Low-energy Coulomb Excitation Research Articles

Shell-model studies relevant for the low-energy Coulomb excitation in Zn isotopes

Shell-model studies relevant for the low-energy Coulomb excitation in Zn isotopes

Low-Energy Coulomb Excitation for the Shell Model

Low-energy Coulomb excitation is capable of providing unique information on static electromagnetic moments of short-lived excited nuclear states, including non-yrast states. The process selectively populates low-lying collective states and is, therefore, ideally suited to study phenomena such as shape coexistence and the development of exotic deformation (triaxial or octupole shapes). Historically, these experiments were restricted to stable isotopes. However, the advent of new facilities providing intense beams of short-lived radioactive species has opened the possibility to apply this powerful technique to a much wider range of nuclei. The paper discusses the observables that can be measured in a Coulomb-excitation experiment and their relation to the nuclear structure parameters with an emphasis on the nuclear shape. Recent examples of Coulomb-excitation studies that provided outcomes relevant for the Shell Model are also presented.

Onset of triaxial deformation in Zn66 and properties of its first excited 0+ state studied by means of Coulomb excitation

The electromagnetic structure of Zn66 at low excitation energy was investigated via low-energy Coulomb excitation at INFN Legnaro National Laboratories, using the Gamma Array of Legnaro Infn Laboratories for nuclEar spectrOscopy (GALILEO) γ-ray spectrometer coupled to the SPIDER (Silicon PIe DEtectoR). A set of reduced E2, E3, and M1 matrix elements was extracted from the collected data using the gosia code, yielding 12 reduced transition probabilities between the low-spin states and the spectroscopic quadrupole moment of the 21+ state. The B(E2) values for transitions depopulating the 02+ state have been determined for the first time, allowing for the lifetime of this state to be deduced and, consequently, the ρ2(E0;02+→01+) monopole transition strength to be extracted. In addition, the B(E3;31−→01+) value has been determined for the first time in a Coulomb excitation experiment. The obtained results resolve the existing discrepancies between literature lifetimes and demonstrate that Zn66 cannot be described by using simple collective models. Therefore, new state-of-the-art beyond-mean-field and large-scale shell-model calculations were performed in order to interpret the structure of this nucleus. Both the experimental and theoretical results suggest that the triaxial degree of freedom has an important impact on electromagnetic properties of Zn66, while the unique features of the 02+ state indicate its distinct and rather isolated structure.

Applications of Rutherford backscattering analysis methods to nuclear physics experiments

Target properties such as thickness and composition are essential ingredients in nuclear physics experiments, therefore, dedicated analyses to evaluate them before and/or after the measurement are often performed. In some experimental techniques, the exploited detectors allow for the evaluation of these properties on-line, i.e. directly during the experiment. In this paper, we report on the use of analysis methods coming from the Rutherford backscattering spectroscopy technique to obtain on-line information on the target used in a nuclear physics experiment. This measurement was performed at INFN LNL by exploiting the low-energy Coulomb excitation technique. The results have been compared with an independent Rutherford backscattering spectroscopy analysis of the same target performed at INFN LABEC in Florence.

SPIDER: A Silicon PIe DEtectoR for low-energy Coulomb-excitation measurements

SPIDER is a new array of segmented silicon detectors for low-energy Coulomb-excitation experiments, designed as an ancillary device for modern γ-ray spectrometers such as GALILEO and AGATA. Currently, it is used at the INFN Legnaro National Laboratories (LNL) for experiments with the GALILEO γ-ray array and the stable beams provided by the Tandem-XTU, ALPI-PIAVE accelerator complex. In this paper, a detailed description of SPIDER is presented, as well as the outcomes from the first in-beam experiment of the array coupled with GALILEO. In particular, radiation damage and cross-talk/charge-sharing effects induced by energetic heavy ions in SPIDER are investigated and the capabilities of the array to perform on-line Rutherford back-scattering analysis of the exploited target are presented. The material reported here can be used to plan future experiments with the GALILEO-SPIDER setup with the presently available stable beams at LNL and paves the way for future experimental campaigns with the radioactive beams provided in the near future by the SPES facility at LNL.

Coulomb excitation studies at LNL with the SPIDER-GALILEO set-up

Low-energy Coulomb excitation is one of the simplest and most known tools to study the nuclear shape; for this reason it is nowadays widely used at radioactive beam facilities. The Selective Production of Exotic Species (SPES) facility, for the acceleration of radioactive beams will soon provide the first exotic beams at the Laboratori Nazionali di Legnaro (LNL) in Italy. To this end a new particle detector (Silicon PIe DEtectoR) to be used for Coulomb excitation studies has been installed at LNL. SPIDER has been coupled to the GALILEO array of germanium detectors, and a number of experiments have been already successfully performed. This paves the way for future experiments with the radioactive beams provided by the SPES facility.

Shape coexistence in 94Zr studied via Coulomb excitation

In recent years, a number of both theoretical and experimental investigations have been performed focusing on the zirconium isotopic chain. In particular, state-of-the-art Monte Carlo shell-model calculations predict shape coexistence in these isotopes. In this context, the 94Zr nucleus, which is believed to possess a nearly spherical ground state, is particularly interesting since the purported deformed structure is basedon the low-lying 02+ state, making it amenable for detailed study. In order to provide definitive conclusionson the shapes of the low-lying states, two complementary experiments to study 94Zr by means of low-energy Coulomb excitation were performed. This data will allow the quadrupole moments of the 21,2+ levels to be extracted as well as for the deformation parameters of the 01,2+ states to be determined and, thus, definitive conclusions to be drawn on the role of shape coexistence in this nucleus for the first time. The first experiment was performed at the INFN Legnaro National Laboratory with the GALILEO-SPIDER setup, which, for the first time, was coupled with 6 lanthanum bromide scintillators (LaBr3:Ce) in order to maximize the γ-ray detection effciency. The second experiment was performed at the Maier-Leibnitz Laboratory (MLL) in Munich and used a Q3D magnetic spectrograph to detect the scattered 12C ions following Coulomb excitation of 94Zr targets.

Localizing the Shape Transition in Neutron-Deficient Selenium.

Neutron-deficient selenium isotopes are thought to undergo a rapid shape change from a prolate deformation near the line of beta stability towards oblate deformation around the line of N=Z. The point at which this shape change occurs is unknown, with inconsistent predictions from available theoretical models. A common feature in the models is the delicate nature of the point of transition, with the introduction of even a modest spin to the system sufficient to change the ordering of the prolate and oblate configurations. We present a measurement of the quadrupole moment of the first-excited state in radioactive ^{72}Se-a potential point of transition-by safe Coulomb excitation. This is the first low-energy Coulomb excitation to be performed with a rare-isotope beam at the reaccelerated beam facility at the National Superconducting Cyclotron Laboratory. By demonstrating a negative spectroscopic quadrupole moment for the first-excited 2^{+} state, it is found that any low-spin shape change in neutron-deficient selenium does not occur until ^{70}Se.

Electromagnetic Properties of $^{45}$Sc Studied by Low-energy Coulomb Excitation

Electromagnetic Properties of $^{45}$Sc Studied by Low-energy Coulomb Excitation

Nuclear shapes studied with low-energy Coulomb excitation

Coulomb excitation is one of the rare methods available to obtain information on static electromagnetic moments of short-lived excited nuclear states, including collective non-yrast levels. It is thus an ideal tool to study shape coexistence and shape evolution throughout the nuclear chart. Historically, these experiments were limited to stable isotopes, however the advent of new facilities, providing intense beams of short-lived radioactive species, has opened the possibility to apply this powerful technique to a much wider range of nuclei. Here, we present some recent complex Coulomb-excitation studies and use the example of superdeformed states in 42Ca to demonstrate the sensitivity of the method to second-order effects such as relative signs of electromagnetic matrix elements and quadrupole moments.

JANUS — A setup for low-energy Coulomb excitation at ReA3

A new experimental setup for low-energy Coulomb excitation experiments was constructed in a collaboration between the National Superconducting Cyclotron Laboratory (NSCL), Lawrence Livermore National Laboratory (LLNL), and the University of Rochester and was commissioned at the general purpose beam line of NSCL’s ReA3 reaccelerator facility. The so-called JANUS setup combines γ-ray detection with the Segmented Ge Array (SeGA) and scattered particle detection using a pair of segmented double-sided Si detectors (Bambino 2). The low-energy Coulomb excitation program that JANUS enables will complement intermediate-energy Coulomb excitation studies that have long been performed at NSCL by providing access to observables that quantify collectivity beyond the first excited state, including the sign and magnitude of excited-state quadrupole moments. In this work, the setup and its performance will be described based on the commissioning run that used stable 78Kr impinging onto a 1.09 mg/cm2208Pb target at a beam energy of 3.9 MeV/u.

Doppler-shift attenuation lifetime measurement of the Ar3621+ level

At TRIUMF, the TIGRESS Integrated Plunger device and its suite of ancillary detector systems have been implemented for charged-particle tagging and light-ion identification in coincidence with γ-ray spectroscopy for Doppler-shift lifetime studies and low-energy Coulomb excitation measurements. As a test of the device, the lifetime of the first 2+ excited state in Ar36 was measured from the γ-ray line shape of the 21+→0g.s.+ transition using the Doppler-shift attenuation technique following Coulomb excitation. The line-shape signatures, vital for precision lifetime measurements, were significantly improved by enhanced reaction-channel selectivity using a complementary approach of kinematic gating and digital rise-time discrimination of recoiling charged particles in a silicon PIN diode array. The lifetime was determined by comparisons between the data and simulated line shapes generated using our TIGRESS Coulomb excitation code as an input to the Lindhard method, which was then extended and included as a class in geant4. The model-independent lifetime result of 490±50 fs corresponds to a reduced quadrupole transition strength of B(E2;21+→0g.s.+)=56±6e2fm4 and agrees well with previous intermediate energy Coulomb excitation measurements, thereby resolving reported discrepancies in the 21+ level lifetime in this self-conjugate nucleus.5 MoreReceived 13 April 2017Revised 28 June 2017DOI:https://doi.org/10.1103/PhysRevC.96.024305©2017 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasElectromagnetic transitionsLifetimes & widthsNuclear structure & decaysProperties20 ≤ A ≤ 38TechniquesRadiation detectorsShell modelNuclear Physics

Shape coexistence in neutron-rich strontium isotopes at N = 60

The structure of neutron-rich Sr nuclei was investigated by low-energy Coulomb excitation of radioactive beams at the REX-ISOLDE facility, CERN, with the MINIBALL spectrometer. The results support the scenario of a shape transition at N = 60, giving rise to the coexistence of a highly deformed prolate and a spherical configuration in 98Sr with low configuration mixing. They are discussed in the context of systematics of quadrupole moments and transition probabilities in the N = 60 region.

First measurement with a new setup for low-energy Coulomb excitation studies at INFN LNL

A new segmented particle detector, SPIDER, has been designed to be used as an ancillary device with the GALILEO γ-ray spectrometer, as well as with other multi-detector γ-ray arrays that will be available at LNL in the future (e.g. AGATA). To commission the SPIDER-GALILEO experimental setup, a multi-step Coulomb excitation experiment was carried out with a 240 MeV beam of 66Zn produced by the Tandem-XTU accelerator at INFN Laboratori Nazionali di Legnaro. The measured particle and γ-ray spectra are compared with the results of detailed GEANT4 simulations which used the Coulomb excitation cross sections, estimated with the computer code GOSIA, as an input. The preliminary results indicate that precise transition probabilities will be obtained which are essential for solving discrepancies reported in the literature for this nucleus.

Low-energy Coulomb excitation of Sr96,98 beams

The structure of neutron-rich 96,98Sr nuclei was investigated by low-energy safe Coulomb excitation of radioactive beams at the REX-ISOLDE facility, CERN, with the MINIBALL spectrometer. A rich set of transitional and diagonal E2 matrix elements, including those for non-yrast structures, has been extracted from the differential Coulomb-excitation cross sections. The results support the scenario of a shape transition at N = 60, giving rise to the coexistence of a highly deformed prolate and a spherical configuration in 98Sr, and are compared to predictions from several theoretical calculations. The experimental data suggest a significant contribution of the triaxal degree of freedom in the ground state of both isotopes. In addition, experimental information on low-lying states in 98Rb has been obtained.

Superdeformed and Triaxial States in ^{42}Ca.

Shape parameters of a weakly deformed ground-state band and highly deformed slightly triaxial sideband in ^{42}Ca were determined from E2 matrix elements measured in the first low-energy Coulomb excitation experiment performed with AGATA. The picture of two coexisting structures is well reproduced by new state-of-the-art large-scale shell model and beyond-mean-field calculations. Experimental evidence for superdeformation of the band built on 0_{2}^{+} has been obtained and the role of triaxiality in the A∼40 mass region is discussed. Furthermore, the potential of Coulomb excitation as a tool to study superdeformation has been demonstrated for the first time.

Structure of low-lying states inSm140studied by Coulomb excitation

The electromagnetic structure of $^{140}$Sm was studied in a low-energy Coulomb excitation experiment with a radioactive ion beam from the REX-ISOLDE facility at CERN. The $2^+$ and $4^+$ states of the ground-state band and a second $2^+$ state were populated by multi-step excitation. The analysis of the differential Coulomb excitation cross sections yielded reduced transition probabilities between all observed states and the spectroscopic quadrupole moment for the $2_1^+$ state. The experimental results are compared to large-scale shell model calculations and beyond-mean-field calculations based on the Gogny D1S interaction with a five-dimensional collective Hamiltonian formalism. Simpler geometric and algebraic models are also employed to interpret the experimental data. The results indicate that $^{140}$Sm shows considerable $\gamma$ softness, but in contrast to earlier speculation no signs of shape coexistence at low excitation energy. This work sheds more light on the onset of deformation and collectivity in this mass region.

Coulomb excitation studies of shape coexistence in atomic nuclei

Low-energy Coulomb excitation provides a well-understood means of exciting atomic nuclei and allows measuring electromagnetic moments that can be directly related to the nuclear shape. The availability of radioactive ion beams (RIBs) at energies near the Coulomb barrier has made it possible to study shape coexistence in a variety of short-lived exotic nuclei. This review presents a short overview of the methods related to multi-step Coulomb excitation experiments, followed by a discussion of several examples. The focus is on two mass regions where recent Coulomb excitation experiments have contributed to the quantitative understanding of shape coexistence: nuclei with mass near the N = Z line and nuclei with near neutron number N = 60. Experimental results are summarized and their significance for understanding shape coexistence is discussed. Experimental observables such as quadrupole moments and electromagnetic transition strengths represent furthermore important benchmarks for advancing theoretical nuclear structure models. With several new RIB facilities planned and under construction, Coulomb excitation will remain to be an important tool to extend the studies of nuclear shapes toward more exotic systems, and to obtain a more comprehensive and quantitative understanding of shape coexistence.

Study of Octupole Collectivity in $^{146}$Nd and $^{148}$Sm Using the New Coulomb Excitation Set-up at ALTO

For certain combinations of protons and neutrons in atomic nuclei, a rise of a reflection asymmetry is expected. Experimental E3 strengths, which as a function of the neutron number peak at around N approximate to 8 8 and N approximate to 1 3 4, indicate enhanced octupole correlations as predicted by theory. Low-energy Coulomb excitation is a highly successful method for establishing the evolution of nuclear shapes, through the measurement of cross sections, to populate excited states that can be directly related to the static and dynamic moments of the charge distribution of the nucleus. A Coulomb excitation experiment at the ALTO facility, Orsay was performed recently to study collective properties of Nd-146 and Sm-148. In particular, the strengths of the and matrix elements will provide a clear distinction between octupole vibration and rigid deformation.

Low-energy Coulomb excitation of 62Fe and 62Mn following in-beam decay of 62Mn

Sub-barrier Coulomb-excitation was performed on a mixed beam of $^{62}$Mn and $^{62}$Fe, following in-trap $\beta^{-}$ decay of $^{62}$Mn at REX-ISOLDE, CERN. The trapping and charge breeding times were varied in order to alter the composition of the beam, which was measured by means of an ionisation chamber at the zero-angle position of the Miniball array. A new transition was observed at 418~keV, which has been tentatively associated to a $(2^{+},3^{+})\rightarrow1^{+}_{g.s.}$ transition. This fixes the relative positions of the $\beta$-decaying $4^{+}$ and $1^{+}$ states in $^{62}$Mn for the first time. Population of the $2^{+}_{1}$ state was observed in $^{62}$Fe and the cross-section determined by normalisation to the $^{109}$Ag target excitation, confirming the $B(E2)$ value measured in recoil-distance lifetime experiments.