Attitude errors, accelerometer bias, the gravity disturbance vector, and their coupling are the primary factors obstructing strapdown airborne vector gravimetry. This paper takes the geocentric inertial frame as a reference and solves the kinematic equations of its motion and its errors of the body frame and local geographic frame in the Lie group, respectively; the attitude accuracy is improved through a high-precision navigation algorithm. The constant accelerometer bias is estimated through Kalman filtering and is deducted from the accelerometer output to eliminate its influence. Based on the EGM2008 model, the low-frequency components of the gravity disturbance vector are corrected. The gravity disturbance vectors after model data fusion were low-pass filtered to obtain the ultimate results. This method was applied to flight experimental data in the South China Sea, and a gravity anomaly accuracy of better than 0.5 mGal, a northward gravity disturbance accuracy of 0.85 mGal, and an eastward gravity disturbance accuracy of 4.0 mGal were obtained, with a spatial resolution of approximately 4.8 km.