Magnon Signal Research Articles

Axion and dark fermion electromagnetic form factors in superfluid He4

Condensed matter materials have shown great potential in searching for light dark matter (DM) via detecting the phonon or magnon signals induced by the scattering of DM off the materials. In this paper, we study the possibility of detecting electromagnetic form factors of fermionic DM and axionlike particles (ALPs) using superfluid He4. The phonon induced by a sub-GeV fermionic DM scattering off the superfluid can be described using the effective field theory with the interaction between DM and the bulk He4. Signals arising from the electromagnetic form factors of light DM in the presence of an external electric field are calculated. Projected constraints on the charge radius, anapole moment, and magnetic moment of the DM are derived with 1 kg·yr exposure. The phonon signal induced by the scattering of ALPs off the superfluid is also calculated, which can put competitive and the first direct detection bounds on ALP-photon-dark photon couplings in the projected experiments. Published by the American Physical Society 2024

Reversing the magnetization of 50-nm-wide ferromagnets by ultrashort magnons in thin-film yttrium iron garnet.

Spin waves (magnons) can enable neuromorphic computing by which one aims at overcoming limitations inherent to conventional electronics and the von Neumann architecture. Encoding magnon signal by reversing magnetization of a nanomagnetic memory bit is pivotal to realize such novel computing schemes efficiently. A magnonic neural network was recently proposed consisting of differently configured nanomagnets that control nonlinear magnon interference in an underlying yttrium iron garnet (YIG) film [Papp et al., Nat. Commun., 2021, 12, 6422]. In this study, we explore the nonvolatile encoding of magnon signals by switching the magnetization of periodic and aperiodic arrays (gratings) of Ni81Fe19 (Py) nanostripes with widths w between 50 nm and 200 nm. Integrating 50-nm-wide nanostripes with a coplanar waveguide, we excited magnons having a wavelength λ of ≈100 nm. At a small spin-precessional power of 11 nW, these ultrashort magnons switch the magnetization of 50-nm-wide Py nanostripes after they have propagated over 25 μm in YIG in an applied field. We also demonstrate the magnetization reversal of nanostripes patterned in an aperiodic sequence. We thereby show that the magnon-induced reversal happens regardless of the width and periodicity of the nanostripe gratings. Our study enlarges substantially the parameter regime for magnon-induced nanomagnet reversal on YIG and is important for realizing in-memory computing paradigms making use of magnons with ultrashort wavelengths at low power consumption.

Magnon-Assisted Magnetization Reversal of Ni81Fe19 Nanostripes on Y3Fe5O12 with Different Interfaces.

Magnetic bit writing by short-wave magnons without conversion to the electrical domain is expected to be a game-changer for in-memory computing architectures. Recently, the reversal of nanomagnets by propagating magnons was demonstrated. However, experiments have not yet explored different wavelengths and the nonlinear excitation regime of magnons required for computational tasks. We report on the magnetization reversal of individual 20 nm thick Ni81Fe19 (Py) nanostripes integrated onto 113 nm thick yttrium iron garnet (YIG). We suppress direct interlayer exchange coupling by an intermediate layer, such as Cu and SiO2. By exciting magnons in YIG with wavelengths λ down to 148 nm we observe the reversal of the integrated ferromagnets in a small external field of 14 mT. Magnons with a small wavelength of λ = 195 nm, i.e., twice the width of the Py nanostripes, induced the reversal at a spin-precessional power of only about 1 nW after propagating over 15 μm in YIG. Such small power value has not been reported so far. Considerations based on dynamic dipolar coupling explain the observed wavelength dependence of the magnon-induced reversal efficiency. For an increased power, the stripes reversed in an external field of only about 1 mT. Our findings are important for the practical implementation of nonvolatile storage of broadband magnon signals in YIG by means of bistable nanomagnets without the need of an appreciable global magnetic field.

Numerical Model for 32-Bit Magnonic Ripple Carry Adder

In CMOS-based electronics, the most straightforward way to implement a summation operation is to use the ripple carry adder (RCA). Magnonics, the field of science concerned with data processing by spin-waves and their quanta magnons, recently proposed a magnonic half-adder that can be considered as the simplest magnonic integrated circuit. Here, we develop a computation model for the magnonic basic blocks to enable the design and simulation of magnonic gates and magnonic circuits of arbitrary complexity and demonstrate its functionality on the example of a 32-bit integrated RCA. It is shown that the RCA requires the utilization of additional regenerators based on magnonic directional couplers with embedded amplifiers to normalize the magnon signals in-between the half-adders. The benchmarking of large-scale magnonic integrated circuits is performed. The energy consumption of 30 nm-based magnonic 32-bit adder can be as low as 961aJ per operation with taking into account all required amplifiers.

Magnon transport and thermoelectric effects in ultrathin Tm3Fe5O12 /Pt nonlocal devices

The possibility of electrically exciting and detecting magnon currents in magnetic insulators has opened exciting perspectives for transporting spin information in electronic devices. However, the role of the magnetic field and the nonlocal thermal gradients on the magnon transport remain unclear. Here, by performing nonlocal harmonic voltage measurements, we investigate magnon transport in perpendicularly magnetized ultrathin ${\mathrm{Tm}}_{3}{\mathrm{Fe}}_{5}{\mathrm{O}}_{12}$ (TmIG) films coupled to Pt electrodes. We show that the first harmonic nonlocal voltage captures spin-driven magnon transport in TmIG, as expected, and the second harmonic is dominated by thermoelectric voltages driven by current-induced thermal gradients at the detector. The magnon diffusion length in TmIG is found to be ${\ensuremath{\lambda}}_{\mathrm{m}}\ensuremath{\sim}0.3\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}\mathrm{m}$ at 0.5 T and gradually decays to ${\ensuremath{\lambda}}_{\mathrm{m}}\ensuremath{\sim}0.2\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}\mathrm{m}$ at 0.8 T, which we attribute to the suppression of the magnon relaxation time due to the increase of the Gilbert damping with field. By performing current-, magnetic field-, and distance-dependent nonlocal and local measurements we demonstrate that the second harmonic nonlocal voltage exhibits five thermoelectric contributions, which originate from the nonlocal spin Seebeck effect and the ordinary, planar, spin, and anomalous Nernst effects. Our work provides a guide on how to disentangle magnon signals from diverse thermoelectric voltages of spin and magnetic origin in nonlocal magnon devices, and establish the scaling laws of the thermoelectric voltages in metal/insulator bilayers.

Quantum theory of magnon excitation by high energy electron beams

The role of magnon inelastic scattering in high energy electron diffraction of spin unpolarised electron beams, including vortex beams, is investigated theoretically for a Heisenberg ferromagnet. The interaction is between the atomic magnetic dipoles in the specimen and orbital angular momentum (OAM) of the electron beam. Magnon inelastic scattering by vortex beams is allowed despite many atoms along the magnon spin wave experiencing mixed OAM states. The scattering cross-section is however independent of the vortex beam winding number. In the case of planes waves in ferromagnetic iron, the magnon diffuse scattered intensity is significantly smaller than phonons in the energy loss range currently accessible by state-of-the-art monochromated electron energy loss spectroscopy (EELS). Nevertheless, it is shown that the long-range magnetic field of the atomic dipoles has a similar role to dipole scattering in phonon excitation. This means that magnons could, in principle, be detected using aloof beam EELS, where long acquisition times can be realised without any specimen beam damage, an important pre-requisite for detecting the weak magnon signal.

Electrically switchable van der Waals magnon valves

Van der Waals magnets have emerged as a fertile ground for the exploration of highly tunable spin physics and spin-related technology. Two-dimensional (2D) magnons in van der Waals magnets are collective excitation of spins under strong confinement. Although considerable progress has been made in understanding 2D magnons, a crucial magnon device called the van der Waals magnon valve, in which the magnon signal can be completely and repeatedly turned on and off electrically, has yet to be realized. Here we demonstrate such magnon valves based on van der Waals antiferromagnetic insulator MnPS3. By applying DC electric current through the gate electrode, we show that the second harmonic thermal magnon (SHM) signal can be tuned from positive to negative. The guaranteed zero crossing during this tuning demonstrates a complete blocking of SHM transmission, arising from the nonlinear gate dependence of the non-equilibrium magnon density in the 2D spin channel. Using the switchable magnon valves we demonstrate a magnon-based inverter. These results illustrate the potential of van der Waals anti-ferromagnets for studying highly tunable spin-wave physics and for application in magnon-base circuitry in future information technology.

Solids of quantum Hall skyrmions in graphene

Partially filled Landau levels host competing orders, with electron solids prevailing close to integer fillings before giving way to fractional quantum Hall liquids as the Landau level fills. Here, we report the observation of an electron solid with noncolinear spin texture in monolayer graphene, consistent with solidification of skyrmions---topological spin textures characterized by quantized electrical charge. In electrical transport, electron solids reveal themselves through a rapid metal-insulator transition in the bulk electrical conductivity as the temperature is lowered, accompanied by the emergence of strongly nonlinear dependence on the applied bias voltage. We probe the spin texture of the solids using a modified Corbino geometry that allows ferromagnetic magnons to be launched and detected. We find that magnon transport is highly efficient when one Landau level is filled ($\nu=1$), consistent with quantum Hall ferromagnetic spin polarization; however, even minimal doping immediately quenches the the magnon signal while leaving the vanishing low-temperature charge conductivity unchanged. Our results can be understood by the formation of a solid of charged skyrmions near $\nu=1$, whose noncolinear spin texture leads to rapid magnon decay. Data near fractional fillings further shows evidence for several fractional skyrmion crystals, suggesting that graphene hosts a vast and highly tunable landscape of coupled spin and charge orders.

Impact of electromagnetic fields and heat on spin transport signals in Y3Fe5O12

Exploring new strategies to perform magnon logic is a key requirement for the further development of magnon-based spintronics. In this work, we realize a three-terminal magnon transport device to study the possibility of manipulating magnonic spin information transfer in a magnetic insulator via localized magnetic fields and heat generation. The device comprises two parallel Pt wires as well as a Cu center wire that are deposited on the ferrimagnetic insulator Y$_{3}$Fe$_{5}$O$_{12}$. While the Pt wires act as spin current injector and detector, the Cu wire is used to create local magnetostatic fields and additional heat, which impact both the magnetic configuration and the magnons within the Y$_{3}$Fe$_{5}$O$_{12}$ below. We show that these factors can create a non-local signal that shows similar features as compared to an electrically induced magnon flow. Furthermore, a modulation of the spin transport signal between the Pt wires is observed, which can be partly explained by thermally excited spin currents of different polarization. Our results indicate a potential way towards the manipulation of non-local magnon signals, which could be useful for magnon logic.

New Insights about CuO Nanoparticles from Inelastic Neutron Scattering.

Inelastic Neutron Scattering (INS) spectroscopy has provided a unique insight into the magnetodymanics of nanoscale copper (II) oxide (CuO). We present evidence for the propagation of magnons in the directions of the ordering vectors of both the commensurate and helically modulated incommensurate antiferromagnetic phases of CuO. The temperature dependency of the magnon spin-wave intensity (in the accessible energy-range of the experiment) conforms to the Bose population of states at low temperatures (T ≤ 100 K), as expected for bosons, then intensity significantly increases, with maximum at about 225 K (close to TN), and decreases at higher temperatures. The obtained results can be related to gradual softening of the dispersion curves of magnon spin-waves and decreasing the spin gap with temperature approaching TN on heating, and slow dissipation of the short-range dynamic spin correlations at higher temperatures. However, the intensity of the magnon signal was found to be particle size dependent, and increases with decreasing particle size. This “reverse size effect” is believed to be related to either creation of single-domain particles at the nanoscale, or “superferromagnetism effect” and the formation of collective particle states.

Time-Resolved Measurements of Surface Spin-Wave Pulses at Millikelvin Temperatures

In this work, we experimentally investigate the propagation of pulsed magnetostatic surface spin-wave (magnon) signals in an yttrium iron garnet (YIG) waveguide at millikelvin temperatures. Our measurements are performed in a dilution refrigerator at microwave frequencies. The excellent signal-to-noise ratio afforded by the low-temperature environment allows the propagation of the pulses to be observed in detail. The work gives insight both into low-temperature magnon dynamics in YIG and the potential application of systems of propagating magnons to solid-state quantum information processing.

Topological Magnon Modes in Patterned Ferrimagnetic Insulator Thin Films.

Manipulation of magnons opens an attractive direction in the future energy-efficient information processing devices. Such quasi-particles can transfer and process information free from the troublesome Ohmic loss in conventional electronic devices. Here, we propose to realize topologically protected magnon modes using the interface between the patterned ferrimagnetic insulator thin films of different configurations without the Dzyaloshinskii-Moriya interaction. The interface thus behaves like a perfect waveguide to conduct the magnon modes lying in the band gap. These modes are immune to backscattering even in sharply bent tracks, robust against the disorders, and maintain a high degree of coherence during propagation. We design a magnonic Mach-Zehnder interferometer, which realizes a continuous change of magnon signal with varying external magnetic field or driving frequency. Our results pave a new way for realizing topologically protected magnon waveguide and finally achieving a scalable low-dissipation spintronic devices and even the magnonic integrated circuit.

Observation of Ultrafast Magnon Dynamics in Antiferromagnetic Nickel Oxide by Optical Pump-Probe and Terahertz Time-Domain Spectroscopies

We have studied the ultrafast magnon dynamics in an antiferromagnetic 3d-transition-metal monoxide, nickel oxide (NiO), using optical pump-probe spectroscopy and terahertz time-domain spectroscopy (THz-TDS). THz damped magnon oscillations were observed in the Faraday rotation signal and in the transmitted THz electric field via optical pump-probe spectroscopy and THz-TDS, respectively. The magnon signals were observed in both the optical pump-probe spectroscopy and THz-TDS experiments, which shows that both Raman- and infrared-active modes are included in the NiO magnon modes. The magnon relaxation rate observed using THz-TDS was found to be almost constant up to the Neel temperature T N (= 523 K) and to increase abruptly near that temperature. This shows that temperature-independent spin-spin relaxation dominates up to T N . In our experiment, softening of the magnon frequency near T N was clearly observed. This result shows that the optical pump-probe spectroscopy and THz-TDS have high frequency resolution and a high signal to noise ratio in the THz region. We discuss the observed temperature dependence of the magnon frequencies using three different molecular field theories. The experimental results suggest that the biquadratic contribution of the exchange interaction plays an important role in the temperature dependence of the sublattice magnetization and the magnon frequency in cubic antiferromagnetic oxides.

Coherent Two-Dimensional Terahertz Magnetic Resonance Spectroscopy of Collective Spin Waves.

We report a demonstration of two-dimensional (2D) terahertz (THz) magnetic resonance spectroscopy using the magnetic fields of two time-delayed THz pulses. We apply the methodology to directly reveal the nonlinear responses of collective spin waves (magnons) in a canted antiferromagnetic crystal. The 2D THz spectra show all of the third-order nonlinear magnon signals including magnon spin echoes, and 2-quantum signals that reveal pairwise correlations between magnons at the Brillouin zone center. We also observe second-order nonlinear magnon signals showing resonance-enhanced second-harmonic and difference-frequency generation. Numerical simulations of the spin dynamics reproduce all of the spectral features in excellent agreement with the experimental 2D THz spectra.

Magnon propagation in a nanometric magnetic cluster chain: Effects of additional clusters near the chain

A fundamental understanding of nanoscaled materials has become an important challenge for any technical applications. For magnetic nanoparticles, the investigations are in particular stimulated by the magnetic storage devices. In this paper we present a theory of the magnon propagation in a nanometric chain and of the effects of neighbor magnetic clusters. We show that with an appropriate choice of the additional clusters, it is possible to control the transmission spectrum of the magnons. The additional clusters can also create a resonator with zero of transmission. This model could be useful to construct device to transmit or stop the magnon signal.

Inelastic Neutron Scattering Signal from Deconfined Spinons in a Fractionalized Antiferromagnet

We calculate the contribution of deconfined spinons to inelastic neutron scattering (INS) in the fractionalized antiferromagnet (AF*), introduced elsewhere. We find that the presence of free spin-1/2 charge-less excitations leads to a continuum INS signal above the Néel gap. This signal is found above and in addition to the usual spin-1 magnon signal, which to lowest order is the same as in the more conventional confined antiferromagnet. We calculate the relative weights of these two signals and find that the spinons contribute to the longitudinal response, where the magnon signal is absent to lowest order. Possible higher-order effects of interactions between magnons and spinons in the AF* phase are also discussed.

Ballistic propagation of magnons in MnF2

Abstract We present evidence of ballistic transport of energy by high energy, large wave vector magnons in the antiferromagnet MnF 2 . Non-equilibrium magnons are created in broad frequency bands by heat pulses or in narrow frequency bands, throughout the Brillouin zone, by pumping the far-infrared (FIR) two magnon absorption bands. The ballistic magnon signal is extracted from the total observed signal and used to calculate the magnon velocity as a function of magnon energy. The results compare favorably with theory. Non-ballistic signals are interpreted with respect to magnon decay processes.

Ballistic propagation of large wave vector magnons in magnetically ordered materials (invited)

We present evidence of ballistic transport of energy by high-energy, large wave vector magnons in the antiferromagnet MnF2. Nonequilibrium magnons are created by heat pulses or by selective laser excitation throughout the Brillouin zone, using the magnon sideband or far-infrared (FIR) two-magnon absorptions. The ballistic magnon signal is extracted from the total observed signal and used to calculate the magnon velocity as a function of magnon energy. The results compare favorably with theory. Implications of our results to various types of magnetically ordered lattices are discussed.

Optical observation of evanescent surface magnons in thin magnetic films

A new type of nonpropagating surface-wave-like magnon has been detected in yttrium iron garnet films (YIG) in a magnetostatic wave (MSW) device structure using Brillouin light scattering. The measurements were carried out on a YIG film stripline device operated at 2–4 GHz. With an applied magnetic field parallel to the stripline, magnon signals were observed at fields above the surface wave band edge. Theory shows that highly localized, evanescent surface modes can exist at such fields, but only when a ground plane is present; the bandwidth in field or frequency is inversely proportional to the separation between the film and the ground plane. The observed evanescent wave band limits are in good agreement with the theoretical values.

Brillouin light scattering on yttrium iron garnet films in a magnetostatic wave device structure

Brillouin light scattering (BLS) has been used for the direct detection of magnetostatic wave (MSW) excitations in a MSW microwave device structure. The results are for a signal-to-noise enhancer device which consists of a yttrium iron garnet (YIG) film on a gadolinium gallium garnet substrate. The YIG film is in contact with a 30-μm-wide stripline and the static magnetic field is parallel to the stripline. MSW excitations were observed over the frequency range 2– 4 GHz. At low power, magnetostatic surface waves (MSSW) were excited with propagation perpendicular to the stripline and field direction. At high power, parametric half-frequency magnons were also observed. The measured magnon dispersion for the MSSW excitations, determined using the wave vector selective capabilities of the BLS spectrometer, is in good agreement with theory. The measured intensity profiles for MSW excitations at low-power levels show strong MSSW excitations over the entire surface wave band. At high power, the scattering intensity for surface MSW excitations saturates and is accompanied by a strong parametric magnon signal.