Local Tropopause Research Articles

Distribution of cross-tropopause convection within the Asian monsoon region from May through October 2017

Abstract. We constructed a database of cross-tropopause convection in the Asian monsoon region for the months of May through October of 2017 using overshooting tops (OTs), deep convective features that penetrate the local cirrus anvil layer and the local tropopause, with Meteosat-8 geostationary satellite detections. The database of 40 918 OTs represents a hemispheric record of convection covering the study domain from 10∘ S to 55∘ N and from 40 to 115∘ E. With this database, we analyzed the geographic, monthly, and altitude distribution of this convection and compared it to the convective distributions represented by satellite observations of outgoing longwave radiation (OLR) and precipitation. We find that cross-tropopause convection is most active during the months of May through August (with daily averages of these months above 300 OTs per day) and declines through September and October. Most of this convection occurs within Northern India and Southern India, the Bay of Bengal, and the Indian Ocean regions, which together account for 75.1 % of all OTs. We further identify distinct, differing seasonal trends within the study subregions. For the Northern India, Southern India, and Bay of Bengal regions, the distribution of OTs follows the development of the Asian monsoon, with its north–south movement across the study period. This work demonstrates that when evaluating the effects of convection on lower stratospheric composition over the Asian monsoon region, it is important to consider the impact of cross-tropopause convection specifically, as well as the contributions from both land-based and oceanic regions due to the significant geographic and monthly variation in convective activity.

Comparison of inorganic chlorine in the Antarctic and Arctic lowermost stratosphere by separate late winter aircraft measurements

Abstract. Stratospheric inorganic chlorine (Cly) is predominantly released from long-lived chlorinated source gases and, to a small extent, very short-lived chlorinated substances. Cly includes the reservoir species (HCl and ClONO2) and active chlorine species (i.e., ClOx). The active chlorine species drive catalytic cycles that deplete ozone in the polar winter stratosphere. This work presents calculations of inorganic chlorine (Cly) derived from chlorinated source gas measurements on board the High Altitude and Long Range Research Aircraft (HALO) during the Southern Hemisphere Transport, Dynamic and Chemistry (SouthTRAC) campaign in austral late winter and early spring 2019. Results are compared to Cly in the Northern Hemisphere derived from measurements of the POLSTRACC-GW-LCYCLE-SALSA (PGS) campaign in the Arctic winter of 2015/2016. A scaled correlation was used for PGS data, since not all source gases were measured. Using the SouthTRAC data, Cly from a scaled correlation was compared to directly determined Cly and agreed well. An air mass classification based on in situ N2O measurements allocates the measurements to the vortex, the vortex boundary region, and midlatitudes. Although the Antarctic vortex was weakened in 2019 compared to previous years, Cly reached 1687±19 ppt at 385 K; therefore, up to around 50 % of total chlorine was found in inorganic form inside the Antarctic vortex, whereas only 15 % of total chlorine was found in inorganic form in the southern midlatitudes. In contrast, only 40 % of total chlorine was found in inorganic form in the Arctic vortex during PGS, and roughly 20 % was found in inorganic form in the northern midlatitudes. Differences inside the two vortices reach as much as 540 ppt, with more Cly in the Antarctic vortex in 2019 than in the Arctic vortex in 2016 (at comparable distance to the local tropopause). To our knowledge, this is the first comparison of inorganic chlorine within the Antarctic and Arctic polar vortices. Based on the results of these two campaigns, the differences in Cly inside the two vortices are substantial and larger than the inter-annual variations previously reported for the Antarctic.

CALIPSO Aerosol-Typing Scheme Misclassified Stratospheric Fire Smoke: Case Study From the 2019 Siberian Wildfire Season

In August 2019, a 4-km thick wildfire smoke layer was observed in the lower stratosphere over Leipzig, Germany, with a ground-based multiwavelength Raman lidar. The smoke was identified by the smoke-specific spectral dependence of the extinction-to-backscatter ratio (lidar ratio) measured with the Raman lidar. The spaceborne CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) lidar CALIOP (Cloud–Aerosol Lidar with Orthogonal Polarization) detected the smoke and classified it as sulfate aerosol layer (originating from the Raikoke volcanic eruption). In this article, we discuss the reason for this misclassification. Two major sources for stratospheric air pollution were active in the summer of 2019 and complicated the CALIPSO aerosol typing effort. Besides intense forest fires at mid and high northern latitudes, the Raikoke volcano erupted in the Kuril Islands. We present two cases observed at Leipzig, one from July 2019 and one from August 2019. In July, pure volcanic sulfate aerosol layers were found in the lower stratosphere, while in August, wildfire smoke dominated in the height range up to 4–5 km above the local tropopause. In both cases, the CALIPSO aerosol typing scheme classified the layers as sulfate aerosol layers. The aerosol identification algorithm assumes non-spherical smoke particles in the stratosphere as consequence of fast lifting by pyrocumulonimbus convection. However, we hypothesize (based on presented simulations) that the smoke ascended as a results of self-lifting and reached the tropopause within 2–7 days after emission and finally entered the lower stratosphere as aged spherical smoke particles. These sphercial particles were then classified as liquid sulfate particles by the CALIPSO data analysis scheme. We also present a successful case of smoke identification by the CALIPSO retrieval method.

Quantifying the Source Term and Uniqueness of the August 12, 2017 Pacific Northwest PyroCb Event

AbstractA pyrocumulonimbus (pyroCb) firestorm event known as the Pacific Northwest Event (PNE), on August 12, 2017, is examined with a focus on newly reported details of the pyroconvective injections, transport pathway, and young‐plume altitude. Because PNE and a subsequent pyroCb event in Australia have been compared to classic stratospheric volcanic plumes, a prime motivation for this work was to exhaustively characterize the beginning of PNE, and to show how it compared to major stratospheric plumes from prior events. We find and report direct evidence that PNE pyroconvection involved seven discrete storms, at least two of which injected a plume to at least 13.7 km, up to 2.5 km above the local tropopause. The morning after, stratospheric smoke was observed above the tropopause to altitudes as great as 16 km. We also quantify for the first time that PNE was preceded by a pyroCb injection one day earlier, generating a plume noteworthy on its own but overwhelmed by the PNE smoke. Our comparison of PNE with five earlier pyroCb events reveals that PNE was not distinctive with respect to its injection and nascent plume height. However, it did produce the greatest known ultraviolet absorbing aerosol index and plume longevity as of 2017.

Lower-stratospheric aerosol measurements in eastward-shedding vortices over Japan from the Asian summer monsoon anticyclone during the summer of 2018

Abstract. Eastward air-mass transport from the Asian summer monsoon (ASM) anticyclone in the upper troposphere and lower stratosphere (UTLS) often involves eastward-shedding vortices, which can cover most of the Japanese archipelago. We investigated the aerosol characteristics of these vortices by analysing data from two lidar systems in Japan, at Tsukuba (36.1∘ N, 140.1∘ E) and Fukuoka (33.55∘ N, 130.36∘ E), during the summer of 2018. We observed several events with enhanced particle signals at Tsukuba at 15.5–18 km of altitude (at or above the local tropopause) during August–September 2018, with a backscattering ratio of ∼ 1.10 and particle depolarization of ∼ 5 % (i.e. not spherical, but more spherical than ice crystals). These particle characteristics may be consistent with those of solid aerosol particles, such as ammonium nitrate. Each event had a timescale of a few days. During the same study period, we also observed similar enhanced particle signals in the lower stratosphere at Fukuoka. The upper troposphere is often covered by cirrus clouds at both lidar sites. Backward trajectory calculations for these sites for days with enhanced particle signals in the lower stratosphere and days without indicate that the former air masses originated within the ASM anticyclone and the latter more from edge regions. Reanalysis carbon monoxide and satellite water vapour data indicate that eastward-shedding vortices were involved in the observed aerosol enhancements. Satellite aerosol data confirm that the period and latitudinal region were free from the direct influence of documented volcanic eruptions and high-latitude forest fires. Our results indicate that the Asian tropopause aerosol layer (ATAL) over the ASM region extends east towards Japan in association with the eastward-shedding vortices and that lidar systems in Japan can detect at least the lower-stratospheric portion of the ATAL during periods when the lower stratosphere is undisturbed by volcanic eruptions and forest fires. The upper-tropospheric portion of the ATAL is either depleted by tropospheric processes (convection and wet scavenging) during eastward transport or is obscured by much stronger cirrus cloud signals.

Upward transport into and within the Asian monsoon anticyclone as inferred from StratoClim trace gas observations

Abstract. Every year during the Asian summer monsoon season from about mid-June to early September, a stable anticyclonic circulation system forms over the Himalayas. This Asian summer monsoon (ASM) anticyclone has been shown to promote transport of air into the stratosphere from the Asian troposphere, which contains large amounts of anthropogenic pollutants. Essential details of Asian monsoon transport, such as the exact timescales of vertical transport, the role of convection in cross-tropopause exchange, and the main location and level of export from the confined anticyclone to the stratosphere are still not fully resolved. Recent airborne observations from campaigns near the ASM anticyclone edge and centre in 2016 and 2017, respectively, show a steady decrease in carbon monoxide (CO) and increase in ozone (O3) with height starting from tropospheric values of around 100 ppb CO and 30–50 ppb O3 at about 365 K potential temperature. CO mixing ratios reach stratospheric background values below ∼25 ppb at about 420 K and do not show a significant vertical gradient at higher levels, while ozone continues to increase throughout the altitude range of the aircraft measurements. Nitrous oxide (N2O) remains at or only marginally below its 2017 tropospheric mixing ratio of 333 ppb up to about 400 K, which is above the local tropopause. A decline in N2O mixing ratios that indicates a significant contribution of stratospheric air is only visible above this level. Based on our observations, we draw the following picture of vertical transport and confinement in the ASM anticyclone: rapid convective uplift transports air to near 16 km in altitude, corresponding to potential temperatures up to about 370 K. Although this main convective outflow layer extends above the level of zero radiative heating (LZRH), our observations of CO concentration show little to no evidence of convection actually penetrating the tropopause. Rather, further ascent occurs more slowly, consistent with isentropic vertical velocities of 0.7–1.5 K d−1. For the key tracers (CO, O3, and N2O) in our study, none of which are subject to microphysical processes, neither the lapse rate tropopause (LRT) around 380 K nor the cold point tropopause (CPT) around 390 K marks a strong discontinuity in their profiles. Up to about 20 to 35 K above the LRT, isolation of air inside the ASM anticyclone prevents significant in-mixing of stratospheric air (throughout this text, the term in-mixing refers specifically to mixing processes that introduce stratospheric air into the predominantly tropospheric inner anticyclone). The observed changes in CO and O3 likely result from in situ chemical processing. Above about 420 K, mixing processes become more significant and the air inside the anticyclone is exported vertically and horizontally into the surrounding stratosphere.

Assessment of Observational Evidence for Direct Convective Hydration of the Lower Stratosphere

AbstractIn situ and remote sensing observations of water vapor are analyzed to assess the evidence for direct convective hydration of the lower stratosphere. We have examined several hundred balloon‐borne and airborne in situ measurements of lower stratospheric humidity in the tropics and northern midlatitudes. We find that the tropical lower stratospheric H2O enhancements above the background occur quite infrequently, and the height of the enhancements is within about 1 km of the cold‐point tropopause. Following Schwartz et al. (2013, https://doi.org/10.1002/grl.50421), we examine the anomalously high (above 8 ppmv) water vapor mixing ratios retrieved by the Aura Microwave Limb Sounder (MLS) at 100‐ and 82‐hPa pressure levels, and we determine their vertical location relative to the local tropopause based on both Global Forecast System (GFS) operational analysis and the ERA5 reanalysis temperature data. We find that essentially all of the >8‐ppmv MLS water vapor measurements over the extratropical North American monsoon region are above the relatively low lapse‐rate tropopause in the region, and most are above the local cold‐point tropopause. Over the Asian monsoon region, most (80/90%) of the high H2O values occur below the relatively high‐altitude local lapse‐rate/cold‐point tropopause. Anomalously high MLS water vapor retrievals at 100 and 82 hPa almost never occur in the deep tropics. We show that this result is consistent with the in situ observations given the broad vertical averaging kernel of the MLS measurement. The available evidence suggests that direct hydration of the lower stratosphere is important over North America during the monsoon season but likely has limited impact in the tropics.

Observational evidence of moistening the lowermost stratosphere via isentropic mixing across the subtropical jet

Abstract. Isentropic mixing across and above the subtropical jet is a significant mechanism for stratosphere–troposphere exchange. In this work, we show new observational evidence on the role of this process in moistening the lowermost stratosphere. The new measurement, obtained from the Spatial Heterodyne Observations of Water (SHOW) instrument during a demonstration flight on the NASA's ER-2 high-altitude research aircraft, captured an event of poleward water vapour transport, including a fine-scale (vertically <∼1 km) moist filament above the local tropopause in a high-spatial-resolution two-dimensional cross section of the water vapour distribution. Analysis of these measurements combined with ERA5 reanalysis data reveals that this poleward mixing of air with enhanced water vapour occurred in the region of a double tropopause following a large Rossby wave-breaking event. These new observations highlight the importance of high-resolution measurements in resolving processes that are important to the lowermost-stratosphere water vapour budget.

Estimate of Turbulent Energy Dissipation Rate From the VHF Radar and Radiosonde Observations in the Antarctic

AbstractThis study estimated the turbulent kinetic energy dissipation rates (TKEDRs) from 1‐year observations of the Program of the Antarctic Syowa Mesosphere‐Stratosphere‐Troposphere/Incoherent Scatter radar (PANSY radar) from October 2015 to September 2016 and compared the results with estimates from radiosonde measurements based on Thorpe's method. The radar‐based estimates showed that the TKEDR at Syowa Station was on the order of 10−5–10−3 m2/s3 in the altitude range of 1.5–19 km. Taking the proportional constant for Thorpe's method (the ratio of the Thorpe scale to Ozmidov scale) as unity, the radiosonde‐based measurements show values of TKEDR larger than radar‐based estimates by a factor of 2–5. The difference in the TKEDR between radiosonde‐ and radar‐based estimates is larger in the middle and upper troposphere than in the stratosphere. According to previous observational and numerical studies, Thorpe's method tends to overestimate the TKEDR for deep overturning layers. It is confirmed that the depth of the overturning layer is negatively correlated with the difference between radiosonde‐ and radar‐based estimates. The seasonal variation was also examined. An analysis using the distance from the local tropopause level showed that the local maximum in the TKEDR around the tropopause is particularly clear in austral summer. This is likely connected to the seasonality in the gravity wave activity in the Antarctic stratosphere.

Extreme levels of Canadian wildfire smoke in the stratosphere over central Europe on 21–22 August 2017

Abstract. Light extinction coefficients of 500 Mm−1, about 20 times higher than after the Pinatubo volcanic eruptions in 1991, were observed by European Aerosol Research Lidar Network (EARLINET) lidars in the stratosphere over central Europe on 21–22 August 2017. Pronounced smoke layers with a 1–2 km vertical extent were found 2–5 km above the local tropopause. Optically dense layers of Canadian wildfire smoke reached central Europe 10 days after their injection into the upper troposphere and lower stratosphere which was caused by rather strong pyrocumulonimbus activity over western Canada. The smoke-related aerosol optical thickness (AOT) identified by lidar was close to 1.0 at 532 nm over Leipzig during the noon hours on 22 August 2017. Smoke particles were found throughout the free troposphere (AOT of 0.3) and in the pronounced 2 km thick stratospheric smoke layer at an altitude of 14–16 km (AOT of 0.6). The lidar observations indicated peak mass concentrations of 70–100 µg m−3 in the stratosphere. In addition to the lidar profiles, we analyzed Moderate Resolution Imaging Spectroradiometer (MODIS) fire radiative power (FRP) over Canada, and the distribution of MODIS AOT and Ozone Monitoring Instrument (OMI) aerosol index across the North Atlantic. These instruments showed a similar pattern and a clear link between the western Canadian fires and the aerosol load over Europe. In this paper, we also present Aerosol Robotic Network (AERONET) sun photometer observations, compare photometer and lidar-derived AOT, and discuss an obvious bias (the smoke AOT is too low) in the photometer observations. Finally, we compare the strength of this record-breaking smoke event (in terms of the particle extinction coefficient and AOT) with major and moderate volcanic events observed over the northern midlatitudes.

Tropospheric ozone seasonal and long-term variability as seen by lidar and surface measurements at the JPL-Table Mountain Facility, California

Abstract. A combined surface and tropospheric ozone climatology and interannual variability study was performed for the first time using co-located ozone photometer measurements (2013–2015) and tropospheric ozone differential absorption lidar measurements (2000–2015) at the Jet Propulsion Laboratory Table Mountain Facility (TMF; elev. 2285 m), in California. The surface time series were investigated both in terms of seasonal and diurnal variability. The observed surface ozone is typical of high-elevation remote sites, with small amplitude of the seasonal and diurnal cycles, and high ozone values, compared to neighboring lower altitude stations representative of urban boundary layer conditions. The ozone mixing ratio ranges from 45 ppbv in the winter morning hours to 65 ppbv in the spring and summer afternoon hours. At the time of the lidar measurements (early night), the seasonal cycle observed at the surface is similar to that observed by lidar between 3.5 and 9 km. Above 9 km, the local tropopause height variation with time and season impacts significantly the ozone lidar observations. The frequent tropopause folds found in the vicinity of TMF (27 % of the time, mostly in winter and spring) produce a dual-peak vertical structure in ozone within the fold layer, characterized by higher-than-average values in the bottom half of the fold (12–14 km), and lower-than-averaged values in the top half of the fold (14–18 km). This structure is consistent with the expected origin of the air parcels within the fold, i.e., mid-latitude stratospheric air folding down below the upper tropospheric sub-tropical air. The influence of the tropopause folds extends down to 5 km, increasing the ozone content in the troposphere. No significant signature of interannual variability could be observed on the 2000–2015 de-seasonalized lidar time series, with only a statistically non-significant positive anomaly during the years 2003–2007. Our trend analysis reveals however an overall statistically significant positive trend of 0.3 ppbv year−1 (0.6 %) in the free troposphere (7–10 km) for the period 2000–2015. A classification of the air parcels sampled by lidar was made at 1 km intervals between 5 and 14 km altitude, using 12-day backward trajectories (HYSPLIT, Hybrid Single Particle Lagrangian Integrated Trajectory Model). Our classification revealed the influence of the Pacific Ocean, with air parcels of low ozone content (43–60 ppbv below 9 km), and significant influence of the stratosphere leading to ozone values of 57–83 ppbv down to 8–9 km. In summer, enhanced ozone values (76 ppbv at 9 km) were found in air parcels originating from Central America, probably due to the enhanced thunderstorm activity during the North American Monsoon. Influence from Asia was observed throughout the year, with more frequent episodes during spring, associated with ozone values from 53 to 63 ppbv at 9 km.

Anomalies of Northern Hemisphere ozone associated with a tropopause‐lower stratosphere teleconnection during summer

ABSTRACTUsing the ozone data set from the satellite observations and the atmospheric reanalysis data sets during 1979–2005, we examine the variability of a tropopause‐lower stratosphere (TS) teleconnection a and its relationship with the ozone change over the Northern Hemisphere (NH) during summer. The TS teleconnection has an approximate opposite phase to that in the upper‐troposphere Asian‐Pacific Oscillation (APO), and the TS teleconnection index (the TS index) is also related well to the APO index. Corresponding to a higher TS index, the ozone generally decreases in the NH mid‐high latitudes (near 40°N and the Far East of Russia). This link between the TS teleconnection and the ozone is physically supported by the changes of the background atmospheric circulation. When the TS index is higher, the decrease of the ozone is closely associated with an increase of the local tropopause height. The upward and downward motion variations in the upper troposphere and the lower stratosphere in the east and west parts of the anomalous anticyclones associated with the TS index strengthen the exchanges of the ozone between the troposphere and the lower stratosphere, which may cause a decrease of the ozone. The horizontal advection of the ozone could also contribute to the ozone decreases over these regions.

A novel tropopause-related climatology of ozone profiles

Abstract. A new ozone climatology, based on ozonesonde and satellite measurements, spanning the altitude region between the earth's surface and ~60 km is presented (TpO3 climatology). This climatology is novel in that the ozone profiles are categorized according to calendar month, latitude and local tropopause heights. Compared to the standard latitude–month categorization, this presentation improves the representativeness of the ozone climatology in the upper troposphere and the lower stratosphere (UTLS). The probability distribution of tropopause heights in each latitude–month bin provides additional climatological information and allows transforming/comparing the TpO3 climatology to a standard climatology of zonal mean ozone profiles. The TpO3 climatology is based on high-vertical-resolution measurements of ozone from the satellite-based Stratospheric Aerosol and Gas Experiment II (in 1984 to 2005) and from balloon-borne ozonesondes from 1980 to 2006. The main benefits of the TpO3 climatology are reduced standard deviations on climatological ozone profiles in the UTLS, partial characterization of longitudinal variability, and characterization of ozone profiles in the presence of double tropopauses. The first successful application of the TpO3 climatology as a priori in ozone profile retrievals from Ozone Monitoring Instrument on board the Earth Observing System (EOS) Aura satellite shows an improvement of ozone precision in UTLS of up to 10% compared with the use of conventional climatologies. In addition to being advantageous for use as a priori in satellite retrieval algorithms, the TpO3 climatology might be also useful for validating the representation of ozone in climate model simulations.

Simultaneous occurrence of polar stratospheric clouds and upper-tropospheric clouds caused by blocking anticyclones in the Southern Hemisphere

Abstract. Previous studies have reported that polar stratospheric clouds (PSCs) are frequently observed simultaneously with upper-tropospheric clouds (UCs) in the Southern Hemisphere. However, it has not yet been examined whether the UCs that simultaneously occur with PSCs are actually located below the height of the tropopause, which is modified by tropospheric disturbances. Furthermore, the mechanism of this simultaneous occurrence has not yet been clarified. This study statistically examines the simultaneous appearance of PSCs and UCs using the Cloud-Aerosol Lidar and Pathfinder Satellite Observation (CALIPSO) for the five austral winters of 2007–2011. From correlation analyses and statistical dependence tests, it is shown that the simultaneous occurrence frequencies of clouds with an altitude range of 15–25 km and 9–11 km are significant. The analyses based on tropopause-relative altitude suggest that the occurrence frequency of clouds at altitudes higher than 6 km above the local tropopause (i.e., PSCs) is significantly correlated with that of clouds around and slightly above the tropopause. These results indicate that the UCs observed simultaneously with PSCs reported in previous case studies are likely located around and slightly above the tropopause rather than in the troposphere. It is also shown that the simultaneous occurrence of PSCs and UCs is frequently associated with blocking highs that have large horizontal scales (several thousand kilometers) and tall structure (up to a height of ~15 km). The longitudinal variation of blocking high frequency accords well with that of the simultaneous occurrence frequency of PSCs and UCs. This fact suggests that the blocking highs provide a preferable condition for such simultaneous occurrences. Moreover, the composition of PSCs is investigated as a function of relative longitude of the anticyclones including blocking highs. It was discovered that relatively high proportions of STS (super-cooled ternary solutions), Ice, and Mix2 (mixture of nitric acid trihydrate and STS) types are distributed towards the windward, near, and leeward side of anticyclones in westerly background flows, respectively.

On the temporal and spatial structure of troposphere-to-stratosphere transport in the lowermost stratosphere over the Asian monsoon region during boreal summer

This study produced a novel characterization of the troposphere-to-stratosphere transport (TST) over the Asian monsoon region during boreal summer, using a comprehensive analysis of 60-day backward trajectories initialized in the stratosphere. The trajectory datasets were derived from the high-resolution Lagrangian particle dispersion model (FLEXPART) simulation driven by the wind fields acquired from the National Center for Environmental Prediction (NCEP). The results indicate that the distribution of residence time (tTST) of tropopause-crossing trajectories in the lowermost stratosphere represents a horizontal signature of the Asian summer monsoon. Vertically, the distribution of tTST can be roughly separated into two layers: a consistent lower layer with tTST <5 days forming a narrow band, corresponding to a layer ∼3 km thick following the location of the tropopause, and an upper layer at a larger distance from the local tropopause. The maximum residence time was ∼20 days, especially within the Asian high anticyclone consistent with its confinement effects. In general, the overall geographical distribution of dehydration points was not coincident with the location of tropopause crossing. TST trajectories, which were initialized in the stratosphere, underwent their Lagrangian cold points mostly in the tropics and subtropics 1–4 days after the TST event; they were characterized by a wide range of temperature differences, with a mean value of 3–12 K. The vertical extent of the influence of tropospheric intrusion on the Asian monsoon region in the stratosphere exhibited a peak at ∼16.5–18.5 km, and the uppermost height was ∼21 km.

In-situ observation of Asian pollution transported into the Arctic lowermost stratosphere

Abstract. On a research flight on 10 July 2008, the German research aircraft Falcon sampled an air mass with unusually high carbon monoxide (CO), peroxyacetyl nitrate (PAN) and water vapour (H2O) mixing ratios in the Arctic lowermost stratosphere. The air mass was encountered twice at an altitude of 11.3 km, ~800 m above the dynamical tropopause. In-situ measurements of ozone, NO, and NOy indicate that this layer was a mixed air mass containing both air from the troposphere and stratosphere. Backward trajectory and Lagrangian particle dispersion model analysis suggest that the Falcon sampled the top of a polluted air mass originating from the coastal regions of East Asia. The anthropogenic pollution plume experienced strong up-lift in a warm conveyor belt (WCB) located over the Russian east-coast. Subsequently the Asian air mass was transported across the North Pole into the sampling area, elevating the local tropopause by up to ~3 km. Mixing with surrounding Arctic stratospheric air most likely took place during the horizontal transport when the tropospheric streamer was stretched into long and narrow filaments. The mechanism illustrated in this study possibly presents an important pathway to transport pollution into the polar tropopause region.

Effect that jet streams have on the vertical ozone distribution and characteristics of tropopause inversion layer in the far east region

The paper describes a lidar and presents the results of lidar sensing of the vertical ozone distribution (VOD); the lidar measurements are analyzed together with data from a network of meteorological stations situated along the 132° E meridian. VODs over Primorye and Japan in the winter period are compared. An analysis showed that an interrelation exists between the subtropical jet stream and the structures of VOD and tropopause inversion layer. Specifically, the region of the VOD local maximum above the tropopause is in the upper part of the tropopause inversion layer and the width of the maximum depends on the distance from the core of the subtropical jet stream. It is found that the local ozone minimum in the lower stratosphere corresponds to the local minimum of the squared Brunt-Vaisala frequency within this same altitude range in the winter season, when two tropopauses frequently overlap. It is conjectured that the local ozone maximum and tropopause inversion layer may be associated with mixing processes in the layer where stratospheric and tropospheric circulation cells come into contact near the core of the subtropical jet stream.

On the Wind and Turbulence in the Lower Atmosphere above Complex Terrain

Numerical modeling and studies of the wind fields at the junction of three continents: over the complex terrains of the South-east Europe, Asia Minor, Middle East, Caucasus and over the Black, Caspian and Medi-terranean seas have been carried out for the first time. Traveling synoptic scale vortex wave generation and subsequent evolution of orographic vortices are discovered. Wind fields, spatial distribution of the coefficients of subgrid scale horizontal and vertical turbulence and the Richardson number are calculated. It is shown that the local relief, atmospheric hydrothermodynamics and air-proof tropopause facilitate the generation of β-mesoscale vortex and turbulence amplification in the vicinity of the atmospheric boundary layer and tropopause. Also turbulence parameters distribution in the troposphere has the same nature as in the stratosphere and mesosphere: turbulence coefficients, stratification of the vertical profiles of the Richardson number, thickness of the turbulent and laminar layers.

Dynamic formation of extreme ozone minimum events over the Tibetan Plateau during northern winters 1987–2001

Wintertime extreme ozone minima in the total column ozone over the Tibetan Plateau (TP) between 1978 and 2001 are analyzed using observations from the Total Ozone Mapping Spectrometer (TOMS), Global Ozone Monitoring Experiment (GOME), and reanalysis data from both National Centers for Environmental Prediction and European Centre for Medium‐Range Weather Forecasts. Results show that total column ozone reduction in nine persistent (lasting for at least 2 days) and four transient events can be substantially attributed to ozone reduction in the upper troposphere and lower stratosphere region (below 25 km). This reduction is generally caused by uplift of the local tropopause and northward transport of tropical ozone‐poor air associated with an anomalous anticyclone in the upper troposphere. These anticyclonic anomalies are closely related to anomalous tropical deep convective heating, which is, however, not necessarily phase locked with the tropical Madden‐Julian Oscillation as in our earlier case study. Considering stratospheric processes, the selected 13 events can be combined into nine independent events. Moreover, five of the nine independent events, especially the persistent events, are coupled with contributions from stratospheric dynamics between 25 and 40 km, i.e., 15%–40% derived from GOME observations for events in November 1998, February 1999, and December 2001. On the basis of these events, stratospheric column ozone reduction over the TP region can be attributed to the dynamics (development and/or displacement) of the two main stratospheric systems, namely, the polar vortex and the Aleutian High. The effect of a “low‐ozone pocket” inside the Aleutian High on the total column ozone in East Asia requires further study.

Transport timescales and tracer properties in the extratropical UTLS

Abstract. A comprehensive evaluation of seasonal backward trajectories initialized in the northern hemisphere lowermost stratosphere (LMS) has been performed to investigate the factors that determine the temporal and spatial structure of troposphere-to-stratosphere-transport (TST) and it's impact on the LMS. In particular we explain the fundamental role of the transit time since last TST (tTST) for the chemical composition of the LMS. According to our results the structure of the LMS can be characterized by a layer with tTST&lt;40 days forming a narrow band around the local tropopause. This layer extends about 30 K above the local dynamical tropopause, corresponding to the extratropical tropopause transition layer (ExTL) as identified by CO. The LMS beyond this layer shows a relatively well defined separation as marked by an aprupt transition to longer tTST indicating less frequent mixing and a smaller fraction of tropospheric air. Thus the LMS constitutes a region of two well defined regimes of tropospheric influence. These can be characterized mainly by different transport times from the troposphere and different fractions of tropospheric air. Carbon monoxide (CO) mirrors this structure of tTST due to it's finite lifetime on the order of three months. Water vapour isopleths, on the other hand, do not uniquely indicate TST and are independent of tTST, but are determined by the Lagrangian Cold Point (LCP) of air parcels. Most of the backward trajectories from the LMS experienced their LCP in the tropics and sub-tropics, and TST often occurs 20 days after trajectories have encountered their LCP. Therefore, ExTL properties deduced from CO and H2O provide totally different informations on transport and particular TST for the LMS.