Light-induced Dipole-dipole Interactions Research Articles

Tunable light-induced dipole-dipole interaction between optically levitated nanoparticles.

Arrays of optically trapped nanoparticles have emerged as a platform for the study of complex nonequilibrium phenomena. Analogous to atomic many-body systems, one of the crucial ingredients is the ability to precisely control the interactions between particles. However, the optical interactions studied thus far only provide conservative optical binding forces of limited tunability. In this work, we exploit the phase coherence between the optical fields that drive the light-induced dipole-dipole interaction to couple two nanoparticles. In addition, we effectively switch off the optical interaction and observe electrostatic coupling between charged particles. Our results provide a route to developing fully programmable many-body systems of interacting nanoparticles with tunable nonreciprocal interactions, which are instrumental for exploring entanglement and topological phases in arrays of levitated nanoparticles.

Disorder-assisted excitation localization in chirally coupled quantum emitters

One-dimensional quantum emitters with chiral couplings can exhibit nonreciprocal decay channels, along with light-induced dipole-dipole interactions mediated via an atom-waveguide interface. When the position disorders are introduced to such atomic array, we are able to identify the dynamical phase transition from excitation delocalization to localization, with an interplay between the directionality of decay rates and the strength of light-induced dipole-dipole interactions. Deep in the localization phase, its characteristic length decreases and saturates toward a reciprocal coupling regime, leading to a system dynamics whose ergodicity is strongly broken. We also find an interaction-driven re-entrant behavior of the localization phase and a reduction of level repulsion under strong disorder. The former coincides with a drop in the exponent of power-law decaying von Neumann entropy, which gives insights to a close relation between the preservation of entanglement and nonequilibrium dynamics in open quantum systems, while the latter presents a distinct narrow distribution of gap ratios in this particular disordered system.

Superatom Picture of Collective Nonclassical Light Emission and Dipole Blockade in Atom Arrays.

We show that two-time, second-order correlations of scattered photons from planar arrays and chains of atoms display nonclassical features that can be described by a superatom picture of the canonical single-atom g_{2}(τ) resonance fluorescence result. For the superatom, the single-atom linewidth is replaced by the linewidth of the underlying collective low light-intensity eigenmode. Strong light-induced dipole-dipole interactions lead to a correlated response, suppressed joint photon detection events, and dipole blockade that inhibits multiple excitations of the collective atomic state. For targeted subradiant modes, the nonclassical nature of emitted light can be dramatically enhanced even compared with that of a single atom.

Collective Shift in Resonant Light Scattering by a One-Dimensional Atomic Chain.

We experimentally study resonant light scattering by a one-dimensional randomly filled chain of cold two-level atoms. By a local measurement of the light scattered along the chain, we observe constructive interferences in light-induced dipole-dipole interactions between the atoms. They lead to a shift of the collective resonance despite the average interatomic distance being larger than the wavelength of the light. This result demonstrates that strong collective effects can be enhanced by structuring the geometrical arrangement of the ensemble. We also explore the high intensity regime where atoms cannot be described classically. We compare our measurement to a mean-field, nonlinear coupled-dipole model accounting for the saturation of the response of a single atom.

Near-Resonant Light Scattering by a Subwavelength Ensemble of Identical Atoms.

We study theoretically the scattering of light by an ensemble of N resonant atoms in a subwavelength volume. We consider the low intensity regime so that each atom responds linearly to the field. While N noninteracting atoms would scatter N^{2} more than a single atom, we find that N interacting atoms scatter less than a single atom near resonance. In addition, the scattered power presents strong fluctuations, either from one realization to another or when varying the excitation frequency. We analyze this counterintuitive behavior in terms of collective modes resulting from the light-induced dipole-dipole interactions. We find that for small samples and sufficiently large atom number, their properties are governed only by their volume.

Transmission of near-resonant light through a dense slab of cold atoms

The optical properties of randomly positioned, resonant scatterers is a fundamentally difficult problem to address across a wide range of densities and geometries. We investigate it experimentally using a dense cloud of rubidium atoms probed with near-resonant light. The atoms are confined in a slab geometry with a sub-wavelength thickness. We probe the optical response of the cloud as its density and hence the strength of the light-induced dipole-dipole interactions are increased. We also describe a theoretical study based on a coupled dipole simulation which is further complemented by a perturbative approach. This model reproduces qualitatively the experimental observation of a saturation of the optical depth, a broadening of the transition and a blue shift of the resonance.

Homogenization of an ensemble of interacting resonant scatterers

We study theoretically the concept of homogenization in optics using an ensemble of randomly distributed resonant stationary atoms with density $\rho$. The ensemble is dense enough for the usual condition for homogenization, viz. $\rho\lambda^3 \gg 1$, to be reached. Introducing the coherent and incoherent scattered powers, we define two criteria to define the homogenization regime. We find that when the excitation field is tuned in a broad frequency range around the resonance, none of the criteria for homogenization is fulfilled, meaning that the condition $\rho\lambda^3\gg 1$ is not sufficient to characterize the homogenized regime around the atomic resonance. We interpret these results as a consequence of the light-induced dipole-dipole interactions between the atoms, which implies a description of scattering in terms of collective modes rather than as a sequence of individual scattering events. Finally, we show that, although homogenization can never be reached for a dense ensemble of randomly positioned laser-cooled atoms around resonance, it becomes possible if one introduces spatial correlations in the positions of the atoms or non-radiative losses, such as would be the case for organic molecules or quantum dots coupled to a phonon bath.

Coherent Scattering of Near-Resonant Light by a Dense Microscopic Cold Atomic Cloud.

We measure the coherent scattering of light by a cloud of laser-cooled atoms with a size comparable to the wavelength of light. By interfering a laser beam tuned near an atomic resonance with the field scattered by the atoms, we observe a resonance with a redshift, a broadening, and a saturation of the extinction for increasing atom numbers. We attribute these features to enhanced light-induced dipole-dipole interactions in a cold, dense atomic ensemble that result in a failure of standard predictions such as the "cooperative Lamb shift". The description of the atomic cloud by a mean-field model based on the Lorentz-Lorenz formula that ignores scattering events where light is scattered recurrently by the same atom and by a microscopic discrete dipole model that incorporates these effects lead to progressively closer agreement with the observations, despite remaining differences.

Nonresonance mechanisms of biological effects of coherent and incoherent light

Two mechanisms of the nonresonance action of light on biological systems are considered. The first of them is caused by gradient effects arising upon interaction of a biological system with spatially inhomogeneous radiation. The second mechanism is determined by light-induced dipole-dipole interactions between biological particles. The first mechanism is characteristic of coherent radiation. A speckle structure arising upon interaction of coherent light with a biological system gives rise to gradient forces, which depend on the intensity of the incident light and the properties of an object. It is shown that the action of the gradient forces on microparticles causes a selective increase in the kinetic energy of the particles. Due to random pulsations of speckles in living tissue, this effect is equivalent to an increase in the “partial” temperature of the particles, which depends on their size and properties. The second mechanism manifests itself both upon coherent and upon incoherent irradiation of a biological object. This mechanism is determined by interactions between oscillating dipole moments of neighboring particles (cells, organelles, biomolecules) induced by incident radiation. The second mechanism is shown to be observed for linearly polarized radiation only. For each mechanism, the forces acting on biological particles are calculated.

Magnetic soliton and soliton collisions of spinor Bose-Einstein condensates in an optical lattice

We study the magnetic soliton dynamics of spinor Bose-Einstein condensates in an optical lattice which results in an effective Hamiltonian of anisotropic pseudospin chain. A modified Landau-Lifshitz equation is derived and exact magnetic soliton solutions are obtained analytically. Our results show that the time-oscillation of the soliton size can be controlled in practical experiment by adjusting of the light-induced dipole-dipole interaction. Moreover, the elastic collision of two solitons is investigated.

Spin waves in a Bose-Einstein--condensed atomic spin chain.

The spin dynamics of atomic Bose-Einstein condensates confined in a one-dimensional optical lattice is studied. The condensates at each lattice site behave like spin magnets that can interact with each other through both the light-induced dipole-dipole interaction and the static magnetic dipole-dipole interaction. We show how these site-to-site dipolar interactions can distort the ground-state spin orientations and lead to the excitation of spin waves. The dispersion relation of the spin waves is studied and possible detection schemes are proposed.

Self-trapping and self-focusing of a coherent atomic beam

Light-induced dipole-dipole interaction in a coherent atomic-field results in an effective nonlinearity for atoms. This nonlinearity can induce self-trapping and self-focusing of a coherent atomic beam undergoing propagation through a traveling-wave laser beam; we show how such a scheme could be realized and evaluate the critical density required for atomic self-trapping and self-focusing. An analogy to optical self-trapping and self-focusing is discussed.