Mid-infrared Fiber Research Articles

Mid-infrared pulsed fiber laser source at 4.3 µm based on a CO2-filled anti-resonant hollow-core silica fiber

Fiber lasers in the mid-infrared (mid-IR) band are of great interest due to their wide range of applications such as manufacturing, defense, spectroscopy, and free-space communication. Due to the immaturity of the soft glass fiber fabrication technology and the limitation of the type of doped rare earth, laser power scaling and wavelength expansion above 4 µm are greatly limited. Lasers based on gas-filled hollow-core fibers (HCFs) have proved to be an effective way of generating mid-IR lasers. We demonstrate a pulsed 4.3 µm laser source based on a CO2-filled HCF for the first time. The pulse energy characteristics and output spectrum of the mid-IR laser have been investigated. The maximum pulse energy of the mid-IR laser is 236 nJ. The maximum average power of the mid-IR laser is 297.8 mW with a slope efficiency of 17.3%. A step-tunable mid-IR output is achieved from 4293.718 nm to 4392.085 nm including 8 emission lines. Furthermore, the time-domain and frequency-domain properties of the mid-IR laser have been studied to understand laser operation better. This work has an important reference value for the development of pulsed mid-IR fiber gas laser sources.

Mid-infrared enhanced Raman soliton generation in an erbium-doped ZBLAN with record energy and peak power

The advancement of tunable ultrafast sources in the mid-infrared spectrum would bring about significant progress in various scientific fields. This study suggests a gain-modulation technique to increase the peak power and pulse energy of mid-infrared tunable Raman solitons. By utilizing a high-power 2-2.23 µm Raman soliton pulse as a pump source, mid-infrared Raman solitons within the 2-3.2 µm tuning range can be generated in a segment of Er3+: ZBLAN fiber. Additionally, the introduction of 976 nm pump light into the Er3+: ZBLAN fiber leverages the gain of Er3+ to amplify the frequency shift velocity and pulse energy of the Raman soliton. Consequently, the frequency shift range of the Raman soliton is extended to 3.5 µm, with peak power and pulse energy reaching 0.93 MW and 107 nJ, respectively. These achievements represent the highest peak power and energy levels of Raman solitons generated in mid-infrared fibers to date.

InAs/GaSb superlattice SESAM mode-locked fluoride fiber laser at 2.8 µm.

We demonstrate a mode-locked fluoride fiber laser operating at 2.8 µm using an InAs/GaSb superlattice (SL) semiconductor saturable absorber mirror (SESAM). Z-scan measurements show that the SL saturable absorber layer possesses off-bandgap nonlinearity near 2.8 µm, with a saturation fluence of 15.9 µJ/cm2, a single-pass modulation depth of 2.4%, and a damage threshold of 10.4 mJ/cm2. Using this high-damage-threshold SESAM, we achieved a maximum average output power of 1.16 W from the 2.8 µm mode-locked Er:ZBLAN fiber laser, with a pulse duration of 28.1 ps. Continuous mode-locking operation at an average power of 224 mW was sustained for 36 h without interruption, demonstrating the reliability of the InAs/GaSb SL SESAM for the development of mid-infrared mode-locked fluoride fiber lasers.

Fluoride and chalcogenide glass fiber components for mid-infrared lasers and amplifiers: Breakthroughs, challenges, and future perspective

Since the early 1990s, when researchers began to explore rare-earth-doped mid-infrared glass fibers, fiber laser systems have emerged as promising high-brightness light sources with wavelengths beyond 2.5 μm for applications in spectroscopy and sensing, optical communications and ranging, and processing of complex materials and bio-tissues, to name a few. Despite a substantial research effort over the years, mid-infrared fiber lasers and amplifiers have yet to reach the maturity required for widespread and/or industrial use. The well-known advantages of fiber lasers over their bulk counterparts, namely superior stability and beam quality, compactness, cost-efficiency, flexibility, and maintenance-free operation, can only be fully harnessed in the mid-infrared wavelength range with the development of non-existent yet essential fiber-based components made of advanced fluoride or chalcogenide-glass materials. This Perspective reports on the recent significant achievements that have been made in the design and fabrication of in-fiber and fiber-pigtailed components for fully integrated mid-infrared fiber laser systems. Building upon a comprehensive overview of the mechanical, thermodynamic, and optical properties of fluoride and chalcogenide glass fibers, as well as their interaction with light, we aim to highlight current challenges and opportunities and provide an informed forecast of future advancements in mid-infrared all-fiber laser research.

Physical mechanisms of femtosecond laser induced refractive index change in direct-written mid-infrared fiber Bragg gratings

Physical mechanisms of femtosecond laser induced refractive index change in direct-written mid-infrared fiber Bragg gratings

Generation of a MW-class tunable Raman soliton up to 3.8 µm in a fluorotellurite fiber.

We report the generation of MW-class tunable Raman solitons of 3.3-3.8 µm in a fluorotellurite fiber. The pump source of the mid-infrared fiber is a 2.15-2.3 µm Raman soliton source which has the highest peak-power Raman soliton (3.8 MW) ever achieved in a silica fiber. Fluorotellurite fiber is characterized by its short length and high nonlinearity, preventing the Raman soliton pulse broadening that occurs with fiber dispersion. The Raman soliton shifted to 3.8 µm while still maintaining an ultra-narrow pulse width of 70.4 fs with 1.36 W output power and 1.17 MW peak power. To the best of our knowledge, this is the highest peak-power Raman soliton obtained in a mid-infrared fiber.

4.8-μm CO-filled hollow-core silica fiber light source

Mid-infrared (MIR) fiber lasers are important for a wide range of applications in sensing, spectroscopy, imaging, defense, and security. Some progress has been made in the research of MIR fiber lasers based on soft glass fibers, however, the emission range of rare-earth ions and the robustness of the host materials are still a major challenge for MIR fiber lasers. The large number of gases provide a variety of optical transitions in the MIR band. When combined with recent advances in low-loss hollow-core fiber (HCF), there is a great opportunity for gas-filled fiber lasers to further extend the radiation to the MIR region. Here, a 4.8-μm CO-filled silica-based HCF laser is reported for the first time. This is enabled by an in-house manufactured broadband low-loss HCF with a measured loss of 1.81 dB/m at 4.8 μm. A maximum MIR output power of 46 mW and a tuning range of 180 nm (from 4644 to 4824 nm) are obtained by using an advanced 2.33-μm narrow-linewidth fiber laser. This demonstration represents the longest-wavelength silica-based fiber laser to date, while the absorption loss of bulk silica at 4824 nm is up to 13, 000 dB/m. Further wavelength expansion could be achieved by changing the pump absorption line and optimizing the laser structure.

Enhanced 3 μm emission in Ho3+/Yb3+ co-doped bismuth-fluoride glasses by Gd2O3

In this work, (100-b)(45Bi2O3-40GeO2-15BaF2)-bGd2O3-2Yb2O3-0.5Ho2O3 glass was prepared to use a high-temperature melting method(where b= 0, 2.5, 5, 7.5, 10). The absorption and fluorescence spectra indicate that the optimal Gd2O3 content is 7.5 mol% (BGBG7.5HY), with an Ω2 value of 6.20×10−20 cm2 for the main glass, which is superior to that of BGBG0HY glass. This suggests that the incorporation of Gd2O3 enhances the mid-infrared emission capacity. Raman spectroscopy studies demonstrate that the introduction of Gd₂O₃ results in a substantial influx of oxygen atoms into the glass network, accompanied by a transition of [BiO₆] to [BiO₃] within the glass mesh. This is evidenced by a notable redshift of the characteristic peaks at 509 cm−1 and 677 cm−1 in comparison to BGB glass. The introduction of Gd2O3 also expands the distance between Ho3+/Yb3+ ions, inhibits rare earth ion clusters, improves the Ho3+ luminescence center environment, and thus enhances the 3 μm emission performance of bismuth fluoride glass. The maximum emission cross section is 1.82 × 10−20 cm2 and the maximum gain coefficient is 3.71 cm−1. The results show that the bismuth fluoride glass prepared in this paper is an excellent gain material for mid-infrared fiber lasers.

Heavy metal fluoride glasses: A tutorial review

Heavy metal fluoride glasses are the backbone of modern mid-infrared fiber technology. In the last few years, optical fibers made of fluorozirconate, fluoroaluminate, and fluoroindate glasses have reached the high level of reliability that is required for their widespread use in industrial and medical applications, which explains the rapid growth of this technology. In this tutorial review, the author, who was part of the team that discovered heavy metal fluoride glasses exactly fifty years ago, provides a summary of the glass synthesis process and elucidates the most important physical properties of heavy metal fluoride glasses. Finally, a brief overview of their main application areas is presented.

High-power hollow-core fiber gas laser at 3.1 µm with a linear-cavity structure.

Mid-infrared hollow-core fiber (HCF) gas lasers based on a population inversion regime of gas molecules have made advanced development in recent years, but mostly with single-pass cavity-free structures. Here, we demonstrated a 3.1 µm high-power acetylene-filled HCF continuous wave (CW) laser and a self-Q-switched pulse laser with a linear-cavity structure. This configuration not only facilitates the transformation of amplified spontaneous emission into the laser output but also enhances the coherence of the light source and imparts distinct cavity mode characteristics. Harnessing a homemade high-power 1535 nm single-frequency fiber laser that served as the pump source, a CW laser output of 8.23 W at 3.1 µm was achieved, which is over three orders of magnitude higher than those in reported works so far. The corresponding slope efficiency of 31.8% and beam quality of Mx 2 = 1.18 and My 2 = 1.15 were characterized. When the gas pressure was up to 50 mbar, the laser generated a 3.1 µm self-Q-switched pulse with an output power of 1.98 W as well as a pulse width of 45 ns under the repetition rate of 4.59 MHz. To the best of our knowledge, this is the first time that an HCF gas laser achieves a self-Q-switched pulse. Future studies will aim to further optimize the experimental setup, potentially enabling the direct generation of picosecond pulses in the mid-infrared wavelength band.

Acetone Gas Sensing Using a Hybrid Mid-Infrared Fluoride Fiber Laser

Acetone Gas Sensing Using a Hybrid Mid-Infrared Fluoride Fiber Laser

Chalcogenide mid‐infrared 3 × 1 fiber combiner for highly efficient 2–5 µm power and wavelength combining

AbstractFiber combiner is an effective device to enhance the power level or broaden the spectral wavelengths through a single monolithic output aperture, by fusing multiple fibers together. This is particularly important in mid‐infrared (MIR) 2–5 µm range, in which the output power of a single laser is limited. Due to the high MIR transmission, chalcogenide glass is an ideal host for constructing MIR fiber combiner. In this study, we report the design, fabrication, and characterization of a homemade 3 × 1 chalcogenide glass fiber combiner. The fiber combiner includes a 3 × 1 As–S input fiber bundle and an output fiber. The input fiber bundle was made by tapering three As–S multimode fibers with a core diameter of 200 µm and a cladding diameter of 250 µm. The taper reduction ratio R was 2, and the length of the taper transition region was ∼2 cm. The output fiber with core diameter of 360 µm and cladding diameter of 570 µm was then spliced with the tapered end of the fiber bundle. The total length of the combiner was ∼53 cm. The measurement of power combination at 4.56 µm indicated that the transmission efficiency of three ports reached 80%, whereas the power combining efficiency of the combiner was measured to be ∼48%. In addition, efficient wavelength combining over one octave has been demonstrated, by launching three different lasers at 2.1, 3.39, and 4.56 µm through the 3 × 1 combiner. It proves that chalcogenide fiber combiner is promising for the applications of high‐level power combination and broadband wavelength combining in MIR 2–5 µm range.

Indium selenide for mode-locked pulse generation in a Mid-infrared Er:ZBLAN fiber laser

Two-dimensional materials are increasingly recognized for their distinctive nonlinear optical properties. Indium selenide (InSe), a notable optoelectronic material, demonstrates unique advantages in terms of nonlinear absorption behavior, making it a promising candidate in mid-infrared mode-locked lasers. By preparing a InSe saturable absorber (SA) and applying it in a Er: ZBLAN fiber laser, we demonstrate a stable mode-locked mid-infrared fiber laser at 2.8 μm. The obtained mode-locked pulses have a repetition frequency and pulse duration of 29.875 MHz and 13.6 ps, respectively. The obtained maximum value of pulse energy is 4.3 nJ. The signal-to-noise ratio (SNR) is 55 dB, indicating the high stability of the laser system. Our experimental results validate that InSe is a promising SA in the near 3 μm band. This work paves the way for further investigations and applications of InSe-based devices in nonlinear optics and mode-locked laser systems.

2.1–2.2 μm wavelength-tunable cascade gain modulation Raman fiber laser

We present a theoretical and experimental analysis of a mid-infrared wavelength-tunable cascade gain modulation Raman fiber laser. Our simulation model incorporates the Generalized Nonlinear Schrödinger Equation with the fiber Bragg grating transmission functions. Utilizing the pulse tracking method, we investigate and analyze the impact of pump pulse width and Raman gain fiber length on the first and second order Raman laser thresholds. Additionally, we exhibit the evolution process of the pulse and optical spectrum at a constant pump pulse energy. Furthermore, we present the output pulse width and energy, and the Raman laser center wavelength as a function of the pump pulse energy. Subsequently, using the optimal theoretical values of pump pulse width and Raman gain fiber length, we experimentally achieve the gain modulation Raman fiber laser. With a 1990 nm laser pumping, the Raman laser can produce a 2172 nm laser with a pulse width of 1.25 µs and a single pulse energy of approximately 400 nJ. When tuning the pump laser wavelength from 1950 nm to 2030 nm, the gain modulation Raman laser wavelength can vary from 2130 nm to 2215 nm. Importantly, our experimental results closely align with the theoretical predictions. This study provides valuable insights for the investigation of gain modulation Raman fiber lasers.

Prediction of mid-infrared 2.72 μm lasing in heavily Er3+-doped fluorotellurite glass

Fluorotellurite glasses heavily doped with Er3+ are prepared in less demanding conditions as compared with fluoride glasses. Specifically, the effects of PbF2 added in the system of AlF3–MgF2–CaF2–SrF2–BaF2–TeO2 (AMCSBYT) are systematically studied on the correlation between glass structure and mid-infrared (MIR) luminescent properties of Er3+. These PbF2-modified glasses with an improved thermal stability and a noticeably reduced phonon energy as compared with telluride glasses exhibit an intense MIR emission at 2.72 μm and a long radiative decay lifetime. Calculation and analysis based on the Judd-Ofelt theory provide deeper insights into the interdependence of luminescent properties and glass structure. Numerical simulation is conducted for a MIR fiber laser based on the experimental data derived from the proposed glass. The 2.72 μm lasing output of 0.68 W is predicted with a slope efficiency of 3.38 %. It is expected that the performance of the fiber laser can be further optimized such that the output power can be increased over 1.0 W. The results emphasize the potential of the PbF2-modified fluorotellurite glass as a promising gain material for 2.72 μm fiber lasers.

From 393 to 1167 nm Tunable Third-Harmonic Generation in a Mid-Infrared Tellurite Optical Fiber

From 393 to 1167 nm Tunable Third-Harmonic Generation in a Mid-Infrared Tellurite Optical Fiber

Compact and efficient high-power mid-infrared supercontinuum fiber laser source based on a noise-like pulse and germania fiber

Here, we demonstrate a compact and efficient high-power mid-infrared supercontinuum (MIR-SC) laser source based on a tunable noise-like pulse (NLP) fiber laser system and a short section of single-mode germania-core fiber (GCF). The NLP all-polarization-maintaining fiber laser system can deliver the maximum output power of ∼30.6 W and a broadband spectrum (∼1.8-2.7 µm) with a compact single-stage fiber amplifier. By directly pumping only ∼6.5 cm-long GCF with a core diameter of ∼3.5 µm, a MIR-SC (spectral coverage of ∼1.5-3.3 µm) with a maximum power of ∼25.2 W and a power conversion efficiency ∼81.2% is obtained, which represent the highest power and efficiency in any single-mode GCF-based MIR-SCs, to the best of our knowledge. Our study contributes to the high-power MIR-SC laser source with compact all-fiber configuration, and will prompt its practical applications.

Mid-infrared seven-core chalcogenide fiber with ultra-large mode field area and high beam quality

A seven-core chalcogenide fiber with an ultra-large mode field for mid-infrared range of 2.5–11 μm is designed and fabricated. Through manipulation of the core radius and pitch in the seven-core configuration, we are engaged in a comprehensive exploration of crosstalk characteristics and the mode field area (MFA). In addition, the relationship between the parameters of seven-core fiber for infrared and the beam quality of the output laser is analyzed for the first time. A theoretical MFA of 8914 μm2 can be calculated with a core radius of 24 μm and the pitch of 50 μm. This impressive MFA is realized through the deployment of an improved drilling technique in the fabrication of a Ge–As–Se seven-core fiber. The fiber has a relatively low loss at the wavelength range of 2.5–11 μm, and the minimum loss is 1.4 dB m−1 at 8.5 μm. The measured MFA of the fiber at 10.6 μm is 7364 μm2, which is 6.2 times higher than that of traditional stepped single-core fiber, but slightly lower than the theoretical value. The power delivery capability of the fiber has been significantly improved about two times compared with that of single-core fiber. The output beam quality factor M 2 is calculated as 1.13. In all, the seven-core fiber exhibits substantial potential for high-power laser propagation with high quality and flexibility.

Efficient Pulsed Raman Laser with Wavelength above 2.1 μm Pumped by Noise‐Like Pulse

Herein, the efficiently high‐power pulsed Raman lasers with wavelength above 2.1 μm are experimentally demonstrated relying on the stimulated Raman scattering. A tailored high‐power noise‐like pulse (NLP) fiber laser system centered at ≈1953 nm with a maximum output power of ≈10.9 W is served as the pump source. By directly pumping a section of highly Ge‐doped silica fiber, the first pulsed Raman laser (centered at≈2139 nm) and the second pulsed Raman laser (centered at ≈2353 nm) with maximum output powers of ≈3.8 and ≈0.25 W are obtained, respectively, which represent the highest output powers of NLP at these wavelength regions, to the best of knowledge. Moreover, a high spectral purity of ≈94.3% of the first Raman laser is obtained, which indicates the significantly potential application of NLP in pulsed Raman laser. The midinfrared NLP fiber laser source will have potential applications in transparent polymer materials processing and midinfrared spectroscopy.

Short review and prospective: chalcogenide glass mid-infrared fibre lasers

Rare-earth ion doped, silica glass, optical fibre amplifiers have transformed the world by enabling high speed communications and the Internet. Fibre lasers, based on rare-earth ion doped silica glass optical fibres, achieve high optical powers and are exploited in machining, sensing and medical surgery. However, the chemical structure of silica glass fibres limits the wavelength of laser operation to < 2.5 µm, which excludes the mid-infrared longer wavelength range of 3–50 µm. Rare-earth ion doping of fluoride glasses enables manufacture of fibre lasers up to a limiting 3.92 µm wavelength, but the fluoride glass chemical structure again prevents operation at longer wavelengths. Optical fibre lasers that are constructed from different rare-earth ion doped chalcogenide glass fibres will potentially operate across the 4–10 µm wavelength range, where suitable high-power lasers currently do not exist. We present a short review here of our recent work in achieving first time, continuous wave, mid-infrared fibre lasing beyond 5 μm wavelength in Ce3+-doped selenide chalcogenide fibre. We place this disruptive breakthrough into the wider fibre laser context, and also present the unprecedented advances in new cross-sector applications that will be enabled by mid-infrared fibre lasers in the 4–10 µm wavelength range. To surpass the few mW power output of the Ce3+-doped chalcogenide glass fibre lasing achieved to date, the glass quality of the doped chalcogenide fibres must now be improved, similar to the challenges originally facing the first glass fibre lasers based on silica.