Lidar Ratio Research Articles

Large-Scale Network-Based Observations of a Saharan Dust Event across the European Continent in Spring 2022

Between 14 March and 21 April 2022, an extensive investigation of an extraordinary Saharan dust intrusion over Europe was performed based on lidar measurements obtained by the European Aerosol Research Lidar Network (EARLINET). The dust episode was divided into two distinct periods, one in March and one in April, characterized by different dust transport paths. The dust aerosol layers were studied over 18 EARLINET stations, examining aerosol characteristics during March and April in four different regions (M-I, M-II, M-III, and M-IV and A-I, A-II, A-III, and A-IV, respectively), focusing on parameters such as aerosol layer thickness, center of mass (CoM), lidar ratio (LR), particle linear depolarization ratio (PLDR), and Ångström exponents (ÅE). In March, regions exhibited varying dust geometrical and optical properties, with mean CoM values ranging from approximately 3.5 to 4.8 km, and mean LR values typically between 36 and 54 sr. PLDR values indicated the presence of both pure and mixed dust aerosols, with values ranging from 0.20 to 0.32 at 355 nm and 0.24 to 0.31 at 532 nm. ÅE values suggested a range of particle sizes, with some regions showing a predominance of coarse particles. Aerosol Optical Depth (AOD) simulations from the NAAPS model indicated significant dust activity across Europe, with AOD values reaching up to 1.60. In April, dust aerosol layers were observed between 3.2 to 5.2 km. Mean LR values typically ranged from 35 to 51 sr at both 355 nm and 532 nm, while PLDR values confirmed the presence of dust aerosols, with mean values between 0.22 and 0.31 at 355 nm and 0.25 to 0.31 at 532 nm. The ÅE values suggested a mixture of particle sizes. The AOD values in April were generally lower, not exceeding 0.8, indicating a less intense dust presence compared to March. The findings highlight spatial and temporal variations in aerosol characteristics across the regions, during the distinctive periods. From 15 to 16 March 2022, Saharan dust significantly reduced UV-B radiation by approximately 14% over the ATZ station (Athens, GR). Backward air mass trajectories showed that the dust originated from the Western and Central Sahara when, during this specific case, the air mass trajectories passed over GRA (Granada, ES) and PAY (Payerne, CH) before reaching ATZ, maintaining high relative humidity and almost stable aerosol properties throughout its transport. Lidar data revealed elevated aerosol backscatter (baer) and PLDR values, combined with low LR and ÅE values, indicative of pure dust aerosols.

Polarization lidar observations of diurnal and seasonal variations in the atmospheric mixing layer above a tropical rural place gadanki, India

This study presents the daily and seasonal variation of the atmospheric mixing layer height (MLH) over Gadanki, India (13.45°N, 79.18°E), a tropical rural location based on polarization lidar observations. The observations spanned the years 2009–2014, encompassing 303 instances, and coinciding with radiosonde and surface weather station measurements. The MLH was determined through the analysis of aerosol profiles and confirmed with the MLH values derived from radiosonde data. The lidar depolarization ratio was employed to characterize aerosol shape. This study aims to establish a connection between aerosol backscatter and its shape through lidar observations, considering diurnal and seasonal variations, while also identifying the influencing factors. This study illustrates four distinct case studies conducted during different seasons to depict aerosol behavior in both convectively active and non-active periods. These case studies unveil the influence of aerosol shape on water intake and subsequent residual layer and cloud formation. The observed fluctuations in MLH and aerosol shape suggest a dynamic relationship between local meteorology and long-range aerosol transport.

The algorithm of microphysical-parameter profiles of aerosol and small cloud droplets based on the dual-wavelength lidar data

Abstract. This study proposed an inversion method for atmospheric-aerosol or cloud microphysical parameters based on dual-wavelength lidar data. The matching characteristics between aerosol and cloud particle size distributions and gamma distributions were studied using aircraft observation data. The feasibility of the retrieval of the particle effective radius from lidar ratios and backscatter ratios was simulated and studied. A method for inverting the effective radius and number concentration of atmospheric aerosols or small cloud droplets using the backscatter ratio was proposed, and the error sources and applicability of the algorithm were analyzed. This algorithm was suitable for the inversion of uniformly mixed and single-property aerosol layers or small cloud droplets. Compared with the previous study, this algorithm could quickly obtain the microphysical parameters of atmospheric particles and has good robustness. For aerosol particles, the inversion range that this algorithm can achieve is 0.3–1.7 µm. For cloud droplets, it is 1.0–10 µm. An atmospheric-observation experiment was conducted using the multi-wavelength lidar developed by Xi'an University of Technology, and a thin cloud layer was captured. The microphysical parameters of aerosol and clouds during this process were retrieved. The results clearly demonstrate the growth of the effective radius and number concentration.

A near-global multiyear climate data record of the fine-mode and coarse-mode components of atmospheric pure dust

Abstract. A new four-dimensional, multiyear, and near-global climate data record of the fine-mode (submicrometer in terms of diameter) and coarse-mode (supermicrometer in terms of diameter) components of atmospheric pure dust is presented. The separation of the two modes of dust in detected atmospheric dust layers is based on a combination of (1) the total pure-dust product provided by the well-established European Space Agency (ESA) “LIdar climatology of Vertical Aerosol Structure” (LIVAS) database and (2) the coarse-mode component of pure dust provided by the first step of the two-step POlarization LIdar PHOtometer Networking (POLIPHON) technique, developed in the framework of the European Aerosol Research Lidar Network (EARLINET). Accordingly, the fine-mode component of pure dust is extracted as the residual between the LIVAS total pure dust and the coarse-mode component of pure dust. Intermediate steps involve the implementation of regionally dependent lidar-derived lidar ratio values and AErosol RObotic NETwork (AERONET)-based climatological extinction-to-volume conversion factors, facilitating conversion of dust backscatter into extinction and subsequently extinction into mass concentration. The decoupling scheme is applied to observations from the Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) at 532 nm. The final products consist of the fine mode and coarse mode of atmospheric pure dust, quality-assured profiles of backscatter coefficient at 532 nm, extinction coefficient at 532 nm, and mass concentration for each of the two components. The datasets are established primarily with the original L2 horizontal (5 km) and vertical (60 m) resolution of the Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) along the CALIPSO orbit path and secondly in averaged profiles of seasonal–temporal resolution, 1° × 1° spatial resolution, and the original vertical resolution of CALIPSO, focusing on the latitudinal band extending between 70° S and 70° N and covering more than 15 years of Earth observations (June 2006–December 2021). The quality of the CALIPSO-based fine-mode and coarse-mode dust products is assessed through the use of AERONET fine-mode and coarse-mode aerosol optical thickness (AOT) interpolated to 532 nm and the AERosol properties – Dust (AER-D) campaign airborne in situ particle size distributions (PSDs) as reference datasets during atmospheric conditions characterized by dust presence. The near-global fine-mode and coarse-mode pure-dust climate data record is considered unique with respect to a wide range of potential applications, including climatological, time series, and trend analysis over extensive geographical domains and temporal periods, validation of atmospheric dust models and reanalysis datasets, assimilation activities, and investigation of the role of airborne dust in radiation and air quality.

Reply to: “Comment on ‘Stratospheric Aerosol Composition Observed by the Atmospheric Chemistry Experiment Following the 2019 Raikoke Eruption’ by Boone et al.” by Ansmann et al.

AbstractThe question of stratospheric aerosol type following the Raikoke eruption is revisited. Raman lidar measurements suggest the aerosols are predominately smoke, while Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE‐FTS) results indicate the aerosols are predominately sulfate aerosols. The suggested mechanism of smoke particles self‐lofting into the stratosphere is inconsistent with observations in 2020, when more severe Siberian fires failed to invoke a response even vaguely similar to 2019. A side‐by side comparison of the Sarychev and Raikoke eruptions invalidates model calculations that suggest sulfate aerosols should be at levels too low to explain the observed aerosol loading. Structure in infrared absorption spectra provides conclusive evidence of composition, a unique fingerprint for identifying aerosol type. Such information cannot be misinterpreted so long as there is sufficient resolution and spectral coverage. ACE‐FTS infrared aerosol spectra often have an order of magnitude stronger absorption than that of background sulfate aerosols. These spectra can be accurately reproduced by laboratory measured sulfate aerosol spectroscopic information, providing unambiguous identification of the aerosols as sulfate. Visual inspection of thousands of infrared aerosol spectra from the period following the Raikoke eruption indicates the aerosols in the lower stratosphere are predominately sulfate, with no indication of smoke. The lidar study's identification of the aerosols as smoke was based primarily on observed lidar ratios that were more consistent with a material that absorbed significantly at the lidar wavelengths, inconsistent with expectations for sulfate aerosols. However, this could indicate the presence of a substance dissolved in the sulfate aerosols absorbing at those wavelengths rather than smoke particles.

Enhancing mobile aerosol monitoring with CE376 dual-wavelength depolarization lidar

Abstract. We present the capabilities of a compact dual-wavelength depolarization lidar to assess the spatiotemporal variations in aerosol properties aboard moving vectors. Our approach involves coupling the lightweight Cimel CE376 lidar, which provides measurements at 532 and 808 nm and depolarization at 532 nm, with a photometer to monitor aerosol properties. The assessments, both algorithmic and instrumental, were conducted at ATOLL (ATmospheric Observatory of LiLle) platform operated by the Laboratoire d'Optique Atmosphérique (LOA), in Lille, France. An early version of the CE376 lidar co-located with the CE318-T photometer and with a multi-wavelength Raman lidar were considered for comparisons and validation. We developed a modified Klett inversion method for simultaneous two-wavelength elastic lidar and photometer measurements. Using this setup, we characterized aerosols during two distinct events of Saharan dust and dust smoke aerosols transported over Lille in spring 2021 and summer 2022. For validation purposes, comparisons against the Raman lidar were performed, demonstrating good agreement in aerosol properties with relative differences of up to 12 % in the depolarization measurements. Moreover, a first dataset of CE376 lidar and photometer performing on-road measurements was obtained during the FIREX-AQ (Fire Influence on Regional to Global Environments and Air Quality) field campaign deployed in summer 2019 over the northwestern USA. By lidar and photometer mapping in 3D, we investigated the transport of released smoke from active fire spots at William Flats (northeast WA, USA). Despite extreme environmental conditions, our study enabled the investigation of aerosol optical properties near the fire source, distinguishing the influence of diffuse, convective, and residual smoke. Backscatter, extinction profiles, and column-integrated lidar ratios at 532 and 808 nm were derived for a quality-assured dataset. Additionally, the extinction Ångström exponent (EAE), color ratio (CR), attenuated color ratio (ACR), and particle linear depolarization ratio (PLDR) were derived. In this study, we discuss the capabilities (and limitations) of the CE376 lidar in bridging observational gaps in aerosol monitoring, providing valuable insights for future research in this field.

Characteristics and seasonal variations of cirrus clouds from ground-based lidar and satellite observations over Shouxian Area, China

This study investigates the macroscopic and optical properties of cirrus clouds in the 32N region from July 2016 to May 2017, leveraging data from ground-based lidar observations and CALIOP to overcome the inconsistencies in detected cirrus cloud samples. Through extensive data analysis, statistical characteristics of cirrus clouds were discerned, revealing lidar ratio values of 28.5 ± 10.8 from ground-based lidar and 27.4 ± 11.2 from CALIOP. Validation with a decade of CALIOP data (2008-2018) confirmed these findings, presenting a consistent lidar ratio of 27.4 ± 12.0. A significant outcome of the analysis was the identification of a positive correlation between the lidar ratio and cloud centroid temperature, indicating a gradual decrease in the lidar ratio as temperatures dropped. The study established a fundamental consistency in their macroscopic properties, including cloud base height, cloud top height, cloud thickness, cloud centroid height, and cloud centroid temperature. The results for ground-based lidar (CALIOP) are: 10.0 ± 2.1 km (10.0 ± 2.2 km), 11.8 ± 2.1 km (11.5 ± 2.3 km), 1.87 ± 0.83 km (1.52 ± 0.71 km), and 10.5 ± 2.2 km, -46.9 ± 9.7°C (-47.1 ± 10.0°C).These properties exhibited seasonal variations, with cirrus clouds reaching higher altitudes in summer and lower in winter, influenced by the height of the tropopause. The optical properties of cirrus clouds were also analyzed, showing an annual average optical depth of 0.31 ± 0.35 for ground-based lidar and 0.32 ± 0.44 for CALIOP. The study highlighted the distribution of subvisible, thin, and thick cirrus clouds, with a notable prevalence of subvisible clouds during summer, suggesting their frequent formation above 14 km. Furthermore, the study observed linear growth in geometric thickness and optical depth up to 2.5 km from CALIOP and 2.9 km from ground-based lidar. Maximum optical depth was observed at cloud centroid temperatures of -35°C for CALIOP and -40°C for ground-based lidar, with optical depth decreasing as temperatures fell. This suggests that fully glaciated cirrus clouds exhibit the highest optical depth at warmer temperatures, within the complete glaciation temperature range of -35°C to -40°C.

Assessing Lidar Ratio Impact on CALIPSO Retrievals Utilized for the Estimation of Aerosol SW Radiative Effects across North Africa, the Middle East, and Europe

North Africa, the Middle East, and Europe (NAMEE domain) host a variety of suspended particles characterized by different optical and microphysical properties. In the current study, we investigate the importance of the lidar ratio (LR) on Cloud-Aerosol Lidar with Orthogonal Polarization–Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIOP-CALIPSO) aerosol retrievals towards assessing aerosols’ impact on the Earth-atmosphere radiation budget. A holistic approach has been adopted involving collocated Aerosol Robotic Network (AERONET) observations, Radiative Transfer Model (RTM) simulations, as well as reference radiation measurements acquired using spaceborne (Clouds and the Earth’s Radiant Energy System-CERES) and ground-based (Baseline Surface Radiation Network-BSRN) instruments. We are assessing the clear-sky shortwave (SW) direct radiative effects (DREs) on 550 atmospheric scenes, identified within the 2007–2020 period, in which the primary tropospheric aerosol species (dust, marine, polluted continental/smoke, elevated smoke, and clean continental) are probed using CALIPSO. RTM runs have been performed relying on CALIOP retrievals in which the default and the DeLiAn (Depolarization ratio, Lidar ratio, and Ångström exponent)-based aerosol-speciated LRs are considered. The simulated fields from both configurations are compared against those produced when AERONET AODs are applied. Overall, the DeLiAn LRs leads to better results mainly when mineral particles are either solely recorded or coexist with other aerosol species (e.g., sea-salt). In quantitative terms, the errors in DREs are reduced by ~26–27% at the surface (from 5.3 to 3.9 W/m2) and within the atmosphere (from −3.3 to −2.4 W/m2). The improvements become more significant (reaching up to ~35%) for moderate-to-high aerosol loads (AOD ≥ 0.2).

An iterative algorithm to simultaneously retrieve aerosol extinction and effective radius profiles using CALIOP

Abstract. The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on board the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite has been widely used in climate and environment studies to obtain the vertical profiles of atmospheric aerosols. To retrieve the vertical profile of aerosol extinction, the CALIOP algorithm assumes column-averaged lidar ratios based on a clustering of aerosol optical properties measured at surface stations. On one hand, these lidar ratio assumptions may not be appropriate or representative at certain locations. One the other hand, the two-wavelength design of CALIOP has the potential to constrain aerosol size information, which has not been considered in the operational algorithm. In this study, we present a modified inversion algorithm to simultaneously retrieve aerosol extinction and effective radius profiles using two-wavelength elastic lidars such as CALIOP. Specifically, a lookup table is built to relate the lidar ratio with the Ångström exponent calculated using aerosol extinction at the two wavelengths, and the lidar ratio is then determined iteratively without a priori assumptions. The retrieved two-wavelength extinction at each layer is then converted to the particle effective radius assuming a lognormal distribution. The algorithm is tested on synthetic data, Raman lidar measurements and then finally the real CALIOP backscatter measurements. Results show improvements over the CALIPSO operational algorithm by comparing with ground-based Raman lidar profiles.

Tropospheric sulfate from Cumbre Vieja (La Palma) observed over Cabo Verde contrasted with background conditions: a lidar case study of aerosol extinction, backscatter, depolarization and lidar ratio profiles at 355, 532 and 1064 nm

Abstract. In September 2021, volcanic aerosol (mainly freshly formed sulfate plumes) originating from the eruption of Cumbre Vieja on La Palma, Canary Islands, Spain, crossed Cabo Verde at altitudes below 2 km. On 24 September 2021, an extraordinary large aerosol optical depth (AOD) close to 1 (daily mean at 500 nm) was observed at Mindelo, Cabo Verde. This event provided favorable conditions to obtain lidar-derived profiles of extinction and backscatter coefficients, lidar ratio, and depolarization ratio at 355, 532 and 1064 nm in the sulfate aerosol plume. A novel feature of the lidar system operated at Mindelo is the availability of extinction, lidar ratio and depolarization measurements at 1064 nm in addition to the standard wavelengths of 355 and 532 nm. Having measurements of these parameters at all three wavelengths is a major advantage for the aerosol characterization and in aerosol typing efforts as the lidar ratio and the particle linear depolarization ratio are key parameters for this purpose. In this article, we present the key results of the lidar observations obtained on one specific day, namely on 24 September 2021 at 04:38–05:57 UTC, including the first ever measurements of the particle extinction coefficient, the lidar ratio and the depolarization ratio at 1064 nm for volcanic sulfate, and discuss the findings in terms of aerosol optical properties and mass concentrations by comparison with a reference observation (16 September 2021) representing the typical background conditions before the start of the eruptions. We found an unusual high particle extinction coefficient of 721 ± 51, 549 ± 38 and 178 ± 13 Mm−1, as well as an enhanced lidar ratio of 66.9 ± 10.1, 60.2 ± 9.2 and 30.8 ± 8.7 sr at 355, 532 and 1064 nm, respectively, in the sulfate-dominated planetary boundary layer (PBL). The particle linear depolarization ratio was ≤ 0.9 % at all respective wavelengths. It is the first time that lidar-derived intensive aerosol optical properties could be derived for volcanic sulfate at all three wavelengths, and thus it is a highly valuable data set for global aerosol characterization. The lidar analysis also revealed a sulfate-related AOD of about 0.35 ± 0.03 at 532 nm of the total PBL-related AOD of 0.43. The rest of the AOD contribution was caused by a lofted Saharan dust layer extending from 1.4 to 5 km and leading to a total AOD of 0.79 at 532 nm. Volcanic ash contribution to the observed aerosol plumes could be mostly excluded based on trajectory analysis and the observed optical properties. Peak mass concentration was 178.5 ± 44.6 µg m−3 in the volcanic-influenced and sulfate-dominated polluted PBL, showing the hazardous potential of such sulfate plumes to significantly worsen local air quality even at remote locations.

Synergy between Short-Range Lidar and In Situ Instruments for Determining the Atmospheric Boundary Layer Lidar Ratio

Short-range elastic backscatter lidar (SR-EBL) systems are remote sensing instruments for studying low atmospheric boundary layer processes. This work presents a field campaign oriented to filling the gap between the near-surface aerosol processes regarding aerosol radiative properties and connecting them with the atmospheric boundary layer (ABL), centering attention on the residual layer and the ABL transition periods. A Colibri Aerosol Lidar (CAL) instrument, based on the short-range lidar with high spatio-temporal resolution, was used for the first time in the ACTRIS AGORA facility (Andalusian Global Observatory of the Atmosphere) in Granada (Spain). This study showed the possibility of combining lidar and in situ measurements in the lowermost 150 m. The results address, on the one hand, the characterization of the short-range lidar for developing a method to find the calibration constant of the system and to correct the incomplete overlap to further data exploitation. On the other hand, relevant radiative properties such as the temporal series of the aerosol lidar ratio and extinction coefficient were quantified. The campaign was divided in three different periods based on the vehicular emission peak in the early mornings, namely, before, during, and after the emission peak. For before and after the emission peak data classification, aerosol properties presented closer values; however, large variability was obtained after the emission peak reaching the maximum values of extinction and a lidar ratio up to 51.5 ± 11.9 (Mm)−1 and 36.0 ± 10.5 sr, respectively. During the emission peaks, the values reached for extinction and lidar ratio were up to 136.8 ± 26.5 (Mm)−1 and 119.0 ± 22.7 sr, respectively.

Characterization of dust aerosols from ALADIN and CALIOP measurements

Abstract. Atmospheric aerosols have pronounced effects on climate at both regional and global scales, but the magnitude of these effects is subject to considerable uncertainties. A major contributor to these uncertainties is an incomplete understanding of the vertical structure of aerosol, largely due to observational limitations. Spaceborne lidars can directly observe the vertical distribution of aerosols globally and are increasingly used in atmospheric aerosol remote sensing. As the first spaceborne high-spectral-resolution lidar (HSRL), the Atmospheric LAser Doppler INstrument (ALADIN) on board the Aeolus satellite was operational from 2018 to 2023. ALADIN data can be used to estimate aerosol extinction and co-polar backscatter coefficients separately without an assumption of the lidar ratio. This study assesses the performance of ALADIN's aerosol retrieval capabilities by comparing them with Cloud-Aerosol LIdar with Orthogonal Polarization (CALIOP) measurements. A statistical analysis of retrievals from both instruments during the June 2020 Saharan dust event indicates consistency between the observed backscatter and extinction coefficients. During this extreme dust event, CALIOP-derived aerosol optical depth (AOD) exhibited large discrepancies with Moderate Resolution Imaging Spectroradiometer (MODIS) Aqua measurements. Using collocated ALADIN observations to revise the dust lidar ratio to 63.5 sr, AODs retrieved from CALIOP are increased by 46 %, improving the comparison with MODIS data. The combination of measurements from ALADIN and CALIOP can enhance the tracking of aerosols' vertical transport. This study demonstrates the potential for spaceborne HSRL to retrieve aerosol optical properties. It highlights the benefits of spaceborne HSRL in directly obtaining the lidar ratio, significantly reducing uncertainties in extinction retrievals.

Effect of wind speed on marine aerosol optical properties over remote oceans with use of spaceborne lidar observations

Abstract. Marine aerosol affects the global energy budget and regional weather. The production of marine aerosol is primarily driven by wind at the sea–air interface. Previous studies have explored the effects of wind on marine aerosol, mostly by examining the relationships between aerosol optical depth (AOD) and surface wind speed. In this paper, utilizing the synergy of aerosol and wind observations from Aeolus, the relationships between the marine aerosol optical properties at 355 nm and the instantaneous co-located wind speeds of remote oceans are investigated at two vertical layers (within and above the marine atmospheric boundary layer (MABL)). The results show that the enhancements of the extinction and backscatter coefficients caused by wind are larger within the MABL than above it. The correlation models between extinction and backscatter with wind speed were established using power-law functions. The slope variation points occur during extinction and backscatter coefficients increasing with wind speed, indicating that the wind-driven enhancement of marine aerosol involves two phases: a rapid-growth phase with high wind dependence, followed by a slower-growth phase after the slope variation points. We also compared the AOD–wind relationship acquired from Aeolus with CALIPSO-derived results from previous research. The variation in the lidar ratio with wind speed is examined, suggesting a possible “increasing–decreasing–increasing” trend of marine aerosol particle size as wind speed increases. This study enhances the comprehension of the correlation between marine aerosol optical properties and wind speed by providing vertical information and demonstrating that their relationships are more complex than a linear or exponential relation.

1064 nm rotational Raman polarization lidar for profiling aerosol and cloud characteristics

The vertical profiles of aerosol or mixed-phase cloud optical properties (e.g. extinction coefficient) at 1064 nm are difficult to obtain from lidar observations. Based on the techniques of rotational Raman signal at 1058 nm described by Haarig et al. [ Atmos. Meas. Tech. 9, 4269 (2016)10.5194/amt-9-4269-2016 ], we have developed a novel rotational Raman polarization lidar at 1064 nm at Wuhan University. In this design, we optimized the central wavelength of the rotational Raman channel to 1056 nm with a bandwidth of 6 nm to increase the signal-to-noise ratio and minimize the temperature dependence of the extracted rotational Raman spectrum. And then separated elastic polarization channels (1064 nm Parallel, P and 1064 nm Cross, S) into near range (low 1064 nm P and 1064 nm S) and far range detection channels (high 1064 nm P and 1064 nm S) to extend the dynamic range of lidar observation. Silicon single photon avalanche diodes (SPAD) working at photon counting mode were applied to improve the quantum efficiency and reduce the electronic noise, which resulted in quantum efficiency of 2.5%. With a power of 3 W diode pumped pulsed Nd:YAG laser and aperture of 250 mm Cassegrain telescope, the detectable range can cover the atmosphere from 0.3 km to the top troposphere (about 12-15 km). To the best of our knowledge, the design of this novel lidar system is described and the mixed-phase cloud and aerosol optical properties observations of backscatter coefficients, extinction coefficients, lidar ratio and depolarization ratio at 1064 nm were performed as demonstrations of the system capabilities.

Aerosol and cloud data processing and optical property retrieval algorithms for the spaceborne ACDL/DQ-1

Abstract. The new-generation atmospheric environment monitoring satellite DQ-1, launched successfully in April 2022, carries the Aerosol and Carbon Detection Lidar (ACDL), which is capable of globally profiling aerosol and cloud optical properties with high accuracy. The ACDL/DQ-1 is a high-spectral-resolution lidar (HSRL) that separates molecular backscatter signals using an iodine filter and has 532 nm polarization detection and dual-wavelength detection at 532 and 1064 nm, which can be utilized to derive aerosol optical properties. The methods have been specifically developed for data processing and optical property retrieval according to the specific characteristics of the ACDL system and are introduced in detail in this paper. Considering the different signal characteristics and different background noise behaviors of each channel during daytime and nighttime, the procedures of data pre-processing, denoising process and quality control are applied to the original measurement signals. The aerosol and cloud optical property products of the ACDL/DQ-1, including the total depolarization ratio, backscatter coefficient, extinction coefficient, lidar ratio and color ratio, can be calculated by the retrieval algorithms presented in this paper. Two measurement cases with use of the ACDL/DQ-1 on 27 June 2022 and the global averaged aerosol optical depth (AOD) from 1 June to 4 August 2022 are provided and analyzed, demonstrating the measurement capability of the ACDL/DQ-1.

Validation of initial observation from the first spaceborne high-spectral-resolution lidar with a ground-based lidar network

Abstract. On 16 April 2022, China successfully launched the world's first spaceborne high-spectral-resolution lidar (HSRL), which is called the Aerosol and Carbon Detection Lidar (ACDL), on board the Atmospheric Environment Monitoring Satellite known as Daqi-1 (DQ-1). The ACDL is expected to precisely detect the three-dimensional distribution of aerosol and cloud globally with high spatial–temporal resolutions. To assess the performance of the newly launched satellite lidar, the ACDL-retrieved observations were compared with ground-based lidar measurements of atmospheric aerosol and cloud over northwest China from May to July 2022 using the Belt and Road lidar network (BR-lidarnet) initiated by Lanzhou University in China and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) lidar observations. A total of six cases in the daytime and nighttime, including clear days, dust events, and cloudy conditions, were selected for further analysis. Moreover, profiles of the total attenuated backscatter coefficient (TABC) and the volume depolarization ratio (VDR) at 532 nm measured by the ACDL, the CALIPSO lidar, and ground-based lidar are compared in detail. Comparison is made between the 532 nm extinction coefficient and lidar ratio obtained from ACDL HSRL retrieval and the Raman retrieval results obtained from BR-lidarnet. The achieved results revealed that the ACDL observations were in good agreement with the ground-based lidar measurements during dust events with a relative deviation of about −10.5 ± 25.4 % for the TABC and −6.0 ± 38.5 % for the VDR. Additionally, the heights of the cloud top and bottom from these two measurements were well matched and comparable. Compared with the observation of CALIPSO, the ACDL also shows high consistency. This study proves that the ACDL provides reliable observations of aerosol and cloud in the presence of various climatic conditions, which helps to further evaluate the impacts of aerosol on climate and the environment, as well as on the ecosystem in the future.

Optical Characterization of Marine Aerosols Using a Morphologically Realistic Model With Varying Water Content: Implications for Lidar Applications and Passive Polarimetric Remote Sensing

AbstractRetrieving the physical properties and water content of marine aerosols requires understanding the links between the particles' optical and microphysical properties. By using a morphologically realistic model with varying salt mass fractions fm, describing the transition from irregularly shaped, dry salt crystals to brine‐coated geometries, optical properties relevant to polarimetric remote sensing are computed at wavelengths of 532 and 1,064 nm. The extinction cross section and its color ratio depend on particle size, but are insensitive to changes in fm; thus, measured extinction coefficients at two wavelengths contain information on both particle number and size. The lidar ratio's dependence on both size and wavelength has implications for inverting the lidar equation. The results suggest that active observations of the backscattering cross section's color ratio and the depolarization ratio, as well as, passive observations of the degree of linear polarization offer avenues to obtain the water content of marine aerosols.

Geometrical and optical properties of cirrus clouds in Barcelona, Spain: analysis with the two-way transmittance method of 4 years of lidar measurements

Abstract. In this paper a statistical study of cirrus geometrical and optical properties based on 4 years of continuous ground-based lidar measurements with the Barcelona (Spain) Micro Pulse Lidar (MPL) is analysed. First, a review of the literature on the two-way transmittance method is presented. This method is a well-known lidar inversion method used to retrieve the optical properties of an aerosol–cloud layer between two molecular (i.e. aerosol and cloud-free) regions below and above, without the need to make any a priori assumptions about their optical and/or microphysical properties. Second, a simple mathematical expression of the two-way transmittance method is proposed for both ground-based and spaceborne lidar systems. This approach of the method allows the retrieval of the cloud optical depth, the cloud column lidar ratio and the vertical profile of the cloud backscatter coefficient. The method is illustrated for a cirrus cloud using measurements from the ground-based MPL and from the spaceborne Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). Third, the database is then filtered with a cirrus identification criterion based on (and compared to) the literature using only lidar and radiosonde data. During the period from November 2018 to September 2022, 367 high-altitude cirrus clouds were identified at 00:00 and 12:00 UTC, of which 203 were successfully inverted with the two-way transmittance method. The statistical results of these 203 high-altitude cirrus clouds show that the cloud thickness is 1.8 ± 1.1 km, the mid-cloud temperature is −51 ± 8 ∘C and the linear cloud depolarization ratio is 0.32 ± 0.13. The application of the transmittance method yields an average cloud optical depth (COD) of 0.36 ± 0.45 and a mean effective column lidar ratio of 30 ± 19 sr. Statistical results of the errors associated with the two-way transmittance method retrievals are also provided. The highest occurrence of cirrus is observed in spring and the majority of cirrus clouds (48 %) are visible (0.03 < COD < 0.3), followed by opaque (COD > 0.3) with a percentage of 38 %. Together with results from other sites, possible latitudinal dependencies have been analysed together with correlations between cirrus cloud properties. For example, we noted that in Barcelona the COD correlates positively with the cloud base temperature, effective column lidar ratio and linear cloud depolarization ratio and negatively with the cloud base height.

Optical and Microphysical Properties of the Aerosols during a Rare Event of Biomass-Burning Mixed with Polluted Dust

A rare event of mixed biomass-burning and polluted dust aerosols was observed over Athens, Greece (37.9° N, 23.6° E), during 21–26 May 2014. This event was studied using a synergy of a 6-wavelength elastic-Raman-depolarization lidar measurements, a CIMEL sun photometer, and in situ instrumentation. The FLEXPART dispersion model was used to identify the aerosol sources and quantify the contribution of dust and black carbon particles to the mass concentration. The identified air masses were found to originate from Kazakhstan and Saharan deserts, under a rare atmospheric pressure system. The lidar ratio (LR) values retrieved from the Raman lidar ranged within 25–89 sr (355 nm) and 35–70 sr (532 nm). The particle linear depolarization ratio (δaer) ranged from 7 to 28% (532 nm), indicating mixing of dust with biomass-burning particles. The aerosol optical depth (AOD) values derived from the lidar ranged from 0.09–0.43 (355 nm) to 0.07–0.25 (532 nm). An inversion algorithm was used to derive the mean aerosol microphysical properties (mean effective radius (reff), single scattering albedo (SSA), and mean complex refractive index (m)) inside selected atmospheric layers. We found that reff was 0.12–0.51 (±0.04) µm, SSA was 0.94–0.98 (±0.19) (at 532 nm), while m ranged between 1.39 (±0.05) + 0.002 (±0.001)i and 1.63 (±0.05) + 0.008 (±0.004)i. The polarization lidar photometer networking (POLIPHON) algorithm was used to estimate the vertical profile of the mass concentration for the dust and non-dust components. A mean mass concentration of 15 ± 5 μg m−3 and 80 ± 29 μg m−3 for smoke and dust was estimated for selected days, respectively. Finally, the retrieved aerosol microphysical properties were compared with column-integrated sun photometer CIMEL data with good agreement.

HETEAC-Flex: an optimal estimation method for aerosol typing based on lidar-derived intensive optical properties

Abstract. This study introduces a novel methodology for the characterization of atmospheric aerosol based on lidar-derived intensive optical properties. The proposed aerosol-typing scheme is based on the optimal estimation method (OEM) and allows the identification of up to four different aerosol components of an aerosol mixture, as well as the quantification of their contribution to the aerosol mixture in terms of relative volume. The four aerosol components considered in this typing scheme are associated with the most commonly observed aerosol particles in nature and are assumed to be physically separated from each other and, therefore, can create external mixtures. Two components represent absorbing and less-absorbing fine-mode particles, and the other two components represent spherical and non-spherical coarse-mode particles. These components reflect adequately the most frequently observed aerosol types in the atmosphere: combustion- and pollution-related aerosol, sea salt, and desert dust, respectively. In addition, to consolidate the calibration and validation efforts for the upcoming EarthCARE mission, the typing scheme proposed here is in accordance with the Hybrid End-To-End Aerosol Classification (HETEAC) model of EarthCARE. The lidar-derived optical parameters used in this typing scheme are the lidar ratio and the particle linear depolarization ratio at two distinct wavelengths (355 and 532 nm), the backscatter-related color ratio for the wavelength pair of 532/1064 nm and the extinction-related Ångström exponent for the wavelength pair of 355/532 nm. These intensive optical properties can be combined in different ways, making the methodology flexible, thus allowing its application to lidar systems with different configurations (e.g., single wavelength or multiwavelength, Raman, high spectral resolution). The typing scheme was therefore named HETEAC-Flex due to its compatibility with EarthCARE's HETEAC and its methodological flexibility. The functionality of the typing scheme is demonstrated by its application to three case studies based on layer-averaged optical properties.