Active metasurface device capable of complex modulation in the visible light range is demonstrated. To realize complex modulation, a liquid crystal (LC) of twisted nematic mode on a plasmonic antenna metasurface, where resonance wavelength is sensitive to its geometry and nearby optical environment, is integrated. For the LC process on the metasurface, the alignment characteristics of the material exposed to the LC on the metasurface are first identified and the polyimide alignment layer is omitted. The LC works in twisted nematic mode to enhance complex modulation characteristics. The complex reflectivity coefficient is measured while varying the voltage applied to both the antenna and metal electrode in the visible light region. Complex reflectivity into a doughnut shape with a small voltage variation of 3.1 V on the antenna electrode and 2.5 V on the metal electrode is successfully modulated. The largest complex modulation is achieved at a wavelength of 660 nm, with phase and reflectivity amplitude modulations of 0–2π radian in a doughnut shape and 0.3 and 0.6, respectively. So far true holographic experience is limited by high‐order overlapping and twin images. Through this approach, a technical method is suggested for overcoming such obstacles and accomplishing advanced holographic display.