AbstractGeopolymer concrete (GPC) is a rising eco-conscious substitute for traditional cement-based concrete, bringing the construction industry closer to sustainability. Self-compacting geopolymer concrete (SCGC) enhances the concrete flowability and fills the congested reinforced areas without vibrators in concrete structures such as bridges, tunnels and canals. This study aims to analyze the impact of silicon dioxide nanoparticles (NS) on the rheological and mechanical properties of SCGC to optimize the dosage of NS in SCGC. For this purpose, NS (0–6%) blended in partially distributed binders of fly ash and ground granulated blast furnace slag (50:50) with 0.5 alkaline binder ratio, 2% superplasticizers (9 kg m−3) (MasterGlenium SKY 8233) and 12% extra water (54 kg m−3). Sodium silicate solution and sodium hydroxide ratio of 2.5 was used for this study. It is observed that SCGC with 3% NS replacement complied with the guidelines of EFNARC. According to the T50cm slump flow test, V-funnel test, and L-box test results meet the guidelines of up to 4% NS replacement, and 3% NS addition offers excellent mechanical properties in SCGC. This study concluded that the replacement of 3% of NS improved the fresh and hardened properties of SCGC, which can apply to construction.