Nanometer-thick Yttrium Iron Garnet Research Articles

Propagating spin-wave spectroscopy in a liquid-phase epitaxial nanometer-thick YIG film at millikelvin temperatures

Performing propagating spin-wave spectroscopy of thin films at millikelvin temperatures is the next step toward the realization of large-scale integrated magnonic circuits for quantum applications. Here, we demonstrate spin-wave propagation in a 100 nm-thick yttrium-iron-garnet (YIG) film at temperatures down to 45 mK, using stripline nanoantennas deposited on YIG surface for electrical excitation and detection. The clear transmission characteristics over the distance of 10 μ m are measured and the extracted spin-wave group velocity and the YIG saturation magnetization agree well with the theoretical values. We show that the gadolinium-gallium-garnet (GGG) substrate influences the spin-wave propagation characteristics only for the applied magnetic fields beyond 75 mT, originating from a GGG magnetization up to 62 kA / m at 45 mK. Our results show that the developed fabrication and measurement methodologies enable the realization of integrated magnonic quantum nanotechnologies at millikelvin temperatures.

Dispersionless Propagation of Ultrashort Spin-Wave Pulses in Ultrathin Yttrium Iron Garnet Waveguides

We study experimentally the propagation of nanosecond spin-wave pulses in microscopic waveguides made of nanometer-thick yttrium iron garnet films. For these studies, we use microfocus Brillouin light-scattering spectroscopy, which provides the possibility to observe propagation of the pulses with high spatial and temporal resolution. We show that, for most spin-wave frequencies, dispersion leads to broadening of the pulse by several times at propagation distances of 10 \textmu{}m. However, for certain frequency interval, the dispersion broadening is suppressed almost completely resulting in a dispersionless pulse propagation. We show that the formation of the dispersion-free region is caused by the competing effects of the dipolar and the exchange interaction, which can be controlled by the variation of the waveguide geometry. These conclusions are supported by micromagnetic simulations and analytical calculations. Our findings provide a simple solution for the implementation of high-speed magnonic systems that require undisturbed propagation of short information-carrying spin-wave pulses.

Frequency Filtering with a Magnonic Crystal Based on Nanometer-Thick Yttrium Iron Garnet Films

Magnonics rely on the wave nature of the magnetic excitations to process information, an approach that is common to many fields such as photonics, phononics, and plasmonics. Nevertheless, magnons, the quanta of spin-wave excitations, have the unique advantage to be at frequencies that are lying between a few GHz to tens of GHz, that is, in the technologically relevant radio-frequency bands for 4G and 5G telecommunications. Furthermore, their typical wavelengths are compatible with on-chip integration. Here, we demonstrate radio-frequency signal filtering by a micron-scale magnonic crystal (MC) based on a nanopatterned 20 nm-thick film of yttrium iron garnet with a minimum feature size of 100 nm where the Bragg vector is set to be kB = 2.1 μm–1. We map the intensity and the phase of spin waves (SWs) propagating in the periodic magnetic structure using phase-resolved microfocus Brillouin light-scattering spectroscopy. Based on these maps, we obtain the SW dispersion and the attenuation characteristics. Efficient filtering is obtained with a frequency selectivity of 20 MHz at an operating frequency of 4.9 GHz. The results are analyzed by performing time- and frequency-resolved full-scale micromagnetic simulations of the MC that reproduce quantitatively the complexity of the harmonic response across the magnonic band gap and allow the identification of the relevant SW-quantized modes, thereby providing an in-depth insight into the physics of SW propagation in periodically modulated nanoscale structures.

Nanometer-thick YIG-based magnonic crystals: Bandgap dependence on groove depth, lattice constant, and film thickness

We report on bandgap tuning in magnonic crystals made of nanometer-thick yttrium iron garnet (YIG) films with CoFeB-filled grooves via a variation of the groove depth, lattice constant, and film thickness. Using broadband spin-wave spectroscopy, we demonstrate bandgap widening in a 260-nm-thick YIG crystal when the grooves are deepened from half to full film thickness. Importantly, low-loss spin-wave transmission in the allowed bands of the magnonic crystal is almost unaffected by the patterning of fully discrete YIG stripes. Downscaling of the YIG film thickness to 35 nm decreases the bandgap size through a flattening of the spin-wave dispersion relation. We show that a reduction in the lattice constant effectively compensates for this trend. Our experimental results are corroborated by micromagnetic simulations, providing relevant information for the design of ultrathin YIG-based magnonic crystals with optimized bandgaps and spin-wave transmission properties.

Propagating spin waves in nanometer-thick yttrium iron garnet films: Dependence on wave vector, magnetic field strength, and angle

We present a comprehensive investigation of propagating spin waves in nanometer-thick yttrium iron garnet (YIG) films. We use broadband spin-wave spectroscopy with integrated coplanar waveguides (CPWs) and microstrip antennas on top of continuous and patterned YIG films to characterize spin waves with wave vectors up to 10 rad/$\mu$m. All films are grown by pulsed laser deposition. From spin-wave transmission spectra, parameters such as the Gilbert damping constant, spin-wave dispersion relation, group velocity, relaxation time, and decay length are derived and their dependence on magnetic bias field strength and angle is systematically gauged. For a 40-nm-thick YIG film, we obtain a damping constant of $3.5 \times 10^{-4}$ and a maximum decay length of 1.2 mm. Our experiments reveal a strong variation of spin-wave parameters with magnetic bias field and wave vector. Spin-wave properties change considerably up to a magnetic bias field of about 30 mT and above a field angle of $\theta_{H} = 20^{\circ}$, where $\theta_{H} = 0^{\circ}$ corresponds to the Damon-Eshbach configuration.

Low-loss YIG-based magnonic crystals with large tunable bandgaps

Control of spin waves in magnonic crystals is essential for magnon-based computing. Crystals made of ferromagnetic metals offer versatility in band structure design, but strong magnetic damping restricts their transmission efficiency. Yttrium iron garnet (YIG) with ultralow damping is the palpable alternative, yet its small saturation magnetization limits dipolar coupling between discrete units. Here, we experimentally demonstrate low-loss spin-wave manipulation in magnonic crystals of physically separated nanometer-thick YIG stripes. We enhance the transmission of spin waves in allowed minibands by filling the gaps between YIG stripes with CoFeB. Thus-formed magnonic crystals exhibit tunable bandgaps of 50–200 MHz with nearly complete suppression of the spin-wave signal. We also show that Bragg scattering on only two units produces clear frequency gaps in spin-wave transmission spectra. The integration of strong ferromagnets in nanometer-thick YIG-based magnonic crystals provides effective spin-wave manipulation and low-loss propagation, a vital parameter combination for magnonic technologies.

Exchange-torque-induced excitation of perpendicular standing spin waves in nanometer-thick YIG films

Spin waves in ferrimagnetic yttrium iron garnet (YIG) films with ultralow magnetic damping are relevant for magnon-based spintronics and low-power wave-like computing. The excitation frequency of spin waves in YIG is rather low in weak external magnetic fields because of its small saturation magnetization, which limits the potential of YIG films for high-frequency applications. Here, we demonstrate how exchange-coupling to a CoFeB film enables efficient excitation of high-frequency perpendicular standing spin waves (PSSWs) in nanometer-thick (80 nm and 295 nm) YIG films using uniform microwave magnetic fields. In the 295-nm-thick YIG film, we measure intense PSSW modes up to 10th order. Strong hybridization between the PSSW modes and the ferromagnetic resonance mode of CoFeB leads to characteristic anti-crossing behavior in broadband spin-wave spectra. We explain the excitation of PSSWs by exchange coupling between forced magnetization precessions in the YIG and CoFeB layers. If the amplitudes of these precessions are different, a dynamic exchange torque is generated, causing the emission of spin waves from the interface. PSSWs form when the wave vector of the spin waves matches a perpendicular confinement condition. PSSWs are not excited if exchange coupling between YIG and CoFeB is eliminated by a 10 nm Ta spacer layer. Micromagnetic simulations confirm the exchange-torque-driven mechanism.

Chemical solution synthesis and ferromagnetic resonance of epitaxial thin films of yttrium iron garnet

Cubic Yttrium Iron Garnet (YIG) is a technologically important material due to its excellent magneto-optical properties, high electrical resistivity, and a very narrow ferromagnetic resonance, which makes it particularly suitable for applications in filters and resonators at microwave frequencies. These properties depend on the precise stoichiometry and distribution of Fe${}^{3+}$ ions among the octahedral/tetrahedral sites of a complex structure, which required the use of high-vacuum deposition methods for the fabrication of high-quality YIG thin films. In this paper the authors report the synthesis of nanometer-thick epitaxial films of YIG by a simple water-based chemical method. The films show a long spin relaxation time, comparable to that obtained from high-vacuum physical deposition methods. These results demonstrate that chemical methods can compete to develop nanometer-thick YIG films with the quality required for spintronic devices and other high-frequency applications.

Characterization of spin wave propagation in (1 1 1) YIG thin films with large anisotropy

We report on long-range spin wave (SW) propagation in nanometer-thick yttrium iron garnet (YIG) film with an ultralow Gilbert damping. The knowledge of a wavenumber value is essential for designing SW devices. Although determining the wavenumber in experiments like Brillouin light scattering spectroscopy is straightforward, quantifying the wavenumber in all-electrical experiments has not been widely commented upon so far. We analyze magnetostatic spin wave (SW) propagation in YIG films in order to determine the SW wavenumber excited by the coplanar waveguide. We show that it is crucial to consider the influence of magnetic anisotropy fields present in YIG thin films for precise determination of SW wavenumber. With the proposed methods we find that experimentally derived values of are in perfect agreement with that obtained from electromagnetic simulation only if anisotropy fields are included.

High-efficiency control of spin-wave propagation in ultra-thin yttrium iron garnet by the spin-orbit torque

We study experimentally with submicrometer spatial resolution the propagation of spin waves in microscopic waveguides based on the nanometer-thick yttrium iron garnet and Pt layers. We demonstrate that by using the spin-orbit torque, the propagation length of the spin waves in such systems can be increased by nearly a factor of 10, which corresponds to the increase in the spin-wave intensity at the output of a 10 μm long transmission line by three orders of magnitude. We also show that, in the regime, where the magnetic damping is completely compensated by the spin-orbit torque, the spin-wave amplification is suppressed by the nonlinear scattering of the coherent spin waves from current-induced excitations.

Interface effects in nanometer-thick yttrium iron garnet films studied by magneto-optical spectroscopy

The properties of nanometer-thick yttrium iron garnet (YIG) films are strongly influenced by interfaces. This work employs spectral ellipsometry (SE) and magneto-optic polar Kerr rotation (PKR) to characterize YIG films with thickness, t, from 6 nm to 30 nm grown on Gd3Ga5O12 (GGG) substrates oriented parallel to (111) plane. The films display a surface roughness of 0.35 nm or lower. The analysis of the SE data at the photon energies of 1 eV < E < 6.5 eV provided the t and permittivity values. The PKR at 1.3 eV < E < 4.5 eV is reasonably explained with the optical model for the YIG film/GGG substrate system. Even better agreement is achieved by assuming a 1.07-nm-thick layer sandwiched between YIG and GGG that has Fe3+ sublattice magnetization opposite to that in the YIG volume. This suggests the existence of antiferromagnetic coupling between the Gd3+ and tetrahedral Fe3+.

Short-Wavelength Spin Waves in Yttrium Iron Garnet Micro-Channels on Silicon

Yttrium iron garnet (YIG) has been widely used in spin wave studies thanks to its low Gilbert damping constant. However, most high-quality YIG films are grown on gadolinium gallium garnet (GGG) substrate, which makes it difficult to integrate with existing semiconductor technology. We show spin wave excitation in a nanometer-thick YIG micro-channel on silicon substrate. The YIG is grown by pulsed laser deposition (PLD) in high-purity oxygen followed by rapid thermal annealing at 800°C after deposition. Using meander coplanar waveguides at submicrometer scale, spin waves with wavelength down to 1 μm are excited. By measuring the linewidth of the spin wave reflection spectra, a Gilbert damping constant α = 1.9×10 -3 was obtained.

Thickness- and temperature-dependent magnetodynamic properties of yttrium iron garnet thin films

The magnetodynamical properties of nanometer-thick yttrium iron garnet films are studied using ferromagnetic resonance as a function of temperature. The films were grown on gadolinium gallium garnet substrates by pulsed laser deposition. First, we found that the damping coefficient increases as the temperature increases for different film thicknesses. Second, we found two different dependencies of the damping on film thickness: at room temperature, the damping coefficient increases as the film thickness decreases, while at T = 8 K, we find the damping to depend only weakly on the thickness. We attribute this behavior to an enhancement of the relaxation of the magnetization by impurities or defects at the surfaces.

Optical spectroscopy of sputtered nanometer-thick yttrium iron garnet films

Nanometer (nm)-thick yttrium iron garnet (Y3Fe5O12, YIG) films present interest for spintronics. This work employs spectral ellipsometry and magneto-optic Kerr effect (MOKE) spectra to characterize nm-thick YIG films grown on single-crystal Gd3Ga5O12 substrates by magnetron sputtering. The thickness (t) of the films ranges between 10 nm and 40 nm. Independent on t, the polar MOKE hysteresis loops saturate in the field of about 1.8 kOe, consistent with the saturation magnetization in bulk YIG (4πMs ≈ 1.75 kG). The MOKE spectrum measured at photon energies between 1.3 eV and 4.5 eV on the 38-nm-thick film agrees with that measured on single-crystal YIG bulk materials. The MOKE spectrum of the 12-nm-thick film still preserves the structure of the bulk YIG but its amplitude at lower photon energies is modified due to the fact that the radiation penetration depth exceeds 20 nm. The t dependence of the MOKE amplitude is consistent with MOKE calculations. The results indicate that the films are stoichiometric, strain free, without Fe2+, and preserve bulk YIG properties down to t ≈ 10 nm.

Pseudomorphic Yttrium Iron Garnet Thin Films With Low Damping and Inhomogeneous Linewidth Broadening

Nanometer-thick yttrium iron garnet films, grown on gadolinium gallium garnet substrates by pulsed laser deposition, exhibit remarkably high crystallinity and atomically smooth surfaces. The pseudomorphic growth mechanism leads to large negative out-of-plane uniaxial anisotropy, narrow resonance linewidths, and minimal damping. Magnetic resonance measurements indicate that both the Gilbert damping parameter and inhomogeneous linewidth broadening $\Delta H_{pp,0}$ are consistently low for films of various thicknesses. Even at film thickness $\approx 20$ nm, we attain $\alpha \approx 2\times 10^{-4}$ and $\Delta H_{pp,0} \approx 1$ Oe, which are among the lowest values ever reported.

Electric control of magnetization relaxation in thin film magnetic insulators

Control of magnetization relaxation in magnetic insulators via interfacial spin scattering is demonstrated. The experiments use nanometer-thick yttrium iron garnet (YIG)/Pt layered structures, with the Pt layer biased by an electric voltage. The bias voltage produces a spin current across the Pt thickness. As this current scatters off the YIG surface, it exerts a torque on the YIG surface spins. This torque can reduce or enhance the damping and thereby decrease or increase the ferromagnetic resonance linewidth of the YIG film, depending on the field/current configuration.