Multi-octave Supercontinuum Generation Research Articles

Multioctave supercontinuum generation and frequency conversion based on rotational nonlinearity.

The field of attosecond science was first enabled by nonlinear compression of intense laser pulses to a duration below two optical cycles. Twenty years later, creating such short pulses still requires state-of-the-art few-cycle laser amplifiers to most efficiently exploit "instantaneous" optical nonlinearities in noble gases for spectral broadening and parametric frequency conversion. Here, we show that nonlinear compression can be much more efficient when driven in molecular gases by pulses substantially longer than a few cycles because of enhanced optical nonlinearity associated with rotational alignment. We use 80-cycle pulses from an industrial-grade laser amplifier to simultaneously drive molecular alignment and supercontinuum generation in a gas-filled capillary, producing more than two octaves of coherent bandwidth and achieving >45-fold compression to a duration of 1.6 cycles. As the enhanced nonlinearity is linked to rotational motion, the dynamics can be exploited for long-wavelength frequency conversion and compressing picosecond lasers.

Multioctave supercontinua from shock-coupled soliton self-compression

Fiber-optic multioctave supercontinuum generation is a unique resource for ultrafast optical science, enabling ultrabroadband frequency-comb technologies and paving the way for the photonics of subcycle field wave forms. Extension of these methods to the midinfrared spectral range encounters numerous challenges, calling for radically new approaches in fiber optics and short-pulse generation technologies, as well as for closing the gaps in our understanding of optical nonlinearities in the midinfrared range. Here, we confront these challenges by showing that multioctave supercontinua spanning from the ultraviolet to the midinfrared range can be generated by shock-wave-coupled soliton self-compression of ultrashort midinfrared pulses in a gas-filled antiresonance-guiding hollow-core photonic-crystal fiber. Analysis of the fiber output spectra, measured within a broad range of gas pressures and input driver energies, shows that multioctave supercontinuum generation in this setting becomes possible due to soliton self-compression coupled to shock-wave pulse self-steepening, yielding extraordinarily short, sub-half-cycle field transients.

Deep-UV to Mid-IR Supercontinuum Generation driven by Mid-IR Ultrashort Pulses in a Gas-filled Hollow-core Fiber

Supercontinuum (SC) generation based on ultrashort pulse compression constitutes one of the most promising technologies towards ultra-wide bandwidth, high-brightness, and spatially coherent light sources for applications such as spectroscopy and microscopy. Here, multi-octave SC generation in a gas-filled hollow-core antiresonant fiber (HC-ARF) is reported spanning from 200 nm in the deep ultraviolet (DUV) to 4000 nm in the mid-infrared (mid-IR) having an output energy of 5 μJ. This was obtained by pumping at the center wavelength of the first anti-resonant transmission window (2460 nm) with ~100 fs pulses and an injected pulse energy of ~8 μJ. The mechanism behind the extreme spectral broadening relies upon intense soliton-plasma nonlinear dynamics which leads to efficient soliton self-compression and phase-matched dispersive wave (DW) emission in the DUV region. The strongest DW is observed at 275 nm which corresponds to the calculated phase-matching wavelength of the pump. Furthermore, the effect of changing the pump pulse energy and gas pressure on the nonlinear dynamics and their direct impact on SC generation was investigated. This work represents another step towards gas-filled fiber-based coherent sources, which is set to have a major impact on applications spanning from DUV to mid-IR.

Multi-octave supercontinuum generation in YAG pumped by mid-infrared, multi-picosecond pulses.

High-energy, multi-octave supercontinuum (SC) generation in bulk media pumped with picosecond pulses in the mid-infrared, though pivotal in a myriad of applications, poses severe constraints due to wavelength scaling of the critical power criterion and the propensity to induce avalanche-ionization-seeded breakdown mechanisms. Here, we demonstrate a simple experimental geometry, relying on a very low numerical aperture for the pump pulse, and a crystal length commensurate with the Rayleigh length of the focusing geometry, generating a multi-octave, stable SC in yttrium aluminum garnet (YAG). The SC ranges from 500nm to 3.5μm (measured at -30 dB with spectral components at wavelengths up to 4.5μm) when pumped by a 3ps pulse centered at 2.05μm in the anomalous dispersion regime. We also investigate the dynamics of filament formation in this interaction regime by monitoring the spectral and temporal evolution of the pulse during its propagation through the length of the crystal.

Ultrafast supercontinuum generation in bulk condensed media

Nonlinear propagation of intense femtosecond laser pulses in bulk transparent media leads to a specific propagation regime, termed femtosecond filamentation, which in turn produces dramatic spectral broadening, or superbroadening, termed supercontinuum generation. Femtosecond supercontinuum generation in transparent solids represents a compact, efficient and alignment-insensitive technique for generation of coherent broadband radiation at various parts of the optical spectrum, which finds numerous applications in diverse fields of modern ultrafast science. During recent years, this research field has reached a high level of maturity, both in understanding of the underlying physics and in achievement of exciting practical results. In this paper we overview the state-of-the-art femtosecond supercontinuum generation in various transparent solid-state media, ranging from wide-bandgap dielectrics to semiconductor materials and in various parts of the optical spectrum, from the ultraviolet to the mid-infrared spectral range. A particular emphasis is given to the most recent experimental developments: multioctave supercontinuum generation with pumping in the mid-infrared spectral range, spectral control, power and energy scaling of broadband radiation and the development of simple, flexible and robust pulse compression techniques, which deliver few optical cycle pulses and which could be readily implemented in a variety of modern ultrafast laser systems.

Resonance-enhanced multi-octave supercontinuum generation in antiresonant hollow-core fibers

Ultrafast supercontinuum generation in gas-filled waveguides is an enabling technology for many intriguing applications ranging from attosecond metrology towards biophotonics, with the amount of spectral broadening crucially depending on the pulse dispersion of the propagating mode. In this study, we show that structural resonances in a gas-filled antiresonant hollow core optical fiber provide an additional degree of freedom in dispersion engineering, which enables the generation of more than three octaves of broadband light that ranges from deep UV wavelengths to near infrared. Our observation relies on the introduction of a geometric-induced resonance in the spectral vicinity of the ultrafast pump laser, outperforming gas dispersion and yielding a unique dispersion profile independent of core size, which is highly relevant for scaling input powers. Using a krypton-filled fiber, we observe spectral broadening from 200 nm to 1.7 μm at an output energy of ∼ 23 μJ within a single optical mode across the entire spectral bandwidth. Simulations show that the frequency generation results from an accelerated fission process of soliton-like waveforms in a non-adiabatic dispersion regime associated with the emission of multiple phase-matched Cherenkov radiations on both sides of the resonance. This effect, along with the dispersion tuning and scaling capabilities of the fiber geometry, enables coherent ultra-broadband and high-energy sources, which range from the UV to the mid‐infrared spectral range.

Comparative study of multioctave supercontinuum generation in fused silica, YAG, and LiF in the range of anomalous group velocity dispersion

We present spectral measurements that uncover the detailed dynamics of the supercontinuum generation in fused silica, YAG, and LiF crystals when pumped with 100 fs pulses with a central wavelength of 2.3 μm, which falls into the range of anomalous group velocity dispersion of the media. The multi-octave supercontinuum spectra, which span from the ultraviolet to the mid-infrared, are recorded by means of high-dynamic range measurements over the entire wavelength range covered by the supercontinuum radiation. The spectral dynamics versus the input pulse energy uncovers different mechanisms of spectral broadening, which are characterized by the occurrence of specific but well-distinguished spectral signatures and which are interpreted in terms of plasma-induced and anomalous group velocity dispersion-induced compression of the driving pulse.

Multi-octave supercontinuum generation with IR radiation filamentation in transparent solid-state media

Supercontinuum generation from the near to far IR during radiation filamentation in solid-state media in an anomalous dispersion region is theoretically investigated. The initial search for appropriate media with the use of an interference model showed that the widest IR spectrum is generated in media with high values of zero group velocity dispersion wavelength with the pump wavelength located not far from it. Halides belong to one of such media groups. The possibility of generation of a very wide supercontinuum in calcium fluoride (0.52–3.35 μm, which corresponds to 2.7 octaves), sodium chloride (0.7–7.6 μm, 3.5 octaves), and potassium iodide (0.66–22 μm, 5.1 octaves) is demonstrated by numerical simulation. Also, pulse self-compression down to 13 fs at the 5-μm central wavelength (about single period) has been observed in potassium iodide. The mechanisms of multi-octave supercontinuum generation are discussed.

Multi-octave supercontinuum generation from mid-infrared filamentation in a bulk crystal

We present supercontinuum generation pumped by femtosecond mid-infrared pulses in a bulk homogeneous material. The spectrum extends from 450 nm into the midinfrared, and carries high spectral energy density (3 pJ/nm–10 nJ/nm). The supercontinuum has high shot-to-shot reproducibility and preserves the carrier-to-envelope phase. Our result paves the way for compact supercontinuum sources with unprecedented bandwidth.

Multi-octave supercontinuum generation from mid-infrared filamentation in a bulk crystal

In supercontinuum generation, various propagation effects combine to produce a dramatic spectral broadening of intense ultrashort optical pulses. With a host of applications, supercontinuum sources are often required to possess a range of properties such as spectral coverage from the ultraviolet across the visible and into the infrared, shot-to-shot repeatability, high spectral energy density and an absence of complicated pulse splitting. Here we present an all-in-one solution, the first supercontinuum in a bulk homogeneous material extending from 450 nm into the mid-infrared. The spectrum spans 3.3 octaves and carries high spectral energy density (2 pJ nm−1–10 nJ nm−1), and the generation process has high shot-to-shot reproducibility and preserves the carrier-to-envelope phase. Our method, based on filamentation of femtosecond mid-infrared pulses in the anomalous dispersion regime, allows for compact new supercontinuum sources.