In space optical communication, owing to the influence of atmospheric turbulence, optical beams lose focus and become phase-distorted, which reduces the communication quality. Considering the polarization dependence of liquid crystal spatial light modulators and the dispersion effect of liquid crystal materials, the energy utilization rate of liquid crystal adaptive optics systems is low. In this study, a dual liquid crystal spatial light modulator adaptive optics system based on the GS algorithm is used to correct the wavefront distortion of a signal beam under different atmospheric turbulence intensities, and the Strehl ratio (SR) is used as the evaluation index. The simulation results show that the SR of the corrected system can be increased from 0.23, 0.41, and 0.72 to 0.77, 0.89, and 0.95, respectively. The corrected beam spot was more concentrated and the light intensity at the center of the beam spot was stronger. The experimental results show that, after the distortion wavefront is corrected by the dual liquid crystal spatial light modulator, the average gray value of the 10 × 10 pixels in the center of the spot increases from 159.3, 113.1, and 58.4 to 253.4, 247.7, and 198.3, respectively.