Light-absorbing Particles In Snow Research Articles

The Spatio-Temporal Variability in the Radiative Forcing of Light-Absorbing Particles in Snow of 2003–2018 over the Northern Hemisphere from MODIS

Light-absorbing particles (LAPs) deposited on snow can significantly reduce surface albedo and contribute to positive radiative forcing. This study firstly estimated and attributed the spatio-temporal variability in the radiative forcing (RF) of LAPs in snow over the northern hemisphere during the snow-covered period 2003–2018 by employing Moderate Resolution Imaging Spectroradiometer (MODIS) data, coupled with snow and atmospheric radiative transfer modelling. In general, the RF for the northern hemisphere shows a large spatial variability over the whole snow-covered areas and periods, with the highest value (12.7 W m−2) in northeastern China (NEC) and the lowest (1.9 W m−2) in Greenland (GRL). The concentration of LAPs in snow is the dominant contributor to spatial variability in RF in spring (~73%) while the joint spatial contributions of snow water equivalent (SWE) and solar irradiance (SI) are the most important (>50%) in winter. The average northern hemisphere RF gradually increases from 2.1 W m−2 in December to 4.1 W m−2 in May and the high-value area shifts gradually northwards from mid-altitude to high-latitude over the same period, which is primarily due to the seasonal variability of SI (~58%). More interestingly, our data reveal a significant decrease in RF over high-latitude Eurasia (HEUA) of −0.04 W m−2 a−1 and northeastern China (NEC) of −0.14 W m−2 a−1 from 2003 to 2018. By employing a sensitivity test, we find the concurrent decline in the concentration of LAPs in snow accounted for the primary responsibility for the decrease in RF over these two areas, which is further confirmed by in situ observations.

Snow Albedo Feedbacks Enhance Snow Impurity‐Induced Radiative Forcing in the Sierra Nevada

This study employs a fully coupled meteorology‐chemistry‐snow model to investigate the impacts of light‐absorbing particles (LAPs) on snow darkening in the Sierra Nevada. After comprehensive evaluation with spatially and temporally complete satellite retrievals, the model shows that LAPs in snow reduce snow albedo by 0.013 (0–0.045) in the Sierra Nevada during the ablation season (April‐July), producing a midday mean radiative forcing of 4.5 W m−2 which increases to 15–22 W m−2 in July. LAPs in snow accelerate snow aging processes and reduce snow cover fraction, which doubles the albedo change and radiative forcing caused by LAPs. The impurity‐induced snow darkening effects decrease snow water equivalent and snow depth by 20 and 70 mm in June in the Sierra Nevada bighorn sheep habitat. The earlier snowmelt reduces root‐zone soil water content by 20%, deteriorating the forage productivity and playing a negative role in the survival of bighorn sheep.

Satellite-based radiative forcing by light-absorbing particles in snow across the Northern Hemisphere

Abstract. Snow is the most reflective natural surface on Earth and consequently plays an important role in Earth's climate. Light-absorbing particles (LAPs) deposited on the snow surface can effectively decrease snow albedo, resulting in positive radiative forcing. In this study, we used remote-sensing data from NASA's Moderate Resolution Imaging Spectroradiometer (MODIS) and the Snow, Ice, and Aerosol Radiative (SNICAR) model to quantify the reduction in snow albedo due to LAPs before validating and correcting the data against in situ observations. We then incorporated these corrected albedo-reduction data in the Santa Barbara DISORT (Discrete Ordinate Radiative Transfer) Atmospheric Radiative Transfer (SBDART) model to estimate Northern Hemisphere radiative forcing except for midlatitude mountains in December–May for the period 2003–2018. Our analysis reveals an average corrected reduction in snow albedo (ΔαMODIS,correctedLAPs) of ∼ 0.021 under all-sky conditions, with daily radiative forcing (RFMODIS,dailyLAPs) values of ∼ 2.9 W m−2, over land areas with complete or near-complete snow cover and with little or no vegetation above the snow in the Northern Hemisphere. We also observed significant spatial variations in ΔαMODIS,correctedLAPs and RFMODIS,dailyLAPs, with the lowest respective values (∼ 0.016 and ∼ 2.6 W m−2) occurring in the Arctic and the highest (∼ 0.11 and ∼ 12 W m−2) in northeastern China. From MODIS retrievals, we determined that the LAP content of snow accounts for 84 % and 70 % of the spatial variability in albedo reduction and radiative forcing, respectively. We also compared retrieved radiative forcing values with those of earlier studies, including local-scale observations, remote-sensing retrievals, and model-based estimates. Ultimately, estimates of radiative forcing based on satellite-retrieved data are shown to represent true conditions on both regional and global scales.

An Overview of Snow Albedo Sensitivity to Black Carbon Contamination and Snow Grain Properties Based on Experimental Datasets Across the Northern Hemisphere

Black carbon (BC) deposition in snow can trigger a significant reduction in snow albedo and accelerate snowmelt. As a result, numerous snow surveys have performed to measure BC concentrations in snow across the polar regions, the Tibetan Plateau, and other high-mountain regions. This review is aimed to synthesize the current progresses of the potential feedbacks of snow albedo and its sensitivity by BC in snow across the Northern Hemisphere. Generally, BC concentrations in snow are highest in the mid-latitudes of Northern China and North America, and reduce toward higher latitudes (e.g., Greenland and the rest of the Arctic). We found that the snow albedo reduction attributed to low BC contamination (< 20 ng g−1) in older snow (200 μm snow grains) is 1.2%, compared with 0.6% in fresh snow (50 μm snow grains). Non-spherical snow grains exhibit a significantly lower snow albedo reduction (2–6%) due to BC contamination compared with spherical snow grains with 100–500 ng g−1 of BC in the snowpack. Snow–BC–internal mixing reduces the snow albedo (< 10%) more substantially than does external mixing in the case of 50–200 μm snow grains and a given BC concentration (< 2000 ng g−1). Besides the BC and other light-absorbing particles (LAPs), the mixing state of LAPs in snow, snow grain properties, and the scavenging\washing effects are also major challenges in determining snow albedo, which need to be further investigated on a global scale.

Motion of dust particles in dry snow under temperature gradient metamorphism

Abstract. The deposition of light-absorbing particles (LAPs) such as mineral dust and black carbon on snow is responsible for a highly effective climate forcing, through darkening of the snow surface and associated feedbacks. The interplay between post-depositional snow transformation (metamorphism) and the dynamics of LAPs in snow remains largely unknown. We obtained time series of X-ray tomography images of dust-contaminated samples undergoing dry snow metamorphism at around −2 ∘C. They provide the first observational evidence that temperature gradient metamorphism induces dust particle motion in snow, while no movement is observed under isothermal conditions. Under temperature gradient metamorphism, dust particles can enter the ice matrix due to sublimation–condensation processes and spread down mainly by falling into the pore space. Overall, such motions might reduce the radiative impact of dust in snow, in particular in arctic regions where temperature gradient metamorphism prevails.

Radiative forcing by light-absorbing particles in snow

As one of the brightest natural surfaces on Earth, the darkening of snow by light-absorbing particles (LAPs) — dust, black carbon or microbial growth — can trigger albedo feedbacks and accelerate snowmelt. Indeed, an increase in black carbon deposition following the industrial revolution has led to the recognition that LAP radiative forcing has contributed to a reduction in the global cryosphere, with corresponding climatic impacts. This Review synthesizes our current understanding of the distribution of radiative forcing by LAPs in snow, and discusses the challenges that need to be overcome to constrain global impacts, including the limited scope of local-scale observations, limitations of remote sensing technology and the representation of LAP-related processes in Earth system models.

Light-absorbing particles in snow and ice: Measurement and modeling of climatic and hydrological impact

Light absorbing particles (LAP, e.g., black carbon, brown carbon, and dust) influence water and energy budgets of the atmosphere and snowpack in multiple ways. In addition to their effects associated with atmospheric heating by absorption of solar radiation and interactions with clouds, LAP in snow on land and ice can reduce the surface reflectance (a.k.a., surface darkening), which is likely to accelerate the snow aging process and further reduces snow albedo and increases the speed of snowpack melt. LAP in snow and ice (LAPSI) has been identified as one of major forcings affecting climate change, e.g. in the fourth and fifth assessment reports of IPCC. However, the uncertainty level in quantifying this effect remains very high. In this review paper, we document various technical methods of measuring LAPSI and review the progress made in measuring the LAPSI in Arctic, Tibetan Plateau and other mid-latitude regions. We also report the progress in modeling the mass concentrations, albedo reduction, radiative forcing, and climatic and hydrological impact of LAPSI at global and regional scales. Finally we identify some research needs for reducing the uncertainties in the impact of LAPSI on global and regional climate and the hydrological cycle.

Arctic climate response to forcing from light-absorbing particles in snow and sea ice in CESM

Abstract. The presence of light-absorbing aerosol particles deposited on arctic snow and sea ice influences the surface albedo, causing greater shortwave absorption, warming, and loss of snow and sea ice, lowering the albedo further. The Community Earth System Model version 1 (CESM1) now includes the radiative effects of light-absorbing particles in snow on land and sea ice and in sea ice itself. We investigate the model response to the deposition of black carbon and dust to both snow and sea ice. For these purposes we employ a slab ocean version of CESM1, using the Community Atmosphere Model version 4 (CAM4), run to equilibrium for year 2000 levels of CO2 and fixed aerosol deposition. We construct experiments with and without aerosol deposition, with dust or black carbon deposition alone, and with varying quantities of black carbon and dust to approximate year 1850 and 2000 deposition fluxes. The year 2000 deposition fluxes of both dust and black carbon cause 1–2 °C of surface warming over large areas of the Arctic Ocean and sub-Arctic seas in autumn and winter and in patches of Northern land in every season. Atmospheric circulation changes are a key component of the surface-warming pattern. Arctic sea ice thins by on average about 30 cm. Simulations with year 1850 aerosol deposition are not substantially different from those with year 2000 deposition, given constant levels of CO2. The climatic impact of particulate impurities deposited over land exceeds that of particles deposited over sea ice. Even the surface warming over the sea ice and sea ice thinning depends more upon light-absorbing particles deposited over land. For CO2 doubled relative to year 2000 levels, the climate impact of particulate impurities in snow and sea ice is substantially lower than for the year 2000 equilibrium simulation.