Line-focused Beam Research Articles

GEODYNAMIC PROCESSES DURING ASCENT OF A PLUME WITH INTERMEDIATE THERMAL POWER THROUGH THE CONTINENTAL LITHOSPHERE AND DURING ITS ERUPTION ON THE SURFACE

The study is focused on thermochemical mantle plumes with intermediate thermal power (1.15 < Ka < 1.9). Previously we have shown that these plumes are diamondiferous. Based on the laboratory modeling data, the flow structure of a melt in a plume conduit is represented. A plume melts out and ascends from the core – mantle boundary to the bottom of the continental lithosphere. The plume roof moves upwards in the lithosphere because of melting of the lithospheric matter at the plume roof and due to the effect of superlithostatic pressure on the roof, which causes motion in the lithosphere block above the plume roof. The latter manifests itself by uplifting of the ground surface above the plume. As the plume ascends through the lithosphere, the elevation of the surface increases until the plume ascends to critical level xкр, where an eruption conduit is formed. In our model, plume ascent velocity uпл is the rate of melting at the plume roof. Values of uпл and the ascent velocity of a spherical plume roof due to superlithostatic pressure U are calculated. Relationships are found between these velocities and the plume roof depth. The dependence of the velocity of the surface’s rise on the dynamic viscosity of the lithosphere block above the plume is obtained. A relationship is determined between the maximum surface elevation and the lithosphere viscosity. The elevation values are determined for different times and different lithosphere viscosities.The results of laboratory modeling of flow structure at the plume conduit/eruption conduit interface are presented. The flow was photographed (1) in the plane passing through the axes of the plume conduit and the eruption conduit; and (2) in case of the line-focus beam perpendicular to the axial plane. The photographs were used for measuring the flow velocities in the plume conduit and the eruption conduit. Corresponding Reynolds numbers and flow regimes are determined. The relation of dynamic pressure in the eruption conduit to that in the plume conduit is found for intermediate-power plumes. The melt flow velocity in the eruption conduit depends on superlithostatic pressure on the plume roof, plume diameter and kinematic viscosity of the melt. Its values are determined for different kinematic viscosities of melt.

In-process debris removal in femtosecond laser processing

Debris deposited around laser-processed structures, which is a critical issue in high-precision laser processing, should be removed. A new method for laser cleaning of debris was developed. A glass surface was irradiated with a line-focused beam for laser cleaning, together with a focused beam for laser processing. Both beams were formed by computer-generated holograms (CGHs) displayed on a spatial light modulator. The distance between the two beams was controlled with the CGHs, and the time difference was controlled with an optical delay line. These optical structures were the novel aspect of our laser processing system. When two beams were superposed at the same position on a sample, we did not find a suitable beam parameter for debris removal, but we found that the processing area was spatially enlarged depending on the temporal overlap. In contrast, when two beams separated by an adequate distance were radiated on a sample, we found suitable beam parameters for debris removal. Debris removal was effectively performed when the scanning speed of the laser beams was low, because the low scanning speed produced a temperature higher than the glass transition temperature, and the heated and melted debris was ablated due to a smaller ablation threshold than that of the glass substrate. This in-process laser debris removal method has the advantages of needing no additional equipment other than the optics, no additional operations, no special materials, and no specific operating environment.

Large population cell characterization using quantitative phase cytometer

A major challenge in cellular analysis is the phenotypic characterization of large cell populations within a short period of time. Among various parameters for cell characterization, the cell dry mass is often used to describe cell size but is difficult to be measured directly with traditional techniques. Here, we propose an interferometric approach based on line-focused beam illumination for high-content precision dry mass measurements of adherent cells in a non-invasive fashion-we call it quantitative phase cytometry (QPC). Besides dry mass, abundant cellular morphological features such as projected area, sphericity, and phase skewness can be readily extracted from the QPC interferometric data. To validate the utility of our technique, we demonstrate characterizing a large population of ∼104 HeLa cells. Our reported QPC system is envisioned as a promising quantitative tool for label-free characterization of a large cell count at single cell resolution. © 2017 International Society for Advancement of Cytometry.

Ultrasonic microspectroscopy characterization of chemically tempered glass

We evaluated the elastic properties of the compressive stress (CS) layer of chemically tempered glass by ultrasonic microspectroscopy (UMS) in a very high frequency (VHF) range. Two commercial aluminosilicate glass specimens were prepared, and one of them was chemically tempered. Changes in elastic properties in the CS layer with the residual stress introduced by the exchange of Na+ ions for larger K+ ions were estimated by precisely measuring the densities and longitudinal and shear velocities for both the tempered and nontempered specimens. Using a single-layer model for the surface layer, we observed drastic increases in bulk-wave velocities and significant decreases in attenuation coefficients. We determined that the average elastic properties, namely, the elastic constants c11 and c44, and the density of the surface layer, were 9.6 and 7.1, and 1.2% larger than those of the nontempered specimen, respectively. We also estimated the distributions of the elastic properties according to the complementary error function (CEF) for the distribution of K+ ion concentration. Furthermore, using a line-focus-beam (LFB) system, we measured the frequency characteristics of the velocity (VLSAW) of leaky surface acoustic waves (LSAWs) on a water-loaded surface of the tempered specimen and clarified that the distributions of the elastic properties did not follow the CEF. The LFB system can be used for analyzing/determining details of the surface properties and is a promising tool for evaluating and characterizing chemically tempered glass and tempering process conditions.

Holographic laser sweeper for in-process debris removal

Debris deposited around laser-processed structures is a critical issue in high-precision laser processing and should be removed. We demonstrated a new debris removal method that is performed during laser processing. A line-focused beam that is radiated onto a target material simultaneously with a processing beam sweeps away the debris generated by laser ablation. Two physical processes are involved: One is direct photon excitation of the attached debris, similar to laser ablation, due to a smaller ablation threshold of the debris, and the other is blowing away the debris with a laser-induced pressure wave. The laser processing setup for debris sweeping has a simple and practical configuration composed of beam transmission optics from a laser source to the target and a spatial light modulator that displays a computer-generated hologram. This in-process debris removal method has the advantages of needing no additional equipment other than the optics, no additional operations, no special materials, and no specific operating environment.

Current status of protein micro-crystallography at SPring-8

Protein micro-crystallography is one of the most advanced technologies for protein structure analysis. In order to realize this, an undulator beamline, named BL32XU, was constructed at SPring-8. The beamline can provide beam with size of 0.9 x 0.9 µm and photon flux of 6E10 photons/s. The beam size can be easily changed by users from 1 to 10 µm square with the same flux density. Through three years user operation, we have established several key systems for efficient protein micro-crystallography. One of them is the software for precise positioning of micro-crystals in `raster scan'. SHIKA is a program with GUI which searches diffraction spots in a plenty of low dose diffraction images obtained in raster scan. Finally, it generates 2D map of crystal positions based on the number of spots or spot intensities. Parameters and thresholds in peak search have been empirically optimized for LCP crystals and it provides robust results. Another system is for the data collection strategy. Almost all successful data collections were conducted via `helical data collection' on BL32XU using the line-focused beam. The GUI software, named KUMA, enables estimation of an accumulated dose and suggests suitable experimental conditions for helical data collection. The system is proven to be useful for experimental phasing using tiny LCP crystals of membrane proteins[1-3]. Based on them, the rapid and automatic data collection system using protein micro-crystals is under development. The new CCD detector, Rayonix MX225HS, was installed for faster data acquisition in 10 Hz with the pixel size of 78 µm square. The new SHIKA using GPUs is under development for faster and more accurate crystal alignment. Following this step, KUMA system can suggest experimental conditions for each crystal found on the loop. We also report about the effects of higher dose rate in protein crystallography up to the order of 100 MGy/s. This work was supported by Platform for Drug Discovery, Informatics, and Structural Life Science from the Ministry of Education, Culture, Sports, Science and Technology, Japan.

Three-dimensional phase-contrast X-ray microtomography with scanning–imaging X-ray microscope optics

A three-dimensional (3D) X-ray tomographic micro-imaging system has been developed. The optical system is based on a scanning-imaging X-ray microscope (SIXM) optics, which is a hybrid system consisting of a scanning microscope optics with a one-dimensional (1D) focusing (line-focusing) device and an imaging microscope optics with a 1D objective. In the SIXM system, each 1D dataset of a two-dimensional (2D) image is recorded independently. An object is illuminated with a line-focused beam. Positional information of the region illuminated by the line-focused beam is recorded with the 1D imaging microscope optics as line-profile data. By scanning the object with the line focus, 2D image data are obtained. In the same manner as for a scanning microscope optics with a multi-pixel detector, imaging modes such as phase contrast and absorption contrast can be arbitrarily configured after the image data acquisition. By combining a tomographic scan method and the SIXM system, quantitative 3D imaging is performed. Results of a feasibility study of the SIXM for 3D imaging are shown.

Mitigation of X-ray damage in macromolecular crystallography by submicrometre line focusing

Reported here are measurements of the penetration depth and spatial distribution of photoelectron (PE) damage excited by 18.6 keV X-ray photons in a lysozyme crystal with a vertical submicrometre line-focus beam of 0.7 µm full-width half-maximum (FWHM). The experimental results determined that the penetration depth of PEs is 5 ± 0.5 µm with a monotonically decreasing spatial distribution shape, resulting in mitigation of diffraction signal damage. This does not agree with previous theoretical predication that the mitigation of damage requires a peak of damage outside the focus. A new improved calculation provides some qualitative agreement with the experimental results, but significant errors still remain. The mitigation of radiation damage by line focusing was measured experimentally by comparing the damage in the X-ray-irradiated regions of the submicrometre focus with the large-beam case under conditions of equal exposure and equal volumes of the protein crystal, and a mitigation factor of 4.4 ± 0.4 was determined. The mitigation of radiation damage is caused by spatial separation of the dominant PE radiation-damage component from the crystal region of the line-focus beam that contributes the diffraction signal. The diffraction signal is generated by coherent scattering of incident X-rays (which introduces no damage), while the overwhelming proportion of damage is caused by PE emission as X-ray photons are absorbed.

Photoacoustic Imaging with a Line-Focus Laser Beam for Rapid Inspection and Tomographic Characterization of Simulated Surface and Undersurface Defects

A photoacoustic (PA) imaging apparatus using a laser line-focus beam (LFB) was designed to perform rapid inspection and photoacoustic tomographic (PAT) imaging of surface and undersurface defects. 2D-PAT imaging of surface and undersurface defects was demonstrated based on a formulation similar to the X-ray tomography. The obtained PAT images represented forward-projected PA signals collected along the LFB. The reconstructed images were in close agreement with those obtained from laser point-focus beam (PFB) PA imaging. We achieved rapid non-destructive inspection of a surface-simulated defect using a LFB. The reconstructed PA image of the undersurface defect was consistent with that obtained by a plane-thermal wave diffraction model.

Line-focus beam photoacoustic imaging of surface and undersurface defect simulated on a planar specimen

A theoretical formulation of photoacoustic (PA) imaging with a line-focus beam (LFB) for surface and undersurface simulated defect was performed. Equivalence between 2D surface defect photoacoustic tomography (PAT) and X-ray CT was derived. PAT imaging experiment was carried out A second harmonics of a LD-pumped YAG laser was used as a LFB. The laser power was 45mW. The length and width of a laser beam on a specimen was 25 mm times 0.65mm The measured area was 27mm x 27mm, while the reconstructed area was 18mm x 18mm. 64 times 64 resolution image was reconstructed from the rotation and translation scanning. Reconstructed PA image agreed with the PA image obtained with a point-focus PA imaging. The frequency dependence of thermally diffused image agreed well with the theoretical prediction (thermal diffusion length is inversely proportional to the square root of modulation frequency) Under surface PAT image was obtained by a thermal wave diffraction formula, and the simulated image agreed well with the experimental data.

1-04P-11 Imaging of undersurface defect by photoacoustic tomography with a line-focus beam(Poster session 1)

1-04P-11 Imaging of undersurface defect by photoacoustic tomography with a line-focus beam(Poster session 1)

Accurate Velocity Measurement of Periodic Striae of TiO2–SiO2 Glasses by the Line-Focus-Beam Ultrasonic Material-Characterization System

The evaluation of periodic striae layers in TiO2–SiO2 ultra-low-expansion glasses, formed during production, is discussed through the measurement of leaky surface acoustic-wave (LSAW) velocities by the line-focus-beam (LFB) ultrasonic material-characterization system. The averaging effect associated with an LSAW propagation region interacting with periodic striae on a specimen surface was examined at 225 MHz, taking several specimens prepared with inclination angles of θ=0, 2, 5, 10, 20, and 90° to the plane of striae layers with a periodicity of 0.16 mm. LSAW velocities corresponding to TiO2 concentrations in the glass were properly measured for the specimens with θ less than 10°, and the perpendicular specimen (θ=90°) was suitable for accurate determination of the striae periodicities for LSAW propagation perpendicular to the striae plane.

Evaluation method of TiO/sub 2/-SiO/sub 2/ ultra-low-expansion glasses with periodic striae using the LFB ultrasonic material characterization system

Experimental procedures and standard specimens for characterizing and evaluating TiO2-SiO2 ultra-low expansion glasses with periodic striae using the line-focus-beam (LFB) ultrasonic material characterization system are discussed. Two types of specimens were prepared, with specimen surfaces parallel and perpendicular to the striae plane using two different grades of glass ingots. The inhomogeneities of each of the specimens were evaluated at 225 MHz. It was clarified that parallel specimens are useful for accurately measuring velocity variations of leaky surface acoustic waves (LSAWs) excited on a water-loaded specimen surface associated with the striae. Perpendicular specimens are useful for obtaining periodicities in the striae for LSAW propagation perpendicular to the striae plane on a surface and for precisely measuring averaged velocities for LSAW propagation parallel to the striae plane. The standard velocity of Rayleigh-type LSAWs traveling parallel to the striae plane for the perpendicular specimens was numerically calculated using the measured velocities of longitudinal and shear waves and density. Consequently, a reliable standard specimen with an LSAW velocity of 3308.18 +/- 0.35 m/s at 23 degrees C and its temperature coefficient of 0.39 (m/s)/degrees C was obtained for a TiO2-SiO2 glass with a TiO2 concentration of 7.09 wt%. A basis for the striae analysis using this ultrasonic method was established.

Experimental Study for Evaluating Striae Structure of TiO2–SiO2 Glasses Using the Line-Focus-Beam Ultrasonic Material Characterization System

Striae configurations in TiO2–SiO2 ultra-low-expansion glasses caused by variations in TiO2 concentration were investigated through measurement of leaky surface acoustic wave (LSAW) velocities by the line-focus-beam (LFB) ultrasonic material characterization system. LSAW velocity distributions were measured on the surface of a specimen substrate prepared from a large circular plate glass ingot produced by the direct method using a flame hydrolysis process. A subsequent procedure that included polishing the surface of the specimen to reduce the specimen thickness by 40 µm and measuring the LSAW velocity distributions on the surface was repeated five times in order to examine at least one period of the striae. TiO2 concentration variations were clearly observed in the deposit direction of the glass ingot and in its radial direction. The maximum LSAW velocity difference over the whole examined region was 11.7 m/s, corresponding to 0.70 wt % TiO2 concentration. The three-dimensional striae structure revealed that the striae plane in the examined region was almost parallel to the substrate surface but gently curved down in the radial direction. The plane had a slightly convex-shaped cross section layered with a striae periodicity of about 0.16 mm and a curvature radius of about 440 mm, and also existed in a circular form with a curvature radius of about 450 mm. The ultrasonic method will contribute to improvement of characteristics and homogeneity of glass associated with production-process conditions.

Real-time photodisplacement microscope for high-sensitivity simultaneous surface and subsurface inspection

We have developed a new photodisplacement microscope system for practical use that achieves high-sensitivity simultaneous real-time imaging of surface and subsurface structures from a single space-frequency multiplexed interferogram. In this system a linear region of photothermal displacement is excited on the sample surface for subsurface imaging by a line-focused intensity-modulated laser beam. Surface information such as reflectivity and topography along with the displacement is detected with a charge-coupled device sensor-based parallel heterodyne interferometer. Surface and subsurface information components are space-frequency multiplexed into the sensor signal as orthogonal functions based on a frequency-optimized undersampling scheme, allowing each to be discretely reproduced by using a real-time Fourier analysis technique. Preliminary experiments demonstrate that this system is effective, simultaneously imaging reflectivity, topography, and photodisplacement for the detection of subsurface lattice defects in silicon, at a remarkable speed of only 0.26 s/256x256 pixel area. This new microscope is promising for nondestructive hybrid surface and subsurface inspection and other applications.

Evaluation of mass-produced commercial LiTaO/sub 3/ single crystals using the LFB ultrasonic material characterization system

A mass-production line of lithium tantalate (LiTaO3) crystals with a maximum charge number of 60 for surface acoustic wave (SAW) devices was evaluated with the line-focus-beam (LFB) ultrasonic material characterization system. Some serious problems associated with chemical compositions were observed and resolved by measuring the velocities of Rayleigh-type leaky surface acoustic waves (LSAWs), VLSAW, for two groups of LiTaO3 wafers: 21 36 degrees Y X-LiTaO3 wafers selected randomly from crystal ingots grown with different charge numbers in different furnaces, and 14 42 degrees Y X-LiTaO3 wafers obtained at the top, middle, and bottom parts from 5 crystals selected from 39 crystals grown successively in the same furnace and crucible. Using the measured VLSAW and the predetermined relationship between VLSAW and Li2O concentrations, M(Li2O), we estimated the average M(Li2O) controlled in the current mass-production line to be about 48.77 mol% with a maximum difference of 0.75 mol%. The composition for each crystal ingot increased linearly about 0.04 mol% from the top to the bottom, and no dependence on the charge number was observed, as the melt composition used for the mass production was controlled through Curie temperature (TC) measurements. A nearly true congruent composition of 48.49 Li2O-mol% was obtained through the precise VLSAW data for the 42 degrees Y X-LiTaO3 wafers, that was about 0.3 mol% less than the melt composition in the production line. It was also pointed out that the TC measurement conditions, including room temperatures surrounding the measurement systems, should be re-examined for reliable production control. A guideline for more efficient mass production of the crystals has been established concerning the true congruent composition as the starting material.

Theoretical and experimental investigation of ultrasonic waves radiated from a wet surface using a line-focused laser beam

In this paper we use with a theoretical model and experimental study to predict the characteristics of the ultrasonic waves irradiated from a wet surface illuminated by a line-focused laser beam. The theoretical model is developed by assuming normal surface tractions distributed elliptically over the illuminated source. The solutions for both longitudinal and shear waves are obtained using Fourier analysis, in which the transform integral is evaluated asymptotically. The theory was evidenced by the experimental study which allows direct quantitative comparisons between the theoretical and experimental directivity patterns. The effects of beam diameter and frequency of the propagating wave, which are the most influential parameters on the characteristics of the generated wave, are investigated in the experimental work. The experimental results are in strong agreement with the theoretical predictions.

Theoretical and Experimental Investigation of Ultrasonic Waves Radiated from a Wet Surface Using a Line-Focused Laser Beam

Theoretical and Experimental Investigation of Ultrasonic Waves Radiated from a Wet Surface Using a Line-Focused Laser Beam

Wideband high-frequency line-focus PVDF transducer for materials characterization

This paper presents the design, fabrication, operating characteristics and applications of a wideband, high-frequency, line-focus beam transducer we constructed using a 9 μm thick piezoelectric polyvinylidene fluoride (PVDF) film. This transducer possesses a focal length of 2.38 mm and an aperture angle of 84°. The frequency spectrum of the signal measured at the focal point indicates that the transducer has a wide frequency response which extends from 10 MHz to over 100 MHz. When compensated for the frequency-dependent attenuation of the coupling medium, the operational frequency exceeds 150 MHz. The transducer can be operated in a time-resolved pulse mode or in a radio-frequency (rf) tone burst mode. An application of the transducer to determine the anisotropic elastic property of a silicon wafer is demonstrated. The phase velocities of surface acoustic waves (SAW) propagating along various directions on the (0 0 1) surface of cubic silicon are measured and compared to computed values.

A method of determining acoustical physical constants for piezoelectric materials by line-focus-beam acoustic microscopy.

We developed a new method of determining acoustical physical constants (elastic constant, piezoelectric constant, dielectric constant, and density) of piezoelectric materials with high accuracy. This method acquires velocities of leaky surface acoustic waves (LSAWs) excited on the water-loaded specimen surface, measured by line-focus-beam (LFB) acoustic microscopy, and bulk velocities of longitudinal and shear waves, measured with plane-wave transducers replacing the LFB device in the same system, together with the dielectric constants and density measured independently, for a small number of specimens. For LiNbO3 and LiTaO3 crystals, we demonstrated that we could accurately determine the constants by choosing proper propagation directions of LSAWs and bulk waves for three principal X-, Y-, and Z-cut specimens and one rotated Y-cut specimen [(104) plate for LiNbO3 and (012) plate for LiTaOa]. The accuracy is nearly the same as that for the constants determined only from the bulk wave velocities.