To deal with the radio frequency threat posed by modern complex radar networks to aircraft, we researched the unmanned aerial vehicle (UAV) formations radar countermeasures, aiming at the solution of radar jamming resource allocation under system countermeasures. A jamming resource allocation method based on an improved firefly algorithm (FA) is proposed. Firstly, the comprehensive factors affecting the level of threat and interference efficiency of radiation source are quantified by a fuzzy comprehensive evaluation. Besides, the interference efficiency matrix and the objective function of the allocation model are determined to establish the interference resource allocation model. Finally, A mutation operator and an adaptive heuristic are integtated into the FA algorithm, which searches an interference resource allocation scheme. The simulation results show that the improved FA algorithm can compensate for the deficiencies of the FA algorithm. The improved FA algorithm provides a more scientific and reasonable decision-making plan for aircraft mission allocation and can effectively deal with the battlefield threats of the enemy radar network. Moreover, in terms of convergence accuracy and speed as well as algorithm stability, the improved FA algorithm is superior to the simulated annealing algorithm (SA), the niche genetic algorithm (NGA), the improved discrete cuckoo algorithm (IDCS), the mutant firefly algorithm (MFA), the cuckoo search and fireflies algorithm (CSFA), and the best neighbor firefly algorithm (BNFA).