stability analysis alone. A variation in the ion ∇ B drift direction is observed. A lower pressure gradient, shallower radial electric field well and increased temperature fluctuations are measured in the favorable case. In addition, irregular ELMs are present. This difference is more pronounced in electron cyclotron resonance heating (ECRH) plasmas compared to plasmas with combined neutral beam injection and ECRH. A comparative analysis between two discharges, featuring similar plasma parameters but varied shaping, suggests that an interplay between other parameters, such as magnetic shear, the timing of the auxiliary heating and shaping, might play a strong role in low- to high-confinement transitions. While the low shaping discharge maintained L-mode, the high shaping discharge entered H-mode with ELMs, contrary to expectations.

Contribution of Metastable Oxygen Spectra to Fluctuated Waveform Tails after Breakdown Time in Air under Positive and Negative Impulse Voltages

In this study, we explored the correlation between fluctuated waveform tails under both positive and negative impulse voltages and their corresponding spectral lines during millisecond observations of arc discharge. We examined impulse voltages in ±100, ±125, and ±150 kV across 3, 3.5, and 4 cm gaps using spectroscopic analysis focused on oxygen excitations. Six selected spectra in ±100, ±125, and ±150 kV at 3.5 cm and two negative spectra of −100 kV at 3 and 4 cm were analyzed by identifying spectral lines in the wavelength range of 200–900 nm. The results revealed a correlation between the fluctuated waveform tails and spectral lines in positive voltage discharges, which were almost similar, while in negative voltage discharges, this correlation was found only in −100 kV at 3 and 4 cm. We concluded that during the spark phase for both positive and negative voltage discharges, symmetrical fluctuation in the waveform tails was observed after breakdown time, especially above the voltage level of the recombination phase. This suggested the presence of energetic oxygen excited states in the 200–400 nm range, with higher peak intensity than the O I line at 777.417 nm, observed in most positive impulse voltage discharges and at −100 kV with 3 and 4 cm gaps, contributing to rapid breakdown.

Advancing spectroscopic understanding of HOCS+: Laboratory investigations and astronomical implications

Sulphur-bearing species play crucial roles in interstellar chemistry, yet their precise characterisation remains challenging. Here, we present laboratory experiments aimed at extending the high-resolution spectroscopy of protonated carbonyl sulphide (HOCS+), a recently detected molecular ion in space. Using a frequency-modulated free-space absorption spectrometer, we detected rotational transitions of HOCS+ in an extended negative glow discharge with a mixture of H2 and OCS, extending the high-resolution rotational characterisation of the cation well into the millimetre wave region (200–370 GHz). Comparisons with prior measurements and quantum chemical calculations revealed an overall agreement in the spectroscopic parameters. With the new spectroscopic dataset in hand, we re-investigated the observations of HOCS+ towards G+0.693−0.027, which were initially based solely on Ka = 0 lines contaminated by HNC34S. This re-investigation enabled the detection of weak Ka ≠ 0 transitions, free from HNC34S contamination. Our high-resolution spectroscopic characterisation also provides valuable insights for future millimetre and submillimetre astronomical observations of these species in different interstellar environments. In particular, the new high-resolution catalogue will facilitate the search for this cation in cold dark clouds, where very narrow line widths are typically observed.

Mitigation of PBDE net discharge in hazardous waste thermal treatment system through reintroducion of sludge and fly ash into GASMILD operations

The presence of polybrominated diphenyl ethers (PBDEs) in consumer products, waste treatment processes, and treated ashes poses a significant environmental threat. Due to the lack of research on the removal of PBDEs during waste incineration, this study investigated the effectiveness of a Hazardous Waste Thermal Treatment System (HAWTTS) utilizing reburning of sludge and fly ash (SFA) with gasification-moderate or intense low-oxygen dilution (GASMILD) combustion for PBDE removal. The closed-loop treatment of sludge and ash within the HAWTTS provides a potential pathway for near-zero PBDE emissions. The GASMILD combustion addresses potential combustion issues associated with fly ash recirculation. The system achieved an impressive overall removal efficiency of 98.4% for PBDEs, with minimal stack emissions (2.45 ng/Nm³) and a negative net discharge rate (−1.02 μg/h). GASMILD combustion played a crucial role (92.7%–97.6% destruction) in addressing challenges associated with high-moisture feedstocks and SFA residues. Debromination of highly brominated PBDEs occurred within the incinerator, resulting in an increased proportion of lower brominated PBDEs in the bottom slag compared to the feedstock. Air Pollution Control Devices (APCDs) achieved a total PBDE removal efficiency of 74.4%. However, the hydrophobic nature of PBDEs limited removal efficiency in scrubbers (36.0%) and cyclonic demisters (37.86%). This study demonstrates that reintroducing SFA into the GASMILD combustion process offers an effective and environmentally sustainable strategy for reducing net PBDE levels in hazardous waste. This approach also provides additional benefits such as energy conservation, reduced carbon emissions, and lower operating costs associated with secondary treatment of thermally treated byproducts.

Numerical Simulation of Multibranching Positive and Negative Streamer Discharges Near the Oil-Paper Interface in Dielectric Liquid During Pulsed Voltage

Numerical Simulation of Multibranching Positive and Negative Streamer Discharges Near the Oil-Paper Interface in Dielectric Liquid During Pulsed Voltage

Evolution of the Leader Discharge in Bi‐Directional Propagation System in Altitude‐Triggered Lightning

AbstractOn 18 June 2023, comprehensive observations were conducted to an altitude‐triggered lightning flash. Upward positive leader (UPL) and downward negative leader (DNL) in a bi‐directional development system were detected simultaneously by a high‐speed camera, together with the coordinated measurements of magnetic field and very‐high‐frequency (VHF) emissions. High‐speed images reveal, for the first time, the enhancement of the UPL's propagation speed by DNL in the bi‐directional leader system. Concretely, the upward positive leader initially originates from a suspended wire tip and propagates at a two dimensional (2D) speed of 5.32 × 104 m/s, and after about 6.3 ms, its propagation speed was enhanced to 1.12 × 105 m/s when the stepped DNL started advancing at an average speed of 1.44 × 105 m/s. Additionally, based on the evolution of channel luminosity and the variations of magnetic radiation, it is found that there is a consistency in luminosity variation between the ascending channel and the descending channel in the bi‐directional leader system, and the amplitude of the magnetic field increases when the negative discharges start at the bottom wire end with intensive VHF emissions. Those facts indicate that the DNL has an effect, may be a positive one, on the UPL's development in the early stage of altitude‐triggered lightning.

Positive- and Negative-Polarity Nanosecond-Pulsed Cryogenic Plasma in Liquid Argon

This work reports on observations of positive and negative nanosecond-pulsed discharge in liquid argon. The structures of both positive and negative discharges, their sizes, and the propagation velocities exhibit remarkable similarity. Similar to the streamers in liquid nitrogen and gases, negative streamers require higher applied voltages (electric fields) and propagate to shorter distances. For both polarities, the spectra are almost identical and appear to be a superposition of strongly broadened atomic lines, with preliminary analysis of broadening indicating densities of about 40% that of liquid.

Аномальный грозовой процесс на территории Ростовской области

The work examines the anomalous thunderstorm process that occurred on the territory of the Rostov region on June 27, 2023. This thunderstorm process was observed in other regions of the North Caucasus, but the greatest intensity of thunderstorm activity was observed in the territory of the Rostov region, where the thunderstorm lasted more than a day. The analysis of thunderstorm activity was carried out using data from the lightning direction network of the Federal State Budgetary Institution "High Mountain Geophysical Institute". During the day, about 60,000 lightning strikes were recorded in this territory, of which 7,635 were ground strikes. Of the registered 7635 ground-based lightning discharges in the Rostov region, negative lightning amounted to 6625, and positive lightning – 1010. The share of negative lightning discharges from the total number of ground-based lightning discharges in the specified territory was 87 %. The largest number of negative lightning (more than 70 %) had values up to 20 kA. More than 50 % of positive lightning discharges had values from 21 to 40 kA. The average value of the negative polarity currents was -19.19 kA, and the positive polarity was +39.7 kA. Such a large-scale thunderstorm process is a consequence of regional climate change. When carrying out lightning protection measures for facilities in the Rostov region, it is recommended to take into account abnormal values of thunderstorm activity.

Subnanosecond Electromagnetic Pulse Generated by a Long Spark Discharge: Lightning Implication

AbstractThe effects of generating pulsed radiation by a long spark discharge are important for the development of lightning models and applications related to lightning protection. In experiments with a Marx generator simulating a lightning discharge, we detected the radiation in the form of a single ultrawideband electromagnetic pulse (UWB EMP) about 200 ps in duration, and rising time about 100 ps. UWB EMP generation occurs during the breakdown of a “rod–rod” 4 m long gap. Pulses of almost unipolar shape are observed in more than half of all positive discharges. EMP emission occurs before the main stage, and corresponds to the start of the upward leader from a grounded electrode. In negative discharges, pulses are also observed, but less frequently and with a smaller amplitude. The UWB EMPs, given their large amplitude (more than 100 V/m at a distance of 90 m from the discharge), can be considered as possible new lightning damage factors.

Experiments and modelling of negative triangularity ASDEX Upgrade plasmas in view of DTT scenarios

The paper presents experimental and modelling results of a comparison of negative (NT) and positive (PT) triangularity ASDEX Upgrade (AUG) discharges using the plasma shapes presently foreseen in the DTT tokamak, under construction in Italy. This work is part of a broader effort of investigation to understand whether the good properties observed in NT scenarios in DIII-D and TCV may be extrapolated to the DTT device and more generally to DEMO future operations. The experimental results have shown a practical gain of running these AUG plasmas with only ECRH and mixed NBI+ECRH phases in negative triangularity, even if they access the H-mode. Indeed, the NT electron kinetic profiles recover in all cases the PT electron pressures inside mid-radius due to reduced transport in the region ρtor=0.7−0.9 , while exhibiting lower individual ELM (Edge Localised Mode) energy losses. The ion pressure and expected fusion performance are comparable in the case of similar densities. Integrated modelling has been performed using the transport solver ASTRA and the quasi-linear turbulent model TGLF, investigating the transport properties of these discharges. The modelling reproduces the experiments qualitatively with reasonable accuracy. Nonetheless, the heat transport in NT cases is partially overestimated. This may be because TGLF uses the Miller equilibrium, which approximates the magnetic flux surfaces as up-down symmetric. In the caseof these asymmetric NT shapes, the simulated outer surfaces lose part of the tilt with respect to the z-axis, reducing the upper δ < 0 effect. A numerical test to discern the impact of the geometry by symmetrically flipping the shape has shown a beneficial effect of the negative triangularity on heat transport.

Negative Medium-Voltage Direct Current Discharges in Air under Simulated Sub-Atmospheric Pressures for All-Electric Aircraft

The increase in the global temperature due to greenhouse gas emissions is a major concern to the world. To achieve the goal of zero emissions by 2050 in the USA the practical realization of all-electric vehicles, particularly all-electric aircraft (AEA), is important. For the design of electrical power systems (EPSs) in all-electric aircraft, a bipolar medium-voltage direct current (MVDC) system of ±5 kV is being investigated. However, several challenges manifest when using such voltages in a low-pressure environment. One of the main challenges is the partial discharge (PD) behavior of the insulation. It is important to study the PD behavior of the insulation by simulating the aviation environment in the lab. This work aimed to study the partial discharge behavior of air under a negative DC voltage in a needle-to-plane electrode geometry by simulating the aviation pressures in the lab. The partial discharge inception voltage (PDIV) and the breakdown voltage (BDV) show an obvious pressure-dependent variation. Regression analysis was performed to better understand the relationship between the PDIV and pressures. Plots were drawn for the average discharge current at each voltage step until breakdown. This paper’s findings can provide valuable insight into the design of EPS for an AEA. To the best of our knowledge, such a study has not been carried out to date.

The impact of magnesium content on lithium-magnesium alloy electrode performance with argyrodite solid electrolyte

Solid-state lithium-based batteries offer higher energy density than their Li-ion counterparts. Yet they are limited in terms of negative electrode discharge performance and require high stack pressure during operation. To circumvent these issues, we propose the use of lithium-rich magnesium alloys as suitable negative electrodes in combination with Li6PS5Cl solid-state electrolyte. We synthesise and characterise lithium-rich magnesium alloys, quantifying the changes in mechanical properties, transport, and surface chemistry that impact electrochemical performance. Increases in hardness, stiffness, adhesion, and resistance to creep are quantified by nanoindentation as a function of magnesium content. A decrease in diffusivity is quantified with 6Li pulsed field gradient nuclear magnetic resonance, and only a small increase in interfacial impedance due to the presence of magnesium is identified by electrochemical impedance spectroscopy which is correlated with x-ray photoelectron spectroscopy. The addition of magnesium aids contact retention on discharge, but this must be balanced against a decrease in lithium diffusivity. We demonstrate via electrochemical testing of symmetric cells at 2.5 MPa and 30∘C that 1% magnesium content in the alloy increases the stripping capacity compared to both pure lithium and higher magnesium content alloys by balancing these effects.

A large-scale filament-free planar plume generated by an argon plasma jet in a gas-confined barrier discharge geometry

Large-scale plumes in a plasma jet are desirable for fast processing of materials with large surface, which are normally composed of discharge filaments. A filamentary plume may cause nonuniform treatment or even damage to vulnerable samples. In this Letter, an argon plasma jet in a gas-confined barrier discharge geometry is proposed to generate a large-scale filament-free plume. Results indicate that the filament-free plume can only be sustained in a relatively low voltage amplitude (Vp), which transits to the filamentary plume with increasing Vp. There is only one negative discharge per voltage cycle for the filament-free plume, while both positive and negative discharges for the filamentary plume. Fast photography reveals that the negative discharge is diffuse, originating from the propagation of a negative streamer. On the contrary, the positive discharges are filamentary. Optical emission spectroscopy indicates that the filament-free plume has lower electron density, electron excitation temperature, and molecular vibrational temperature compared to the filamentary plume, while gas temperature keeps at a low value with varying Vp.

Time-resolved characteristics of a nanosecond pulsed multi-hollow needle plate packed bed dielectric barrier discharge

In this paper, self-designed multi-hollow needle electrodes are used as a high-voltage electrode in a packed bed dielectric barrier discharge reactor to facilitate fast gas flow through the active discharge area and achieve large-volume stable discharge. The dynamic characteristics of the plasma, the generated active species, and the energy transfer mechanisms in both positive discharge (PD) and negative discharge (ND) are investigated by using fast-exposure intensified charge coupled device (ICCD) images and time-resolved optical emission spectra. The experimental results show that the discharge intensity, number of discharge channels, and discharge volume are obviously enhanced when the multi-needle electrode is replaced by a multi-hollow needle electrode. During a single voltage pulse period, PD mainly develops in a streamer mode, which results in a stronger discharge current, luminous intensity, and E/N compared with the diffuse mode observed in ND. In PD, as the gap between dielectric beads changes from 0 to 250 μm, the discharge between the dielectric bead gap changes from a partial discharge to a standing filamentary micro-discharge, which allows the plasma to leave the local area and is conducive to the propagation of surface streamers. In ND, the discharge only appears as a diffusion-like mode between the gap of dielectric beads, regardless of whether there is a discharge gap. Moreover, the generation of excited states and is mainly observed in PD, which is attributed to the higher E/N in PD than that in ND. However, the generation of the radical in ND is higher than in PD. It is not directly dominated by E/N, but mainly by the resonant energy transfer process between metastable and . Furthermore, both PD and ND demonstrate obvious energy relaxation processes of electron-to-vibration and vibration-to-vibration, and no vibration-to-rotation energy relaxation process is observed.

Unravelling K intercalation on graphene and its variants through two-dimensional cluster expansion modeling

In this study, we investigate K ordering and its impact on K intercalation and storage capacity in graphite, bilayer and single-layer graphene through two-dimensional cluster expansion implemented in first-principles calculations with van der Waals corrections. For graphite, similar to the Li counterpart, K intercalation exhibits a multistage feature as the K concentration increases from C2 to KC8. However, beyond KC8, K atoms become crowded in graphite, resulting in a negative discharge voltage. For bilayer and single-layer graphene, a noticeable displacement of K from original hexagonal sites occurs at higher K concentrations compared to graphite. K intercalation in graphite after the initial segment (from C2 to KC8) leads to an increase in interlayer distance, while in bilayer graphene causes much larger elongation in interlayer distance. The calculated overpotential for K intercalation on bilayer and single-layer graphene is found to be 0.17 and 0.13 V, respectively, which is lower than the overpotential (0.86 V) observed on graphite. The charge redistribution between K and carbon layers indicates that bilayer and single-layer graphene offer pseudo-capacitance, facilitating faster charge transfer and higher K capacity. The above observation suggests the graphene structures have a superior K-storage capacity compared to graphite.